Large-scale collisional energy transfer in laser-pumped metastable Ca atoms: Excitation of resonance states of Ca II

We report the first experimental observation of the excitation of the 4p ² P _{3/2, 1/2} resonance states of Ca II (located at 74 720.4 and 74 497.5 cm^–1 above the ground state of Ca I) following pulsed-laser pumping of the 4s ^{2 1} S _O–4s4p ³P₁ intercombination transition of Ca I (E _ex = 15 210 cm^–1). Large scale collisional transfer of energy between the laser-excited atoms is believed to be responsible for this. This is possibly because sufficient time is available (_rad of the 4s4p ³ P ₁ state is approximately 350 µs) for collisions to build such a high level of excitation. Some interesting additional features of the fluorescence spectra of the laser-pumped Ca vapor, such as temperature dependence of the fluorescence intensities and evolution in time of some selected states, are also presented.     

Detailed simulation of recombination XUV laser experiments

The detailed simulation of recombination XUV laser experiments is described and the calculation of gain as measured by two different experimental techniques is discussed. It is shown that a reasonable comparison between simulation and experiment can only be obtained if the self-trapping of the Lyman line is neglected.     

Single picosecond UV pulse generation by mode-locking of an excimer laser-pumped dye laser

A single picosecond ultraviolet pulse has been generated based on mode-locking of a dye laser pumped by a long pulse XeCl laser to serve as the input source for a high-power ps KrF laser system. A short-pulse uv dye laser (BBQ) pumped by an additional XeCl laser was used to selectively amplify a single pulse from a mode-locked pulse train with the pulse separation of 3.2 ns. The amplified single pulse was frequency-doubled to 248 nm with the pulse duration of 20 ps.     

Influence of cavity configuration on the pulse energy of a high-pressure molecular fluorine laser

We report an investigation of a high-pressure molecular fluorine laser operating at 158 nm. Several cavity configurations were studied, including one employing a roof prism as the high reflector. A maximum VUV pulse energy of 237 mJ, corresponding to a specific output of 3.3 J/1 was obtained when the laser was operated as a double-ended device. With single-ended operation the largest output energy was 176 mJ at a specific output of 2.5 J/1.     

Orange,red and deep-red flashlamp-pumped Pr3+:LiYF4 laser with improved output energy and efficiency

Three laser transitions (607.2 nm, 639.5 nm, 720.9 nm) in a flashlamp-pumped Pr³⁺:LiYF₄ laser at room temperature are investigated. Cerium ions (Ce³⁺) doped into the fused-quartz envelope of the flashlamp efficiently transfer strong UV radiation from pumping light into the absorption region of Pr³⁺ ions ( = 420–480 nm), so that the slope efficiency of all three laser emissions could be increased by almost 100% compared to excitation with a pure quartz flashlamp. At a pump energy of 30 J the output energy of these three laser emissions reached 4.7 mJ, 87 mJ and 30 mJ.     

Solid-state active media of tunable organic- compound lasers pumped with a laser. II. A copper vapor laser

The lasing properties of organic compounds in a polymethylmethacrylate matrix pumped by a copper vapor laser are studied. The results demonstrate that the transverse pumping scheme of solid-state laser-active media with the copper vapor laser is promising compared to the longitudinal pumping scheme from the viewpoint of the lifetime parameters. Received: 6 February 2002 / Published online: 2 May 2002     

Excited-state absorption in Er: BaY2F8 and Cs3Er2Br9 and comparison with Er: LiYF4

The influence of Excited-State Absorption (ESA) on the green laser transition and the overlap of Ground-State Absorption (GSA) and ESA for 970 nm upconversion pumping in erbium is investigated in Er³⁺ : BaY₂F₈ and Cs₃Er₂Br₉. Results are compared to Er³⁺ : LiYF₄. In Er³⁺: BaY₂F₈, a good overlap between GSA and ESA is found at 969 nm in one polarization direction. The emission cross section at 550 nm is a factor of two smaller than in LiYF₄. In Cs₃Er₂Br₉, the smaller Stark splitting of the levels shifts the wavelengths of the green emission and ESA from⁴ I _{1 3/2} off resonance. It enhances, however, ground-state reabsorption. The emission cross section at 550 nm is comparable to LiYF₄. Upconversion leads to significant green fluorescence from² H _9/2. A significant population of the⁴ I _11/2 level and ESA at 970 nm are not present under 800 nm pumping.     

