Nuclear structure of low-lying 0+ states in Ge and Se isotopes

The following meanlives of levels in⁷²Se have been measured using the recoildistance Doppler-shift method:Τ(2⁺, 862 keV)=3.1±0.6 ps,Τ(2⁺′, 1317 keV)=12.5±2.6 ps,Τ(4⁺, 1638 keV)=1.2±0.3 ps andΤ(6⁺, 2469 keV)≦0.7 ps. These meanlives yield sixB(E2) values which are discussed together with the known data of the depopulation of the excited 0⁺′ state at 937 keV. Systematics of 0⁺′ states in the mass region 70?A?100 show that the low excitation energy of the 0⁺′ states is correlated with subshell closures. This suggests that the previous interpretation of the 0⁺′ state in⁷²Se as a rotational band head is questionable.     

Structure of excited states in100Mo and102Mo from spectroscopy using18O induced reactions

The lifetimes have been determined for the 2⁺, 0^+～ and 4⁺ states in¹⁰⁰Mo and¹⁰²Mo using the recoil-distance Doppler-shift method. The states have been excited in¹⁰⁰Mo by Coulomb excitation and in¹⁰²Mo by the two-neutron transfer reaction induced by¹⁸O ions on a¹⁰⁰Mo target. The study of the excitation function for the elastic and inelastic scattering on the ground and first excited 2⁺ state in¹⁰⁰Mo at beam energies between 20 and 61 MeV shows that 40 MeV is the highest incident energy for pure Coulomb excitation. Above this energy nuclear absorption sets in and nuclear scattering contributes to the excitation of the 2⁺ state of¹⁰⁰Mo. From the lifetimes of the 2⁺ and 4⁺ states deformation parameters of ¦β¦= 0.21 and ¦β¦=0.31 for¹⁰⁰Mo and¹⁰²Mo respectively were deduced. The 0^+′ levels are not shape isomeric states, as suggested earlier, but they decay by enhancedE2 transitions to the first 2⁺ states. From a comparison with similar states in other transitional nuclei it is suggested that they are band heads forβ vibrational bands.     

Lifetime of the 2755 keV 15/2− state in43Ca

Using the recoil distance Doppler shift method, we measured the lifetime of the 2755 keV 15/2^? state in⁴³Ca populated in the reaction²⁸Si(¹⁸0,2p n) to beΤ=39 ±5 ps. We also remeasured the lifetime of the 2751 keV 4⁺ state in⁴²Ca excited in the reaction²⁸Si(¹⁶O,2p) to beΤ=3.8±0.4ps. Effective charges derived fromE2 transition between (f _7/2)^v high-spin states are discussed.     

Static electric quadrupole interaction of Ta- and Hf-ions in barium and lead titanate

The static electric quadrupole interaction of¹⁸¹Ta and¹⁷⁸Hf in polycrystalline barium and lead titanate at the site of titanium has been measured using time differential PAC and the Mössbauer effect. The electric field gradients (EFG) at room temperature at the¹⁸¹Ta nucleus are ¦V _zz¦=(3.6±0.2)·10¹⁷V/cm² in BaTiO₃ and ¦V _zz¦=(14.6±0.6)·10¹⁷ V/cm² in PbTiO₃. The temperature dependence of the quadrupole interaction has been studied giving the following EFG values: ¦V _zz¦=(2.4±0.2)·10¹⁷ V/cm² in the monoclinic and ¦V _zz¦=(1.1±0.3)·10¹⁷ V/cm² in the rhomboedral phase of BaTiO₃, and ¦V _zz¦=(15.7±0.6)·10¹⁷ V/cm² for¹⁸¹Ta/PbTiO ₃ at 77 °K. The EFG of¹⁷⁸Hf in PbTiO₃ has been derived from a Mössbauer effect experiment to beV _zz=+(10.7±0.5)·10¹⁷ V/cm². The results are compared with EFG's calculated in a point charge model and with experimental EFG's measured at⁴⁴Sc and⁵⁷Fe in the same titanates by other authors. Contributions of covalent bonds to the effective EFG's in perovskit crystals are discussed.     

