Experimental evidence for the vortex glass phase in untwinned, proton irradiated YBa2Cu3O7-delta

We report on magnetoresistance measurements of the effects of 9 MeV proton irradiation on a clean, untwinned single crystal of YBa2Cu3O7-delta. For the first time, evidence for a vortex glass transition is detected in an untwinned single crystal of YBa2Cu3O7-delta with induced pointlike disorder, in which the first order vortex melting transition is completely suppressed after proton irradiation. Our results suggest that a sufficiently high pinning disorder is required in order for the vortex glass phase to be observed.     

Two crossovers in the Pseudogap regime of YBa 2Cu 3O (7-delta) superconductors observed by ultrafast spectroscopy

We have investigated the temperature dependence of the optical reflectivity on a femtosecond scale in a near optimally doped YBa 2Cu 3O (7-delta) superconductor. The combined study of the lattice and carrier dynamics at temperatures above T(c) allows us to identify two crossover temperatures in the normal state, giving evidence for an inhomogeneity of the pseudogap regime. These crossovers exhibit a clear hysteresis behavior depending on the direction of temperature change. The carrier and lattice dynamics within the crossover regimes show distinct differences from and similarities to the superconducting state, which may help in choosing between the competing theories for the pseudogap state.     

Evidence of doping-dependent pairing symmetry in cuprate superconductors

Scanning tunneling spectroscopy studies reveal long-range spatial homogeneity and predominantly d(x(2)-y(2))-pairing spectral characteristics in under- and optimally doped YBa2Cu 3O (7-delta) superconductors, whereas STS on YBa2(Cu 0.9934Zn 0.0026Mg (0.004))3O (6.9) exhibits microscopic spatial modulations and strong scattering near the Zn or Mg impurity sites, together with global suppression of the pairing potential. In contrast, in overdoped (Y 0.7Ca (0.3))Ba 2Cu 3O (7-delta), (d(x(2)-y(2))+s)-pairing symmetry is found, suggesting significant changes in the superconducting ground state at a critical doping value.     

Broken particle-hole symmetry at atomically flat a-axis YBa2Cu3O7-delta interfaces

We have studied quasiparticle tunneling into atomically flat a-axis films of YBa(2)Cu(3)O(7-delta) and DyBa(2)Cu(3)O(7-delta) through epitaxial CaTiO3 barriers. The junction heterostructures were grown by oxide molecular beam epitaxy and were carefully optimized using in situ monitoring techniques, resulting in unprecedented crystalline perfection of the superconductor-insulator interface. Below T(c), the tunneling conductance shows the evolution of a large unexpected asymmetrical feature near zero-bias. This is evidence that superconducting YBCO crystals, atomically truncated along the lobe direction with a titanate layer, have intrinsically broken particle-hole symmetry over macroscopically large areas.     

Mott gap excitations in twin-free YBa2Cu3O7-delta (Tc=93 K) studied by resonant inelastic x-ray scattering

Mott gap excitations in the optimally doped high-T(c) superconductor YBa(2)Cu(3)O(7-delta) (T(c)=93 K) have been studied by the resonant inelastic x-ray scattering method. Anisotropic spectra in the ab plane are observed in a twin-free crystal. The excitation from the one-dimensional CuO chain is enhanced at 2 eV near the zone boundary of the b* direction, while the excitation from the CuO2 plane is broad at 1.5-4 eV and almost independent of the momentum transfer. Theoretical calculations based on the one-dimensional and two-dimensional Hubbard model reproduces the observed spectra when different values of the on-site Coulomb energy are assumed. The Mott gap of the CuO chain site is found to be much smaller than that of the CuO2 plane site.     

Critical points in heavy ion irradiated untwinned YBa(2)Cu3O(7-delta) crystals

The critical points in untwinned YBa(2)Cu(3)O(7-delta) crystals with dilute columnar defects are investigated. We find a convergence of a first order vortex melting line with an irreversibility line associated with the onset of the Bose glass critical regime at the lower critical point. In addition, we find that columnar defects raise the upper critical point, implying that vortex line meandering is a basic feature controlling its position.     

Electronic transport in underdoped YBa2Cu3O7-delta nanowires: evidence for fluctuating domain structures

We have measured the transport properties of a series of underdoped YBa(2)Cu(3)O(7-delta) nanowires fabricated with widths of 100-250 nm. We observe large telegraphlike fluctuations in the resistance between the pseudogap temperature T* and the superconducting transition temperature T(c), consistent with the formation and dynamics of a domain structure. We also find anomalous hysteretic steps in the current-voltage characteristics well below T(c).     

