Two-octave spectral broadening of subnanojoule Cr:forsterite femtosecond laser pulses in tapered fibers

Spectral broadening of femtosecond Cr:forsterite laser pulses is enhanced due to the use of tapered fibers. Supercontinuum generation with unamplified subnanojoule femtosecond Cr:forsterite laser pulses is observed for the first time. With 40-fs 0.6-nJ pulses of 1.25-μm Cr:forsterite laser radiation coupled into a tapered fiber having a taper waist diameter of about 2 μm and a taper waist length of 90 mm, we observed the spectra spanning more than two octaves at the output of the fiber in the regime of anomalous group-velocity dispersion. This result opens the way for the creation of compact femtosecond Cr:forsterite laser plus tapered fiber systems for optical metrology and biomedical applications. Received: 23 October 2001 / Accepted: 16 January 2002 / Published online: 14 March 2002     

All-solid-state Cr:forsterite laser generating 14-fs pulses at 1.3 mum

We report the generation of 14-fs pulses at 1.3mum with 80-mW average power at 100-MHz repetition rate by an all-solid-state Kerr-lens mode-locked Cr:forsterite laser. The laser spectrum covers wavelengths of 1230-1580 nm, with a FWHM of 250 nm. Since 1.3-mum wavelengths are close to the zero dispersion wavelength of Cr:forsterite, higher-order dispersion is the main factor limiting pulse durations. We use specially designed and fabricated double-chirped mirrors in combination with high-index PBH71 prisms to compensate for the intracavity dispersion over almost 300 nm.     

Spectral superbroadening of subnanojoule Cr:Forsterite femtosecond laser pulses in a tapered fiber

Spectral superbroadening of subnanojoule femtosecond Cr:forsterite laser pulses is demonstrated for the first time in experiments with a tapered fiber. Coupling 40-fs 0.6-nJ pulses of 1.25-μm Cr:forsterite laser radiation into a tapered fiber with a taper waist diameter of about 2 μm and a taper waist length of 90 mm, we observed the spectra spanning more than two octaves at the output of the fiber. These experimental results open new horizons for the creation of compact femtosecond systems based on Cr:forsterite lasers and tapered fibers for optical metrology and biomedical applications.     

Microjoule supercontinuum generation by stretched megawatt femtosecond laser pulses in a large-mode-area photonic-crystal fiber

Microjoule supercontinuum generation is demonstrated using a large-mode-area photonic-crystal fiber (PCF) pumped by an amplified stretched-pulse output of a mode-locked Cr:forsterite laser. A PCF with a mode area of 380 μm² is employed to transform 300-fs Cr:forsterite laser pulses with a peak-power of a few megawatts into a supercontinuum radiation with a spectrum spanning from 700 to 1800 nm and a total energy of 1.15 μJ.     

Two-photon absorption-induced effects in femtosecond coherent anti-Stokes Raman-scattering microspectroscopy of silicon photonic components

We study the effects related to two-photon absorption (TPA) in the microspectroscopy of the silicon photonic components based on coherent anti-Stokes Raman scattering (CARS) of femtosecond pulses. With 300-fs pulses of 1.24-μm Cr:forsterite laser radiation delivering pump and probe fields and a frequency-shifted soliton output of a large-mode area photonic-crystal fiber employed as a Stokes field, pronounced TPA effects have been observed in the CARS microspectroscopy of silicon components for pump-pulse intensities exceeding 10 GW/cm².     

Femtosecond Cr:forsterite laser diode pumped by a double-clad fiber

We present a compact, all-solid-state femtosecond Cr:forsterite laser. The laser is pumped by diodes through a double-clad fiber. Kerr-lens mode locking is initiated and stabilized by a semiconductor saturable-absorber mirror with a single InGaAs quantum well. This system generates transform-limited 80-fs pulses near 1.3microm . An average power of 68 mW with fluctuation of much less than 1% is obtained with 3.8 W of absorbed pump power. The stability, efficiency, compactness, and potential for scaling to higher power of this system make it an attractive short-pulse source for applications.     

