Fission neutron multiplicity versus fragment mass and kinetic energy

High spin states of ¹²⁷ Ba have been investigated by means of the OSIRIS anti-compton γ -spectrometer. Five new bands, 48levels and 77transitions were found. Spin suggestions for four bandheads could be given. On ground of these suggestions routhians and alignments were compiled for the observed bands, giving a first insight into the high spin structure of this nucleus.     

Nuclear dissipation,fission probability and neutron multiplicity prior to fission

We discuss the effects of nuclear dissipation on fission probabilities that are characteristic of a diffusion model of the fission process. Reproducing the experimental fission probabilities at low excitation energies fixes the ratioa _f/a_n of the level density parameters for a given strength of the reduced dissipation coefficientβ. These low energy constraints ona _f/a_n andβ balance the effects of transients on neutron multiplicities prior to fission at higher excitation energies. For the competitive decay of¹⁵⁸Er formed in the reaction¹⁶O+¹⁴²Nd at 207 MeV we show that dueto transients only the multiplicity of pre-fission neutrons is enhanced with respect to the prediction of the statistical model in a manner consistent with our earlier general analysis.     

Systematics on fission fragment mass distribution of neutron induced 235U fission

Based on the neutron induced fission fragment mass distribution data up to     

Systematics on fission fragment mass distribution of neutron induced 235U fission

Based on the neutron induced fission fragment mass distribution data up to neutron energy 20 MeV measured with the double kinetic energy method (KEM) and the radio active method (RAM), the systematics of fission fragment mass distribution was investigated by using 5 Gaussian model and the systematics parameters were obtained by fitting the experimental data. With the systematics, the yields of any mass A and at any energy in the region from 0 to 20 MeV of neutron energy can be calculated. The calculated results could well reproduce the experimental data measured with KEM, but show some systematical deviation from the data measured by RAM, which reflects some systematical deviations between the two kinds of measured data.The error of systematics yield was calculated in an exact error transformation way, including from the error of the experimental yield data to the error of the discrete parameters, then to the systematics parameters,and at last to the yield calculated with systematics.     

An estimate of the internal excitation energy in fission

A comparison of the potential energy at scission with experimental post-scission data yields an estimate of 7 MeV and an upper bound of 25 MeV for the internal excitation energy at scission. Complete damping during the descent to scission can be ruled out.     

Research on the prompt neutron multiplicity of fission fragments for 235U(n,f)

According to some experimental and evaluated data, the total excitation energy partitioning way between both of the fission fragments was given with a semi-empirical method. With the calculated energy partitioning way, the prompt neutron multiplicity as a function of fragment mass, (-v)(A), for neutron-induced fission of 235U at En=0.0253 eV, 3 MeV, and 5 MeV was calculated. The results are checked with the total average prompt neutron multiplicities (-v) and compared with the experimental and evaluated data.     

Dependence of mass fission asymmetry on the compound excitation energy

The influence of the excitation energy of compound fissioning nucleus on the potential deformation energy as a function of the fission and asymmetry coordinates has been investigated. The Fermi distribution of nucleons at a certain temperature is assumed and taken into account in the Strutinsky shell-correction method. It has been found that the structure of the potential energy surface becomes smoother with increasing excitation energy and shell effects disappear at a compound-nuclear temperature of 2.0 to 2.5 MeV.     

Fission fragment angular distributions for neutron fission of 232Th and their interpretation with a triple-humped fission barrier

The fission fragment angular distributions have been measured for the neutron fission of ²³²Th at a number of energies near the neutron threshold. An exhaustive search has been made for a set of transition states and barrier parameters that would simultaneously fit the angular distributions and reproduce quantitatively the structure seen in the neutron fission cross section. No satisfactory fit to both types of data could be obtained with a double-humped fission barrier. However, use of a triple-humped fission barrier does provide a reasonable fit to all the experimental data.     

Bayesian evaluation of energy dependent neutron induced fission yields

From both the fundamental and applied perspectives, fragment mass distributions are important observables of fission. We apply the Bayesian neural network(BNN) approach to learn the existing neutron induced fission yields and predict unknowns with uncertainty quantification. Comparing the predicted results with experimental data, the BNN evaluation results are found to be satisfactory for the distribution positions and energy dependencies of fission yields. Predictions are made for the fragment ...     

Determination of the characteristics of a double monochromator in neutron powder diffractometers with allowance for spatial effects

Analytical expressions for the characteristics of double monochromators have been derived on the basis of a universal mathematically correct approach developed previously. These expressions are combined with simple geometric diagrams added to explain the features of instrument operation.     