Phase-coherence effects in vortex transport entropy

Nernst and electrical resistivity measurements in superconducting YBa2Cu3O7-delta and Bi2Sr2CaCu2O8+delta with and without columnar defects show a distinctive thermodynamics of the respective liquid vortex matter. At a field-dependent high temperature region in the H-T phase diagram, the Nernst signal is independent of structural defects in both materials. At lower temperatures, in YBa2Cu3O7-delta, defects contribute only to the vortex mobility, and the transport entropy is that of a system of vortex lines. The transition to lower temperatures in Bi2Sr2CaCu2O8+delta has a different origin; the maximum in the Nernst signal when decreasing temperature is not associated with transport properties but with the entropy behavior of pancake vortices in the presence of structural defects.     

Nernst effect and disorder in the normal state of high-T(c) cuprates

We have studied the influence of disorder induced by electron irradiation on the Nernst effect in optimally and underdoped YBa2Cu3O(7-delta) single crystals. The fluctuation regime above T(c) expands significantly with disorder, indicating that the T(c) decrease is partly due to the induced loss of phase coherence. In pure crystals the temperature extension of the Nernst signal is found to be narrow whatever the hole doping, contrary to data reported in the low-T(c) cuprate families. Our results show that the presence of intrinsic disorder can explain the enhanced range of the Nernst signal found in the pseudogap phase of the latter compounds.     

Anisotropic vortex plasticity in the liquid state of YBa2Cu3O7: evidence for quenched c-axis vortex correlation length

A generalized methodology, based on anisotropic angular dependent magnetoresistance measurements, is presented to deconvolute the contributions to the vortex activation energy (i.e., plastic and pinning energies) in the vortex liquid state of high temperature superconductors. Experimental evidence is given for the appearance of a partially entangled liquid vortex state in YBa 2Cu 3O (7) when random quenched and correlated disorders compete, as in twinned melt textured YBa 2Cu 3O (7) quasisingle crystals with Y 2BaCuO (5) precipitates. The hallmark of this new phase is a quench of the c-axis vortex correla-tion length.     

Superconducting gap and strong in-plane anisotropy in untwinned YBa2Cu3O(7-delta)

With significantly improved sample quality and instrumental resolution, we clearly identify in the ( pi,0) photoemission spectra from YBa(2)Cu(3)O(6.993), in the superconducting state, the long-sought "peak-dip-hump" structure. This advance allows us to investigate the large a-b anisotropy of the in-plane electronic structure including, in particular, a 50% difference in the magnitude of the superconducting gap that scales with the energy position of the hump feature. This anisotropy, likely induced by the presence of the CuO chains, raises serious questions about attempts to quantitatively explain the YBa(2)Cu(3)O(7-delta) data from various experiments using models based on a perfectly square lattice.     

Intrinsic d-wave effects in YBa(2)Cu(3)O(7-delta) grain boundary Josephson junctions

We have measured the angular dependence of the Josephson critical current density (J(C)) in c-axis tilt biepitaxial grain boundary YBa(2)Cu(3)O(7-delta) junctions. We observe for the first time intrinsic d-wave pairing symmetry effects manifested as an oscillatory dependence of J(C) on angle. This intrinsic effect is evident even though spontaneous currents, possibly induced by faceting or barrier impurities, are observed in the grain boundaries.     

Depth-resolved profile of the magnetic field beneath the surface of a superconductor with a few nm resolution

The variation of a magnetic field as a function of depth beneath the surface of an YBa(2)Cu(3)O(7-delta) thin film in the Meissner state has been measured using low energy muons. The depth of implantation was varied from 20-150 nm by tuning the energy of the implanted muons from 3-30 keV. These are direct measurements of the penetration of a magnetic field beneath a superconducting surface which illustrate the power of low energy muons for near surface studies in superconductivity and magnetism.     

Observation of splintered Josephson vortices at grain boundaries in YBa(2)Cu(3)O(7-delta)

We have directly observed well-separated Josephson vortex splinters with unquantized magnetic flux at asymmetric 45 degrees grain boundaries in YBa(2)Cu(3)O(7-delta) films by imaging magnetic flux with scanning SQUID microscopy. The existence of these splinter vortices has been predicted and is well described by a model based on dx(2)(-y(2)) pairing symmetry and facetting of the grain boundary on a length scale shorter than the Josephson penetration depth.     

