基于二次谐波产生技术的BaTiO3薄膜对称性研究

光学二次谐波产生技术是研究材料极化特性和对称性的重要工具,利用搭建的显微二次谐波产生光路,对生长在SrTiO3衬底上的BaTiO3薄膜样品进行了二次谐波产生测试.结果 表明,BaTiO3薄膜在面内方向具有二重旋转对称性.在四种偏振模式下测量了样品的二次谐波信号,结果表明,随着基频光入射功率的变化,二次谐波强度的图样也发...     

非线性左手材料中的二次谐波

基于电磁场理论，推导了无耗非线性左手材料中二次谐波的曼利－诺关系，及相位匹配条件下正向基波与逆向二次谐波的能量转换过程及其空间分布.验证了可将无耗非线性左手材料的入射面作为反射镜，把能量以二次谐波的形式反射.同时分别给出有限厚度介质板中基波和二次谐波的场强分布数值结果，验证了结论的正确性.最后从相位失配角度说明了相位匹配是分析非线性左手材料二次谐波的重要条件.这为研究左手材料的非线性理论奠定了基础.     

磁诱导的光学二次谐波及其应用

介绍一种新近发展起来的，利用光学非线性效应来进行磁学测量的实验方法－－磁诱导的光学二次谐波。该方法不仅对于表面的对称性及磁性结构具有极高的探测灵敏度，更重要的是它还是现在极少数可对多层薄膜的界面进行研究的技术，这为当今非常活跃的磁性单层、多摹研究工作提供了一个强有力的手段。     

二次谐波产生过程中准相位匹配条件的研究

从耦合波基本方程出发,在实空间严格推导出二次谐波产生(SHG)过程中的准相位匹配(QPM)条件.讨论了满足QPM条件时,SHG的转换效率以及相位失配角随波传播距离的变化.着重研究了非线性极化率的周期性调制对提高SHG转换效率的贡献.     

二次谐波产生中入射啁啾脉冲对相位的影响

讨论了基波为叔率啁啾脉冲的二次谐波产生过程，结果表明选取合适的啁啾参量可以提高二次谐波的光强，但同时会使其波形和相位发生变化，三次相位的畸变主要取决于入射的基波啁啾脉冲，而与相位匹配的失谐量关系不大。     

锗薄膜透射光学二次谐波研究

本文采用固定入射角，改变入射光偏振方位角的方法从实验上了研究了锗薄膜的透射光学二次谐波产生及其变化规律，并从理论上推导了产生透射二次谐波的表达式，最后拟合求得描述面谐波电流的唯象参数ａ。     

掺半花菁二氧化硅薄膜光学二次谐波产生

报道了用溶胶 凝胶技术制备掺入半花菁染料的二氧化硅薄膜．在不加电场极化条件下，由半花菁分子的自取向导致光学二次谐波产生，定量测得厚度为50nm薄膜的二阶非线性系数χ^（2）为6.6pm/V，并初步研究了半花菁分子自取向的机理 关键词：     

LB膜的变入射角透射光学二次谐波产生研究

给出了不同基频光和倍频光偏振态组合情况下，淀积在固体基板上的Ｌａｎｇｍｕｉｒ－Ｂｌｏｄｇｅｔｔ单分子层膜在面对入射光方向和背对入射光方向时，反射及透射光学二次谐波产生随入射角变化关系的理论公式。在此基础上，对一种芪盐ＬＢ膜样品进行变入射角的透射二次谐波产生研究。     

双轴晶体中非共线相位匹配二次谐波产生现象分析

激光束与其散射光束在晶体中发生非线性和频作用，在满足非共线相位匹配条件时，可观察到二次谐波环的现象。本文以拆射率主轴坐标ｘｏｚ平面为例，推导出了双轴晶体中环参数的近似表达式。并用计算机得出了精确数值解，与实验观察到环的形状完全一致，提出了一种寻找最佳二次谐波产生方向的方法。     

双轴晶体中二次谐波产生的最佳相位匹配条件

从二次谐波产生的理论出发，讨论了双轴晶体中二次谐波产生的相位匹配条件，推导了有效非线性光学系数的精确计算公式，以有机非线性光学晶体二苯甲酮为例，给出了对两种基波(1064μm和0808μm)二次谐波产生的相位匹配条件的数值模拟及相应的有效非线性光学系数的精确计算结果，并确定出相应的最佳相位匹配条件. 关键词： 二次谐波产生 最佳相位匹配 有效非线性光学系数 二苯甲酮晶体     

准相位匹配周期极化钼酸钆制备及倍频效应

根据准相位匹配原理，对钼酸钆晶体用于准相位匹配倍频过程的周期性畴结构进行了设计，当入射基频光为l.064pm时，所需的钼酸钆晶体畴结构周期为5．54μm。利用外电场极化，当外电场为2．5kV／mm时，钼酸钆晶体的畴结构反转时间tc=500～600μs。当外电场脉冲幅值为2．5kV／mm、脉冲延续时间t=0．6～0．8tc时，在钼酸钆晶体中制备得到了周期畴结构。当Nd：YAG纳秒激光器输出准连续功率为7～10mW的l.064μm激光通过具有周期畴结构的样品时，获得了0．532μm的倍频光输出。     

Second Harmonic Generation in TlInS2 Crystals

The temperature dependence of the generation of the second optical harmonic in TlInS₂ crystals in the vicinity of the phase transitions high–temperature–incommensurate–polar phases is investigated. It is shown that radiation in the incommensurate phase occurs only when the fundamental wave propagates along the axis of the superstructure of a crystal and the presence of radiation for certain geometries of the experiment confirms the symmetry group C ₂ ³ of the low–temperature polar phase. The dependence of the spectra on the periodic temperature change is attributed to the occurrence of long–lived metastable states.     

