共查询到17条相似文献,搜索用时 359 毫秒
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低对称性非线性光学晶体硼酸铋(BIBO)的1064nm三倍频性质 总被引:2,自引:2,他引:0
采用高温溶液法成功生长出高光学质量的硼酸铋 (BIBO)晶体 ,尺寸达到 2 4mm× 19mm× 35mm ,质量为4 8g。对BIBO晶体进行了定向 ,并测量了该晶体的主轴折射率。讨论了BIBO晶体的 10 6 4nm三倍频性质 ,包括相位匹配角、有效非线性光学系数deff、容限角、走离角等。结果表明 ,BIBO晶体的最佳三倍频方向为 (137.7°,130°) ,其有效非线性光学系数值达到 3.6 0 pm/V ,属I类相位匹配。就主平面内的相位匹配方向而言 ,(14 6 .4°,90°)具有最大的有效非线性光学系数值 ,为 3.16pm/V。在 10 6 4nm的腔外三倍频实验中 ,(14 6 .4° ,90°)BIBO晶体的转换效率达到 39.5 % ,角度容限半宽为 0 .2 2mrad·cm ,该数值与 0 .175mrad·cm的计算值基本符合。由于(33.6°,90°)BIBO晶体的有效非线性光学系数较小 (0 .31pm/V) ,其三倍频转换效率小于 5 %。 相似文献
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基于非线性光学频率变换理论,采用已报道的利用非线性光学差频方法产生可调谐太赫兹波的实验条件作为理论分析的实验模型,计算模拟出在不同相位匹配条件下,GaSe和ZnGeP2晶体差频的相位匹配角、走离角、允许角和有效非线性系数,并对计算结果进行了分析比较,总结出对应输出不同太赫兹波长的最佳相位匹配方式.计算结果为利用非线性晶体差频产生可调谐太赫兹辐射的实验研究提供深入和全面的理论基础.
关键词:
太赫兹波
GaSe晶体
2晶体')" href="#">ZnGeP2晶体
差频 相似文献
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介绍了一种基于新型非线性晶体Ba1-xB2-y-zO4SixAlyGaz 的可调谐深紫外飞秒激光光源. 从理论上分析了基频光和倍频光在通过非线性晶体时所造成的空间走离和群速度失配, 为了补偿空间走离以及波长调谐过程中晶体折射造成的光束偏离现象, 将两块相同的倍频晶体成镜像放置来产生二次谐波. 并调节延迟线的长度来补偿基频光和倍频光之间的群速度失配, 从而提高和频转换效率. 然后通过和频方式进行三倍频和四倍频来突破晶体相位匹配条件的限制, 产生了波长低于200 nm的深紫外飞秒激光. 利用钛宝石激光器提供基频光光源, 最终在250–300 nm, 192.5–210 nm 范围内获得了高重频、可调谐超短脉冲紫外和深紫外激光. 并在基频光波长为800 nm时, 得到的二倍频、三倍频和四倍频的功率分别为1.28 W, 194 mW和5.8 mW, 相对于前一级的转换效率依次为46.14%, 15.16%和3%. 采用互相关法测量得到266.7 nm紫外激光的脉冲宽度约为640.4 fs. 相似文献
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量子光学频率梳在量子计算、量子信息以及高精度量子测量等领域都有重要的价值,同步泵浦光学参量振荡器是制备量子光频梳最主要的手段.本文采用中心波长为815 nm、脉冲宽度为130 fs的锁模飞秒脉冲激光二次谐波泵浦Ⅰ类共线BiB3O6晶体以制备真空压缩态量子光频梳,给出了同步泵浦光学参量振荡器中空间走离效应对获得量子光频梳压缩度的影响.研究表明,随着晶体长度的增加,压缩度的增长会受到空间走离效应限制,经计算在晶体长度为1.49 mm时压缩达到最大.在此基础上,本文实验研究了在四种晶体长度下获得的真空压缩态量子光频梳的压缩特性,当BiB3O6长度为1.5 mm时获得了(3.6±0.2) dB的最大真空压缩,考虑损耗后为(7.0±0.2) dB,实验结果与理论分析相符.该研究揭示了飞秒脉冲光在非线性晶体中存在的空间走离效应是影响量子光频梳压缩特性的重要因素,为优化量子光频梳的实验测量提供了指导. 相似文献
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描述了在BBOⅠ类相位匹配的飞秒光参量放大(OPA)中,利用非共线结构和倾斜抽运光的脉 冲波面来完全补偿三波群速失配的方法.理论计算了三波群速匹配时,非共线角、相位匹配 角、抽运光的脉冲波面倾斜角随信号光波长的变化,并分析了对抽运光光斑尺寸的要求和对 空间走离长度的影响.结果表明,利用该方法不仅能够实现最大的参量带宽,而且能够完全 补偿飞秒OPA中三波的群速失配.此外,选取合适的抽运光光斑尺寸和非线性晶体的长度对提 高参量增益也至关重要.
