共查询到20条相似文献,搜索用时 15 毫秒
1.
D. P. Kozlenko S. V. Trukhanov E. V. Lukin I. O. Troyanchuk B. N. Savenko 《The European Physical Journal B - Condensed Matter and Complex Systems》2007,58(4):361-365
The crystal and magnetic structures of the oxygen deficient manganites
La0.7Sr0.3MnO3-d (d = 0.15, 0.20) have been studied by means
of powder neutron diffraction over the 0–5.2 GPa pressure and 10–290 K
temperature ranges. La0.7Sr0.3MnO2.85 exhibits a coexistence
of rhombohedral
and tetragonal (I4/mcm) crystal structures and below
Tg ~ 50 K a spin glass state is formed.
La0.7Sr0.3MnO2.80 exhibits a tetragonal (I4/mcm) crystal structure.
Below Tg ~ 50 K a phase separated magnetic state is formed,
involving coexistence of C-type AFM domains with spin glass domains. In both
compounds the crystal structure and magnetic states remain stable upon
compression. The factors leading to the formation of different magnetic
states in La0.7Sr0.3MnO3-d (d = 0.15, 0.20) and their specific
high pressure behavior, contrasting with that of the stoichiometric
A0.5Ba0.5MnO3 (A = Nd, Sm) compounds showing pressure-induced
suppression of the spin glass state and the appearance of the FM state, are analysed. 相似文献
2.
J. Badro J.P. Itié A. Polian 《The European Physical Journal B - Condensed Matter and Complex Systems》1998,1(3):265-268
X-ray diffraction (XRD) experiments have been carried out on quartz-like GaPO4 at high pressure and room temperature. A transition to a high pressure disordered crystalline form occurs at 13.5 GPa. Slight
heating using a YAG infrared laser was applied at 17 GPa in order to crystallize the phase in its stability field. The structure
of this phase is orthorhombic with space group Cmcm. The cell parameters at the pressure of transition are a
=7.306?, b
=5.887? and c
=5.124?.
Received: 7 October 1997 / Received in final form: 17 November 1997 / Accepted: 18 November 1997 相似文献
3.
A. Sacchetti M. Weller H. R. Ott Y. Ōnuki 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,66(3):307-313
We report a study of the low-temperature high-pressure phase diagram of the intermetallic compound PrCu2, by means of molecular-field calculations and 63,65Cu nuclear-quadrupole-resonance (NQR) measurements under pressure. The pressure-induced magnetically-ordered phase can be
accounted for by considering the influence of the crystal electric field on the 4f electron orbitals of the Pr3+ ions and by introducing a pressure-dependent exchange interaction between the corresponding local magnetic moments. Our experimental
data suggest that the order in the induced antiferromagnetic phase is incommensurate. The role of magnetic fluctuations both
at high and low pressures is also discussed. 相似文献
4.
F. Morales M. Monteverde M. Núñez-Regueiro 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,65(4):511-514
We measure electrical transport on networks of single wall nanotube of different origin as a function of temperature T, voltage V
and pressure P. We observe Luttinger liquid (LL) behavior, a conductance ∝Tα and a dynamic conductance ∝Vα. We observe a sample dependent P variation of the α parameters, interpreted as Fermi level changes due to pressure induced
charge transfer. We show how, through standard four-leads and crossed configuration methods, it is possible to determine αbulk and αend, respectively. We study and discuss the pressure and doping level dependences of the number of channels N, the LL parameter g
and the intra-rope tube-tube coupling constant U within a phenomenological model. 相似文献
5.
K. Araki T. Goto Y. Nemoto T. Yanagisawa B. Lüthi 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,61(3):257-259
The temperature dependence of the elastic constants in
Tb3Ga5O12 was measured and analysed with a simple crystal
field model. The magneto-elastic coupling constants have been deduced from
this experiment. The coupling constant gΓ5, related to the
c44 mode, is anomalously large. These coupling constants are important
for the interpretation of the phonon Hall effect. 相似文献
6.
The melting temperatures of H2, D2; N2 and CH4 are analysed. The computed results are in very good agreement with the experimental data in each solid. Further, the analysis
indicates the presence of the melting maximum in these solids. 相似文献
7.
In the present work, we developed a new kind of electrorheological (ER) materials, metal cations modified amorphous TiO2 gels. The static yield stress of Sn4+ modified amorphous TiO2 gel based ER fluid with a volume fraction = 38% reaches 26.2 kPa at E = 3.5 kV/mm. The result shows that metal cations can significantly enhance the ER activity of amorphous TiO2 gels. We then proposed a novel ER effect mechanism (metal cations enhanced polarization mechanism) to clarify the experimental results. We believe that it is the metal cations that enhanced the polarization of the polar groups (-OH) which results in the corresponding enhancement of the interfacial polarization. 相似文献
8.