Cascaded Second Harmonic Generation for Deep-UV Radiations with a 2D Nonlinear Photonic Quartz Crystal

Harmonic generation can broaden the laser wavelength in a great scope and is rich in physics, but the efficient cascaded second harmonic generation especially those directly deep into deep-ultraviolet (DUV) with one single crystal seems to be impossible, due to the extremely strict phase-matching conditions and relative narrow bandgap of present nonlinear optical crystals. Here, this work designs a nonlinear photonic quartz crystal where the phase difference of interacted light waves is manipulated in two dimensions and realizes an unprecedented cascaded phase-matched 2nd–5th harmonic generation simultaneously with the photon energy up to 6 eV, representing the shortest wavelength by cascaded second harmonic generation in the solid-state nonlinear medium. The generated light is located in the visible-DUV region with a total conversion efficiency of 2.7%. The present nonlinear photonic quartz scheme not only provides a multi-wavelength solid-state laser source applied in modern devices but also develops a new route for studying the light-matter nonlinear interaction in the DUV region.     

基于周期性极化铌酸锂倍频的光学电压传感方法

从光学电压传感器的原理出发,在周期性极化铌酸锂(PPLN)晶体倍频(SHG)效应基础上,提出了一种新的光学电压传感方法,讨论了周期性极化铌酸锂不同长度、不同占空比对该电压传感性能的影响,并给出了图示。结果表明：当周期性极化铌酸锂长度一定,在占空比为0．3或0．7时,灵敏度最高;在占空比趋于0．5,但不等于0．5时,电压测量范围最大;长度增加,灵敏度提高,但测量范围变小。这些结果为制作此类传感器提供了可靠的理论依据。     

聚焦光场激发下中心对称球形粒子的二次谐波产生

在聚焦光场矢量衍射理论的基础上,利用贝塞尔函数的微分递推关系,推导了聚焦光场的梯度变化表达式。根据中心对称材料二次谐波产生的唯象模型,研究了单个中心对称球形纳米颗粒在聚焦光场激发下的二次谐波产生,考察了表面响应和体效应产生的二次谐波辐射分布随着数值孔径增大的变化规律,并利用聚焦光场及其梯度场分布特性讨论差异产生的原因。研究结果表明,激发光场的聚焦程度对体响应的影响更为显著。     

Second Harmonic Generation in 1D Nonlinear Plasma Photonic Crystals

In this paper, a 1D nonlinear plasma photonic crystal (NPPC) structure composed of polarized ferroelectric crystals and nonlinear plasma periodic alternation is proposed. The transfer matrix method is employed to analyze the second harmonic generation (SHG) problem of this structure. In the designed NPPCs, the fundamental wave (FW) operates in the gigahertz (GHz) band and the nonlinear plasma is controlled by an external high-intensity control wave (CW). Numerical simulations are performed to investigate the effects of different incident angles and external CW intensities on the total conversion efficiency (T-con) of the second harmonic wave (SHW). Additionally, the internal electric field distribution and incident light intensity within the nonlinear structure are analyzed. The importance of the relationship between the FW frequency and photonic band gap (PBG) in enhancing SHG is summarized. The results demonstrate that the optimal structure can be obtained by changing the structural parameters, such that the FW and SHW are tuned to the edge of the PBG. At this point, the electromagnetic field density is large, the group velocity is small, the local field is enhanced, and the nonlinear optical interaction is increased, resulting in a significant increase in the T-con of the SHW.     

Second Harmonic Generation in Bis Typed Organic Compounds

In systematic research on a series of new nonlinear organic materials, we found that Bis (4-nitrophenoxy) methane (BNPM) showed a large intensity of second harmonic light, which was 4.4 times as large as that of urea crystal by powder technique and easily crystallized from a solution. The crystal structure of BNPM, obtained by the X-ray diffraction method, was orthorhombic, space group P2₁2₁2 (point group 222), with unit-sell dimension a = 10.205 Å; b = 12.854 Å; c = 4.8822 Å. In addition, we found that the absorption edge of BNPM was 430 nm with a 0.9-mm-thick crystal, and we observed the second harmonic light with BNPM single crystal at the wavelength of 1064 nm and in the range from 906 nm to 990 nm.     

二次谐波中的饱和效应和乘性噪声

研究了单模激光中产生的二次谐波的统计性质,用全饱和激光理论导出了二次谐波光子计数ｍ的几率分布函数、二次阶乘矩和三次阶矩的表达式,同实验值比较,理论与实验在阈值附近符合得很好。研究结果表明,激光场基波和二次谐波的涨落随空腔衰减常数的增大而减小;当激光场中含有乘性噪声时,乘性噪声增强基波的涨落,同时抑制二次谐波的涨落。