有限尺寸方靶等离子体离子注入动力学的三维粒子模拟研究

采用三维粒子模拟模型研究了有限尺寸方靶等离子体浸没离子注入过程中的鞘层动力学行为,得到了鞘层尺寸和方靶表面的注入剂量、注入能量以及注入角度等信息,并与二维无限长方靶注入结果进行了对比.模拟结果表明,与无限长方靶不同,有限尺寸方靶周围鞘层很快扩展为球形,但鞘层厚度明显减小.在模拟的50ω^-1_pi时间尺度内靶表面注入剂量很不均匀,中心区域注入剂量最小,四个边角附近位置注入剂量最大.这种剂量不均匀性是由于鞘层扩展为球形,使得鞘层内离子被聚焦并注入到边角附 关键词： 等离子体浸没离子注入 数值模拟 三维粒子模拟 有限尺寸方靶     

表面凹陷对等离子体浸没离子注入均匀性的影响

利用二维流体模型和数值计算方法模拟了等离子体浸没离子注入（ＰⅢ）Ｋ ,具有圆弧凹槽的平面靶周围的鞘层扩展情况,计算了鞘层扩展过程中的电热分布、离子速度和离子密度变化获得了沿靶表面的离子入射角度和注入剂量的分布情况,为等离子体浸没离子注入处理复杂形状靶提供了理论基础。     

梯形管内壁等离子体离子注入鞘层扩展MATLAB-PIC数值模拟

基于MATLAB利用Particle-in-cell模型,对梯形管内壁等离子体离子注入过程,进行了二维数值模拟.计算结果表明在中心电极附近出现了"阳极鞘层",该鞘层内部不存在离子,而且在鞘层边缘离子密度最高.在上下管壁上的离子注入剂量呈现"m"形分布.通过对注入过程中等离子体密度分布和不同时间段管壁不同位置离子注入剂量的跟踪,发现"阳极鞘层"扩展行为是导致"m"形分布的原因.由于梯形管形状的不对称性,"阳极鞘层"的边缘向梯形长底方向扩展较快.在注入初始时刻离子注入的能量很低,随着时间延长离子能量逐渐升高,这是由离子初始位置决定的.可见梯形管自身形状决定了鞘层形状和最终的离子注入能量和剂量分布.     

增强辉光放电等离子体离子注入的三维PIC／MC模拟

采用三维粒子模拟／蒙特卡洛模型自洽地模拟了增强辉光放电等离子体离子注入过程中离子产生和注入,获得了放电空间的离子总数、电势分布、等离子体密度分布和离子入射剂量等信息．模拟结果表明,5μs时鞘层达到稳定扩展,15μs时离子的产生与注入达到平衡,证实了增强辉光放电等离子体离子注入能在一定条件下实现白持的辉光放电．注入过程中,在点状阳极正下方存在一个高密度的等离子体区域,证实了电子聚焦效应．除靶台边缘外,离子的注入速率稳定且入射剂量均匀．脉冲负偏压提高时注入速率增加但入射剂量的均匀性变差．     

射频低压等离子体电子能量分布函数的探针诊断

本文对于无内电极放电的射频低压等离子体,采用探针电流调制法,设计并建立了三探针诊断电子能量分布函数的测量系统,测量了压力在10^-3—10^-1Torr下氮气等离子体的电子能量分布函数。从理论和实验上研究了探针鞘层上射频干扰电压对测量电子能量分布函数的影响,给出了确定射频干扰值以及对射频干扰的影响进行修正的方法,并采用该方法对实验数据进行了修正,得到了正确的电子能量分布函数。根据所得到的电子能量分布函数计算的电子平均能量,与由探针伏安特性计算得到的电子平均能量相差不超过5％,该结果间接证明了本文实验测量系统的可靠性以及对射频干扰影响进行修正的正确性。     

