X‐ray fluorescence induced by standing waves in the grazing‐incidence and grazing‐exit modes: study of the Mg–Co–Zr system

The characterization of Mg–Co–Zr tri‐layer stacks using X‐ray fluorescence induced by X‐ray standing waves, in both the grazing‐incidence (GI) and the grazing‐exit (GE) modes, is presented. The introduction of a slit in the direction of the detector improves the angular resolution by a factor of two and significantly improves the sensitivity of the technique for the chemical characterization of the buried interfaces. By observing the intensity variations of the Mg Kα and Co Lα characteristic emissions as a function of the incident (GI mode) or detection (GE mode) angle, it is shown that the interfaces of the Si/[Mg/Co/Zr]_×30 multilayer are abrupt, whereas in the Si/[Mg/Zr/Co]_×30 multilayer a strong intermixing occurs at the Co‐on‐Zr interfaces. An explanation of this opposite behavior of the Co‐on‐Zr and Zr‐on‐Co interfaces is given by the calculation of the mixing enthalpies of the Co–Mg, Co–Zr and Mg–Zr systems, which shows that the Co–Zr system presents a negative value and the other two systems present positive values. Together with the difference of the surface free energies of Zr and Co, this leads to the Mg/Zr/Co system being considered as a Mg/Co_xZr_y bi‐layer stack, with x/y estimated around 3.5.     

Spectroscopy and dynamics of neutral atoms in superfluid helium

Optical spectra and radiative lifetimes of neutral atoms in superfluid helium have been studied. The absorption and emission spectra of Ag, Mg, Yb, Al, Ga, and In were found to exhibit shifts and broadening typical of atoms residing in microscopic He bubbles, showing that this type of trapping is fairly general. The radiative lifetimes measured for these atoms are close to the free space values, indicating that the surrounding bubble hardly perturbs the electronic orbitals during photo emission. One exception observed in Sr is discussed, where competing autoionization substantially decreases the lifetime of a high excited triplet state. A transient non-bubble state with sharp, free atom like spectra is seen during the first few s after dispersion for many atomic species. The dynamics of this state are unusual, with for example very short radiative lifetimes measured for light alkali atoms.     

First observation of two-electron one-photon transitions in single-photon K-shell double ionization

Experimental evidence for the correlated two-electron one-photon transitions (1s(-2)→2s(-1)2p(-1)) following single-photon K-shell double ionization is reported. The double K-shell vacancy states in solid Mg, Al, and Si were produced by means of monochromatized synchrotron radiation, and the two-electron one-photon radiative transitions were observed by using a wavelength dispersive spectrometer. The two-electron one-photon transition energies and the branching ratios of the radiative one-electron to two-electron transitions were determined and compared to available perturbation theory predictions and configuration interaction calculations.     

Measurement of temperature, density, and particle transport with localized dopants in wire-array Z pinches

Axially localized NaF dopants are coated onto Al cylindrical wire arrays in order to act as spectroscopic tracers in the stagnated z-pinch plasma. Non-local-thermodynamic-equilibrium kinetic models fit to Na K-shell lines provide an independent measurement of the density and temperature that is consistent with spectroscopic analysis of K-shell emissions from Al and an alloyed Mg dopant. Axial transport of the Na dopant is observed, enabling quantitative study of instabilities in dense z-pinch plasmas.     

Spectroscopic diagnosis of the temperature profile of an Al:MgZ-pinch

We consider the question of how the temperature profile of a Z-pinch plasma can be determined and/or constrained by the requirement that its observed K-shell spectrum be replicated. As a case study we employ spatially integrated, time-resolved K-shell data obtained from the implosion of 30-wire Al:Mg alloy arrays on the Saturn driver at Sandia National Laboratories. Given the measured pinch size, its K-shell power and line intensities are compared with the predictions of a collisional-radiative-equilibrium plasma model whose temperature profile is varied in seeking agreement with the data. The Al data rules out a large range of possible temperature profiles, but two quite different temperature distributions can both match the measurements. These are: a uniform temperature, or, one with a sharply dropping temperature near the pinch outer edge. However, the measured ratio of the Mg α resonance lines to those of Al, even though time-integrated, excludes the possibility of a uniform temperature distribution     

