The Relation Between Barrier Structure and Current Uniformity in YBCO Josephson Junctions

Electromagnetic transport measurements were combined with high-resolution electron microscopy observations to study the relation between structure and local critical currents in YBa₂Cu₃O_7–x (YBCO) Josephson junctions. The spatial variation of the critical current J(x) along the length of the boundary for interface engineered Josephson junctions and bicrystal grain boundary Josephson junctions was determined using a phase retrieval algorithm. The current distribution solutions were found to be highly uniform along the length of interface engineered junctions in contrast to solutions for grain boundary junctions. The latter showed significant spatial oscillations in the critical current as well as areas along the boundary that carried no current. Microstructural evaluation of interface engineered junctions fabricated using identical processing parameters to the junctions used for transport measurements suggest that the uniform current distribution is controlled by a highly uniform barrier layer formed between the superconducting electrodes. Microstructural evaluation of grain boundary junctions similar to the junctions used for transport measurements show considerable variations of the grain boundary structure within a single junction.     

Tunneling spectroscopy and order parameter symmetry of hole- and electron-doped cuprate superconductors

In tunneling spectroscopy of superconductors the density of states close to the surface or the interface to an insulating tunneling barrier is probed. For d-wave superconductors the particle–hole coherence results in interesting new phenomena at surfaces such as the formation of bound surface states at the Fermi level by Andreev reflection due to a sign change of the order parameter field in different k -directions. The probing of these states represents a phase-sensitive experiment allowing the determination of the order parameter symmetry in superconductors. We summarize the present experimental status with respect to the study of high-temperature superconductors (HTS). We discuss theoretically predicted consequences of a dominating d-wave order parameter in the hole-doped HTS on their tunneling spectra as well as on the physics of high-temperature superconductor Josephson junctions. A comparison of the tunneling spectra obtained for hole- and electron-doped HTS leads to the conclusion that the former have a d-wave, whereas the latter most likely have an anisotropic s-wave order parameter. We also address some unsettled questions related to the presence of a state with broken time-reversal symmetry at surfaces and interfaces of d-wave HTS and discuss specific features of d-wave tunnel junctions that have been predicted theoretically but still not been confirmed in experiments.     

Ca‐doped Ba2Cu3O7–δ bicrystal junctions fabricated on asymmetric SrTiO3 substrates

Bicrystal grain–boundary Josephson junctions of Ca–doped YBa₂Cu₃O_7–δ that is Y_0.7Ca_0.3Ba₂Cu₃O_7–δ were fabricated on three bicrystal SrTiO₃ (001) substrates with asymmetric 30°, 40° and 45° orientations. An enhancement of the critical current density in these Ca–doped junctions was observed when compared with normal YBCO grain–boundary junctions with similar angular orientations. The observed increase in the critical current density is large for the junctions fabricated on the asymmetric 30° bicrystal substrate and small or negligible, for those on the asymmetric 45° bicrystal substrate. The critical current was modulated by a magnetic field applied in the plane of the junctions. However, the Fraunhofer pattern observed due to the applied magnetic field deviates from the ideal one.     

Josephson and quasiparticle currents in tunneling junctions between partially dielectrized (partially gapped) superconductors with spin density waves

The current-voltage characteristics (CVC) are calculated for the Josephson, interference, and quasiparticle components of the current through a tunneling junction formed by two superconductors with spin density waves (SDW). The treatment is based on the model of partial dielectrization (gapping) of the Fermi surface and the assumption of pinning of the spin density waves. The following particular cases are studied in detail: asymmetric SDW superconductor-ordinary superconductor junctions and symmetric junctions between two identical SDW superconductors. The positions and nature of the singularities in the CVC are determined. For a symmetric contact the possibility of the existence of asymmetric CVC’s is predicted. The calculations are in qualitative agreement with the experimentally observed behavior of the CVC’s of tunneling junctions and microcontacts containing the SDW superconductor with heavy fermions URu₂Si₂. Fiz. Tverd. Tela (St. Petersburg) 41, 1743–1749 (October 1999)     

Spin-charge gauge compositeness of electron in HTS: Hints from metal-insulator crossover and entropy behavior

We show that the coexistence of Fermi arcs and metal-insulator crossover of the in-plane resistivity can give a hint of a peculiar “gauge compositeness” of the electron in hole-doped high T_c cuprates and a similar hint also comes from the negative intercept at T=0 of the electronic entropy extrapolated from moderate temperatures in the “pseudogap phase”. An implementation of this “compositeness” within the spin-charge gauge approach is outlined and is employed to discuss the above phenomena.     