Self-compensation of thermal lens in high-power diode pumped solid-state lasers

We present a comprehensive model to describe the optic-thermal coupling in the diode pumped solid-state lasers (DPSSL). The thermal transition of particles at the upper laser level leads the heat-generation of laser crystals to depend on shape of the laser beam, while the laser field is also influenced by the temperature because of the thermal excitation of doped particles among various Stark levels. These effects, together with the usual thermal-optic effect that induces a fluctuation of the refraction index by an inhomogeneous temperature distribution, cause a complicated coupling between the laser field and the temperature field. We show that the optic-thermal coupling plays an important role in high-power DPSSL with larger size beam. That effect may yield a self-compensation for the thermal lens and improve the beam quality.     

Theoretical treatment of relaxation oscillations in quasi-three-level systems

The study of the temporal and spectral behavior of relaxation oscillations in quasi-three-level systems allows the direct measurement of the absolute value and spectral profile of laser-transition absorption and emission cross sections, simultaneously and independently, not requiring the usual assumption of Boltzman distributions for the intermanifold sublevels.On leave from the General Physics Institute, Russian Academy of Sciences, Moscow, Russia     

Energetic and thermal performance of high-gain diode-side-pumped Nd:YAG rods

We investigated the energetic and thermal performance of a diode-side-pumped Nd:YAG rod laser with up to 50 W power deposited as excess heat into a 3-mm-diameter, 10-cm-length rod. The rod design produces an extremely flat gain profile resulting in “textbook” expressions of thermal lensing and birefringence. Thermal and energetic measurements are compared to corresponding “textbook” theoretical expressions. Discrepancies between various published thermo-mechanical YAG parameters are resolved by a self-consistent set of measured and calculated data for rod thermal lens focal lengths, birefringence depolarization and ratio of heat to stored energy (χ). Measured thermal and energetic performance under lasing and nonlasing conditions are presented, which agree with published theoretical expressions and measurements. Compensation of rod thermal lensing with simple spherical concave lenses is demonstrated. In addition various methods for compensating birefringence depolarization are theoretically and experimentally analyzed and compared. Received: 19 July 1999 / Revised version: 22 October 1999 / Published online: 23 February 2000     

Threshold and saturation properties of a solid-state XeF (C-A) excimer laser

A dielectric laser cavity of 1 cm length has been optimized for high gain (7 cm^–1) operation which is achieved in XeF doped Ar crystals. Mode structures on the C-A spectral distribution around 540 nm and far field transverse mode patterns are reported. Photchemical gain burning is observed in the spectral mode structures. The dependence of the laser threshold on pump energy, pumped length and on cavity losses is studied. XeF densities of 7×10¹⁷ cm^–3 and distributed losses of 1.2 cm^–1 are derived. The measured quantum efficiency of 14% and the saturation behaviour are consistently described. Losses by transient aborption and two photon absorption are discussed.     

Gain Measurement and Anomalous Decrease of Peak Gain at Long Wavelength for InAs/GaAs Quantum-Dot Lasers

Mode gain spectrum is measured by the Fourier series expansion method for InAs/GaAs quantum-dot （QD） lasers with seven stacks of QDs at different injection currents. Gain spectra with distinctive peaks are observed at the short and long wavelengths of about 1210nm and 1300nm. For a QD laser with the cavity length of 1060μm, the peak gain of the long wavelength first increases slowly or even decreases with the injection current as the peak gain of the short wavelength increases quickly, and finally increases quickly before approaching the saturated values as the injection current further increases.     

Femtosecond noncollinear and collinear parametric generation and amplification in BBO crystal

Measurements of intensity and frequency noise of an injection-locked 5-W Nd:YAG laser are presented and compared with the predictions of models. We show that the output of the injection-locked laser has very low levels of noise, and that the measurements support the predictions of the models. Thus these models can confidently be used to predict the performance of high-power, injection-locked lasers being developed for gravity wave detection. Received: 31 January 2000 / Revised version: 18 March 2000 / Published online: 16 June 2000     

Intensity and frequency noise characteristics of two coherently-added injection-locked Nd:YAG lasers