各向异性超导体的Ginzburg-Landau理论

本文内容主要有二个方面 :1 )由各向同性均匀系的BCS理论扩展到各向异性非均匀系 ,并给出各向异性非均匀系的完整的GL方程式 ,定出了各个宏微观参量间的关系式。2 )结合层状结构氧化物超导体的导电层与非导电层相间的特征等 ,用有效调制势模型和电子有效质量近似 ,将各向同性均匀系的BCS理论较具体地扩展到各向异性非均匀系并进行深化研究。扩展理论所给出的临界温度和能隙方程公式 ,主要的热力学性质和电磁性质公式等应用到YBaCuO超导体上 ,理论结果与实验结果均相符 ,并也给出各向异性非均匀系的完整的GL方程式 ,与上面 1所给出的形式相同 ,也定出了各个宏微观参量间的关系 ,应用到YBaCuO超导体的一些主要性质上也与实验结果相符。     

Electrical resistivity anisotropy from self-organized one dimensionality in high-temperature superconductors

We investigate the manifestation of stripes in the in-plane resistivity anisotropy in untwinned single crystals of La2-xSrxCuO4 ( x = 0.02-0.04) and YBa(2)Cu(3)O(y) ( y = 6.35-7.0). It is found that both systems show strongly temperature-dependent in-plane anisotropy in the lightly hole-doped region and that the anisotropy in YBa(2)Cu(3)O(y) grows with decreasing y below approximately 6.60 despite the decreasing orthorhombicity, which gives most direct evidence that electrons self-organize into a macroscopically anisotropic state. The transport is found to be easier along the direction of the spin stripes already reported, demonstrating that the stripes are intrinsically conducting in cuprates.     

各向异性超导体的Ginzburg-Landau理论

本文内容主要有二个方面：1）由各各同性均匀系的BCS理论扩展到各向异性非均匀系，并给出各种异性非均匀系的完整的GL方程式，定出了各个宏微观参量间的关系式。2）结合层状结构氧化物超导体的导电层在导电层相间的特征等，用有效调制势模型和电子有效质量近似，交各向同性均匀系的BCS理论较具体的扩展到各向异性非均匀系并进行深化研究，扩展理论所给出的临界温度和能隙方程公式，主要的热力学性质和电磁性质公式等应用到YBaCuO超导体上，理论结果与实验结果均相符，并也给出各向异性非均匀系的完整的GL方程式，与上面1所给出的形式相同，也定出了各个宏微观参量间的关系，应用到YBaCuO超导体的一些主要性质上也与实验结果相符。     

Crystal-lattice coupling to the vortex-melting transition in YBa(2)Cu(3)O(7-delta)

Distinct discontinuities in the thermal expansion of the crystal lattice are observed at the melting transition of the vortex lattice in a naturally untwinned reversible YBa(2)Cu3O(7-delta) single crystal using high-resolution dilatometry. This coupling between the vortex transition and the crystal lattice demonstrates that the crystal lattice is more than a mere host for the vortices, and it is attributed to a strong pressure dependence of the superconducting transition temperature and thus to the condensation energy at the vortex-melting temperature.     

Influence of pair breaking and phase fluctuations on disordered high Tc cuprate superconductors

Electron irradiation has been used to introduce point defects in a controlled way in underdoped and optimally doped YBa(2)Cu(3)O(7-delta) crystals. This technique allows us to perform very accurate measurements of T(c) and of the ab plane resistivity in a wide range of defect contents x(d) down to T(c)=0. The variation of T(c) and of the transition width with x(d) do not follow current predictions of pair-breaking theories. The data are rather compatible, at least for the highly damaged regime, with the expected influence of phase fluctuations. These results open new questions about the evolution of the defect induced T(c) depression over the phase diagram of the cuprates.     

Anomalous proximity effect in gold coated (110) YBa2Cu3O7-delta films: penetration of the Andreev bound states

Scanning tunneling spectroscopy of (110)YBa(2)Cu(3)O(7-delta)/Au bilayers reveal a proximity effect markedly different from the conventional one. While proximity-induced mini-gaps rarely appear in the Au layer, the Andreev bound states clearly penetrate into the metal. Zero bias conductance peaks are measured on Au layers thinner than 7 nm with a magnitude similar to those detected on the bare superconductor films. The peaks then decay abruptly with Au thickness and disappear above 10 nm. This length is shorter than the normal coherence length and corresponds to the (ballistic) mean free path.