Alpha decay of the new isotopes 188,189Po

New neutron-deficient isotopes ^188,189Po have been produced in the complete fusion reaction of ⁵²Cr ions with a ¹⁴²Nd target at the velocity filter SHIP. The evaporation residues were separated in-flight and subsequently identified on the basis of α-γ and α-conversion electron coincidence measurements and of α-α position and time correlations. In ¹⁸⁹Po a ground state to ground state α decay with E_α1= 7540(20) keV, T_1/2= 5(1) ms and two fine structure α-decays at E_α2= 7264(15) keV and E_α3= 7316(15) keV have been observed. In ¹⁸⁸Po (T_1/2= 400⁺²⁰⁰ ₋₁₅₀μs) a ground state to ground state α decay at E_α= 7915(25) keV and a fine structure α decay at E_α= 7350(40) keV have been found. Improved data on the α-decay of ¹⁸⁹Bi were obtained. Received: 15 October 1999     

Alpha decay of new neutron deficient gold,mercury, and thallium isotopes

In fusion evaporation reactions of a⁹²Mo beam with targets of neutron deficient Rb — Mo isotopes very neutron deficient isotopes of elements between Au and Po have been produced. The new isotopes^{173, 174}Au,^{175, 176}Hg, and¹⁷⁹Tl were identified by alpha spectroscopy. The mass excess value of¹⁷⁶Hg could be linked to known values of theN?Z=16 chain. The location of the new isotopes with respect to the proton drip line is discussed. A new high energyα transition of (7.20±0.02) MeV andT _1/2=(1.4±0.5) ms has been found in the reaction⁹²Mo+⁸⁹Y→¹⁸¹Tl^* at an excitation energy of 37 MeV. It is tentatively assigned to isotopes produced in 2-particle evaporation channels.     

Alpha decay studies of new neutron-deficient francium isotopes and their daughters

Neutron-deficient francium isotopes were produced by proton-induced spallation reactions and investigated by alpha spectroscopy following on-line mass separation. The new isotopes^{201, 202}Fr were identified and their half-lives measured. An improved value for the half-life of²⁰³Fr was obtained. Alpha branching ratios were determined for^{198m, g, 199}At. The derivation of the mass excess of²⁰²Fr and the systematics of alpha energies and reduced widths are discussed.     

Alpha decay of neutron-deficient isotopes of tungsten

Three neutron-deficient isotopes of tungsten have been produced by the reactions of ²⁴Mg on targets of ¹⁴⁷Sm and ¹⁴⁴Sm. They are ¹⁶⁴W, E_α = 5.153 MeV, $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 6.3 s}$; ¹⁶³W, E_α = 5.385 MeV, $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 2.5}\text{s}$; and ¹⁶²W, E_α = 5.53 MeV, $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{< 0.25}\text{s}$.     

Alpha decay studies of neutron-deficient radium isotopes

Neutron-deficient isotopes of radium have been produced in the reactions ³⁵Cl + ¹⁷⁵Lu, ⁴⁰Ar + ^170,171Yb, and ³⁶Ar + ^170,171Yb and separated in-flight with a gas-filled recoil separator. The activities have been identified on the basis of correlated alpha decay chains. The alpha particle energy E_α and the half-life T_1/2 of an isomeric state of the new isotope, ^203mRa, have been determined to be (7615±20) keV and (33 _?10 ⁺²² ), respectively. An assignment of another decay with E_α = (7577±20) keV and T_1/2 = (1.1 _?0.5 ^+5.0 ) ms to ^203g Ra is made on the basis of one observed three-decay chain. Tentative evidence for the production of the new isotope ²⁰²Ra is also given. The values E_α = (7860±60) keV and T_1/2 = (0.7 _?0.3 ^+3.3 ) ms were measured. Improved decay data have been obtained for ²⁰⁴Ra. The results are E_α = (7484±10) keV and T_1/2 = (59 _?9 ⁺¹² ). Earlier findings concerning the decay of two states in ²⁰⁵Ra and an isomer in ²⁰⁷Ra have been confirmed. Approximate values for cross sections have been determined for ²⁰²Ra, produced using the ³⁶Ar + ¹⁷⁰Yb reaction and for ²⁰³Ra, ²⁰⁴Ra, and ²⁰⁵Ra using the ³⁵Cl + ¹⁷⁵Lu reaction. The results are 2 nb (²⁰²Ra), 4 nb (²⁰³Ra), 40 nb (²⁰⁴Ra), and 800 nb (²⁰⁵Ra).     

