Natural radiative lifetimes in the2S1/2 and2D5/2,3/2 sequences of aluminum

Natural radiative lifetimes have been measured for the 3s ² ns ² S _1/2 (n≦10) and 3s ² nd ² D _5/2,3/2 (n≦11) sequences of aluminum using pulsed laser excitation of an atomic beam. The investigated states were populated from the ground configuration using UV pulses of wavelength down to 210 nm produced by a Nd: YAG- or an excimer-pumped dye-laser system. TheS-state lifetimes increase regularily with increasing principal quantum number but this is not the case for theD sequence.     

Constants of quenching of 5s 22 D 5/2, 3/2 CdII levels by argon

Constants of quenching of the CdII ion Beutler levels by argon were experimentally determined. Excited cadmium ions in the 5s ^{2 2} D _{5/2, 3/2} states were produced by sputtering metal cadmium with alpha-particles at a temperature of 240°C. The quenching constants for the 5s ^{2 2} D _5/2 and 5s ^{2 2} D _3/2 CdII ion levels were found to be 1.3×10^?10 and 1.8×10^?10 cm³ s^?1, respectively.     

Lifetime measurements of Rydberg states in the 6snd 1 D 2-series of BaI

We have measured the lifetimes of 10 Rydberg states from 6s8d ¹ D ₂ to 6s 17d ¹D₂ in the Ba I spectrum by time-resolved recording of the exponential decay of the resonance fluorescence in an atomic beam. The excitation was performed by use of two pulsed dye lasers simultaneously pumped by one nitrogen laser. The lifetime results differ strongly from Coulomb approximation calculations and show deviations from a(n ^*)³-dependence.     

Study of the relaxation of metastable 6p 3 2 D 3 2/0 states of bismuth atoms in a bismuth-vapor laser

A universal absorption technique for studying the kinetics of relaxation of atomic states in the afterglow of a repetitively pulsed discharge in metal vapor lasers is proposed. It uses the measurement of the absorption of narrowband emission of a tunable dye laser and numerical simulation of absorption. The relaxation of metastable 6p ^{3 2} D ₃ ^2/0 states of Bi atoms in the afterglow of a 472.2-nm bismuth vapor laser was studied. The prepulse values of the concentration of metastable atoms n _m were not higher than 10¹¹ cm^?3 and did not impede the improvement of laser characteristics. The afterpulse values of n ^m were ～10¹³ cm^{? 3}.     

Three-photon resonance enhanced excitation spectrum of atomic thallium

We present first measurements on the resonance enhanced three-photon excitation in thallium, using a Nd:YAG laser pumped dye laser in conjunction with a thermionic diode ion detector. The even-parity 6s²ns²S_1/2 (15 ? n ? 31) and nd ²D_5/2 (13 ? n ? 42) Rydberg states have been observed. The measured level energies reveal a dynamic shift from the photoabsorption values, which is decreasing with increasing n, while the asymmetry in the line profile is observed to be increasing with increasing n. In addition, an autoionising level (sp²⁴P_3/2) adjacent to the ionization threshold has been observed and quantitatively analyzed using the Fano’s photoionization cross-section relation for an isolated autoionising resonance.     

Studying(\bar cs) spectroscopy in\bar vN collisions

Charmed strange meson neutrinoproduction is investigated. TheD _s ^? (1970) antineutrino production rate is measured. Two higher \((\bar cs)\) states are seen in the decay channels γD _s ^* (2110) andD ^*K, respectively.     

Lifetimes and oscillator strengths in the triplet system of ZnI

Selective laser excitation was used to measure the radiative lifetimes of the ZnI triplet states 4sns ³ S ₁(n=5–7) and 4snd ³ D ₃,³ D ₂ and³ D ₁(n=4–6). These states were excited from the metastable 4s4p ³ P states, which were collisionally populated in an atomic beam. The values are compared with the results of other experimental methods (beam-foil, pulsed electron excitation, Hanle effect) and with theoretical calculations. The corresponding oscillator strengths are discussed with respect to the astrophysical determination of the Zn photospheric abundance.     