The cross section of the7Be(n,p)7Li reaction at 24.5 keV neutron energy

The 24.5 keV neutrons induced reaction with the⁷Be radioactive nucleus was studied. The value of σ_np=(18±4)b was obtained for the⁷Be(n, p)⁷Li reaction cross section.     

Multihadronic decays and partial widths of the J/Ψ (3100) resonance produced in e+e− annihilation at adone

The reactions e⁺e^?→ hadrons and e⁺e⁺e^?→e⁺e^? have been studied at the J/gY (3100) resonance). The relative weights of the topological cross sections for fixed charged multiplicity are σ₂=(32±5)%, σ₄=(49±8)%, σ₆=(18±3)%, and σ₈=(1±0.6)%. The average pion multiplicities are 〈n_ch〉=3.8±0.3 and 〈n_{π^o〉=3.1±0.8}. The decay widths are Γ_e=(4.6±0.8) keV, Γ_h=(59±24) keV, and Γ=(68±26) keV.     

Properties of excited levels in102Rh by the102Ru(p,nγ) reaction

The level scheme of¹⁰²Rh has been investigated by the¹⁰²Ru(p, nγ) reaction in the proton energy range 3.1 MeV≦E _p≦6 MeV. Excitation functions,γ-γ coincidences and pulsed beam measurements have been performed and a level scheme including 33 excited states up toE _x≈650 keV has been constructed. Theγ-branchings of several levels have also been measured. The lifetimes of 5 excited states have been determined with the centroid-shift method:τ _m(105.2 keV)=(1.3±0.3) ns,τ _m(123.7 keV)=(0.6±0.3) ns,τ _m(178.6 keV)=(1.5±0.3) ns,τ _m(208.7 keV)=(0.5±0.3) ns,τ _m(359.6 keV)=(0.8±0.4) ns. Upper limits have been placed for the lifetimes of 20 other levels.     

Nuclear structure effect on internal conversion ofl-forbidden transitions in139La,141Pr and203Tl

Accurate experimental internal conversion data have been used to study the effect of nuclear penetration in the case of thel-forbidden transitions in¹³⁹La (165.8 keV),¹⁴¹Pr (145.4 keV) and²⁰³Tl (279.2 keV). The nuclear penetration parameterλ and theE2/M 1 mixing ratioδ ² have been deduced by graphical analysis. Following results were obtained:λ=2.8±1.3,δ ² =(8.4 _?8.4 ^+14.0 )·10^?4 for¹³⁹La,λ=1.2±0.6,δ ²=(4.8±0.5)·10^?3 for¹⁴¹Pr, andλ=6.4±1.1,δ ²=1.36±0.12 for²⁰³Tl.     

The spin of the 2,198 keV level in74Ge and multipole mixing ratios of gamma transitions in the decay of74As

Directional-correlation measurements of several cascades in the⁷⁴As decay have been made with a NaI — Ge(Li) detectors system. In the⁷⁴Ge the following cascades were measured: 608–596 keV, 994–1,204 keV, 994-(608)-596 keV and 887-596 keV. The corresponding results give a unique spin assignment of 2 for the 2,198 keV level and determine theE2/M 1 mixing ratios ofδ(608)=3.4±0.4 andδ(994)=?(2.8 ± 0.2). In the⁷⁴Se it was measured the 635-635 keV cascade. The result obtained assigned the spin of the 1,270 keV level as 2 and fixed the E2/M1 mixing ratio of δ(635)=?(2.6 ± 0.2). Also aγ-intensity study has been made to determine the branching ratios of the transitions that deexcite the 1,270 keV level in⁷⁴Se. From these data aI(635)/I(1,270)=12.5 ± 5.0 is obtained.     