Laser heating of solid matter by light-pressure-driven shocks at ultrarelativistic intensities

The heating of solid targets irradiated by 5 x 10(20) W cm(-2), 0.8 ps, 1.05 microm wavelength laser light is studied by x-ray spectroscopy of the K-shell emission from thin layers of Ni, Mo, and V. A surface layer is heated to approximately 5 keV with an axial temperature gradient of 0.6 microm scale length. Images of Ni Ly(alpha) show the hot region has 100 G bar light pressure compresses the preformed plasma and drives a shock into the solid, heating a thin layer.     

A radiochemical study on the existence of dineutron

A radiochemical study has been made to search for dineutron² n produced in the simultaneous two-neutron emission of the excited⁶He nuclei,⁶He^*, induced in the reaction of⁹Be+n→-⁶He^*+α with fast neutrons in a reactor. It was attempted to detect the radio-activity of²⁸Mg as a product of the reaction² n+²⁷Al→²⁸Mg+p. The²⁸Mg radioactivity observed in heterogeneous samples composed of the² n-producing target Be and the² n-detecting target Al separately was not found to be more than that of a side reaction,²⁷Al{(n, p)(n _th, γ)+(n _th, γ)(n, p)}²⁸Mg, whereas it clearly exceeded that of the side reaction in alloy samples made of Be and Al metals. The former experiment gives an upper limit of the production rate of the dineutron in the bound state 1×10^?7 per event of the simultaneous two-neutron emission. A tentative explanation for the excessive²⁸Mg radioactivity observed in the latter experiment is the following two-step process,⁹Be+n→⁶He+α and²⁷Al+⁶He→+²⁸Mg+α+p, rather than the process induced by the dineutron in a virtual state.     

Electron correlation effects in the valence band photoemission spectra of cooper dichloride

He I, He II and Al Kα photoemission measurements of the valence band of CuCl₂ are reported. The presence of the 3d⁸-like satellite indicates the strong correlation effects in the final state and the breakdown of the one-particle model. It is shown that the reduction of the satellite intensity in the valence band compared with the core hole emission is caused by the delocalization of the photo-hole. The satellite intensity in resonance with the super-Coster-Kronig decay is calculated.     

Anomalous photoluminescence and raman scattering behavior in heavily Mg+ ion-implanted InP

Mg⁺ ions were implanted into highly pure InP grown by the liquid encapsulated Czochralski (LEC) method in which the Mg concentration [Mg] was varied between 1×10¹⁵ cm^–3 and 3×10²⁰ cm^–3. Two annealing methods were used: furnace annealing (FA) up to 740° C and flash lamp annealing (rapid thermal annealing, RTA) up to 900° C. For characterization, photoluminescence (PL) spectra were measured between 2K and room temperature together with Raman scattering measurements at room temperature. An emission designated by g, which was attributed to a novel energy state of an isolated acceptor, was found to be produced for a rather low value of [Mg]. In addition, a broad emission denoted by [g–g], which was ascribed to acceptor-acceptor pairs, was observed below bound exciton emissions for moderate values of [Mg]. These features were quite similar to those previously observed in acceptor-doped GaAs when the background concentration of donors is extremely low. Two additional novel emissions located far below the band-to-acceptor emission were also obtained, and each showed a remarkable energy shift towards lower energy with increasing [Mg]. The binding energies of these emissions were estimated from the temperature dependence of PL spectra and the results suggest that they are complex-type radiative recombination centers, presumably donor-acceptor-type centers. A strong broad emission centered near the band-to-acceptor emission was observed for [Mg]=3×10²⁰ cm^–3. This observation indicates a formation of a new material between In, P and Mg, which was also attested by the appearance of a new TO-like Raman signal for [Mg] greater than 1×10¹⁹ cm^–3. A substantial difference of PL and Raman spectra was revealed for the two annealing methods, suggesting that the annealing behaviour of ion-implanted InP should be investigated more extensively in order to establish reliable annealing procedures.Dedicated to H.-J. Queisser on the occasion of his 60th birthday     