介质靶表面的充电效应对等离子体浸没离子注入过程中鞘层特性的影响

针对等离子体浸没离子注入技术在绝缘体表面制备硅薄膜工艺，采用一维脉冲鞘层模型描述介质靶表面的充电效应对鞘层厚度、注入剂量及靶表面电位等物理量的影响.数值模拟结果表明：随着等离子体密度的增高，表面的充电效应将导致鞘层厚度变薄、表面电位下降以及注入剂量增加，而介质的厚度对鞘层特性的影响则相对较小. 关键词： 等离子体浸没离子注入 脉冲鞘层 绝缘介质 充电效应     

超短超强激光导引及对电子加速的影响

使用粒子模拟程序对30 fs超短超强激光在均匀与抛物型两种密度分布等离子体中的传输, 以及在稳定传输状态下尾场的电子注入与加速形成的电子能谱进行了模拟与分析. 固定入射激光束斑尺寸, 在(0.4-2)×10¹⁹/cm³等离子体密度范围, 对比分析了归一化峰值强度从1-6范围的激光脉冲在上述两种密度分布等离子 体中传输时激光束斑尺寸的演化, 结果表明抛物型分布的等离子体密度通道能够对超短超强脉冲实现良好的导引, 有利于高能电子加速. 对于较高密度情况,即使在均匀等离子体中依靠相对论自聚 焦等机制也可以实现良好的自导引传输,有利于实验简化以及产生更大电量的加速电子.     

用离焦4f差分干涉仪测量等离子体壳层电子密度

 将环型横向剪切干涉仪置于两个镜头之间,由此设计出一种新型的离焦4f差分干涉仪,该干涉仪同时具有分离光路的剪切量和条纹空间频率分别可调的优点以及共光路结构的稳定性和易于调节的优点,使得在测量大密度梯度等离子体的密度分布时,可以在不降低空间分辨率的条件下仍保证干涉条纹可读。在DPF装置上进行了实验,获得了等离子体壳层的干涉图样,计算了等离子体的径向电子密度分布,在内电极端面上方测量到的最高电子密度约为1.2×10¹⁹ cm^-3,外围等离子体壳层的电子密度约为2×10¹⁸ cm^-3。     

等离子体源离子注入鞘层随时空演化的数值模拟

在等离子体源离子注入装置中(PSⅡ),靶被直接放入均匀等离子体源中,并在其上加负高压脉冲,从而使靶的周围形成了一个只存在离子的等离子体鞘层,离子以较高速度注入靶中。利用冷流体方程和泊松方程组成的非线性方程组对一维平面几何鞘层时空演化过程进行数值模拟,所采用的负高电势脉冲波形为方波和梯形波,得到了电子密度、离子密度、电势分布的时空演化曲线,并首次对梯形波下降沿时间内鞘层时空演化作了详细讨论。     

空心圆管端点附近等离子体源离子注入过程中鞘层的时空演化

等离子体源离子注入过程中，鞘层的演化规律直接影响到离子注入到材料中的深度进而影响材料表面的性质和结构，对材料的不同部位这种影响是不同的.利用无碰撞两维流体动力学模型，研究了有限上升时间的电压脉冲作用下，共轴放置附加零电极的半无限空心圆管端点附近等离子体源离子注入过程中，鞘层的时空演化规律.通过计算得到了鞘层内随时间变化的电势分布和离子密度分布，计算了端点附近材料表面处的离子流密度分布和注入剂量分布随时间的变化规律.计算机模拟结果显示了空心圆管内部、外部及端点表面处的离子流密度分布和注入剂量分布存在很大差异.     

电磁脉冲在实验室等离子体中传播时间的实验研究

利用矢量网络分析仪，对频域9—11 GHz的电磁脉冲在实验室稳态无磁场等离子体中传播时间的问题进行了实验研究.实验发现当等离子体密度在0.65—1.43×10¹¹ cm^-3范围内时，电磁脉冲通过该等离子体传播的时间将会小于该电磁脉冲在真空中传播同样距离所需要的时间，在密度约为1.10×10¹¹ cm^-3时，这两个时间差会出现一个极值.进一步的研究表明在此密度范围内，非磁化Xe等离子体中的电磁波色散关系将不再成立. 关键词： 电磁脉冲 脉冲传播时间 等离子体密度 色散关系     

Specific absorbed fractions of electrons and photons for Rad-HUMAN phantom using Monte Carlo method

