Doping dependence of charge order in electron-doped cuprate superconductors

Abstract

In the recent studies of the unconventional physics in cuprate superconductors, one of the central issues is the interplay between charge order and superconductivity. Here the mechanism of the charge-order formation in the electron-doped cuprate superconductors is investigated based on the t-J model. The experimentally observed momentum dependence of the electron quasiparticle scattering rate is qualitatively reproduced, where the scattering rate is highly anisotropic in momentum space, and is intriguingly related to the charge-order gap. Although the scattering strength appears to be weakest at the hot spots, the scattering in the antinodal region is stronger than that in the nodal region, which leads to the original electron Fermi surface is broken up into the Fermi pockets and their coexistence with the Fermi arcs located around the nodal region. In particular, this electron Fermi surface instability drives the charge-order correlation, with the charge-order wave vector that matches well with the wave vector connecting the hot spots, as the charge-order correlation in the hole-doped counterparts. However, in a striking contrast to the hole-doped case, the charge-order wave vector in the electron-doped side increases in magnitude with the electron doping. The theory also shows the existence of a quantitative link between the single-electron fermiology and the collective response of the electron density.     

Incommensurate spin-density modulation in a copper oxide chain compound with commensurate charge order

Neutron diffraction has been used to determine the magnetic structure of Na8Cu5O10, a stoichiometric compound containing chains based on edge-sharing CuO4 plaquettes. The chains are doped with 2/5 hole per Cu site and exhibit long-range commensurate charge order with an onset well above room temperature. Below TN=23 K, the neutron data indicate long-range collinear magnetic order with a spin-density modulation whose propagation vector is commensurate along, and incommensurate perpendicular to, the chains. Competing interchain exchange interactions are discussed as a possible origin of the incommensurate magnetic order.     

Vortex imaging in Co-doped BaFe2As2

We review superconducting vortex imaging in Co-doped BaFe₂As₂ by Bitter decoration and small-angle neutron scattering (SANS). At all measured fields a highly disordered vortex configuration is observed, which is attributed to strong pinning. Further support of this conclusion comes from the absence of a Meissner rim in decoration images obtained close to the sample edge. The evolution of the SANS scattering vector with increasing applied field indicates vortex lattice domains of (distorted) hexagonal symmetry. This is consistent with the decoration images which show small, six fold coordinated ordered vortex domains. The SANS scattered intensity is found to decrease rapidly with increasing field, exceeding the rate expected from estimates of the upper critical field. This is consistent with the large degree of vortex “lattice” disorder.     

Superfluid response in electron-doped cuprate superconductors

We propose a weakly coupled two-band model with dx(2)(-y(2)) pairing symmetry to account for the anomalous temperature dependence of superfluid density rho(s) in electron-doped cuprate superconductors. This model gives a unified explanation to the presence of an upward curvature in rho(s) near T(c) and a weak temperature dependence of rho(s) in low temperatures. Our work resolves a discrepancy in the interpretation of different experimental measurements and suggests that the pairing in electron-doped cuprates has predominately dx(2)(-y(2)) symmetry in the whole doping range.     

Research trends in electron-doped cuprate superconductors

In this review, we look back on some intriguing and puzzling issues in electron-doped cuprate superconductors, such as electron-hole asymmetry, two types of carriers, quantum critical points, order-parameter symmetry, etc. The necessity of study on this family is invoked in comparison with the hole-doped counterparts from several aspects. The related progress, especially in last few years, has been outlined point to point, as well as other hot topics like the discovery of ambipolar superconductors, the applications in superconducting electronics, and the emergency of superconductivity in parent compounds. In perspective, the utilization of blooming advanced techniques, electric double layer transistor and combinatorial film deposition, will bring some new insights into the mechanism such as electron-doped cuprate superconductors.     

Tunneling spectroscopy and order parameter symmetry of hole- and electron-doped cuprate superconductors

In tunneling spectroscopy of superconductors the density of states close to the surface or the interface to an insulating tunneling barrier is probed. For d-wave superconductors the particle–hole coherence results in interesting new phenomena at surfaces such as the formation of bound surface states at the Fermi level by Andreev reflection due to a sign change of the order parameter field in different k -directions. The probing of these states represents a phase-sensitive experiment allowing the determination of the order parameter symmetry in superconductors. We summarize the present experimental status with respect to the study of high-temperature superconductors (HTS). We discuss theoretically predicted consequences of a dominating d-wave order parameter in the hole-doped HTS on their tunneling spectra as well as on the physics of high-temperature superconductor Josephson junctions. A comparison of the tunneling spectra obtained for hole- and electron-doped HTS leads to the conclusion that the former have a d-wave, whereas the latter most likely have an anisotropic s-wave order parameter. We also address some unsettled questions related to the presence of a state with broken time-reversal symmetry at surfaces and interfaces of d-wave HTS and discuss specific features of d-wave tunnel junctions that have been predicted theoretically but still not been confirmed in experiments.     

