基于SiPM和TCMPC的时间分辨拉曼散射测量技术研究

报道了一种基于硅光电信增管(SiPM)的时间相关多光子计数(TCMPC)技术并将其应用于时间分辨拉曼散射测量。相比于常规基于光电倍增管(PMT)或单光子雪崩二极管(SPAD)的时间相关单光子(TCSPC)技术,由于SiPM可以分辨信号脉冲的具体光子数,基于SiPM的TCMPC技术消除了信号脉冲包含的光子数必须小于等于1的限制,光子计数效率提高了10倍以上,大大节省了测量时间。此外,多光子测量比单光子测量能够得到更好的时间分辨率,时间分辨拉曼散射系统的仪器响应函数(IRF)从单光子81.4 ps缩短至双光子59.7 ps,因而可以用更窄的时间门限抑制荧光本底等噪声对拉曼散射测量的影响。使用TCMPC技术测量CCl₄在0.5和1.5 p.e.两个不同光子数阈值的拉曼峰的峰本比,后者较高的光子数阈值能进一步降低SiPM暗计数噪声的影响,增加了拉曼信号测量的信噪比,测量得到的CCl₄ 459 cm-1拉曼峰的峰本比是前者的6.4倍。将所述新的拉曼散射测量技术与基于PMT和锁相放大器(LIA)的传统拉曼散射测量技术进行了比较研究,前者由于可以使用仅有数十皮秒的测量门限,可以有效抑制荧光、环境杂散光和SiPM暗计数等噪声的影响,所得光谱具有更好的峰本比,测得CCl₄的459 cm-1拉曼峰和Si的一阶拉曼峰的峰本比分别是后者的3.9倍和5.5倍。     

A Compact Violet Diode Laser-Based Fluorescence Lifetime Microscope

We have constructed a time-correlated single-photon counting (TCSPC) microscope system using a pulsed violet-laser diode for measuring fluorescence lifetimes below 1 ns. These compact; cool, and fast-pulsed laser diodes are much more suitable for lifetime measurements than the traditional mode-locked lasers used in the past. The laser source (LDH-400, PicoQuant GmbH) is mounted on an optical table above the microscope, and the laser beam is directed into an Olympus BX-60 microscope by means of a dichroic beamsplitter set at 45 degrees. The system operates in backscattering mode with the fluorescence emission passing back through the dichroic beamsplitter and focused into a 100 mm focal length monochromator with a PMT detector. This prototype instrument is compact (80 × 70 × 70 cm) and is nearly fully computer controlled by means of a SPC-730 (Becker & Hickl) PC card. We include preliminary results showing the instrument response function (IRF) of the system, and some of the factors have been adjusted to minimize the temporal width of the IRF. The instrument has been validated using a series of standard fluorophores at different emission wavelengths.     

极微弱脉冲光强度稳定控制技术

实际测量输出光强度随时间变化的随机过程是一个慢过程.将光衰减过程分为固定衰减和可变衰减两部分,设计制作了一种实时监控系统,通过调节自动反馈控制可变衰减器,使得末端固定衰减器的输出脉冲中,单光子脉冲出现的概率等于17.6%,多光子脉冲出现的概率低于2%,保持平均光子输出速率波动不大于0.1%,为量子密码术提供了稳定的准单光子源.     

纠缠光子法绝对定标光电探测器量子效率的研究

为了应对国际上“坎德拉”新定义的动向,开展了利用纠缠光子法测量光电探测器量子效率的研究,并建立了测量装置。装置采用351.1 nm连续激光抽运BBO晶体产生纠缠光子场,然后通过双通道门控计数器组成的符合测量系统在702.2 nm和788.7 nm两个波长点对光电倍增管的量子效率进行了测量。同时对单光子脉冲信号获取、噪声抑制及提取、符合时间特性、偶然符合、暗背景计数和器件透过率等影响测量结果的关键因素进行了实验分析并给出了修正分量,最终在两个波长点量子效率测量不确定度小于0.7%。     

Photon-assisted electronic structure and transport for a quantum dot

This paper investigates theoretically the electronic structure and transport of a two-level quantum dot irradiated under a strong laser field at low temperatures. Using the method of Keldysh equation of motion for nonequilibrium Green functions, it examines the time-averaged density of states and conductance for the system with photon polarization parallel with and perpendicular to the tunnelling current direction respectively. It is demonstrated that, by analysing some numerical examples, more photon sidebands resonance states and multi- and single-photon transitions are found when diagonal matrix elements dominate the interaction, while the electronic transitions due to multiphoton absorption are more or less suppressed when off-diagonal interaction dominates.     

