CH<Subscript>3</Subscript>OH optically pumped by a <Superscript>13</Superscript>CO<Subscript>2</Subscript> laser: new laser lines and assignments

We report 12 new THz (far-infrared) laser lines from methanol (CH₃OH), ranging from 58.1 μm (5.2 THz) to 624.6 μm (0.5 THz). A ¹³CO₂ laser of wide tunability (110 MHz) has been used for optical pumping, allowing access to previously unexplored spectral regions. Optoacoustic absorption spectra were used as a guide to search for new THz laser lines, which have been characterized in wavelength, polarization, offset, relative intensity, and optimum operation pressure. For 20 laser lines previously observed, we have measured the absorption offset with respect to the ¹³CO₂ laser line center. PACS 33.20.Ea; 33.20.Vq; 33.80.-b     

Parametric oscillation of high-power 3-THz pulse by synchronously pumped ZnGeP<Subscript>2</Subscript> crystal: Computer simulation

Possible parametric oscillation of 3-THz pulse at synchronous pumping of the ZnGeP₂ crystal by a train of short second-harmonic pulses from the CO₂ laser has been analyzed. Calculation shows that at changing laser pulse duration τ between 4 and 500 ps and correspondingly pumping energy density (0.5–3.5 J cm⁻²) THz pulse peak power varies from 3 to 70MW with maximum at τ =9 ps.     

Power scaling of a continuous-wave and passively Q-switched Yb:KLu(WO<Subscript>4</Subscript>)<Subscript>2</Subscript> laser end-pumped by a high-power diode

The power scaling capacity of a diode end-pumped Yb:KLu(WO₄)₂ laser, operating in the continuous-wave (cw) and passively Q-switched regimes, has been investigated. A cw output power of 11.5 W was achieved with an optical-to-optical efficiency of 41% with respect to the incident pump power, while the slope efficiency amounts to 60%. The passively Q-switchedoperation yielded an average output power of 4.3 W at the fundamental wavelength of 1031.7 nm, and 1.15 W of Raman radiation at 1139.3 nm. The total slope efficiency for Q-switched operation was 40%. The highest pulse energy, duration, and peak power were 170 μJ, 2.2 ns, and 77.3 kW for the fundamental radiation, and 51 μJ, 2.3 ns, and 22.2 kW for the Raman radiation. PACS 42.55.Rz; 42.55.Xi; 42.55.Ye     

Multiwatt optically pumped ammonia laser operation in the 12–13 μm

Design and operating caracteristics of high pulse repetition rate NH₃ laser producing up to 20 W of average output power are described. The NH₃ laser, operating in the 12–13 μm region was optically pumped with a high pulse repetition rate TEA CO₂ laser. Dependences of the NH₃ laser output on the pump energy, ammonia and buffer gas pressures and pulse repetition rate have been studied. The conversion efficiency of up to 16% has been received.     

Widely tunable PPLN/IOPO driven by a diode-end-pumped Q-switched Nd:YVO<Subscript>4</Subscript> laser

This paper reported a broadband tuning intracavity optical parametric oscillator (IOPO), based on the multiple grating periodical poled lithium niobate (PPLN) pumped by a acoustic-optical (AO) Q-switched Nd:YVO₄ laser. The widely tunable OPO output signal wavelength range from 1390 to 1605 nm, which was obtained by changing PPLN poling period from 27.8 to 31.6 μm at a certain temperature of 46°C, while the continuous tuning range was measured from 1475 to 1592 nm with the PPLN poling period of 30 μm by varying the temperature of nonlinear crystal PPLN from 50 to 120°C. The maximum output power of 0.92 W at 1534 nm with the minimum pulse width of 5.17 ns was generated under the incident pump power of 9.6 W at 808 nm. The corresponding peak power and single pulse energy were calculated to be 5.94 kW and 30.7 μJ, respectively. The M ₂-factor was measured to be 2.01 at the signal power of 0.4 W.     