H. He W. Y. Zhang 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,61(4):457-463
The spin-states of cobalt based perovskite compounds depend sensitively
on the valence state and local crystal environment of Co ions and the
rich physical properties arise from strong coupling among charge, spin,
and orbital degrees of freedom. While extensive studies have been carried
out in the past, most of them concentrated on the isotropic compound
LaCoO3. In this paper, using the unrestricted Hartree-Fock approximation
and the real-space recursion method, we have investigated the competition
of various magnetically ordered spin-states of anisotropic double-layered
perovskite Sr2Y0.5Ca0.5Co2O7. The energy
comparison among these states shows that the nearest-neighbor
high-spin-intermediate-spin ferromagnetically ordered state is the relevant
magnetic ground state of the compound. The magnetic structure and sizes of
magnetic moments are consistent with the recent experimental observation. 相似文献
9.
M. V. Gorev V. S. Bondarev S. I. Raevskaya I. N. Flerov M. A. Malitskaya I. P. Raevskii 《Bulletin of the Russian Academy of Sciences: Physics》2016,80(9):1046-1050
Temperature dependences of specific heat Cp(T) and coefficient of thermal expansion ;(T) for Na0.95Li0.05NbO3 sodium-lithium niobate ceramic samples are investigated in the temperature range of 100–800 K. The Cp(T) and α(T) anomalies at T3 = 310 ± 3 K, T2 = 630 ± 8 K, and T1 = 710 ± 10 K are observed, which correspond to the sequence of phase transitions N ? Q ? S(R) ? T2(S). The effect of heat treatment of the samples on the sequence of structural distortions was established. It is demonstrated that annealing of the samples at 603 K leads to splitting of the anomaly corresponding to the phase transition Q → R/S in two anomalies. After sample heating to 800 K, the only anomaly is observed in both the Cp(T) and ;(T) dependence. Possible mechanisms of the observed phenomena are discussed. 相似文献
10.
11.
J. P. Marques F. Parente P. Indelicato 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2007,41(3):457-465
In this paper, we used the multiconfiguration Dirac-Fock method to compute with high precision the influence of the hyperfine
interaction on the [Ar]
P0 level lifetime in Zn-like ions for stable and some quasi-stable isotopes of nonzero nuclear spin between Z=30 and Z=92. The
influence of this interaction on the
[Ar]
P
P0 separation energy is also calculated for the same ions. 相似文献
12.
T. Okazaki T. Shimada K. Suenaga Y. Ohno T. Mizutani J. Lee Y. Kuk H. Shinohara 《Applied Physics A: Materials Science & Processing》2003,76(4):475-478
Electronic properties of Gd@C82 metallofullerene peapods, (Gd@C82)n@SWNTs, were investigated by electron energy-loss spectroscopy (EELS), scanning tunneling microscopy and spectroscopy (STM/STS),
and field-effect transistor (FET) transport measurements. The results indicate that the electronic structure of Gd@C82 metallofullerene peapods is completely different from that of intact single-walled nanotubes (SWNTs). For example, Gd@C82-peapod-FETs show ambipolar behavior which is not observed in the empty SWNT-FETs under our experimental conditions. Furthermore,
in semiconducting nanotubes the band gap can be varied from ∼0.5 to ∼0.1 eV using inserted Gd@C82 endohedral metallofullerenes with a spatial periodicity of 1.1 to 8.0 nm, depending on the density of the fullerenes. The
present findings suggest that metallofullerene peapods may point the way toward novel electronic devices.
Received: 6 September 2002 / Accepted: 25 October 2002 / Published online: 10 March 2003
RID="*"
ID="*"Corresponding author. Fax: +81-52/789-1169, E-mail: noris@cc.nagoya-u.ac.jp 相似文献
13.
I. A. Leonidov O. N. Leonidova L. A. Perelyaeva R. F. Samigullina S. A. Kovyazina M. V. Patrakeev 《Physics of the Solid State》2003,45(11):2183-2188
The spinel structure of lithium titanate Li4Ti5O12 is refined by the Rietveld full-profile analysis with the use of x-ray and neutron powder diffraction data. The distribution and coordinates of atoms are determined. The Li4Ti5O12 compound is studied at high temperatures by differential scanning calorimetry and Raman spectroscopy. The electrical conductivity is measured in the high-temperature range. It is shown that the Li4Ti5O12 compound with a spinel structure undergoes two successive order-disorder phase transitions due to different distributions of lithium atoms and cation vacancies (□, V) in a defect structure of the NaCl type: (Li)8a[Li0.33Ti1.67]16dO4 → [Li□]16c[Li1.33Ti1.67]16dO4 → [Li1.33□0.67]16c[Ti1.67□0.33]16dO4. The low-temperature diffusion of lithium predominantly occurs either through the mechanism ... → Li(8a) → V(16c) → V(8a) → ... in the spinel phase or through the mechanism ... → Li(16c) → V(8a) → V(16c) → ... in an intermediate phase. In the high-temperature phase, the lithium cations also migrate over 48f vacancies: ... Li(16c) → V(8a, 48f) → V(16c) → .... 相似文献
14.
