Electrooptical effect in YBa2Cu3O6+x films

Optical absorption in YBa₂Cu₃O_6+x metal films carrying a direct current up to 100 mA is investigated. For films with a highly nonlinear I-V curve the current is observed to have a strong influence on interband absorption. The effect is not observed in the region of optical transitions at local levels. The results are analyzed from the standpoint of carrier localization and delocalization processes. Fiz. Tverd. Tela (St. Petersburg) 39, 1747–1749 (October 1997)     

Local magnetism in superconducting YBa2Cu3O6+x

Oxygen-deficient YBa₂Cu₃O_6+x samples were investigated by the muon spin rotation technique in zero external field. In an intermediate oxygen concentration region we find strongly relaxing μSR signals indicating the existence of internal magnetic fields. The strongly relaxing signals were observed only in samples with superconducting transition temperatures below 50 K. As an interpretation of the data we suggest that magnetic ordering and superconductivity coexist in these samples within regions of extensions of a few lattice constants, but not necessarily on the same sites.     

Theoretical study ofμ + site in YBa2Cu3O x site in YBa2Cu3O x

The muon is a useful probe of magnetic fields in superconductors, but knowing the field seen by the muon is often of limited value until we know where the muon is in the crystal lattice. Here we employ two independent theoretical methods to search for candidate muon sites:the potential energy field method, which seeks the minimum of the electrostatic potential of theμ ⁺, and themagnetic dipolar field method, which compares the calculated magnetic field (due to host electronic or nuclear dipolar fields) with the observed local fields at the muon. Work supported by Canadian NRC and NSERC.     

Cluster approach to the problem of hopping with interactions: oxygen transport in YBa2Cu3O6+x

A method for calculation of hopping transport phenomena in lattices which allows for strong interparticle interactions by means of cluster expansion constructions for transport coefficients is presented. The method developed is applied to the oxygen transfer in YBa₂Cu₃O_6+x taking into account interactions both between oxygen ions in lattice sites and between hopping oxygen in the saddle point and surroundings. It is shown that the oxygen mobility μ decreases as the oxygen content increases in contrast to the chemical diffusivityD which rises withx. The effective activation energiesU _eff forD and μ have peculiarities at the phase transition points. At fixedx valuesU _eff of μ falls by ≈ 0.1– 0.15 eV at the ortho-tetraphase transition whileU _eff ofD practically doesn't change. Paper presented at the 5th Euroconference on Solid State Ionics, Benalmádena, Spain, Sept. 13–20, 1998.     

Magnetic properties of undoped YBa 2 Cu 3 O 6 + x system

In the present paper, we study the magnetic properties of bilayer cuprate antiferromagnets. In order to evaluate the expressions for spin-wave dispersion, sublattice magnetization, Néel temperature and the magnetic contribution to the specific heat, the double time Green's function technique has been employed in the random phase approximation (RPA). The spin wave dispersion curve for a bilayer antiferromagnetic system is found to consist of one acoustic and one optic branch. The “optical magnon gap” has been attributed solely to the intra-bilayer exchange coupling (J _⊥ ) as its magnitude does not change significantly with the inter-bilayer exchange coupling (J_z). However J_z is essential to obtain the acoustic mode contribution to the magnetization. The numerical calculations show that the Néel temperature (T _N ) of the bilayer antiferromagnetic system increases with the J_z and a small change in J_z gives rise to a large change in the Néel temperature of the system. The magnetic specific heat of the system follows a T² behaviour but in the presence of J_z it varies faster than T². Received 13 July 2000 and Received in final form 14 May 2001     

Recent progress on neutron studies of YBa2Cu3O6+x

A review is given of recent developments in inelastic neutron scattering experiments on the high temperature superconductor YBa_2Cu_3O_7 and its antiferromagnetic precursor YBa_2Cu_3O_6.2. These include the detection of high energy “optical” spin waves and the determination of the full spin Hamiltonian in YBa_2Cu_3O_6.2, a detailed study of the 40 meV magnetic resonance peak in the superconducting state of YBa_2Cu_3O_7, and experiments on the effect of superconductivity on phonon lifetimes in YBa_2Cu_3O_7. This revised version was published online in August 2006 with corrections to the Cover Date.     

Cu chemistry of YBa2Cu3O6+x investigated by nuclear quadrupole resonance

The nuclear quadrupole resonance (NQR) technique has been utilized to characterize the local oxygen coordination of inequivalent Cu sites in YBa₂Cu₃O_6+x(0 ≤ x ≤ 0.91). Essentially, four distinct NQR lines which correspond to 2, 3,4 oxygen coordinated Cu sites in the Cu-O chains and 5 oxygen coordinated Cu sites in the Cu-O planes have been observed. The zero-field NQR frequencies of these are centered at about 30.1, 24.0, 22.0 and 31.5 MHz for ⁶³Cu, respectively. For the antiferromagnetic ordered state (x ≤ 0.3), antiferromagnetic nuclear resonance (AFNR) has been observed at 90 MHz with quadrupole splittings associated with the moment-bearing Cu sites in the Cu-O planes. The relative intensities of these resonance lines depend on the oxygen content, and this gives us a microscopic understanding of the Cu chemistry of this system.     

Effect of loading on the chemical potential of oxygen atoms in YBa2Cu3O6+x (YBCO) and PrBa2Cu3O6+x (PBCO)

The effect of loading on the chemical potential of oxygen atoms has been studied in the YBCO and PBCO isostructural compounds, with the former exhibiting HTSC, and the latter, not. Application of a load to both YBCO and PBCO in the orthorhombic phase causes an increase in the chemical potential within the 0.5<x<0.8 interval, which is interpreted as a phase-separation region. This effect is associated with an increase in the fraction of an ordered phase possessing a smaller specific volume. It is also related to the additional compressibility of the material. In the tetragonal phase this effect is observed only in YBCO. The absence of the effect in PBCO implies the electron-phonon coupling in this material has a different nature. Fiz. Tverd. Tela (St. Petersburg) 41, 572–576 (April 1999)     

Investigation of superconductivity and magnetism in ceramic YBa2Cu3O6+x

In this work the magnetic and superconducting properties of YBa₂Cu₃O_6+x , ceramic samples are studied with regard to there preparations technology and oxygen content. It is shown that at 0.41≤x≤0.45 the magnetic and superconducting states coexist.