Sub-wavelength micromachining of silica glass by irradiation of CO<Subscript>2</Subscript> laser with Fresnel diffraction

We investigated a simple and productive micromachining method of silica glass by ablation using a TEA CO₂ laser (10.6 μm) with a spatial resolution down to sub-wavelength scale. The silica glass was irradiated by the TEA CO₂ laser light through a copper grid mask with square apertures of 20×20 μm² attached to the silica glass surface. After the irradiation, circular holes with a diameter of several μm were formed on the silica glass surface at the centers of the apertures due to the Fresnel diffraction effect. The minimum diameter of the holes was 3.4 μm. The characteristics of the micromachining are discussed based on the electric field distributions of the CO₂ laser light under the mask using a three-dimensional full-wave electromagnetic field simulation.     

Generation of coherent terahertz phonons by sharp focusing of a femtosecond laser beam in the bulk of crystalline insulators in a regime of plasma formation

The generation of coherent terahertz phonons in a regime of plasma formation by a femtosecond laser radiation with an intensity of 10¹³ W/cm² in the bulk of crystalline quartz has been detected by the method of probing by a probe pulse of the third harmonic. A smooth increase in the frequency of coherent terahertz phonons from 2.2 to 5.5 THz has been detected, along with its subsequent sharp decrease down to 2.2 THz due to an α-β phase transition in crystalline quartz. The generation of 1-THz coherent phonons has been detected in BaF₂ crystals. A smooth variation of the frequency of coherent phonons from 2 to 2.5 THz has been detected in leucosapphire. The generation of coherent phonons during local laser excitation in CaF₂ and LiF crystals develops at the frequencies of 2.3 and 0.1 THz, respectively.     

High-power picosecond LiB3O5 optical parametric oscillators tunable in the blue spectral range

The paper reports on an experimental investigation and numerical analysis of noncritically and critically phasematched LiB₃O₅ (LBO) optical parametric oscillators (OPOs) synchronously pumped by the third harmonic of a cw diode-pumped mode-locked Nd:YVO₄ oscillator–amplifier system. The laser system generates 9.0 W of 355-nm mode-locked radiation with a pulse duration of 7.5 ps and a repetition rate of 84 MHz. The LBO OPO, synchronously pumped by the 355-nm pulses, generates a signal wave tunable in the blue spectral range 457–479 nm. With a power of up to 5.0 W at 462 nm and 1.7 W at 1535 nm the conversion efficiency is 74%. The OPO is characterized experimentally by measuring the output power (and its dependence on the pump power, the transmission of the output coupler and the resonator length) and the pulse properties (such as pulse duration and spectral width). Also the beam quality of the resonant and nonresonant waves is investigated. The measured results are compared with the predictions of a numerical analysis for Gaussian laser and OPO beams. In addition to the blue-signal output visible-red 629-nm radiation is generated by sum-frequency mixing of the 1.535-μm infrared idler wave with the residual 1.064-μm laser radiation. A power of 1.25 W of 1.535-μm idler radiation and 5.7 W of 1.064-μm laser light generated a red 629-nm output power of 2.25 W. Received: 2 February 2000 / Revised version: 28 July 2000 / Published online: 22 November 2000     

Generation of continuously tunable terahertz-wave radiation exploited by stimulated polariton scattering

The characteristics of a coherent tunable terahertz-wave source have been experimentally investigated in detail. By using a difference frequency generation as a result of stimulated Raman scattering by polaritons in MgO:LiNbO₃ crystals, the signal wave was continuously tuned in the range of 1.069–1.075 μm, which corresponded to a terahertz-wave in the wide range from 227 to 104 μm (1.3 to 2.9 THz). The highest output signal pulse energy at the pumping level of 44 mJ/pulse was 1.8 mJ/pulse with 20 mW seeder injection, and the terahertz peak power was 139 mW at the wavelength of 143 μm. This source has the advantages of simple alignment, simplicity of tuning, and compactness that makes the device more attractive.     

Actively Q-switched intracavity frequency-doubled Nd:LuVO<Subscript>4</Subscript>/LBO green laser with an acousto-optic modulator

This work presents experimental results concerning an actively Q-switched intracavity frequency-doubled Nd:LuVO₄/LBO green laser with an acousto-optic modulator operated at the wavelength of 0.53 μm. The green average output power of 2.8 W was obtained at a pump power of 16.3 W and a pulse repetition rate of 20 kHz, resulting in an optical conversion efficiency of 17%. When the pulse repetition rate is operated at 5 kHz, the shortest pulse width and the highest peak power at 0.53 μm were measured to be 26.5 ns and 8.43 kW, respectively.     