Materials and mechanisms of hole superconductivity

The theory of hole superconductivity proposes that there is a single mechanism of superconductivity that applies to all superconducting materials. This paper discusses several material families where superconductivity occurs and how they can be understood within this theory. Materials discussed include the elements, transition metal alloys, high T_c cuprates both hole-doped and electron-doped, MgB₂, iron pnictides and iron chalcogenides, doped semiconductors, and elements under high pressure.     

高温超导GdBa2Cu3O7-δ薄膜双晶晶界结特性研究

在晶界夹角为24°的YSZ人工双晶基片上,采用原位直流磁控溅射法制备了高温超导双晶GdBa₂Cu₃O_7-δ超导薄膜。采用光刻技术在晶界上刻出了尺寸5×5μm²的双晶晶界结。在77K下观测了结的直流I-V特性和在10GHz微波辐射下结的Shapiro台阶。这表明我们的人工双晶晶界结具有约瑟夫森弱连接行为。对结的特性进行了初步的理论分析和在实验基础上的数值模拟,模拟结果与RSJ理论符合较好,表明我们的双晶晶界结基本符合RSJ模型。     

Momentum dependence of pseudogap and superconducting gap in variation theory

To consider the origin of a pseudogap and a superconducting (SC) gap found in the high-T_c cuprates, we evaluated the momentum dependence of the singlet gap corresponding to the pseudogap and the SC gap in the t–J model, using an optimization variational Monte Carlo (VMC) method. In the underdoped regime, the singlet gap is significantly modified from the simple d_x²-y²(d)-wave gap (∝ cos k_x − cos k_y) by the contribution of long-range pairings. Its angular dependence at the quasi Fermi surface is qualitatively consistent with those experimentally observed in both hole and electron-doped cuprates. On the other hand, a SC gap is almost unchanged, preserving the original simple d-wave form. Thus, it seems that the incoherent part of the singlet gap mainly influences the forms of observed gaps.     

Doping dependence of charge order in electron-doped cuprate superconductors

Abstract

In the recent studies of the unconventional physics in cuprate superconductors, one of the central issues is the interplay between charge order and superconductivity. Here the mechanism of the charge-order formation in the electron-doped cuprate superconductors is investigated based on the t-J model. The experimentally observed momentum dependence of the electron quasiparticle scattering rate is qualitatively reproduced, where the scattering rate is highly anisotropic in momentum space, and is intriguingly related to the charge-order gap. Although the scattering strength appears to be weakest at the hot spots, the scattering in the antinodal region is stronger than that in the nodal region, which leads to the original electron Fermi surface is broken up into the Fermi pockets and their coexistence with the Fermi arcs located around the nodal region. In particular, this electron Fermi surface instability drives the charge-order correlation, with the charge-order wave vector that matches well with the wave vector connecting the hot spots, as the charge-order correlation in the hole-doped counterparts. However, in a striking contrast to the hole-doped case, the charge-order wave vector in the electron-doped side increases in magnitude with the electron doping. The theory also shows the existence of a quantitative link between the single-electron fermiology and the collective response of the electron density.     

Conductance anomalies of small tunnel junctions inside the Coulomb gap

A small-capacitance normal tunnel deviates significantly from equilibrium because each tunneling event turns the junction voltage almost upside-down. If such a sudden perturbation occurs locally, Fermi liquid theory guarantees that infinitely many electron-hole pairs should be created near the Fermi surface. It is predicted that such an infrared-divergent shake-up combined with the electromagnetic environment leads to subgap conductance anomalies for two categories of junctions. For symmetric junctions whose electrodes have the same electronic properties, a nonvanishing subgap conductance is shown to be inevitable even if the environmental impedance is infinite. This effect smoothes the current-voltage (I–V) characteristic and shifts the Coulomb offset extrapolated back from the high-voltage part of theI–V curve. For asymmetric junctions, whose electrodes have different electronic affinities, tunneling conductance is enhanced in one direction and suppressed in the other; that is, the junctions exhibit a diode effect. In particular, when the tunneling resistance is much smaller than the resistance quantum and the current flows in the favorable direction, a strong tendency towards establishing phase coherence is shown to emerge, as in Josephson junctions, resulting in infinite differential conductance at zero bias voltage.     