Study of cation tracer diffusion in NaF

Cation tracer diffusion coefficients were measured in pure NaF crystals in the intrinsic ionic conductivity range (876–970 °C). The results can be rationalized satisfactorily in terms of contributions to the observed Na tracer diffusivities arising from both free vacancies and neutral vacancy pairs, the latter contribution amounting to about 53 per cent of the total Na diffusion at the highest measuring temperature. The best-fit defect parameters derived in an earlier conductivity study [21] from this laboratory on similar NaF crystals give for the free vacancy contribution D_v^*(Na) = 4·25 exp (?2·21 eV/kT) cm²s^?1. A combination of these D_v^*(Na) values with the present diffusion data yields for the vacancy-pair contribution D_p^*(Na) = 1·15 × 10⁸exp (?4·04 eV/kT) cm²s^?1. Comparison of the present findings with published values of the anion tracer diffusion coefficient in NaF showed that D_p^* (F) is 2·3 to 4·4 times larger than D_p^*(Na) over the temperature range of our observations, the difference between the two contributions increasing with decreasing temperature. When approximate account is taken of the temperature-dependence of the two pair correlation factors, this last result indicates that the anion jumps into the vacancy pair occur with a higher frequency, and increasingly so at lower temperatures, than do those involving the cations.     

Radiative decay and autoionization in the4 D-states of the 3d 94s5s configuration in CuI

The CuI 3d ⁹4s5s ⁴ D-states, which lie above the ionization limit, were populated by stepwise collisional and laser excitation. With respect to their total angular momentum, the⁴ D-states have completely different decay modes. Whereas the lifetimesτ(⁴ D _7/2)=8.2(4)·10^?9s andτ(⁴ D _1/2)=7.9(6)·10^?9 s are determinrd by radiative transitions and were measured by time-resolved spectroscopy, the lifetimesτ(⁴ D _5/2)=1.59(6)·10^?12s andτ(⁴ D _3/2)=1.28(5)·10^?12s are due to autoionization and were deduced from the widths of the excitation signals observed by ion detection.     

Mössbauer study of the hyperfine and magnetic properties of organo-di-iron electron reservoirs containing a polyaromatic bridging ligand

Organo di-iron electron reservoirs Fe(CP^*)₂(Ar) ⁿ⁺ withn=2, 1, 0, where Cp^* is C₅(CH₃)₅ and where Ar are the following bridges: biphenyl, dihydrophenanthrene, triphenylene, have been studied by Mössbauer spectroscopy in the solid state. Complexes withn=2, with 36e^? in the coordination spheres of the metals, exhibit the usual diamagnetic behaviour of 18e^?, Fe^II mono-iron systems. Complexes withn=1, 37e^?, are delocalized mixed valence (Fe^IIFe^I) with a spin 1/2; the magnetic hyperfine interaction, measured under an external field, shows equal delocalization of the 37^th e^? on the two iron centers and the two bridging carbon atoms of the biphenylene. Complexes withn=0, formally with 38e^?, have a practically temperature-independent quadrupole splitting, and isomer shift values which constrast with the expected behaviour of independent Fe^I, 19e^? centers. This indicates that the 37^th and 38^th electrons are mostly located on the polyaromatic bridge. Spectra obtained in an external field show a negligible magnetic hyperfine interaction and support this conclusion. In the case of biphenyl and dihydrophenanthrene bridges, this electron localization can be related to a strong intramolecular chemical coupling, evidenced by other spectroscopic and X-ray data [1].     

Approximation of the electron excitation cross sections for triplet states excited from the 23 S 1 metastable state in helium

The method of approximated four-parameter representation of the electron-impact cross sections for a helium atom excited from the 2³ S ₁ metastable state into higher triplet states is applied and discussed. The approximation consists in interpolation over the whole set of the cross section values for each helium atomic level measured in our experiments and reported by other researchers. The approximation parameters and the cross sections calculated using these parameters for the maxima of the corresponding excitation functions are presented for 19 triplet levels of the S, P, and D HeI series with n=2–10. The interpolated values are compared to the theoretical cross sections. The serial regularities were investigated for the S, P, and D levels studied and a decrease in the cross sections for excitation from the given metastable state within each series, described by the approximate law Q=Cn ^?5, was revealed. Validity of the similarity relationship and the Bethe approximation for cross sections in the 2³ S?n ³ P series was verified. It is shown that the cross sections for a triplet level excitation from the 2³ S ₁ metastable state exceed the corresponding values for excitation from the ground state of helium by a factor of approximately 10³ for n=2 and 3 and 10 2 for the higher levels. It is concluded that the proposed method of representation of the cross sections for the electron-impact excitation of triplet levels from the metastable state increases accuracy and more importantly, reliability of the final results.     

