Travelling-wave-pumped ultrashort-pulse distributed-feedback dye laser

A travelling-wave pumping scheme is used to excite a distributed feedback dye laser. Output pulse shortening below the resolution limit of the streak camera system (1.9 ps) is observed when the velocity of the travelling pump wave is properly matched to the velocity of the laser emission. The pulse spectrum has been measured simultaneously. It consists of a single line of 4 Å width.     

Subpicosecond,widely tunable distributed feedback dye laser

A simple, achromatic, widely tunable distributed feedback dye laser arrangement is described. It makes use of a microscope objective, which images a transmission grating into the active medium. With this arrangement subpicosecond operation and broad tunability (400–760 nm) is reported.     

A novel picosecond distributed feedback dye laser arrangement for excimer laser pumping

A distributed feedback dye laser arrangement is described which can generate pulses at the subharmonic wavelengths of the main excimer laser lines (308 nm, 248 nm, 193 nm, etc.). The laser can be pumped with broadband lasers, such as the XeCl^* laserpumped dye laser with competing cavities. The laser is designed to be used as a part of a femtosecond, terawatt excimer laser system.     

Novel achromatic distributed feedback dye laser for subpicosecond operation

The optical pump arrangement of distributed feedback dye lasers (DFDLs) having a grating beam splitter is analyzed in detail. The upper limit of the pump spectral bandwidth and beam divergence are given as a function of the length of the excited volume. A novel achromatic pump arrangement is reported which is capable of producing a short, high visibility interference pattern even if a divergent pump source of several nm bandwidth is used. The DFDL pulse duration has an estimated lower limit of 200 fs.     

Characteristics of a hybridly mode-locked cw dye laser

We present experimental and theoretical results on the characteristics and random variations of subpicosecond pulses generated by a synchronously pumped cw dye laser with saturable absorber. The analysis of the power spectra indicates rapid fluctuations of the pulse duration of 40–50%, energy fluctuations of 3%, and a jitter of the repetition time of 0.1% corresponding to an absolute jitter of 12 ps. The latter is caused mainly by the temporal jitter of the pump laser. A mismatch of the lengths of the dye and the pump-laser cavity can result in a nonstationary mode-locking regime with a periodic change of the pulse parameters. The interpretation of the experimental results are supported by computer simulations of the pulse evolution process.     

Astigmatically compensated cw dye laser resonators using lenses

The compensation of the astigmatism of Brewster-angled dye cells can be performed with lenses as well as with spherical mirrors. The advantages of cw dye laser resonators using lenses lie in the linear configuration of the optics and the convenient adjustability of astigmatism compensation. An output efficiency of 30% already at 1.6W pumping power has been observed. In addition, ring laser resonators with lenses have been investigated and they delivered up to 400 mW single mode power in travelling wave operation at less than 2 W pumping power.     

Steady state photoisomer accumulation in the absorber jet of the passively mode-locked femtosecond dye laser

In continuous were passively mode-locked dye lasers a steady state distribution of two isomers of the saturable absorber dye can be established. We report the first intracavity transmission measurement and estimation of the amount of the photoisomer of DODCI in the femtosecond CPM ring laser. Comparison with a simple model based on rate equations allows to estimate the quantum yield of a photo-back reaction. The obtained dependence of the photoisomer concentration on the laser wavelength and pulse energy can be used in theories describing the generation process for adequate estimation of its part in the modelocking regime.     

20 ps pulse generation by an excimer laser pumped double self-Q-switched distributed feedback dye laser

The behaviour of an excimer-laser-pumped distributed feedback dye laser (ELP DFDL) using a mixture of saturable absorber and laser dye as an active medium was studied. In a DFDL self-Q-switching occurs because of the population inversion dependence of the feedback. If the DFDL contains absorber saturation of the absorption by the leading edge of the created laser pulse also causes Q-switching. As a result of this double self-Q-switching, mixing a saturable absorber into the laser dye, the laser pulses become shorter and more stable. This was demonstrated experimentally. Mixing Rhodamine B into the dye solution of a Coumarin 153 ELP DFDL, a six-fold reduction in the pulse duration and a more than two-fold reduction in the pulse energy instability were observed. The experimental results were in good qualitative agreement with the predictions of a simple rate equation model.     

Spatially-hole-burned distributed feedback dye laser produced tunable single picosecond pulses

A new type of distributed feedback dye laser is described in which the Bragg grating is formed by spatial hole-burning. With a simple excimer laser pumped arrangement, single high stability 6 ps pulses were generated. The pulses were nearly transformlimited and were 33 times shorter than the rise time of the pulse which created the Bragg grating.on leave from JATE University, Department of Experimental Physics, Dóm tér 9, H-6720 Szeged, Hungary     

Generation of 320 fs pulses with a distributed feedback dye laser

A new achromatic distributed feedback dye laser (DFDL) arrangement is described. The experimental conditions for subpicosecond pulse generation with the new device were investigated. For the first time, stable generation of subpicosecond pulses (350 fs) at 616 nm was achieved with a DFDL. The simultaneous spectral and autocorrelation measurements showed that the amplified DFDL pulses are nearly transform limited, having a pulse form close to the sech² shape.     