Der Zerfall des125m Xe,des127m Xe und des127g Xe

The decay of^125m Xe produced by the reaction¹²²Te(α, n)^125m Xe using a target enriched in¹²²Te (95.4%) and the decay of^127m Xe produced by the reaction¹²⁷J(d, 2n)^127m Xe have been investigated: ^125m Xe decays with a half-life ofT _1/2=(56±3) sec by ayy- cascade withE _γ1=(140.4 ±0.5) keV andE _γ2=(110.5 ±0.5) keV. The experimental conversion coefficients yield multipolarities ofE3 for the 140.4 keV isomeric transition and predominantlyM1 for the 110.5 keV-transition. ^127m Xe decays with a half-life ofT _1/2=(71±2) sec. The decay also proceeds by aγγ-cascade with an isomeric E3 transition ofE _γ1=(172.5±0.3) keV and a predominantlyM1 transition ofE _γ2=(124.6±0.3) keV. In the decay of^127g Xe an additional branching of the electron capture to a level at (618.1±0.3) keV was observed. The relative probability forK-captureP _K618/P_K375=0.40 ±0.07 yields a total transition energyQ _EC=(664 ±4)keV. A spin of 1/2⁺ was assigned to the ground state.     

The ratio of the quadrupole moments of the isotopes95Mo and97Mo

The spin-lattice relaxation timesT ₁ of the NMR signals of⁹⁵Mo and⁹⁷Mo in aqueous K₂MoO₄ solutions were determined by the inversion recovery technique. To separate the relaxation rates due to electric quadrupole interaction and due to magnetic dipole interaction, pure H₂O and mixtures of H₂O and D₂O were used as solvent. No dependence of the ratio of the relaxation ratesT ₁(⁹⁵Mo)/T ₁(⁹⁷Mo) on the composition of the solvent was to be detected, i.e. the relaxation due to magnetic dipole interaction may be neglected. From the ratio of the relaxation rates the absolute value of the ratio of the quadrupole moments of the molybdenum isotopes was evaluated: ¦Q(⁹⁷Mo)/Q(⁹⁵Mo)¦ = 11.4 ±0.3.     

Double beta decay of 100Mo

Two-neutrino double beta decay of ¹⁰⁰Mo with half-life T _1/2=[7.2±0.9(stat)± 1.8(syst)]×10¹⁸ yr was detected using a liquid argon ionization chamber. With a C.L. of 68% (90%), the bounds on neutrinoless decay and decay with majoron emission were found to be 8.4(4.9)×10²¹ and 4.1(3.2)×10²⁰ yr, respectively. An analysis of all available results provides the average “world” value T _1/2=(8.0±0.7)×10¹⁸ yr for the two-neutrino decay of ¹⁰⁰Mo, and the corresponding nuclear matrix element is M _GT=0.118±0.005.     

Gamma radiation from the ground state decay of95Tc

The 20 h^95gTc decay to levels of⁹⁵Mo has been investigated studyingγ-singles andγγ-coincidences. The first excited state of⁹⁵Mo at 204 keV, previously assumed to be populated in the^95m Tc decay only, is found to be fed by aγ-transition of 870 keV deexciting the level at 1074 keV which is populated in the^95g Tc decay. More over three newγ-transitions of 477, 786 and 1552 keV deexciting the level at 1552 keV have been found. For the levels at 1074 and 1552 keV the range of possibleJ ^π assignments could be reduced.     