The specific absorbed fractions(SAF) for self- and cross-irradiation are effective tools for the internal dose estimation of inhalation and ingestion intakes of radionuclides. A set of SAFs of photons and electrons were calculated using the Rad-HUMAN phantom, which is a computational voxel phantom of a Chinese adult female that was created using the color photographic image of the Chinese Visible Human(CVH) data set by the FDS Team. The model can represent most Chinese adult female anatomical characteristics and can be taken as an individual phantom to investigate the difference of internal dose with Caucasians. In this study, the emission of mono-energetic photons and electrons of 10 ke V to 4 Me V energy were calculated using the Monte Carlo particle transport calculation code MCNP. Results were compared with the values from ICRP reference and ORNL models. The results showed that SAF from the Rad-HUMAN have similar trends but are larger than those from the other two models. The differences were due to the racial and anatomical differences in organ mass and inter-organ distance. The SAFs based on the Rad-HUMAN phantom provide an accurate and reliable data for internal radiation dose calculations for Chinese females.     

平顶线结构光的中心检测算法及光刀平面标定

针对传统线结构光光刀平面标定方法测量精度不高,应用范围小的问题,提出基于平面标靶的线结构光系统光刀平面标定,对无激光的标靶图片进行迭代摄像机标定,有激光的标靶图片进行光刀平面标定.提出光强符合均匀分布的平顶激光检测中心算法,将平顶激光建模为矩形的台阶函数,估计背景亮度和前景亮度,确定亮条纹宽度,再将窗口内的有效像素参与重心计算,得到光条纹中心.用该算法对不同噪声及不同量块的图片进行处理,结果表明,处理后图像的均方根误差分别在0.149pixel和0.176pixel内,表明该算法抗噪声能力强、精度高.用该算法提取光条中心,计算光条在标靶上的位置,根据至少两个姿态下的光条中心三维点,基于最小二乘法拟合光刀平面.通过迭代摄像机标定和光刀平面标定,利用三角测量法,在立体视觉模型下获取物体的三维点云数据.实验测量两个距离为100.5mm的标准球,相机与标准球距离为500mm,比较两球心距离与标准距离,测得平均误差为0.236mm.表明平顶激光检测中心算法切实可行,光刀平面标定方法基本满足要求.     

脉冲激光与碲镉汞相互作用时的冲量耦合

在激光功率密度为４．０×１０８～５．０×１０９Ｗｃｍ－２的范围内，用冲击摆测量了ＮｄＹＡＧ脉冲激光（波长为１．０６μｍ，脉宽为１０ｎｓ）辐照大气中不同面积的ＨｇＣｄＴｅ样品时的冲量耦合系数。从理论上建立了等离子体爆轰模型，对激光结束后等离子体的膨胀过程进行了比较详细的描述，用此模型计算了不同能量的脉冲激光与不同面积的ＨｇＣｄＴｅ相互作用时的冲量耦合系数，计算值与测量值符合得较好。     

Influence of ion species ratio on grid-enhanced plasma source ion implantation

Grid-enhanced plasma source ion implantation (GEPSII) is a newly proposed technique to modify the inner-surface properties of a cylindrical bore. In this paper, a two-ion fluid model describing nitrogen molecular ions N_2^+ and atomic ions N^+ is used to investigate the ion sheath dynamics between the grid electrode and the inner surface of a cylindrical bore during the GEPSII process, which is an extension of our previous calculations in which only N_2^+ was considered. Calculations are concentrated on the results of ion dose and impact energy on the target for different ion species ratios in the core plasma. The calculated results show that more atomic ions N^+ in the core plasma can raise the ion impact energy and reduce the ion dose on the target.     