Alpha decay studies of neutron-deficient radium isotopes

Neutron-deficient isotopes of radium have been produced in the reactions³⁵Cl+¹⁷⁵Lu,⁴⁰Ar+^170,171Yb, and³⁶Ar+^170,171Yb and separated in-flight with a gas-filled recoil separator. The activities have been identified on the basis of correlated alpha decay chains. The alpha particle energy E_α and the half-life T_1/2 of an isomeric state of the new isotope,^203m Ra, have been determined to be (7615±20) keV and (33 _?10 ⁺²² ) ms, respectively. An assignment of another decay with E_α = (7577±20) keV and T_1/2=(1.1 _?0.5 ^+5.0 ) ms to^203g Ra is made on the basis of one observed three-decay chain. Tentative evidence for the production of the new isotope²⁰²Ra is also given. The values E_α = (7860±60) keV and T_1/2=(0.7 _?0.3 ^+3.3 ) ms were measured. Improved decay data have been obtained for²⁰⁴Ra. The results are E_α = (7484±10) keV and T_1/2=(59 _?9 ⁺¹² ) ms. Earlier findings concerning the decay of two states in²⁰⁵Ra and an isomer in²⁰⁷Ra have been confirmed. Approximate values for cross sections have been determined for²⁰²Ra, produced using the³⁶Ar+¹⁷⁰Yb reaction and for²⁰³Ra,²⁰⁴Ra, and²⁰⁵Ra using the³⁵Cl+¹⁷⁵Lu reaction. The results are 2 nb (²⁰²Ra), 4 nb (²⁰³Ra), 40 nb (²⁰⁴Ra), and 800 nb (²⁰⁵Ra).     

Alpha decay of neutron-deficient rhenium and osmium isotopes

Neutron-deficient osmium and rhenium isotopes were produced by bombarding an enriched¹⁴⁴Sm target with beams of²⁷Al and²⁸Si. Previously reported decay data concerning^168,169,170Os were confirmed. Three newα groups, observed in the¹⁴⁴Sm+²⁷Al reaction, were assigned to the decay of^166,167,168Re based on excitation functions,α-energy systematics and theoretical half-life predictions. Their decay properties are: $$\begin{gathered} {}^{166}\operatorname{Re} , E_\alpha = 5,372 (10) keV, T_{1/2} = 2.8 (3) s; \hfill \\ {}^{167}\operatorname{Re} , E_\alpha = 5,136 (8) keV, T_{1/2} = 6.1 (2) s and \hfill \\ {}^{168}\operatorname{Re} , E_\alpha = 4,894 (10) keV, T_{1/2} = 6.9 (8) s. \hfill \\ \end{gathered}$$ It is proposed that twoα groups, observed in the¹⁴⁴Sm+²⁸Si reaction, originate from isomeric states in^168,169Re. Our measured data for the isomeric states are: $$\begin{gathered} {}^{168m}\operatorname{Re} , E_\alpha = 5,250 (10) keV, T_{1/2} = 6.6 (15) s and \hfill \\ {}^{169m}\operatorname{Re} , E_\alpha = 5,050 (10) keV, T_{1/2} = 12.9 (11) s. \hfill \\ \end{gathered} $$      

Alpha decay studies of tellurium,iodine, xenon and cesium isotopes

Very neutron-deficient isotopes in the trans-tin region were produced by reactions of 290 MeV ⁵⁸Ni ions on ⁵⁸Ni targets, and studied by on-line mass separation at GSI. Twelve α-emitters — ^107–110Te, ^110–113I, ^111–113Xe, ¹¹⁴Cs — were identified. Systematics of Q_α values and reduced α-widths for this new island of α-emission are discussed.     