YBCO Josephson junctions based on artificially generated biepitaxial grain boundary

Summary In this paper we report the in-plane fabrication and the characterization of artificially engineered biepitaxial grain boundaries (GB) obtained by partly interposing a MgO seed layer between a bare or even-buffered substrate and a CeO₂ thin layer. The main peculiarity of this technique can be summarized by the capability to locate and engineer a single 45°-tilted GB at any stage of the device preparation. The junctions, realized by patterning the grain boundary occurring in the overhanging YBCO film, show Josephson current modulation in a large temperature range with anI _c R _n value of about 200 μV at 4.2K, theR _n value being constant over the whole superconducting region. Under microwave irradiation, theI–V characteristics display several Shapiro steps while, according to the Resistively Shunted Junction (RSJ) behaviour, the step heights have the typical current biased junction dependence. Paper presented at the ?VII Congresso SATT?, Torino, 4–7 October 1994.     

Charge dynamics in electron-underdoped high-Tc cuprates

We investigate charge dynamics in the antiferromagnetic (AF) phase of electron-doped cuprates by using numerically exact diagonalization technique for an electron-doped t-t′-J model. When AF correlation develops with decreasing temperature, a gap-like behavior emerges in the optical conductivity accompanied by the enhancement of the coherent motion of carriers due to the same sublattice hoppings. This is a remarkable contrast to the behavior of a hole-doped t-t′-J model.     

Spin fluctuation spectrum of electron-doped high-Tc superconductors

The magnetic excitation spectrum of electron-doped copper oxide superconductors is calculated using the Hubbard model on a square lattice. First, the on-site repulsion is treated with the random phase approximation. The spectrum of electron-doped systems in the superconducting state is compared with that of hole-doped systems, and the relationship between the frequency at which a peak grows in the spectrum and the superconducting energy gap at a hot spot (an intersection of the Fermi surface and the magnetic Brillouin zone boundary) is investigated. As compared with the hole-doped systems, the resonance condition is difficult to be satisfied in the electron-doped systems because of the small density of states around the hot spot. Moreover, the correlation effect in the Hubbard model is treated by the fluctuation-exchange approximation (FLEX), and the spin fluctuation spectra in the superconducting state in a wide region of the wave vector and frequency are calculated. We have found that the intensity of the magnetic spectrum at incommensurate wave vectors obtained with the FLEX is considerably weaker than that obtained with the RPA. The validity of the Fermi-liquid approach is also discussed.     

Interlayer magnetotransport study in electron-doped Sm2−x Ce x CuO4−δ

Vortex and pseudogap states in electron-doped Sm_2−x Ce _x CuO_4−δ (x ∼ 0.14) are investigated by the interlayer transport in magnetic fields up to 45 T. To extract intrinsic properties, we fabricated small 30 nm-high mesa structures, sufficiently thin to be free of the recently reported partial decomposition problems. On cooling, the c-axis resistivity ρ_c of the mesa structures reveals a semiconductive upturn above T_c, followed by a sharp superconducting transition at 20 K. When the magnetic fieldH is applied along the c-axis, ρ_c(T) shows a parallel shift without significant broadening, as also observed in the hole-doped underdoped cuprates. Above the transition we observe negative magnetoresistance (MR), which can be attributed to the field suppression of the pseudogap, whose magnitude is as small as 38 K. Our results in thex ∼ 0.14 samples closely correspond to the interlayer transport behavior in the ‘overdoped’ regime of hole-doped Bi₂Sr₂ CaCu₂ O_8+y.     