Prototype of readout electronics for the LHAASO KM2A electromagnetic particle detectors

The KM2A(one kilometer square extensive air shower array) is the largest detector array in the LHAASO(Large High Altitude Air Shower Observatory) project. The KM2 A consists of 5242 EDs(Electromagnetic particle Detectors) and 1221 MDs(Muon Detectors). The EDs are distributed and exposed in the wild. Two channels, anode and dynode, are employed for the PMT(photomultiplier tube) signal readout. The readout electronics designed in this paper aims at accurate charge and arrival time measurement of the PMT signals, which cover a large amplitude range from 20 P.E.(photoelectrons) to 2×10~5 P.E. By using a "trigger-less" architecture, we digitize signals close to the PMTs. All digitized data is transmitted to DAQ(Data Acquisition) via a simplified White Rabbit protocol.Compared with traditional high energy experiments, high precision of time measurement over such a large area and suppression of temperature effects in the wild become the key techniques. Experiments show that the design has fulfilled the requirements in this project.     

Predicting intense-field photoionization of atoms and molecules from their linear photoabsorption spectra in the ionization continuum

We report a new approach to intense-field photoionization that is based on the ad hoc assumption that m photons of energy arriving within a typical electronic response time are effectively equivalent to a single photon of energy . The heuristic model contains no adjustable parameters and unifies apparent multiphoton and field aspects. Moreover, nonsequential, suppressed and above-threshold ionization phenomena become readily understandable. Predicted ionization intensities are in satisfactory agreement with available experimental data ranging from C₆H₆ to Ne^{3 +} , from femtosecond to nanosecond laser pulses, and from ultraviolet to infrared laser radiation.Received: 20 January 2004, Published online: 17 August 2004PACS: 32.80.Rm Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states) - 32.80.Wr Other multiphoton processes - 42.50.Hz Strong-field excitation of optical transitions in quantum systems; multiphoton processes; dynamic Stark shift     

Evaluation of polarization entanglement generated by spontaneous parametric downconversion using photon number counting

Spontaneous parametric downconversion (SPDC) is widely used to generate entangled photon pairs; however, multi-pair emissions degrade the quality of the entanglement. We numerically evaluate polarization-entangled photon pairs created by SPDC. The effects of multi-pair emission events on the visibility of two-photon interference and on the fidelity (the probability overlap for ideal and real states) are analyzed using single-photon detectors that can count the number of incoming photons and discard multiphoton events. Compared with conventional threshold single-photon detectors, photon-number resolving single-photon detectors have higher fidelity for the same or lower visibility.     

光子计数成像技术及其应用

介绍光子计数实时图像采集实验系统，其中的高亮度增益的光子成像头通过超强光力中继透与高帧频电荷耦合器摄像机耦合；分析和介绍了单光子成像模式下系统工作的受限条件和多光子工作模式下系统的主要综合性能指标－读出噪声的测定方法。文中给出在自适应光学弱光波前传感中的应用，光子噪声分布规律以及光的波粒二象性实验验证等例子。     

超导单光子探测器件直流特性研究

超导单光子探测技术是基于超薄超导薄膜的非平衡态热电子效应的一种新型的单光子探测方法。超导单光子探测器(SNSPD)的计数率可达到GHz,时间抖动小于100ps,因而在未来量子通信系统中有着广阔的应用前景。介绍了NbN超导单光子探测器件的工作原理和器件超导性能测试系统;测试了超导单光子探测器件的电阻-温度、电流-电压等特性。并对测试结果进行了分析和讨论。     

Enhancement of ultraweak photon emission with 3 MHz ultrasonic irradiation on transplanted tumor tissues of mice

We investigated photon emissions of various bio-samples which were induced by ultrasonic stimulation. It has been reported that ultrasonic stimulations induced the thermal excitation of the bio-tissues. After ultrasonic stimulation, any measurement of photon radiation in the visible spectral range has not been carried out yet. The instruments consisted of electronic devices for an ultrasonic generator of the frequency 3 MHz and a photomultiplier tube (PMT) system counting photons from bio-tissues. The transplanted tumor tissues of mice were prepared for the experiments and their liver and spleen tissues were also used for the controls. It was found that the continuous ultrasonic stimulations with the electrical power 2300 mW induced ultraweak photon emissions from the tumor tissues. The number of induced photon was dependent of the type of the tissues and the stimulation time intervals. The level of photon emission was increased from the mouse tumor exposed to the ultrasonic stimulations, and the changes were discriminated from those of the spleens and livers.     

基于单光子脉冲时间随机性的光量子随机源

提出了一种基于单光子脉冲时间随机性的光量子随机源。利用衰减成单光子态的光强恒定光源和一个单光子探测器产生单光子随机脉冲,通过连续比较单光子随机脉冲序列中相邻两个脉冲的时间间隔来提取随机位。通过设计高速响应的微通道板单光子探测器和基于现场可编程门阵列(FPGA)的随机位提取电路,获得了超过10Mbit/s的随机位产生速率。通过采用恒比定时和对计数时钟倍频的方法提高时间间隔的测量精度,从而减小随机位序列的相关系数。当光量子随机源的随机位产生速率在10kbit/s以下时,所获得的二进制随机位序列的相关系数小于0.001。运用随机性测试程序ENT和DIEHARD对所获的随机位序列进行测试,测试结果表明序列的随机性非常好且不需要后续处理,完全满足真随机数的标准。     