Charmed particle production in hadron-hadron collisions

In the framework of Quark-Gluon-String Model developed recently in ITEP we calculate spectra of charmed particlesD,D _s,Λ_c,Ξ_c,Ω_c in hadron-hadron collisions taking into account the decays ofS-wave resonances like D^*,D_s ^*,Σ_c,Σ_c ^*,Ξ_c ^*,Ξ_c ^′, and Ω_c ^*. We describe the bulk of the existing data onD, D^*, adΛ _c production in πp andpp collisions and predict the yield of charmed particlesin Σ^?p and Ξ^?p reactions at hyperon beam energies of 340 GeV/c and 600 GeV/c. Because of significant production of baryon resonances our predictions for unfavored fragmentation differ from predictions of other models which do not take resonance production into account.     

Investigation of the mass dependence of self-diffusion coefficients by molecular dynamics calculations: binary and ternary isotopic mixtures of atoms

Extensive molecular dynamics calculations have been used to study for the first time systematically the dependence of the self-diffusion coefficients D_i (i = 1, 2, 3) in binary and ternary atomic isotopic mixtures on the particle mass ratios m*₂ = m ₂/m ₁ and m*₃ = m ₃/m ₁ at different reduced temperatures T* and reduced particle number densities n*, using a Lennard-Jones 12-6 potential and a hard-soft-spheres potential. In addition, the dependence of D_i values of binary mixtures on the mole fraction x ₁ = 1—x ₂ was also investigated for some thermodynamic states. The calculated values of D_i can be represented quantitatively by exponential estimates of the form D_i = D* _i (m*₂)^ex _i in the case of binary mixtures and D_i = D ⁰ _i (m*₂)^{ex _i} (m ₃)^{ext _i} in the case of ternary mixtures. D ⁰ _i are the self-diffusion coefficients in reference mixtures of mass ratios m*₂ = m*₃ = 1. The dependence of the exponents ex _i (m*₂, T*, n*, x ₁) of binary mixtures on m*₂, T*, n*, and x ₁ and the dependence of the exponents ext _i (m*₂, m*₃, n*) of equimolar ternary mixtures at T* = 1.8 on the exponents ex _i of the constituent binary mixtures and on m*₂, m*₃, and n* are discussed.     

Two-photon spectroscopy of ytterbium

Two-photon laser spectra of the Yb vapor have been obtained. Transitions to highly excited 4f¹⁴ 6sns¹S₀ and 4f¹⁴ 6snd ¹D₂ states are seen in direct two-photon excitation. Hybrid resonances involving 4f¹⁴ 6s6p ¹P⁰₁ and 4f¹⁴ 5d6s ³D₂ intermediate states lead to transitions to 4f¹⁴ 6sns¹S₀, 4f¹⁴ 6snp ³P⁰_2,1 and 4f¹⁴ 6snd ¹D₂ levels.     

Durees de vie des niveaux 1D2 ET 1S0 du magnesium

Radiative lifetimes of the excited n¹S₀ (n = 4, 5) and n¹D₂ (n = 3, 4) states in magnesium have been measured by time resolved fluorescence technique using two photon excitation.     

Study off o (995) resonance in the π0π0 decay channel

A high-statistics study of the π⁰π⁰-system produced in the π^- p→π⁰π⁰ n reaction at 38GeV/c has been carried out at the IHEP accelerator using the GAMS-2000 multiphoton spectrometer. A partial-wave analysis which includesS, D ₀, D_? andD ₊ waves has been performed in the |t|-range up to 1 (GeV/c)². TheS ^*/f ₀(980) resonance is seen as a dip in theS-wave amplitude at small |t|. A distinct peak with a mass of 997±5MeV and a width of 48±10MeV is observed in theS-wave at |t|>0.3 (GeV/c)². The production cross sections are measured.     