Proton decay of the isobaric analogs of the ground states of207Pb and208Pb

The proton decays \(\tilde p\) of isobaric analog states of^{207, 208}Pb in the reactions^{207, 208}Pb(p, n) have been studied using a neutron-proton coincidence technique. The width anomaly observed in (p, n) [4] and (p, n \(\tilde p\) ) singles spectra [11] is resolved in the coincident spectra.     

Alpha decay of the new isotope172Au

The first observation of the extremely neutrondeficient nucleus¹⁷²Au is reported, produced using the fusion evaporation reaction⁷⁰Ge+¹⁰⁶Cd→¹⁷⁶Hg^* (E_x?64 MeV). Mass separated evaporation residues were implanted into a double-sided silicon strip detector, and the energy and time of subsequent decay events were recorded. The alpha decay of¹⁷²Au was measured with an energy =6860±10 KeV, corresponding to =7020±10 Kev, and a half-life of 4±1 ms. No evidence was seen for a proton decay branch, implying a limit ofb _p ≤ 2 %.     

Alpha decay of the new isotope 174Hg

Neutron deficient mercury isotopes were produced in the reaction ³⁶Ar + ¹⁴⁴Sm using bombarding energies of 180–230 MeV. Fusion products were separated in-flight from the primary beam using a gas-filled recoil separator. An alpha line with the alpha particle energy and half-life of (7069±11) keV and (2.1 _?0.7 ^+1.8 ) ms, respectively, was assigned to the new mercury isotope ¹⁷⁴Hg.     

Alpha decay studies of very neutron deficient isotopes of Hf,Ta, W,and Re

Very neutron deficient isotopes in the Hf-Re region were produced by bombarding targets of^{107, 109}Ag,^{nat, 108, 110}Pd, and¹⁰³Rh with⁵⁸Ni accelerated by the linear accelerator UNILAC at GSI. After separation from the projectile beam by the velocity filter SHIP, the fusion products were implanted with their full recoil energy into a silicon surface barrier detector. The subsequent alpha decay of the implanted ions was measured with the same detector. In some of the experiments the evaporation residues were implanted into a position sensitive silicon surface barrier detector. With a newly developed position and time correlation technique parent daughter relationships, half lives, andα branching ratios of a large number of isotopes could be determined. In the investigated reactions the eleven new isotopes^161–164Re,¹⁶⁰W,^157–161Ta, and¹⁵⁶Hf could be identified. The measuredQ _α values, half lives, and a branching ratios are discussed. Two new high energyα. transitions of (7,408±10) keV and (7,804±15) keV were also found with half lives of 2.7 ms and 0.52 ms, respectively.A tentative mass and atomic number assignment givesA=153–156 andZ=70–72. The energies of the excited isomeric states are between 2 MeV and 3 MeV. From the systematics of alpha ground state transitions in even nuclei a hindrance of 10⁵ can be deduced for both transitions, possibly indicating orbital angular momenta on the order of 10? for the alpha emitting states. The isomers are proposed to belong to shell model isomers beyond¹⁴⁶Gd.     