关键词:
群速匹配
非共线相位匹配
脉冲波面倾斜
飞秒光参量放大 相似文献
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为了消除群速失配对参量放大的不利影响,描述了利用脉冲波面倾斜与非共线相位匹配相结 合,完全补偿飞秒光参量放大(OPA)中三波群速失配的新方法.计算了在BBOⅠ类、Ⅱ类相 位匹配条件下, 三波实现群速匹配时,相位匹配角、脉冲波面倾斜角以及非共线角随信号 光波长的变化.并分析了三波群速匹配对空间走离长度、参量增益和参量带宽的影响.结果表 明,在BBOⅠ类、Ⅱ类相位匹配条件下,利用该方法均能实现飞秒OPA连续调谐时三波的群速 匹配,从而大大增加了三波的有效互作用长度,为能够获得高增益,窄脉宽的参量光脉冲提 供了理论依据和指导.
关键词:
群速匹配
脉冲波面倾斜
非共线相位匹配
飞秒光参量放大 相似文献
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计算了MgO:LiNbO3晶体中,共线与非共线相位匹配光参量放大产生超短中红外激光脉冲过程中的相位匹配曲线、有效非线性系数以及时间和空间走离情况。结果表明,采用非共线相位匹配方式,可以实现三波间群速度匹配;在抑制了泵浦光与信号光之间的空间走离的同时加大了泵浦光与闲频光之间的空间走离,但这种影响可以忽略;同时非共线角的引入使相位匹配角增大,提高了有效非线性系数。因此,非共线角的引入在不影响空间走离的情况下,有效补偿超短中红外参量放大过程中的时间走离,有利于参量放大转换效率的提高。 相似文献
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We investigate the spontaneous parametric down-conversion (SPDC) process in biaxial nonlinear crystal BiB3O6 (BIBO) with a broadband pump. Under the type I and type II phase-matching conditions, we numerically calculate the influencing factors on SPDC process in BIBO crystal, such as temporal and spatial walk-off, the acceptance angles, and spectral acceptance bandwidth. Comparing the two types of phase-matching, we could conclude that the type II phase-matching in BIBO crystal is better for the SPDC because of zero dispersion and bigger acceptance parameters. These results can be used to construct a system to generate ultra-fast entangled photon pairs. 相似文献
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Second-order nonlinear optical materials for efficient generation and amplification of temporally-coherent and narrow-linewidth terahertz waves 总被引:1,自引:0,他引:1
We have considered forward and backward optical parametric oscillation and amplification, and difference-frequency generation for efficiently generating and amplifying terahertz waves in several second-order nonlinear optical materials. We have used a single crystal of CdSe as an example. We have also investigated GaSe, periodically-poled LiNbO3 and LiTaO3, and diffusion-bonded-stacked GaAs and GaP plates. The advantage of using birefringence in CdSe and GaSe is tunability of the output terahertz frequency. Furthermore, both CdSe and GaSe can be used to achieve the backward parametric oscillation without any cavity. On the other hand, in periodically-poled LiNbO3 and LiTaO3, one can take advantage of large diagonal elements of second-order nonlinear susceptibility tensor. In the diffusion-bonded-stacked GaAs and GaP plates, quasi-phase matching can be achieved by alternatively rotating the plates. We have shown that it is feasible to achieve forward optical parametric oscillation in the THz domain using these plates. The advantage of using coherent parametric processes is possibility of efficiently generating and amplifying temporally-coherent and narrow-linewidth terahertz waves. Compared with a noncollinear configuration, by using the parallel wave propagation configurations, the conversion efficiency can be higher because of longer effective interaction length among all the waves. 相似文献
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We report a femtosecond optical parametric oscillator (OPO) based on the nonlinear material BiB?O? (BIBO) pumped directly by a Kerr lens mode-locked Ti:sapphire laser. Using a 1.5 mm long BIBO crystal cut at θ=11.4° for collinear type I (e→o+o) phase matching in the xz optical plane, femtosecond signal pulses across 1.4-1.6 μm, and idler pulses across 1.6-1.87 μm spectral range are generated, limited by the reflectivity bandwidth of the OPO mirrors. The high nonlinear gain and large spectral acceptance for type I interaction in the xz plane of BIBO permit rapid and continuous tuning across the entire range by simple fine adjustment of OPO cavity delay or through small changes in the pump wavelength, without varying any other parameters. Additionally, owing to the near-zero group velocity mismatch and dispersion, the OPO supports broad spectrum as wide as 33 nm, which results in self-compressed signal pulses. For 150 fs pump pulses, signal pulses with durations down to 106 fs with a time-bandwidth product of 0.48 are obtained without the need for intracavity dispersion compensation. 相似文献