High energy x-ray satellites ofL 2,3 emission bands of Na,Mg, Al,and Si

The x-ray satellites found on the high energy sides of theL _2,3 emission bands of Na, Mg, Al, and Si have previously been attributed to the radiative decay of double ionization states. However, in some recent papers it has been proposed that the satellites in Al and Si may arise from the simultaneous radiative decay of a core ionization state and a volume plasmon. A detailed investigation of the high energy satellites of theL _2,3 x-ray emission bands of Na, Mg, Al, and Si have been made for incident electron energies from 500 eV to 5 keV and the results compared with the double ionization theory. Plasmon involvement is also considered. The present results lend additional support to the first interpretation; namely, that the satellites arise from the radiative decay of atoms with a double vacancy in theL _2,3 (2p) shell and not from the plasma phenomenon.     

利用时间分辨Ar的K壳层发射光谱诊断内爆靶丸芯区电子温度的时间演化过程

在神光Ⅱ装置上的内爆实验中,通过在充氘气(D2)的靶丸中掺入氩(Ar)元素,利用晶体谱仪配条纹相机测量得到了内爆停滞阶段Ar的K壳层发射光谱随时间的变化。在实验中,观测到Ar的Heα,Heβ以及Lyα线发射,持续时间大约200ps。用Heα线与Lyα线强度比值来推断靶丸芯区电子温度。利用碰撞辐射模型,从理论上计算出Heα线与Lyα线强度比值随电子温度、数密度的变化。通过将实验上观测到的Heα线与Lyα线强度比与理论计算值相比较,获得了芯区电子温度随时间的演化。并计算比较了不同电子密度条件下推断出来的电子温度的差异,证明诊断电子温度的方法对电子数密度的变化不敏感。利用逃逸因子修正了自吸收效应,从计算的结果可以看出在目前的实验中Heα线和Lyα线是光学薄的。     

Ratio of single K-shell ionization cross section to double K-shell ionization cross section in heavy-ion-atom collisions

The spectra of Ti Kα X-rays induced by He, C, N and O ions were measured with the use of a Bragg crystal spectrometer. The ratios of the integrated hypersatellite to diagram-plus-satellite X-ray yields were obtained. The previously obtained data on Cr, Fe and Ni Kα X rays induced by N ions were also analysed. It is found that the double K-shell vacancy production cross section is proportional to Z⁴₁.     

Spatially-resolved spectroscopic diagnosing of aluminum wire array Z-pinch plasmas on QiangGuang-I facility

Spatially-resolved crystal spectrometers with a high spectral resolution are developed to diagnose K-shell x-ray radiation from Z-pinch plasmas. These diagnostic apparatuses are successfully applied to aluminum wire array Z-pinch experiments on QiangGuang-I facility, a driver with a pulsed current up to about 1.5 MA in 80 ns. Time-integrated experimental results show that the K-shell x-ray emission lines of aluminum Z-pinch plasmas are dominated by line emissions from helium-like ionisation state. Bright spots that might have higher electron temperature or density are produced randomly in location and size along the z-axis during implosions. According to the experimental data, the electron temperature and the ion density are estimated to be between 250 eV and 310 eV, and between 7.0×10¹⁹cm^-3 and 4.0×10¹⁹ cm^-3 respectively, while the ion temperature is inferred to be about 10.2 keV, which is much higher than the electron temperature.     

超热电子产生Kα辐射的参数影响

 超短超强激光与固体靶相互作用,可以产生大量的Kα特征谱线发射。这种Kα线光源在背光照相、医学成像和超快诊断等方面具有显著优势。为了寻求获得Kα线高产额的方法,利用ITS蒙卡模拟程序,对超短超强激光产生的超热电子在固体靶中产生的Kα线发射进行了模拟。系统研究了Kα线发射强度随出射角度、靶厚度和超热电子温度等参数的变化情况。研究发现在恒定的激光功率密度或超热电子温度下,存在最佳的靶厚度,使得Kα线光子产额最大,并用模拟结果对已有实验数据进行了解释。     

Cold collisions in strong laser fields: partial wave analysis of magnesium collisions

We have developed Monte Carlo wave function simulation schemes to study cold collisions between magnesium atoms in a strong red-detuned laser field. In order to address the strong-field problem, we extend the Monte Carlo wave function framework to include the partial wave structure of the three-dimensional system. The average heating rate due to radiative collisions is calculated with two different simulation schemes which are described in detail. We show that the results of the two methods agree and give estimates for the radiative collision heating rate for ²⁴Mg atoms in a magneto-optical trap based on the ¹S₀–¹P₁ atomic laser cooling transition.     