Luminescence and selective heat radiation of Yb<Subscript>2</Subscript>O<Subscript>3</Subscript> upon the resonant and thermal laser excitation

Yb₂O₃ polycrystals with a size of up to 10 mm are synthesized using the sintering and melting of the ultrapure Yb₂O₃ powders by the CO₂-laser radiation with the power P _L ≤ 100 W at the wavelength λ = 10.6 μm at the melting point T _m = 2703 K, forming due to surface tension in melt, and crystallization in air. The analysis of the polycrystal microstructure using the methods of optical and electron microscopy and X- ray diffractometry shows that perfect oxide crystallites are formed in the course of crystallization after melting-through. The transformation of the luminescence and selective heat radiation (SHR) spectra of the Yb₂O₃ polycrystals is studied under the resonant excitation at λ ≈ 975 nm using a laser diode and the laser heating at the wavelength λ = 10.6 μm. When the resonant excitation power of the Yb³⁺ ions increases from 0.15 to 4.5 W, the Stokes luminescence of the Yb₂O₃ polycrystals is sequentially transformed into SHR and the thermal radiation of the crystal lattice. The transformation of the emission spectra of the Yb₂O₃ polycrystals with an increase in the laser heating intensity by about four orders of magnitude can be represented as the low-temperature heat radiation, spectral burst of the thermodynamically nonequilibrium SHR of the Yb³⁺ ions, and the high-temperature radiation of the crystal lattice. The temperature dependence of the luminescence spectra and SHR of the Yb₂O₃ polycrystals on the intensity of the laser and laser-thermal excitation and the concentration quenching of the Yb³⁺ luminescence in oxides indicate the key role of the interaction of the f-electron shell of the Yb³⁺ ions with the natural oscillations of the crystal lattice in the processes of the multiphonon excitation and nonradiative (multiphonon) and radiative (vibronic) relaxation.     

Tunable terahertz generation from one CO2 laser in a GaSe crystal

Coherent terahertz pulses have been generated at a range of 236.3-1104.5 μm (0.27-1.3 THz) by one CO₂ laser with dual-wavelength output based on collinearly phase-matched different frequency generation (DFG) in a GaSe crystal. This source has the advantages of compact and simplicity for tuning. The output power of the THz pulse and phase-matching conditions were investigated. The maximum single pulse energy of 11 nJ was generated at a frequency of 1.23 THz (243.6 μm), corresponding to a peak output power 182 mW.     

$90^{\circ}$ phase-matched parametric frequency conversion in AgGa1-xInxS2

AgGa_1-xIn_xS₂ with x=0.14±0.01 was found to be 90° phase-matchable for type-I difference-frequency generation (DFG) by mixing the dual-wavelength pulses emitted from an electronically tuned Ti:sapphire laser. Infrared radiation continuously tunable over the range of 4.80–6.98 μm was generated by independently varying the two wavelengths in the 705–932 nm spectral range, and 4.04 μm radiation by mixing a Nd:YAG laser with the Ti:sapphire laser. In addition, this material was found to be noncritically phase-matchable for the second harmonic generation (SHG) of CO₂ laser radiation at 10.591 μm at 203 °C. Sellmeier equations that reproduce well these experimental data are presented. PACS  42.65.-k; 42.65.ky     

Sensory neuron response to emission from a CO<Subscript>2</Subscript> laser

We have built a wavelength-tunable CO₂ laser meeting the requirements for low-intensity laser therapy. At λ = 10.57 μm and 9.24 μm, we observe a physiological effect detectable from the change in the extent of neurite outgrowth from sensory neurons. This makes it possible to study molecular mechanisms for interaction of low-intensity radiation with tissues in a living body. The ATP molecule is considered as the specific molecular target for the action of the radiation.     

