Absolute frequency measurements of wavelength standards 532 nm, 543 nm, 633 nm and 1540 nm

This paper describes the results of absolute frequency measurements of primary wavelength standards 633 nm, 543 nm, 532 nm, (iodine stabilized) and 1540 nm (acetylene stabilized) in CMI. The values obtained with Menlo Systems femtosecond frequency comb in CMI are compared with previous measurements of the same standards in BIPM, BEV and MPQ. Measured sub-Doppler linewidths and relative intensities of several hyperfine spectral components of iodine molecule are also presented.     

1318.8 nm/1338.2 nm simultaneous dual-wavelength Q-switched Nd:YAG laser

A diode-side-pumped simultaneous dual-wavelength Q-switched Nd:YAG laser around 1.3 μm is demonstrated. With the pumping power of 480 W, a peak power of 43 kW was obtained at the repetition rate of 5 kHz. The maximum average output power is up to 43 W with the slope efficiency of 20.5%, and the pulse duration is 200 ns. This dual-wavelength Q-switched laser with high peak power has a balanceable and stable proportion of dual-wavelength output. PACS 42.55.Xi; 42.60.Gd     

High-gain Al2O3:Nd3+ channel waveguide amplifiers at 880 nm, 1060 nm, and 1330 nm

Neodymium-doped aluminum oxide films with a range of Nd³⁺ concentrations are deposited on silicon wafers by reactive co-sputtering, and single-mode channel waveguides with various lengths are fabricated by reactive ion etching. Photoluminescence at 880, 1060, and 1330 nm from the Nd³⁺ ions with a lifetime of 325 μs is observed. Internal net gain at 845–945 nm, 1064, and 1330 nm is experimentally and theoretically investigated under continuous-wave excitation at 802 nm. Net optical gain of 6.3 dB/cm at 1064 nm and 1.93 dB/cm at 1330 nm is obtained in a 1.4-cm-long waveguide with a Nd³⁺ concentration of 1.68×10²⁰ cm^?3 when launching 45 mW of pump power. In longer waveguides a maximum gain of 14.4 dB and 5.1 dB is obtained at these wavelengths, respectively. Net optical gain is also observed in the range 865–930 nm and a peak gain of 1.57 dB/cm in a short and 3.0 dB in a 4.1-cm-long waveguide is obtained at 880 nm with a Nd³⁺ concentration of 0.65×10²⁰ cm^?3. By use of a rate-equation model, the gain on these three transitions is calculated, and the macroscopic parameter of energy-transfer upconversion as a function of Nd³⁺ concentration is derived. The high internal net gain indicates that Al₂O₃:Nd³⁺ channel waveguide amplifiers are suitable for providing gain in many integrated optical devices.     

Zone-plate interferometry at 13 nm wavelength

We report on interferometry using a two-zone-plate common-path interferometer operating at a wavelength of 13 nm. The interferometer was set up with a laser-driven high-harmonic source emitting radiation with the high degree of spatial and temporal coherence necessary for interferometry. The interferometer is suited for investigations of the coherence properties of the light source employed, as well as for simultaneous measurements of the real and imaginary part of the complex index of refraction in the 100 eV regime. This is demonstrated in a proof of principle experiment with a piece of Zr-foil as the phase-shifting and absorbing sample. PACS 41.50.+h; 42.65.Ky; 42.87.Bg; 07.60.Ly     

Laser induced incandescence determination of the ratio of the soot absorption functions at 532 nm and 1064 nm in the nucleation zone of a low pressure premixed sooting flame

In this work, the two-excitation wavelength laser induced incandescence (LII) method has been applied in a low-pressure premixed methane/oxygen/nitrogen flame (equivalence ratio 2.32) to determine the variation of the ratio of the soot absorption functions at 532 nm and 1064 nm E(m,532 nm)/E(m,1064 nm) along the flame. This method relies on the comparison of LII signals measured upon two different excitation wavelengths (here 532 nm and 1064 nm) and with laser fluences selected in such a way that the soot particles are equally laser-heated. The comparison of the laser fluences at 532 nm and 1064 nm leads to an easy determination of E(m,532 nm)/E(m,1064 nm). The reliability of the method is demonstrated for the first time in a low pressure flame in which the soot nucleation zone can be spatially resolved and which contains soot particles acting differently with the laser fluence according to their residence time in the flame. The method is then applied to determine the profile of E(m,532 nm)/E(m,1064 nm) along the flame. A very important decrease of this ratio is observed in the region of nascent soot, while the ratio remains constant at high distance above the burner. Implication on temperature determination from spectrally resolved measurement of flame emission is studied.     