A high-power subpicosecond distributed feedback dye laser system pumped by a mode-locked Nd: YAG laser

The design and operation characteristics of a distributed feedback dye laser (DFDL) system pumped by the second harmonic of a flashlamp pumped mode-locked Nd: YAG laser are described. The DFDL oscillator facilitates a large tuning range with nearly Fourier limited pulse durations of about 1.6 ps. The combined action of saturated absorption and amplification results in a pulse shortening to about 600 fs, with small fluctuations in the pulse duration. Output pulse energies of more than 400 J are achieved, corresponding to a peak power of more than 650 MW. Since the dye amplifiers are pumped by pulses of only 25 ps duration the amplified spontaneous emission (ASE) is very low, typically less than 10^–4.     

Photo-stability of laser dye solutions under Copper-vapour-laser excitation

The photo-stability of laser dyes, Rhodamine-6G, Rhodamine-B, and Kiton-Red, under high repetition rate (6.3 kHz) Copper-vapour-laser (CVL) irradiation has been investigated. Exhaustive photo-bleaching of these dyes in different solvents has been carried out to study the extent to which the dye photo-degraded products would interfere with the lasing process in high-power CVL-pumped dye lasers. Our results indicate that the photo-degradation of dyes occurs predominantly through excited-state intermolecular reactions, involving the singlet state, rather than the process of nonlinear optical absorption in individual molecules. Received: 13 March 2000 / Revised version: 2 August 2000 / Published online: 21 March 2001     

300 Femtosecond pulses at 497 nanometer generated by an excimer laser pumped cascade of distributed feedback dye lasers

The setup is a cascade of 3 lasers: A competing cavity dye laser pumped by a XeCl excimer laser, followed by two distributed feedback dye lasers. The typical durations of the pulses from the lasers are 100 ps, 5 ps, and 300 fs, respectively. The output pulses at 497 nm are amplified up to 500 MW. The shortest pulse duration obtained was 198 fs.     

Pulse generation by distributed feedback dye lasers

Equations describing the pulse generation by distributed feedback dye lasers are derived and solved by analytical methods. The dependence of the laser output on macroscopic parameters is discussed.On leave from the Department of Physics, Friedrich-Schiller-University, DDR-6900, Jena, German Democratic Republic     

A double-wavelength nitrogen-laser-pumped dye laser

A narrow-band tunable double-wavelength dye laser with a bandwidth of 0.1 cm⁻¹ is described. The output at one of the wavelengths is found to be completely linearly polarized in the plane of incidence.     

Undamped undulation superposed on the passive Q-switching pulse of a CO2 laser

An undamped undulation superposed on the pulse tail of the passive Q-switching is observed using HCOOH gas as a saturable absorber. The pulse shapes with the undulation are nicely reproduced through the rate-equation analysis in which the laser gain medium is described as a three-level system. Good agreements between the observation and the calculation are also obtained in the dependence of the period and the width of passive Q-switching pulse on laser parameters. The mechanism of the undulation is interpreted as the relaxation oscillation attributed to the relaxation from the lower laser level. The collisional rate constant of HCOOH molecule is also obtained.     

Efficient single-mode operation of a standing-wave dye laser

The selection of a single longitudinal mode of a dye laser can be achieved with double or triple Michelson reflectors instead of Fabry-Perot etalons inside the laser cavity. These systems can be adapted to commercial multimode dye lasers. They provide a high efficiency and a good geometrical quality of the output beam. With a 7 watt pump power (λ=514.5 nm line of the Ar⁺ laser), a tunable output power of 1 watt was obtained at the peak of R6G, in the main output beam; the total single-mode power, including the auxiliary output beams, exceeded 1.4 watt. These results correspond to efficiencies of 14% and 20%, respectively (24% and 30% slope efficiencies). We discuss in the text why these efficiencies are comparable to those of ring lasers. In the infrared, with a 4.5 watt pump power (red lines of a Kr⁺ laser), 250 mW of single-mode output power in the main output beam was obtained at 780 nm with Oxazine 750.     

A simple and reliable short-pulse dye laser

A simple technique is described that allows the generation of a short pulses (1 ns) from dye lasers pumped by a much longer (7 ns) N₂-laser pulse. Dye-laser pulses, either with a narrow bandwidth or a short duration, can thus be obtained with the same N₂-laser pump.     

High-energy dye laser pumped by wall-ablation lamps

A guideline for the optimum design of linear wall-ablation lamps is presented with a simple empirical formula which describes the luminescent characteristics of lamps. The absolute luminescent efficiency of the wall-ablation lamp was measured. A high-energy dye laser with a quadruple-elliptical cylindrical cavity was constructed using these lamps, and an output energy of 23.3 J (11.6 MW) was obtained with an overall efficiency of 0.31 %. The energy-flow diagram of this laser system was computed with a rate-equation analysis, and the conversion efficiency from electrical input to laser output was determined. One can expect an overall efficiency of about 2 %.     

Spectral purity of pulsed dye lasers

High-spectral purity of pulsed dye lasers is required by many experiments. Unfortunately, the dye laser output is usually accompanied by a spectrally broadband background of spontaneous emission (ASE). We have carried out detailed studies of the ASE background using a dye laser operating with an oscillator, pre- and main amplifier.Dedicated to Prof. Dr. Herbert Welling on the occasion of his 60th birthday