葛根素与牛血清白蛋白相互作用的研究

应用荧光光谱法研究了生理条件下(pH7.4)葛根素(PUE)与牛血清白蛋白(BSA)的相互作用。结果表明,葛根素对BSA荧光的猝灭机制属于形成复合物的静态猝灭过程,求得其猝灭常数为7.29×1012 L·mol-1·s-1,结合常数为5.04×104 L·mol-1;根据Frster非辐射能量转移理论,测得葛根素在BSA中的结合位置与色氨酸残基间的距离为3.35 nm;探讨了葛根素对蛋白质空间结构的影响及其相互作用机理;考察了体内某些共存金属离子对葛根素与BSA结合作用的影响。     

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采用了数值模拟与实验结合的方法研究了用于模拟放射性固体废物玻璃固化的非转移弧型等离子体炬的电、热特性。基于包括电弧室和开放空间在内的3D 模型得到了电弧等离子体和等离子体射流的温度场。根据计算结果,电弧室内的最高温度位于第一阳极内,达到41.77×10 K;弧电压的计算值高于实测值,二者之间的差异随着电流强度的增大而逐渐减小。采用该等离子体炬熔融模拟废物的实验发现,所确定的等离子体炬到炉底的距离能够满足废物熔融的要求,与计算的结果相符合。上述结果表明,数值模拟的结果可以作为等离子体炉工程设计的依据,并可以用作进一步分析等离子体炉炉膛内工艺过程的输入条件。     

Validation of Monte Carlo simulation of 6 MV photon beam produced by Varian Clinac 2100 linear accelerator using BEAMnrc code and DOSXYZnrc code

The Monte Carlo model for the photon-beam output from the Varian Clinac 2100 linear accelerator was validated to compare the calculated to measured PDD and beam dose profiles The Monte Carlo calculation method is considered to be the most accurate method for dose calculation in radiotherapy. The objective of this study is to build a Monte Carlo geometry of Varian Clinac 2100 linear accelerator as realistically as possible. The Monte Carlo codes used in this work were the BEAMnrc code to simulate the photons beam and the DOSXYZnrc code to examinate the absorbed dose in the water phantom. We have calculated percentage depth dose (PDD) and beam profiles of the 6 MV photon beam for the 6 × 6 cm², 10 × 10 cm² and 15 × 15 cm² field sizes. We have used the gamma index technique for the quantitative evaluation to compare the measured and calculated distributions. Good agreement was found between calculated PDD and beam profile compared to measured data. The comparison was evaluated using the gamma index method and the criterions were 3% for dose difference and 3 mm for distance to agreement. The gamma index acceptance rate was more than 97% of both distribution comparisons PDDs and dose profiles and our results were more developed and accurate. The Varian Clinac 2100 linear accelerator was accurately modeled using Monte Carlo codes: BEAMnrc and DOSXYZnrc codes package.     

Metastable state of three-component two-temperature plasma and fireball problem

It has been shown that like-charged particles inside electroneutral plasma can be attracted to each other, in contrast with non-electroneutral plasma considered in the literature, where such particles electrostatically repulse when they have any distance between them. We have calculated an analytical formula for the free energy of electroneutral three-component two-temperature plasma, from the basis of the Poisson–Boltzmann electrostatic equation. It is shown that free energy has a local minimum when the temperature of electrons exceeds 2000 K, when the quantity of electrons is less than 20% of the total quantity of negatively charged particles, when the temperature of ions is 300 K and when the distance between ions is several Debye radii. Plasma of a specified structure, temperature and density can mimic a fireball substance, in contrast with, for example, two-component isothermal plasma which has no minimum free energy at any interparticle distance.     

Ab initio intermolecular potential energy surfaces for the Ar–NCCN van der Waals complexes

The intermolecular potential energy surface of complex pairing argon with cyanogen molecule (NCCN) was calculated using the coupled cluster with single and double and perturbative triple excitations (CCSD(T)) with aug-cc-pvdz basis set extended with a set of mid-bond (3s3p2d1f1g) functions. The interaction energies were calculated by the supermolecular approach with the full counterpoise correction for the basis set superposition error. The calculated potential energies were fitted to an analytical expression. The calculated Ar–NCCN potential energy surface shows a global minimum at 3.35 Å, the distance between argon and centre of mass of cyanogen, for the T-shaped geometry and two local minimum at distance of 5.54 Å for the linear geometry on one side of cyanogen. Finally, the interaction second virial coefficients were calculated using the fitted potential energy surface and were compared with those obtained by the parameters of the Beattie–Bridgeman equation of states of pure argon and cyanogens fluids, approximately.