High-efficiency direct-pumped Nd:YLF laser operating at 1321 nm

We present a high-efficiency Nd: LiYF₄ (Nd:YLF) laser operating at 1321 nm pumped directly into the emitting level, ⁴F_3/2. The linear polarization of the pump diode laser was maintained by a short fiber. At the absorbed pump power of 7.3 W, as high as 3.6 W of continuous-wave output power at 1321 nm is achieved. The slope efficiency with respect to the absorbed pump power was 0.52. To the best of our knowledge, this is the first demonstration of such a laser system. Comparative results obtained for the pump with a diode laser at 806 nm, into the highly absorbing ⁴F_5/2 level, are given in order to prove the advantages of 880 nm wavelength pumping.     

Tunable diode laser spectroscopy of benzene near 1684 nm with a low-temperature VCSEL

We describe the application of a long-wavelength vertical-cavity surface-emitting laser (VCSEL) with extended tuning range to the detection of benzene vapor at atmospheric pressure. A benzene absorption feature centered at 1684.24 nm was accessed by reducing the heat sink temperature of a VCSEL designed for room-temperature operation to −55°C. This allowed us to increase the injection current and thus to extend a single-scan tuning interval up to 46.4 cm⁻¹ or 13.2 nm around a central wavelength of 1687.4 nm. Five absorption lines of methane in the 5903–5950 cm⁻¹ range could be acquired within single laser scans at a repetition rate of 500 Hz. A benzene absorption feature between 5926 and 5948 cm⁻¹ was recorded for concentration measurements at atmospheric pressure using a single-pass 1.2 m absorption cell. A 50 ppmv mixture of CH₄ in N₂ was introduced into the cell along with benzene vapor to calibrate benzene concentration measurements. Benzene mixing ratios down to ∼90 ppmv were measured using a direct absorption technique. The minimum detectable absorbance and detection limit of benzene were estimated to be ∼10⁻⁴ and 30 ppmv, respectively. Using the wavelength modulation technique, we measured a second harmonic sensor response to benzene vapor absorption in air at atmospheric pressure as a function of modulation index. We conclude that a low-temperature monolithic VCSEL operating near 1684 nm can be employed in compact benzene sensors with a detection limit in the sub-ppm range.     

Random fiber laser operating at 1,115 nm

We experimentally demonstrate a random fiber laser operating at 1,115 nm using a LD-pumped Yb-doped fiber laser as the pump source. We achieve about 270 mW lasing output in a 50 km standard communication optical fiber with slope efficiency more than 28 %. A new wavelength is provided for the application of random distributed feedback fiber lasers as light sources.     

224 nm segmented hollow-cathode silver ion laser

The segmented hollow-cathode discharge arrangement is used the first time to excite the 224 nm Ag II laser transition. Quasi-continuous output power of 45 mW is obtained during the 300 s current pulses at optimal discharge conditions (10 hPa of He+4% Ar buffer gas) for discharge current of 3 A. No power saturation is observed up to this current value. An average output power of 0.75 mW is reached using pulse repetition frequency of 190 Hz. The longitudinal mode structure of the TEM₀₀ transversal mode is measured by means of a scanning confocal Fabry–Perot interferometer. Two-mode operation is found to be dominant at high current values. Attempts and suggestions are made to prolong the lifetime of the laser tube. PACS 42.55.Lt; 42.60.Lh; 52.80.-s     

980 nm Yb-doped single-mode fiber laser and its frequency-doubling with BIBO

A quasi-three-level Yb-doped single-mode fiber laser at 980 nm by adopting two 0° fiber ends as cavity mirrors generated a total output power of 1.32 W with the slope efficiency of 75.3%. The fiber length was 36.5 cm close to the optimal theoretical fiber length. The corresponding optical conversion efficiency was 66% from the incident pump power at 946 nm to the laser power at 980 nm. Through frequency-doubling with BIBO crystal, a total output power of 15 mW at 490.8 nm was obtained.     