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Suleyman Cabuk 《哲学杂志》2016,96(2):190-207
The linear and non-linear optical properties of BiAlO3 are studied by employing the density functional perturbation theory within the local density and generalized gradient approximations. The computations are based on the electronic structure obtained within density functional theory. The optical properties such as the dielectric function, refractive index, spectral reflectivity, absorption coefficient and electron energy-loss spectrum are obtained in the energy region of up to 30 eV. The calculated value of the birefringence for BiAlO3 shows that it is a uniaxial negative crystal and has a large birefringence. We also report our studies on the second harmonic generation response coefficient over a large frequency range for BiAlO3 crystal. The predicted second-order optical spectra indicate pronounced structures related to of 1ω and 2ω frequency resonances. Furthermore, the non-linear optic and linear electro-optic coefficients are computed by employing 2n + 1 theorem applied to an electric-field dependent energy functional. The results are compared with the available calculations. 相似文献
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Venkata Ramaiah‐Badarla Adolfo Esteban‐Martin Majid Ebrahim‐Zadeh 《Laser \u0026amp; Photonics Reviews》2013,7(5):L55-L60
A self‐phase‐locked degenerate femtosecond optical parametric oscillator (OPO) based on the birefringent nonlinear material, bismuth triborate, BiB3O6, synchronously‐pumped by a Kerr‐lens‐mode‐locked Ti:sapphire laser at 800 nm is described. By exploiting versatile phase‐matching properties of BiB3O6, including large spectral and angular acceptance for parametric generation and low group velocity dispersion in the optical xz plane, stable self‐phase‐locked degenerate OPO operation centered at 1600 nm is demonstrated using collinear type I (e → oo) interaction in a 1.5‐mm crystal at room temperature. The degenerate OPO output spectrum extends over 46 nm (∼5.4 THz) with 190 fs pulse duration for input pump pulses of 155 fs with a bandwidth of 7 nm. Phase coherence between the pump and degenerate output is verified using f‐2f interferometry, and discrete frequency beats caused by different carrier‐envelope‐offset frequencies are measured using radio frequency measurements. Photo shows a 1.5‐mm BiB3O6 crystal used as a nonlinear gain medium in a degenerate self‐phase‐locked femtosecond OPO operating at room temperature. The green beam is the result of non‐phase‐matched sum‐frequency mixing between the pump light and the sub‐harmonic OPO field at degeneracy. 相似文献
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Comparative investigation of long-wave infrared generation based on ZnGeP2 and CdSe optical parametric oscillators 下载免费PDF全文
Long-wave infrared (IR) generation based on type-II (o→e+o) phase matching ZnGeP2 (ZGP) and CdSe optical parametric oscillators (OPOs) pumped by a 2.05 μm Tm,Ho:GdVO4 laser is reported. The comparisons of the birefringent walk-off effect and the oscillation threshold between ZGP and CdSe OPOs are performed theoretically and experimentally. For the ZGP OPO, up to 419 mW output at 8.04 μm is obtained at the 8 kHz pump pulse repetition frequency (PRF) with a slope efficiency of 7.6%. This ZGP OPO can be continuously tuned from 7.8 to 8.5 μm. For the CdSe OPO, we demonstrate a 64 mW output at 8.9 μm with a single crystal 28 mm in length. 相似文献