光子计数深度获取系统误差机理研究和矫正

采用两路光子时间到达点构建光纤式光子计数伪随机码深度获取系统.为了研究降低深度误差的方法,以高斯函数为激光回波脉冲,计算瞬时概率密度函数,引入"时间行走"效应数学模型,推导深度误差克拉美罗下限.随着激光回波能量的增大,深度误差先降低再增大,并且码长越长,深度误差越小.采用理论推导的累积分布函数,生成光子时间到达点,蒙特卡洛仿真伪随机序列光子探测过程,结果大于理论数值模拟,符合克拉美罗下界原理.17组标定实验表明:由于目标表面特性的不同而导致探测到激光回波中光子数的浮动,该浮动引发光子"时间行走"效应,并带来伪随机码深度获取系统的互相关函数的整体偏移.采用数值拟合方程拟合不同光子计数比例值下的深度误差,测量得到的光子计数比例值,代入拟合的矫正方程,矫正后的深度均方误差下降至1cm.     

A Feasible Add-On Upgrade on a Commercial Two-Photon FLIM Microscope for Optimal FLIM-FRET Imaging of CFP-YFP Pairs

Fluorescence lifetime imaging microscopy (FLIM) based on time-correlated single photon counting (TCSPC) is a widely used method for fluorescence resonance energy transfer (FRET). Here we report a feasible add-on approach to upgrade a commercial two-photon FLIM microscope into a single-photon FLIM microscope which provides optimal FLIM-FRET imaging of FRET pairs consisting of cyan fluorescent proteins (CFPs) as the donor and yellow fluorescent proteins (YFPs) as the acceptor. The capability of the upgraded system is evaluated and discussed, and the imaging performance of the system is demonstrated using FLIM-FRET experiments with a representative CFP-YFP FRET pair (mCerulean-mCitrine).     

基于APD线列的单光子探测计数研究

单光子探测系统可以对单个光子进行探测;探测系统含有探测部分、淬灭电路部分和计数部分;探测部分主要由工作在盖革模式下的雪崩光电二极管组成;在盖革模式下的雪崩光电二极管发生雪崩后不能自然停止,淬灭部分主要为了主动抑制雪崩电流,快速降低雪崩电压,以达到提高探测效率,降低错误计数的目的;APD线列产生多个光子脉冲信号,计数部分的主要功能是对多路光子脉冲信号进行计数、显示并且可以控制每路APD的比较电压,保证每路APD淬灭电路的正常工作。     

甲醛的态选择性多光子电离研究

我们在XeCl准分子激光多光子电离甲醛分子的研究中,获得了甲醛经过2+1和2+2光子共振激发过程而产生的母体离子和高能离解通道的离子CO⁺。在电子轰击和单光子电离中占优势的低能阈离解通道离子HCO⁺,由于态选择性激发的结果而未出现。 关键词：     

用于激光等离子体中X射线测量的单光子计数型CCD的标定

 介绍了单光子计数型CCD的工作原理。实验选择参数准确的X射线放射源前向辐照CCD的像元面,计数由此产生;通过积分获得X射线的强度分布,在CCD处于单光子计数状态下,扣除本底信号,得到该型CCD产生一个计数所需的光子能量,约6.453 eV。标定了该型CCD的探测效率。结果表明：在单光子计数型CCD的有效能区内,对于不同能量的入射光子,其探测效率不同,在5.3 keV处获得最高探测效率66％;随着能量的增大,探测效率降低。标定结果可为激光等离子体研究中定量测量X射线光谱提供实验参考。     

Quantum information-holding single-photon router based on spontaneous emission

In this paper, we propose a single-photon router via the use of a four-level atom system coupled with two one-dimensional coupled-resonator waveguides. A single photon can be directed from one quantum channel into another by atomic spontaneous emission. The coherent resonance and the photonic bound states lead to the perfect reflection appearing in the incident channel. The fidelity of the atom is related to the magnitude of the coupling strength and can reach unit when the coupling strength matches g _a = g _b . This shows that the transfer of a single photon into another quantum channel has no influence on the fidelity at special points.     

Response of photomultiplier tubes to background cosmic radiation

The properties of photomultiplier tubes (PMTs) have been investigated experimentally. The flux of cosmic rays has been used as a source of signals detected directly by a PMT (without a scintillator). The number of detected events versus the size of the PMT’s transparent front window has been studied. To this end, modified FEU-167 multipliers (FEU-167M) have been fabricated in which all parameters have been kept unchanged except for the size of the front window, which has been decreased. It has been found that the number of detected signals is roughly proportional to the surface area of the window. Hence, a signal induced by background cosmic rays arises in the glass of the PMT’s front screen. This circumstance should be taken into consideration when operating with different PMTs.     

单光子探测技术

近年来,以量子密钥分配为代表的各种量子信息技术应用获得了飞速发展,这些应用对单光子探测器的性能提出了非常苛刻的要求,以光电倍增管和雪崩光电二极管为代表的传统单光子探测器件已经无法满足需求。在此背景下,出现了以超导单光子探测器为代表的新型低温单光子探测器件,其性能比现有商用单光子探测器有了本质性的提升。本文综述了迄今为止各种类型的单光子探测器,并指出各自在量子信息技术应用中的优势和不足之处以及发展方向。