Simultaneous generation of a proton beam and terahertz radiation in high-intensity laser and thin-foil interaction

We have observed simultaneously both the fast proton generation and terahertz (THz) radiation in the laser pulse interaction with a 5-μm thick titanium target. In order to control the proton acceleration and THz radiation, we have changed the duration of the amplified spontaneous emission (ASE) preceding the main pulse generated by the high-intensity Ti:sapphire laser. A fast proton beam with the maximal energy of ∼ 490 keV has been realized by reducing the duration of the ASE. Simultaneously, an intense emission of THz radiation is observed for various ASE durations. We propose the antenna mechanism for the THz radiation, according to which the fast electrons moving along the target surface emit the low-frequency electromagnetic wave. PACS 52.25.Os; 52.38.Kd; 52.50.Jm     

Passive Q-switching performance with Co:LMA crystal in a diode-pumped Nd:LuVO<Subscript>4</Subscript> laser

A diode-pumped passively Q-switched Nd:LuVO₄ 1.34 μm laser using Co:LMA saturable absorber was successfully demonstrated. The average output power, pulse width, repetition rate of a-cut and c-cut Nd:LuVO₄ lasers were studied with different output couplers. The maximum average output power of 164 mW was obtained at the pump power of 10.3 W and the narrowest pulse width of 168 ns was achieved at repetition rate of 457 kHz under pump power of 8.59 W in a-cut Nd:LuVO₄ laser with T = 8%.     

Research of Tm (5.5 at %), Ho (0.55 at %):GdVO<Subscript>4</Subscript> laser pumped by diode laser at 800 nm

In this paper, we report a Tm (5.5 at %), Ho (0.55 at %):GdVO₄ laser pumped by diode laser at 800 nm. To our best knowledge, it is the first time that the use of Tm (5.5 at %), Ho (0.55 at %):GdVO₄ crystal among the similar experiments. We observed the influences of LD working temperature i.e. pump wavelength to 2 μm laser conversion efficiency. In the conditions of the continuous wave and 10 kHz acousto-optic Q-switch, high efficiency output of 2.05 μm laser was obtained. With the maximum pump power of 34.6, 13.9, and 13.6 W at 2.05 μm laser output was achieved respectively. Single laser pulse width was 25.6 ns in 10 kHz acousto-optic Q-switched condition.     

Intracavity parametric conversion of radiation from a pulsed Nd:YVO<Subscript>4</Subscript> laser with high-power diode pumping

We have achieved intracavity parametric conversion of the radiation from a laser based on Nd:YVO₄ with high-power diode pumping. An LiF^2- crystal was used as the passive Q-switch for the Nd:YVO₄ laser. We have shown that by using an active element in the master laser with a passive region, we can form pulsed laser beams at a wavelength of 1.57 μm with peak power 3.2 kW and repetition rates up to 80 kHz, with beam quality parameter 1.4–1.8. __________ Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 73, No. 1, pp. 5–8, January–February, 2006.     

High-power,high-quality ZGP OPO pumped by a Tm,Ho:GdVO<Subscript>4</Subscript> laser

We report a ZGP OPO system capable of producing >6 W at a signal wavelength of 3.80 μm and an idler wavelength of 4.45 μm. The pumping source is the Tm,Ho:GdVO₄ laser operated at 2.049 μm with an M ² of 1.07. The ZGP OPO generated a total combined output power of 6.1 W at signal wavelength and idler wavelength under pumping power of 18.3 W, and an M ² of 1.7 for OPO output was obtained.     

Femtosecond laser plasma in CaF<Subscript>2</Subscript> crystal microchannel and effective generation of characteristic X-ray radiation

The dependence of the characteristic X-ray radiation yield from CaF₂ crystal on the formed microchannel depth under highly intensive (I ∼ 3 × 10¹⁵ W/cm²) laser pulses with different contrast was obtained. The maximum of the characteristic X-ray radiation yield at these experimental conditions corresponded to the microchannel depth of 30–50 μm. The efficiency of the laser radiation conversion to the characteristic X-ray radiation increased from 6 × 10⁻⁸ for the surface up to 10⁻⁷ in the microchannel. The dependence of the characteristic X-ray radiation yield on the viewing angle showed that the source of X-ray radiation was located near the surface inside the microchannel.