Incommensurate spin fluctuations in hole-overdoped superconductor KFe2As2

A neutron scattering study of heavily hole-overdoped superconducting KFe2As2 revealed a well-defined low-energy incommensurate spin fluctuation at [π(1 ± 2 δ),0] with δ = 0.16. The incommensurate structure differs from the previously observed commensurate peaks in electron-doped AFe2As2 (A = Ba, Ca, or Sr) at low energies. The direction of the peak splitting is perpendicular to that observed in Fe(Te,Se) or in Ba(Fe,Co)2As2 at high energies. A band structure calculation suggests interband scattering between bands around the Γ and X points as an origin of this incommensurate peak. The perpendicular direction of the peak splitting can be understood within the framework of multiorbital band structure. The results suggest that spin fluctuation is more robust in hole-doped than in electron-doped samples, which can be responsible for the appearance of superconductivity in the heavily hole-doped samples.     

Electronic Raman response in electron-doped cuprate superconductors

The electronic Raman response in the electron-doped cuprate superconductors is studied based on the t-t^′-J model. It is shown that although the domelike shape of the doping dependent peak energy in the B2g symmetry is a common feature for both electron-doped and hole-doped cuprate superconductors, there are pronounced deviations from a cubic response in the B1g channel and a linear response in the B2g channel for the electron-doped case in the low energies. It is also shown that these pronounced deviations are mainly caused by a nonmonotonic d-wave gap in the electron-doped cuprate superconductors.     

电子型掺杂铜氧化物超导体准粒子激发谱研究

文中工作采用t-t′-t″-J模型研究了电子型掺杂铜氧化物超导体在超导序和反铁磁序共存情况下的准粒子激发谱,分别计算了在欠掺杂区、最佳掺杂区和过掺杂区的谱权重,计算结果与角分辨光电子谱实验结果符合较好.     

Quasiparticle scattering interference in electron-doped cuprate superconductors

By considering the nonmonotonic d-wave gap effect, the energy and momentum dependence of quasiparticle scattering interference is studied in the presence of a single impurity. It is shown that the pattern of the quasiparticle scattering peaks in the full Brillouin zone of electron-doped cuprate superconductors is very different from that in the hole-doped case described by the Octet model. This difference is the result of the nonmonotonic d-wave superconducting gap in the electron-doped case. As the energy increases, the position of the local peaks in the Brillouin zone moves rapidly. In particular, the characteristic peaks of the electron-doped cuprate superconductors appear between the antinodal and nodal directions, unlike in the hole-doped case.     

Superconductivity at 22 K in Co-doped BaFe2As2 crystals

Here we report bulk superconductivity in BaFe1.8Co0.2As2 single crystals below Tc=22 K, as demonstrated by resistivity, magnetic susceptibility, and specific heat data. Hall data indicate that the dominant carriers are electrons, as expected from simple chemical reasoning. This is the first example of superconductivity induced by electron doping in this family of materials. In contrast with cuprates, the BaFe2As2 system appears to tolerate considerable disorder in the FeAs planes. First principles calculations for BaFe1.8Co0.2As2 indicate the interband scattering due to Co is weak.     

Incommensurate magnetic order in TbTe3

We report a neutron diffraction study of the magnetic phase transitions in the charge-density wave (CDW) TbTe(3) compound. We discover that in the paramagnetic phase there are strong 2D-like magnetic correlations, consistent with the pronounced anisotropy of the chemical structure. A long-range incommensurate magnetic order emerges in TbTe(3) at T(mag1) = 5.78 K as a result of continuous phase transitions. We observe that near the temperature T(mag1) the magnetic Bragg peaks appear around the position (0, 0, 0.24) (or its rational multiples), that is fairly close to the propagation vector (0,0,0.29) associated with the CDW phase transition in TbTe(3). This suggests that correlations leading to the long-range magnetic order in TbTe(3) are linked to the modulations that occur in the CDW state.     

Evolution of spin dynamics in electron-doped cuprate superconductors

Within the kinetic energy driven superconducting mechanism, the evolution of the magnetic excitations of the electron-doped cuprates in the superconducting state is studied. It is shown that there is a broad commensurate low energy magnetic scattering peak, while the magnetic resonance energy is located among this broad commensurate low energy scattering range. This broad commensurate low energy magnetic scattering disperses outward into a continuous ring-like incommensurate magnetic scattering at high energy.     

H+ irradiation effect in Co-doped BaFe2As2 single crystals

We report the suppression of the critical temperature T_c in single crystalline Ba(Fe_1?xCo_x)₂As₂ at under-, optimal-, and over-doping levels by 3 MeV proton irradiation. T_c decreases and residual resistivity increases monotonically with increasing the dose. The low-temperature resistivity does not show the upturn in contrast with the α-particle irradiated NdFeAs(O,F), which suggests that proton irradiation introduces nonmagnetic scattering centers. Critical scattering rates for all samples obtained by three different ways are much higher than that expected in s±-pairing scenario based on inter-band scattering due to antiferro-magnetic spin fluctuations.     

Fluctuation-exchange study of antiferromagnetism in disordered electron-doped cuprate superconductors

On the basis of the Hubbard model, we extend the fluctuation-exchange (FLEX) approach to investigating the properties of the antiferromagnetic (AF) phase in electron-doped cuprate superconductors. Furthermore, by incorporating the effect of scatterings due to the disordered dopant atoms into the FLEX formalism, our numerical results show that the antiferromagnetic transition temperature, the onset temperature of pseudogap due to spin fluctuations, the spectral density of the single particle near the Fermi surface, and the staggered magnetization in the AF phase as a function of electron doping can consistently account for the experimental measurements.