Coherent addition of two injection-locked Nd:YAG lasers has been performed. A maximum output power of 4.4 W and addition efficiency of 0.94 was achieved, which is the highest power-coupling efficiency ever reported. It was shown experimentally that the frequency and intensity noise level of the coherently-added laser are the same as those of a single injection-locked laser. In particular, no additional intensity noise was observed above the relaxation oscillation frequency of the slave laser, which is suitable for use as the light source for a future gravitational wave detector. The frequency noise of the coherently-added laser was suppressed to 1×10^-4 Hz/ by controlling that of the master laser, and the intensity noise was also suppressed to 1×10^-8 / by controlling the intensity of pump lasers used for the slave lasers. Received: 11 April 2001 / Revised version: 20 June 2001 / Published online: 19 September 2001     

Cross sections of excited-state absorption at 800 nm in erbium-doped ZBLAN fiber

4 I_13/2 and ⁴I_11/2 of erbium is measured in a fluorozirconate fiber in the wavelength range 780–840 nm. Using a pump- and probe-beam technique and choosing the pump wavelength such that the perturbation by pump ESA is minimized in the measurement, it is possible to determine the effective ESA cross sections, despite the fact that the excitation is distributed among two metastable levels. The derived ESA cross sections at 793 nm of 1.4×10^-21 cm² from the ⁴I_13/2 level and less than 0.1×10^-21 cm² from the ⁴I_11/2 level are in reasonable agreement with former results obtained from a rate-equation simulation of the erbium 3-μm laser. The corresponding ESA spectrum under 3-μm lasing conditions is derived. At the strongest ground-state absorption around 799 nm, decreasing ESA from the ⁴I_13/2 level is compensated by increasing ESA from the ⁴I_11/2 level, i.e., ESA losses cannot be avoided when pumping around 800 nm. This result is of relevance for possible high-power diode pumping of an erbium 3-μm double-clad fiber laser. Received: 20 January 1998     

Operation characteristics of the Au-II 690-nm laser transition in a segmented hollow-cathode discharge

Single-mode operation at the Au-II 690-nm transition was obtained in a segmented hollow-cathode discharge laser without the use of any additional frequency-selective device. The pressure of the helium buffer gas, which is responsible for the significant homogeneous broadening of the laser line, was varied between 10 and 20 mbar. The discharge was excited with rectangular current pulses (up to 3 A) six times exceeding the threshold value. The time dependence of the laser output during the 1-ms-long discharge pulses is explained on the basis of the temperature and pressure changes in the tube. The highest small-signal gain at optimal discharge conditions was 11%m⁻¹. Received: 1 July 1999 / Revised version: 4 November 1999 / Published online: 23 February 2000     

The spatial distribution of small signal gain in a segmented hollow cathode discharge laser

Received: 5 February 1997/Revised version: 30 April 1997     

A high power high energy pure N2 laser in the first and second positive systems

Simultaneous high energy lasing in the N₂ first and second positive systems is reported. 20.5 mJ (1.5 MW) UV and 5 mJ (0.4 MW) IR laser pulses were produced in pure N₂. The design is open and easy to improve.     

Theoretical study of a new energy extraction scheme of a chemically pumped pulsed iodine laser amplifier

A new energy extraction scheme of a chemically pumped pulsed large-scale iodine laser based on a high-pressure pulsed singlet oxygen generator is proposed. In previous investigations only low-pressure oxygen generators have been considered. Since they require a high iodine density for an efficient amplifier operation, the lifetime of the stored energy is correspondingly small and thus only small-sized iodine amplifiers appear to be technically feasible. We found, however, that when the singlet oxygen is generated at high-pressure, the iodine density required can be considerably reduced so that the lifetime of the stored energy becomes sufficiently long to fill up large amplifier cells. A numerical model is developed and the extractable energy is theoretically estimated. It is shown that 0.2J/1·pass can be extracted when an input pulse of 20 ns duration (FWHM) and 1 J/cm² fluence is fed into the amplifying medium.     

Numerical study of active mode locking in pulsed solid-state lasers

Transient mode locking of spiking solid-state lasers is studied with the help of two theoretical approaches. The first of them is an extension of the previous transient theory with single-mode rate equations to find the limited spike build-up time depending on the modulation index. The second is based on semiclassical multimode equations describing both spiking behaviour and formation of the picosecond pulse from the initial noise. The derivation of the equations as well as a comparison of results from both approaches are given. The obtained numerical results agree with experimental data. It is shown that the pulsewidth in a spiking laser can approach the small value predicted by the steady-state theory. This minimal pulsewidth can be reached at a smaller modulation index than predicted by the standard transient mode locking theory. The minimal modulation index for generation of good picosecond pulses free of noise is found to be 0.6 in our case. Losses connected with amplitude modulation have a negligible effect on spike build-up time and pulse duration.