Evaluation of hybrid ytterbium–neodymium laser amplification at 1053 nm

We present here the modeling of a hybrid neodymium/ytterbium laser chain. The laser chain is modeled in energy, spectrum and gain for a relevant choice of ytterbium host materials. Special attention is given to spectral matching of both technologies. The model performance is benchmarked by an experimental setup of a Yb:glass regenerative-amplifier. Results indicate Yb:CaF₂ to be the best material for Nd:glass coupling.     

Linewidth studies on Cd+ 636.0 nm and 537.8 nm lines excited in a He-Cd hollow cathode discharge

Hollow cathode (HC) lasers usually operate in a single axial mode without any optical selection. This is attributed to the large homogeneous linewidth of the gain curve due to the relatively high filling pressure of these lasers. Collisional and Doppler broadening (Δν_C and Δν_D) of the Cd⁺ 636 nm and Cd⁺ 538 nm lines (laser transitions of the HeCd⁺ laser) excited in a HC discharge tube were determined using a Fabry–Perot interferometer technique. It was found that in the pressure range 7–25 mbar Δν_D was nearly constant, while, as expected, Δν_C increased linearly with pressure. The broadening constants were α(636 nm)= (47±2) MHz/mbarand α(538 nm)=(11.8±0.5) MHz/mbar. The first constant is large enough to explain single-mode operation of the red HeCd⁺ laser; but in the case of the green laser, the exact reason for the single-mode operation remained unclear. Received: 23 November 2000 / Revised version: 30 March 2001 / Published online: 7 June 2001     

Ablation mechanism of PTFE under 157 nm irradiation

We report time- and mass-resolved measurements on neutral particles emitted from polytetrafluoroethylene (PTFE) during exposure to 157-nm laser radiation at fluences where etching is observed. By comparing the time-of-flight signals over a range of masses, we conclude that (CF₂) _N fragments for N=1–6 are emitted directly from the surface in substantial quantities. In contrast, the monomer (N=2) is the principal product during irradiation at 248 nm, where thermal decomposition is important. The time-of-flight signals of all the (CF₂) _N fragments show fast components with kinetic energies on the order of an electron volt. These high kinetic energies are consistent with photochemical scission of the polymer backbone, where a fraction of the excitation energy is delivered to the fragment as kinetic energy. Although clean etching is observed under these conditions, the great majority of the mass removed from the target appears as much larger fragments that do not reach our detector. The nature of this material and its affect on the velocity distribution of the observed (CF₂) _N fragments is discussed.     

VUV 157 nm laser ablation of composite structures

We report on the laser ablation of composite prismatic structures using a vacuum ultraviolet (VUV) 157 nm F₂ laser. Polycarbonate and CR-39 substrates have been intentionally seeded with silver wires and silicon carbide whiskers respectively. The seed particles remain attached to the underlying substrate after laser ablation, forming composite silver-polycarbonate and silicon carbide-CR-39 interfaces. Strong optical absorption at 157 nm in the polymeric substrates allows precise control over the depth between the base of the substrate and composite interface. The surface roughness of the as-received seed particles has a significant effect on the final surface quality of the ablated structures. The textured surface on the silicon carbide whiskers is resolved on the walls of the ablated structures. This is in contrast to the composite structures formed using silver wires, which have a comparatively smoother surface.     