Measurements on diproton emission from the break-up channels of 23Al and 22Mg

Two-proton relative momentum distributions from the break-up channels ²³Al→p+p+²¹Na and ²²Mg→p+p+²⁰Ne at an energy of 60–70 A MeV have been measured together with two-proton opening angles at the projectile fragment separator beamline (RIPS) in the RIKEN Ring Cyclotron Facility. The results demonstrate the existence of diproton emission component from single-step ²He for highly excited ²³Al and ²²Mg.     

X-ray cross section in helium for electron capture to excited states by C6+ and O8+ ions in the continuum distorted-wave approximation

The projectile X-ray cross sections which are closely related to the total capture cross sections have been calculated in C⁶⁺ + He and O⁸⁺ + He collision processes. The calculated data for K-shell X-ray cross sections for capture to excited states are found to be in good agreement with the recent experimental findings and the existing theoretical calculations.     

Cluster radioactivity in xenon isotopes

Half-life time and branching ratio for cluster decay from various xenon isotopes are studied taking Coulomb and proximity potentials as interacting barrier. Inclusion of proximity potential reduces the height of potential barrier, which closely agrees with the experiments. It is found that⁴He,⁸Be,¹²C and¹⁶O emissions are well within the present upper limit for measurements (T _1/2 10³⁰ s). Our predicted half-life time values lie close to those values reported by Gupta and collaborators based on preformed cluster model (PCM) and also with those values reported by Poenaruet al based on ASAFM. The calculated half-life time shows that⁸Be from¹⁰⁸Xe and¹¹⁰Xe are most favourable for emission (T _1/2 ≈ 10⁸ s). LowestT ^1/2 value for⁸Be emission from¹⁰⁸Xe stress the role of doubly magic¹⁰⁰Sn daughter in cluster decay process. The logarithm of half-life time calculated for⁴He emission from¹¹⁰Xe is −0.39 s which is in good agreement with experimental value which is −0.40 s. Geiger-Nuttall plots for all clusters are studied and are found to be linear. Nuclear structure effect and shell effect are evident from the observed variation in slope and intercept of Geiger—Nuttall plots. It is found that neutron excess in the parent will slow down the cluster decay process.     

K-shell ionization cross section of aluminium induced by low-energy highly charged argon ions

Al K-shell X-ray yields are measured with highly charged Ar^q+ ions (q=12–16) bombarding against aluminium. The energy range of the Ar ions is from 180 to 380 keV. K-shell ionization cross sections of aluminium are also obtained from the yields data. The experimental data is explained within the framework of 2pπ -2pσ rotational coupling. When Ar ions with 2p-shell vacancies are incident on aluminium, the vacancies begin to reduce. Meanwhile, collisions against Al atoms lead to the production of new 2p-shell vacancies of Ar ions. These Ar 2p-shell vacancies will transfer to the 1s orbit of an Al atom via 2pπ-2pσ rotational coupling leading to the emission of a K-shell X-ray of aluminiun. A model is constructed based on the base of the above physical scenario. The calculation results of the model are in agreement with the experimental results.     

Dislocation emission from a crack under mixed mode loading studied by molecular statics

The dislocation emission surface in (k _I,?k _II,?k _III) space is calculated by means of atomistic simulations for the {111}?110? crack in Al. For each relevant combination of loading mode, the precise nature of the dislocations and of the emission process are determined. When appropriate, the analytic formulas proposed by Rice are used by calculating the unstable stacking energy including the effect of the mixed mode loading. Quantitative agreement with the full atomistic calculation is found in the case where dislocations glide in the crack plane. This clearly identifies when and how ab initio data can be introduced in the calculation.