A.-S. Rüetschi D. Jaccard 《The European Physical Journal B - Condensed Matter and Complex Systems》2009,67(1):43-49
High pressure resistivity measurements of the organic compound (TMTTF)2BF4 have been performed in a newly developped Bridgman cell providing good pressure conditions on a wide pressure range. For
the first time in this compound a zero resistance superconducting state is observed between 3 and 4 GPa. At temperatures above
the superconducting transition, the resistivities of the two high quality samples show a different behavior. One sample, provides
indications for a magnetic quantum critical point at the maximum of Tc, whereas in the other antiferromagnetic spin-fluctuations are present above Tc. 相似文献
15.
The elastic, dynamical, and electronic properties of cubic LiHg and Li3Hg were investigated based on first-principles methods. The elastic constants and phonon spectral calculations confirmed the mechanical and dynamical stability of the materials at ambient conditions. The obtained elastic moduli of LiHg are slightly larger than those of Li3Hg. Both LiHg and Li3Hg are ductile materials with strong shear anisotropy as metals with mixed ionic, covalent, and metallic interactions. The calculated Debye temperatures are 223.5 K and 230.6 K for LiHg and Li3Hg, respectively. The calculated phonon frequency of the T2g mode in Li3Hg is 326.8 cm?1. The p states from the Hg and Li atoms dominate the electronic structure near the Fermi level. These findings may inspire further experimental and theoretical study on the potential technical and engineering applications of similar alkali metal-based intermetallic compounds. 相似文献
16.
Vasily Lavrentiev Jiri Vacik Hiroshi Naramoto Kazumasa Narumi 《Applied Physics A: Materials Science & Processing》2009,95(3):867-873
The structure transformation occurring in fullerene film under bombardment by 50 keV C60+ cluster ions is reported. The Raman spectra of the irradiated C60 films reveal a new peak rising at 1458 cm−1 with an increase in the ion fluence. This feature of the Raman spectra suggests linear polymerization of solid C60 induced by the cluster ion impacts. The aligned C60 polymeric chains composing about 5–10 fullerene molecules have been distinguished on the film surface after the high-fluence
irradiation using atomic force microscopy (AFM). The surface profiling analysis of the irradiated films has revealed pronounced
sputtering during the treatment. The obtained results indicate that the C60 polymerization occurs in a deep layer situated more than 40 nm below the film surface. The deep location of the C60 polymeric phase indirectly confirms the dominant role of shock waves in the detected C60 phase transformation. 相似文献
17.
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19.
A. Geddo Lehmann C. Sanna N. Lampis F. Congiu G. Concas L. Maritato C. Aruta A. Yu. Petrov 《The European Physical Journal B - Condensed Matter and Complex Systems》2007,55(4):337-345
Thin films of La0.7Sr0.3MnO3 were grown by
molecular beam epitaxy on (001)LaAlO3 crystals. High resolution X-ray
diffraction analysis proves the presence of twins in the films at room
temperature, showing that the twin structure of the substrate which forms at
the
ferroelastic transition at TF = 813 K
served as a template for the film microstructure. Magnetic measurements
indicate a thermomagnetic irreversibility which is ascribed to the quenched
disorder related to twinning and discussed in terms of coexisting
ferromagnetic and spin disordered regions connected with the undeformed
domain cores and strained domain walls respectively. 相似文献
20.
E. Govea-Alcaide I. García-Fornaris P. Muné R. F. Jardim 《The European Physical Journal B - Condensed Matter and Complex Systems》2007,58(4):373-378
Measurements of the electrical resistivity as a function
of temperature, ρ(T), for different values of applied
magnetic field, Ba (0 ≤ Ba ≤ 50 mT), were performed in
polycrystalline samples of Bi1.65Pb0.35Sr2Ca2
Cu3O10+δ subjected to different uniaxial compacting
pressure (UCP). We have found appreciable differences in the grain
orientation between samples by using X-ray diffractometry. From
the X-ray diffraction patterns performed, in powder and pellet
samples, we have estimated the Lotgering factor along the (00l)
direction, F(00l). The results indicate that F(00l)
increases ~23% with increasing UCP suggesting that grains
of these samples are preferentially aligned along the c-axis,
which is parallel to the compacting direction. The resistive
transition of the samples have been interpreted in terms of the
thermally activated flux-creep model. In addition, the effective
intergranular pinning energy, U0, have been determined for
different applied magnetic field. The magnetic field dependence of
U0, for Ba > 8 mT, was found to follow a H- α
dependence with α = 0.5 for all samples. The analysis of the
experimental data strongly suggested that increasing UCP results
in appreciable changes in both the grain alignment and the grain
connectivity of the samples. We have successfully interpreted the
data by considering the existence of three different
superconducting levels within the samples: the superconducting
grains, the weak-links, and the superconducting clusters. 相似文献