Ion storage technique for very long living states: The decay rate of the 5D 3/2 state of Ba II

The metastable 5D _3/2 state of Ba⁺ is used to demonstrate the possibility of the ion storage technique for the measurement of extremely long lived states. The ions are confined in a r.f. quadrupole trap and excited by a strong pulsed tunable dye laser to the 6P _1/2 state which partially decays into the 5D _3/2 state. Sampling of the time development of the ground state population leads to the determination of the 5D _3/2 decay rate. Using He as a buffer gas at a pressure of about 10^?6 mbar to initially store the ions, varying the gas density and extrapolating to zero pressure, we find for the lifetime \(\tau _{D_{3/2} } = 17.5 \pm 4s\) .     

He5 scattering states in the refined cluster function representation

As a first application of the refined cluster model reaction theory we calculated the scattering states of He⁵ using a specific ansatz for the nucleon-nucleon forces. He⁴-n and H³-d channels are considered only. Our results agree qualitatively with the experimental values if available; in particular we were able to explain the narrow resonance in theD _3/2 He⁴-n channel as a consequence of the strong coupling to theS _3/2 T-d channel.     

A refined potential energy function for the electronic ground state of H2Se

The potential energy surface for the electronic ground state of the hydrogen selenide molecule has been determined previously by Jensen and Kozin [J. Mol. Spectrosc. 160 (1993) 39] in a fitting to experimental data by means of the MORBID computer program. We report here a further refinement of this surface, also made with the MORBID program. With the refined potential surface, we can make predictions of rotation-vibration transition wavenumbers for H₂Se, D₂Se, and HDSe, and with these predictions we can assign weak spectra of these molecules. We assign here two very weak bands of HD⁸⁰Se, ν₁+ν₂+ν₃ and 2ν₁+ν₃. The refinement of the potential energy surface was made possible because (1) the number of vibrational states characterized experimentally for various isotopomers of H₂Se has approximately doubled since 1993, and (2) we now have access to larger computers with which we can fit energy spacings of states with J?8, whereas Jensen and Kozin could only use J?5. In the present work, we fitted rotation-vibration energy spacings associated with 24 vibrational states of H₂⁸⁰Se with v₁?6, v₂?3, and v₃?2; 11 vibrational states of D₂⁸⁰Se with v₁?2, v₂?3, and v₃?2, and 17 vibrational states of HD⁸⁰Se with v₁?3, v₂?3, and v₃?3. The input data set comprised 3611 energy spacings. In the fitting, we could usefully vary 29 potential energy parameters. The standard deviation of the fitting was 0.12 cm⁻¹ and the root-mean-square deviation for 49 vibrational term values was 0.59 cm⁻¹.     

Effects of final state interactions in B^ + \to D_S^ + \bar K^0 decay

We investigate the effects of final state interactions (FSI) contributions in the nonleptonic two body $B^ + \to D_S^ + \bar K^0$ decay, however the hadronic decay of $B^ + \to D_S^ + \bar K^0$ is analyzed by using “QCD factorization” (QCDF) method and final state interaction (FSI). First, the $B^ + \to D_S^ + \bar K^0$ decay is calculated via QCDF method and only the annihilation graphs exist in that method. Hence, the FSI must be seriously considered to solve the $B^ + \to D_S^ + \bar K^0$ decay and the D ⁰π⁺(D ⁰*ρ⁺), D ⁺π⁰(D ⁺*ρ⁰) and D ⁺η _c (D ⁺*J/ψ) via the exchange of K ^+(*), K ^0(*) and D _s ^+(*) mesones are chosen for the intermediate states. To estimate the intermediate states amplitudes, the QCDF method is again used. These amplitudes are used in the absorptive part of the diagrams. The experimental branching ratio of $B^ + \to D_S^ + \bar K^0$ decay is less than 8 × 10^?4 and the predicted branching ratio is 0.23 × 10^?9 in the absence of FSI effects and it becomes 6.74 × 10^?4 when FSI contributions are taken into account.