Effect of entrance channel parameters on fission fragment angular momentum in medium energy fission

Independent isomeric yield ratios of¹³²I were radiochemically determined in alpha particle induced fission of²³⁸U in the energy range 25–44 MeV. Fission fragment angular momenta were deduced from the measured isomeric yield ratios using spin dependent statistical model analysis. It was seen that angular momentum of¹³²I increases with increase of excitation energy and angular momentum of the fissioning nucleus. Comparison of the present data on¹³²I in²³⁸U(α,f) with the literature data for the same product in²³⁸U(p, f) and²³⁸U(γ, f) at various excitation energies show that fragment angular momentum strongly depends on the input angular momentum in the range of excitation energy considered. Experimental fragment angular momentum at all excitation energies were seen to be in agreement with the theoretical values calculated based on thermal equilibration of the various collective rotational degrees after considering the occurence of multichance fission. Thus, strong effect of input angular momentum as well as the statistical equilibration among the various collective rotational degrees of freedom in medium energy fission is corroborated.     

Effect of the initial excitation energy on the average fission lifetime of nuclei

The dependence of the fission time on the initial nuclear excitation energy E _{tot 0} ^* is studied on the basis of a refined combined dynamical and statistical model. It is shown that this dependence may be nonmonotonic, in which case it features a broad maximum. It turns out that the form of the average fission time 〈t _f 〉 as a function of E _{tot 0} ^* depends greatly on the orbital angular momentum L _n carried away by prescission neutrons.     

Isotopic invariance of fission fragment charge distributions for actinide nuclei at excitation energies above 10 MeV

The fragment mass and energy distributions from the proton-induced fission of compound nuclei ²³³Pa, ^{234,236,237,239}Np, ^{239,240,241,243}Am, and ²⁴⁵Bk at proton energy E _p =10.3 and 22.0 MeV have been experimentally studied. It was revealed that the shapes of the asymmetric fission mass distributions are mainly defined by the proton numbers of compound nuclei and demonstrate only a weak dependence on the neutron ones. The detailed study of the fission fragment mass yields for compound nuclei Np and Am isotopic chains has shown that the asymmetric fission fragment charge distributions calculated within the unchanged charge density hypothesis for nuclei with equal Z _C practically coincide.     

Systematic studies of fission fragment kinetic energy distributions by Langevin simulations

Fission fluctuation-dissipation dynamics of heavy nuclei has been studied using Langevin Monte Carlo simulations. The covariant form of the fission transport equation and the coefficients related to it are investigated. To learn about the influence of the dynamics from the ground state to the saddle point on the kinetic energy distributions we have studied various systems and compared the calculations both starting from the ground state and from the saddle point. Both the mean total kinetic energy of the fission fragments and its variances can fit with the experimental values in terms of a finite neck radius as scission condition.This work was supported by the National Natural Science Foundation of China.     

Influence of pre-fission neutron emission on fission fragment angular distribution for the system209Bi +16O

The data of fission fragment anisotropies measured for the system¹⁶O +²⁰⁹Bi in the centre of mass energy region of 73 to 95 MeV have been compared with the saddle point statistical model calculations. The corrections to the nuclear temperature and the spin distribution arising due to pre-fission neutron emission have been made. While the resultant calculations reproduce very well the data in the near- and sub-barrier energy regions, they deviate from the data at higher energies. This observation is similar to what was already reported for¹⁶O +²⁰⁸Pb system.     

Determination of the neutron binding energy of the delayed neutron emitter137Xe

The neutron binding energy of¹³⁷Xe has been deduced to be 4025.2±0.6 keV from a study of the¹³⁶Xe(n, γ)¹³⁷Xe reaction. The importance of a precise value for this quantity is due to the fact that an accurate determination of binding energies of delayed neutron emitters is possible only for⁸⁷Kr and¹³⁷Xe, neighbouring stable isotopes. Nuclear reaction.¹³⁶Xe(n,γ), enriched target; measurede89-01, deduced neutron binding energy, Ge(Li) detector.     

Systematics of the mean energy and the mean multiplicity of prompt neutrons originating from 232Th fission

The cross section for the neutron-induced fission of ²³²Th target nuclei, ?? _f (E _n ), was described within statistical theory. The spectra of the mean multiplicity, $\bar v$ (E _n ), and the mean energy, $\bar E$ (E _n ), of secondary neutrons accompanying ²³²Th fission induced by neutrons of energy extending up to E _n = 20 MeV were analyzed on the basis of the chance structure of the cross section.     

Potential energy surfaces and fission fragment mass yields of even-even superheavy nuclei

Potential energy surfaces and fission barriers of superheavy nuclei are analyzed in a macroscopic-microscopic model. The Lublin-Strasbourg Drop (LSD) model is used to obtain the macroscopic part of the energy, whereas the shell and pairing energy corrections are evaluated using the Yukawa-folded potential; a standard flooding technique is utilized to determine barrier heights. A Fourier shape parametrization containing only three deformation parameters is shown to effectively reproduce the nuclear shapes of nuclei approaching fission. In addition, a non-axial degree of freedom is taken into account to better describe the structure of nuclei around the ground state and in the saddle region. In addition to the symmetric fission valley, a new highly asymmetric fission mode is predicted in most superheavy nuclei. The fission fragment mass distributions of the considered nuclei are obtained by solving 3D Langevin equations.