Metal-insulator crossover in high T c cuprates: A gauge field approach

A metal-insulator crossover appears in the experimental data for in-plane resistivity of underdoped cuprates and a range of superconducting cuprates in the presence of a strong magnetic field suppressing superconductivity. We propose an explanation for this phenomenon based on a gauge field theory approach to the t-J model. In this approach, based on a formal spin-charge separation, the low energy effective action describes gapful spinons (with a theoretically derived doping dependence of the gap m _s ² ∼ δ| ln δ|) and holons with finite Fermi surface (ɛF ∼ tδ) interacting via a gauge field whose basic effect on the spinons is to bind them into overdamped spin waves, shifting their gap by a damping term linear in T, which causes the metal-insulator crossover. The presence of a magnetic field perpendicular to the plane acts by increasing the damping, in turn producing a big positive transverse in-plane magnetoresistance at low T, as experimentally observed.     

The role of the surface depression of the pair potential on the Josephson and quasi-particle tunnelling in high-T c superconductors

Summary We discuss the influence of the intrinsic surface depression of the order parameter on the temperature dependence of the Josephson critical currentI _c(T) and, tentatively, on the quasi-particle tunnelling conductance in a superconductor with a very short coherence length. The comparison with the experiments shows that the presence of a surface-depressed pair potential can explain the large deviations of theI _c(T) from the ideal BCS behaviour that we recently observed in Bi₂Sr₂CaCu₂O_8+x Josephson break junctions and could mimic the presence of a broadening in the Superconductor-Insulator-Normal tunnelling conductance of the same high-T _c superconductor. Paper presented at the ?VII Congresso SATT?, Torino, 4–7 October 1994.     

Variational approach to strong correlation in the photoemission of electron-doped superconductors

We use a variational approach with strictly strong-correlated constraint to gain insight into low-energy states of t-t^′-t^″-J model in the electron-doped regime. Compared with the recent results on the electron-doped cuprates obtained by angle-resolved photoemission spectroscopy (ARPES), we show that based on the long-range ordered antiferromagnetic metallic state prohibiting vacant sites, our results lead to qualitatively similar trends in ARPES spectra and Fermi surface topology. Additionally, the results about the evolution of the energy gap and spectral weight as a function of doping will be discussed.     

Superfluid density in the slave-boson theory

Despite of the success of the slave-boson theory in capturing qualitative physics of high-temperature superconductors like cuprates, it fails to reproduce the correct temperature-dependent behavior of superfluid density, let alone the independence of the linear temperature term on doping in the underdoped regimes of hole-doped cuprate, a common experimental observation in different cuprates. It remains puzzling up to now in spite of intensive theoretical efforts. For electron-doped case, even qualitative treatment is not reported at present time. Here we revisit these problems and provide an alternative superfluid density formulation by using the London relation instead of employing the paramagnetic current-current correlation function. The obtained formula, on the one hand, provides the correct temperature-dependent behavior of the superfluid density in the whole temperature regime, on the other hand, makes the doping dependence of the linear temperature term substantially weaken and a possible interpretation for its independence on doping is proposed. As an application, electron-doped cuprate is studied, whose result qualitatively agrees with existing experiments and successfully explains the origin of d- to anisotropic s-wave transition across the optimal doping. Our result remedies some failures of the slave-boson theory as employed to calculate superfluid density in cuprates and may be useful in the understanding of the related physics in other strongly correlated systems, e.g. Na_xCoO₂·yH₂O and certain iron-based superconductors with dominating local magnetic exchange interaction.     

Doping and temperature dependence of the spin susceptibility in the p-d model

The spin magnetic susceptibility of the p-d model is calculated by means of a perturbation theory in the hybridization term V through a generalized cumulant expansion (GCE). The analysis is approached from the paramagnetic metallic phase. The results qualitatively reproduce some unusual magnetic properties in the normal state of the hole-doped cuprates, supporting the scenario of a Van Hove singularity near the Fermi level. Received 15 October 1998 and Received in final form 24 March 1999     

Electron- and Hole-Doping Effects in Manganites Studied by X-Ray Absorption Spectroscopy

We investigate the electronic structures of hole-doped, La_0.7Ca_0.3MnO₃, and electron-doped, La_0.7Ce_0.3MnO₃, manganites by x-ray absorption near edge structure (XANES) spectroscopy at the O and Mn K-edges. While, the O K-edge XANES results indicate that Ca and Ce doping induce holes in O 2p derived states, the Mn K-edge XANES do not give any evidence for creation of the Mn⁴⁺ (or Mn²⁺) ions by Ca (or Ce) dopants. Such results further questions the validity of double exchange mechanism in understanding the anomalous properties of manganites.