High-repetition-rate, intracavity-pumped KTP OPO at 1572 nm

An efficient, eye-safe, high-repetition-rate, intracavity optical parametric oscillator (IOPO) inside an acousto-optically Q-switched Nd:YVO₄ laser end pumped by a 30-W fiber-coupled diode laser was demonstrated. The pumping, acousto-optically Q-switched Nd:YVO₄ laser gives 3-W average output power at 1064-nm wavelength at 40-kHz repetition rate. An additional separating mirror, x-cut KTP crystal and output coupler highly reflective at 1064-nm and partially transparent at 1572-nm wavelengths form a flat–flat IOPO resonator of 35-mm length. We have achieved 3-ns-duration pulses for 20-mm-long KTP and 4-ns-duration pulses for 30-mm-long KTP, respectively. More than 8-kW-peak-power pulses with an average power of 1.5 W at the signal wavelength for 40-kHz repetition rate were demonstrated. Due to the intracavity spatial cleaning effect, a near diffraction limited signal beam was achieved despite a relatively worse beam quality of the pumping beam. Conversion efficiencies of 50% with respect to Q-switched output at 1064-nm wavelength and 11% with respect to diode pump power were achieved. PACS 42.55.Xi; 42.60.Gd; 42.65.Yj     

8.1 W/670.7 nm and 5.1 W/669.6 nm cw red light outputs by intracavity frequency doubling of a Nd:YAP laser with LBO

In this paper, the continuous-wave intracavity second harmonic generation of a laser diode side-pumped Nd:YAP laser operating in the 1.3-μm region is demonstrated. A type-I critical phase-matched LiB₃O₅ (LBO) crystal was used as the frequency doubler. 8.1 W/670.7 nm and 5.1 W/669.6 nm continuous-wave red light outputs were achieved from the 1341.4-nm laser beam polarized along the c crystalline axis and the 1339.2-nm laser beam polarized along the a crystalline axis, respectively. The stability of the 670.7-nm red laser is better than 3% at the output power of 7 W in an hour.     

Influence of Z-pinch evolution on laser pulse duration at 46.9 nm in Ne-like Ar ions

A capillary discharge 46.9 nm Ne-like Ar laser is achieved with peak current of 20–23 kA. The variation of laser pulse duration with initial Ar pressure and rise-time of main current is reported. Measurements show that the laser pulse durations slightly increase with the increased pressure and increased rise-time of current. A comparison of the experimental results with the calculation of snow-plow model indicates that the increase of laser pulse duration is the result of decreased Z-pinch velocity at the pinch time when the radius of plasma is minimal.     

High-efficiency eye-safe intracavity Raman laser at 1531 nm with SrWO4 crystal

A high-efficiency diode-end-pumped Q-switched eye-safe linearly-polarized intracavity Raman laser at 1531 nm is demonstrated, with Nd:YVO₄ as the laser medium and SrWO₄ as the Raman crystal. The highest average power of 1.93 W is achieved, with an incident pump of 15.6 W and a repetition rate of 35 kHz. The narrowest pulse duration of 4.9 ns and the highest peak power of 32.2 kW are obtained at a repetition rate of 5 kHz.     

Modeling erbium–thulium-co-doped fiber amplifier for 1400–1650 nm band

We present numerical models of tri-valence erbium ion and thulium ion-co-doped fiber amplifiers pumped by 800-nm and 980-nm lasers. The rate and power propagation equations of the models are numerically solved to analyze the gain as a function of co-doping concentrations, fiber length and signal wavelength. The results reveal that with 800-nm or 980-nm pump, gain competition exists between 1470- and 1530-nm bands, which may arise from the pump absorption competition and complicated energy transfer between the two types of active ions, and the results further show that the gain spectra may cover 305 nm (1375–1680 nm) for 800-nm pump and 160 nm (1400–1560 nm) for 980-nm pump. The doping concentrations and fiber length may be tuned to reduce the ripple of the gain spectra.     

Plasma-based X-ray laser at 21 nm for multidisciplinary applications

An overview of recent advances in applications of currently the most energetic X-ray laser at 21 nm is given. The unique parameters of this half-cavity based X-ray laser such as record output energy of 10 mJ, highly symmetric beam, robustness and reproducibility, have made it possible to carry out a number of multidisciplinary scientific projects featuring novel applications of intense coherent X-ray radiation. Selected results obtained in these experiments are reviewed, including X-ray laser probing of dense plasmas, measurements of transmission of focused soft X-ray radiation at intensities of up to 10¹² W cm^-2, measurements of infrared laser ablation rates of thin foils, and ablative microstructuring of solids.