Alpha decay of Cm

An enriched sample of ²⁴⁷Cm (99.4 %) has been used to investigate the -decay scheme of ²⁴⁷Cm. Seven -groups with energies and intensities 5.265 (13.8 %), 5.210 (5.7 %), 5.145 (1.2 %), 4.983 (2.0 %), 4.941 (1.6 %), 4.868 (71.0 %) and 4.818 (4.7 %) were observed. Gamma-singles and γ coincidence spectra showed the presence of 278.0, 287.5, 346.0 and 402.4 keV γ-rays. A two-parameter coincidence experiment established that the sources of the 402.4 and the 287.5 keV γ-rays were 4.868 and 4.983 MeV -groups, respectively. The multipolarity of the 287.5 keV transition was found to be M1. The K conversion coefficient of the 402.4 keV γ-ray indicates an E1 multipolarity for this transition. The levels at 287.5 and 402.4 keV have been assigned to the and Nilsson states, respectively. The half-life of ²⁴⁷Cm was found to be (1.56±0.05) ×10⁷ y from the pulse analysis and mass spectrometric analysis of the sample.     

Neutron particle-hole electric dipole states in 206, 207, 208Pb

Inelastic proton scattering on ²⁰⁶Pb, ²⁰⁷Pb and ²⁰⁸Pb through isobaric analog resonances has been used to study neutron particle-hole excitations with large ground-state γ-branches in these Pb isotopes. Relative (p, p′) cross sections at 90° are extracted for structures selectively excited on the $\text{d}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}\text{,}\text{s}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{and d}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}\text{?}\text{g}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}$ resonances. Interpretation of excitations is ²⁰⁶Pb and ²⁰⁷ Pb in terms of coupling to states in ²⁰⁸Pb is discussed. Branching ratios for 1^?states in ²⁰⁸Pb at 4.84, 5.29, 5.94 and 6.31 MeV and the $\text{1}\text{2}{}^{\mathrm{+}}$ state in ²⁰⁷Pb at 4.63 MeV are deduced.     

Alpha decay of 114Ba

We measured for the first time the α decay of ¹¹⁴Ba. The results are discussed in comparison with theoretical predictions.     

Alpha decay of light nuclei

Theoretical α spectroscopic amplitudes are calculated in jj coupling and isotopic spin formalism. The formulae obtained are applied for calculating the α reduced width amplitudes of the lowest lying 2⁺ levels of ¹⁶O using the shell-model wave functions of Zuker, Buck and McGrory.     

Spontaneous-fission decay properties and production cross-sections for the neutron-deficient nobelium isotopes formed in the 44, 48Ca + 204, 206, 208Pb reactions

Heavy-ion fusion reactions ⁴⁸Ca + ²⁰⁴Pb and ⁴⁴Ca + ²⁰⁸Pb leading to the same compound nucleus ²⁵²No^* were run in attempts to produce new neutron-deficient spontaneous-fission isotopes of ^249,250No using the electrostatic separator VASSILISSA. Production cross-sections for the spontaneous-fission activities with the half-lives 5.6 and 54 μs observed in these reactions are compared with the measured ones for the well-known isotopes of ^{251 - 255}No formed in the heavy-ion fusion reactions ⁴⁸Ca + ²⁰⁶Pb and ⁴⁸Ca + ²⁰⁸Pb. The obtained excitation functions for the reaction products formed after the evaporation of 1-4 neutrons from the corresponding compound No nuclei have been compared with similar data obtained earlier and results of statistical model calculations. Received: 26 July 2002 / Accepted: 5 November 2002 / Published online: 18 March 2003 RID="a" ID="a"e-mail: eremin@sunvas.jinr.ru Communicated by J. ?yst?     

Levels in208Pb populated in the decay of208Tl(ThC″)

Gamma rays in the disintegration of²⁰⁸Tl(ThC″) have been studied with Ge(Li)-Na I(Tl) anti-Compton and coincidence spectrometers. Several new transitions are reported most of which are placed in a decay scheme incorporating excited states in²⁰⁸Pb at 2,614.5, 3,197.6, 3,475.0, 3,708.3, 3,919.8, 3,960.9, 3,998.5, 4,125.3, 4,180.4, 4,296.1 and 4,480.0 keV. According to the present data, the recently reported intensity of 4.5±1.5% of beta groups feeding levels near 4.3 MeV is far too large.