Winkelkorrelationsmessungen an >30y Holmium 166 und Bestimmung desg R -Faktors des 4+-Rotationsniveaus von Erbium 166

The spins of several excited states of Er¹⁶⁶ have been investigated byγγ-angular correlation measurements. The spin sequence 0+, 2+, 4+, 6+ for the ground state rotational band was presumed to be correct. Unique assignments were derived for the states of 1076 keV, 1377 keV and 1785 keV asI=5, 7 and 6 respectively. These results are in agreement with the spins proposed byGallagher jr. andSoloviev. The multipolarities of theγ-transitions of 408 keV, 709 keV, 811 keV and 831 keV were derived as 95%E1+(5±1)%M2, 99·6%E1+(0·4±0·5)%M2, 99·1%E2+(0·9±0·3)%M1, and 96·1%E2+(3·9±1)%M1 respectively. The unusual mixing ratios of the transitions of 811 keV and 831 keV can be understood as a consequence of theK-selection rule. Eachγ-transition from the 1785 keV state should be stronglyK-forbidden and one expects a half-life ofT _1/2≈3·10^?9s. A measurement of the time spectrum of the coincidences between theβ-radiation and the high energyγ-lines gave however:T _1/2(1785 keV state)≦3·10^?10s. The rotation of the angular correlation between the 184 keV line and theγ-group at 820 keV has been measured in an external magnetic field of 53000 gauss as:ω·τ(4+)=0·083±0·006. This value contains small corrections for an additional rotation of the angular correlation of the 831 keV–184 keV triple cascade in the 6+state and for a small attenuation by internal fields. WithT _1/2(4+state)=1·23·10^?10s, andβ=7·08 one gets for theg-factorg _R=+0·266±0·024 in good agreement with recent results for the 2+ state.     

Beta decay of12B and12N to the first excited state of12C (4.44 MeV)

The branching ratios of the beta-decay of¹²B and¹²N to the 4.44 MeV state in¹²C were determined by (βγ-coincidences to be (1.182±0.019)% and (1.898±0.032)% of the total rate, resp. This givesft ^?=(1.407±0.023) · 10⁵ s andft ⁺=(1.406±0.024) · 10⁵ s. For theft-asymmetryδ=(ft ⁺/ft ^?)?1 the valueδ=?(1±14) · 10^?3 was obtained. This is in contrast to other GT mirror transitions which show positiveδ of a few percent.     

Low-lying energy levels in 166Ho

The properties of some low-excited states of ¹⁶⁶Ho have been studied using thin, high resolution Ge detectors. The relative intensities of γ-lines were determined. The directional angular correlation measurements for the 28.23–54.24 keV cascade are in agreement with the 1^?(M1)2^?(E2)0^? spin sequence. The magnetic moment μ = 0.068 ± 0.010 μ_N of the 54.24 keV level was determined by integral perturbed angular correlation (IPAC) in an external magnetic field. This value can be explained by the configuration mixing due to the Coriolis interaction.     

Lifetimes of high-spin levels in39Ar

The high-spin states in³⁹Ar at 2651, 3992, 4543, and 5536 keV were excited in oxygen-induced fusion-evaporation reactions. Mean lifetimes ofτ _m =1.0±0.2, 1.2±0.3, 1.6±0.3, and <1 ps were determined for these levels, respectively, by means of the recoil distance Doppler shift technique. The transition rates are discussed in terms of the Bansal-French weak-coupling model.     

Nuclearg-factors of the first excited states in Ir191 and Ir193

Mössbauer experiments were performed to determine the nuclearg-factor of the 82 keV 1/2⁺ state in Ir¹⁹¹ (g=+1.083±0.009) and the 73 keV 1/2⁺ state in Ir¹⁹³ (g=+0.9400±0.0019). TheE2/M1 mixing parameters of the corresponding (1/2⁺) (E2/M1) (3/2⁺) transitions were found to be ¦δ¦ (Ir¹⁹¹, 82 keV)=0.80±0.06 andδ(Ir¹⁹³, 73 keV)=?0.558±0.005.     

The hyperfine field of99Tc in iron

The magnetic hyperfine field at⁹⁹Tc impurities in Fe has been measured to be ¦H _hf¦=325 (7) kGauss at 298 °K. The technique of time-differential perturbed angular correlations on the 181 keV state of⁹⁹Tc was used.