Self-starting mode locking in a Cr:forsterite laser by use of non-epitaxially-grown semiconductor-doped silica films

We demonstrate RF sputtered, non-epitaxially-grown semiconductor nanocrystallite-doped silica films for mode locking a Cr:forsterite laser. We controlled the size and the optical properties of the nanocrystallites by varying the ratio of InAs to SiO(2) during fabrication. Femtosecond pump-probe measurements were performed to characterize the nonlinear optical properties of these films, revealing their lower saturation fluences. Using the InAs-doped silica films as saturable absorbers permitted self-starting Kerr-lens mode locking (KLM), generating pulses of 25-fs duration with 91-nm spectral bandwidth at 1.3 microm . We also describe saturable-absorber mode-locked operation without KLM and investigate its dependence on intracavity dispersion.     

Broadly tunable femtosecond Cr:LiSAF laser

We demonstrate wavelength tunability of femtosecond pulses over a range of more than 50 nm from a diode-pumped Cr:LiSAF laser. The mode-locking mechanism can be explained by soliton mode locking that is started and stabilized by a broadband semiconductor saturable-absorber mirror designed for low loss over the full reflection bandwidth of the underlying Bragg mirrors, which ultimately limits tunability. We obtain 45-fs pulses at 105-mW average output power and a maximum mode-locked average output power of 125 mW with 60-fs pulses.     

Pump-probe nonlinear absorption spectroscopy of molecular aggregates using chirped frequency-shifted light pulses from a photonic-crystal fiber

Photonic-crystal fibers provide efficient nonlinear-optical transformations of femtosecond Cr: forsterite laser pulses, delivering linearly chirped frequency-shifted broadband light pulses optimized for pump-probe nonlinear absorption spectroscopy of molecular aggregates. The blue-shifted output of a photonic-crystal fiber with a spectrum stretching from 530 to 680 nm is used to probe one-and two-exciton bands of thiacarbocyanine J aggregates in a polymer film excited by femtosecond second-harmonic pulses of the Cr: forsterite laser.     

Microstructure fibers as frequency-tunable sources of ultrashort chirped pulses for coherent nonlinear spectroscopy

Microstructure fibers are shown to allow the creation of new tunable sources for femtosecond nonlinear spectroscopy. These fibers provide a high efficiency of frequency upconversion of regeneratively amplified femtosecond pulses of a Cr:forsterite laser, permitting the generation of subpicosecond anti-Stokes pulses with a smooth temporal envelope and a linear positive chirp. These pulses from a microstructure fiber were used to measure the spectra of coherent anti-Stokes Raman scattering (CARS) of toluene solution by cross-correlating these pulses with the femtosecond second-harmonic output of the Cr:forsterite laser in boxcars geometry (XFROG CARS). PACS 42.65.Wi; 42.81.Qb     

Generation of 0.1-TW 5-fs optical pulses at a 1-kHz repetition rate

A compact all-solid-state femtosecond Ti:sapphire oscillator?amplifier system using no grating-based pulse stretcher produces 20-fs, 1.5-mJ pulses at a 1-kHz repetition rate. The pulses are subsequently compressed in a hollow-fiber chirped-mirror compressor. The system delivers bandwidth-limited 5-fs, 0.5-mJ pulses at 780 nm in a diffraction-limited beam.     

Direct generation of 81 nJ pulses and external compression to a subpicosecond regime with a 4.9 MHz chirped-pulse multipass-cavity Cr⁴⁺:forsterite oscillator

We report direct generation of 81 nJ chirped pulses from a room-temperature, Kerr lens mode-locked Cr??:forsterite oscillator operating at 1258 nm. To increase the pulse energy, the pulse repetition rate of the short x-type resonator was lowered from 143 to 4.9 MHz by the addition of a q-preserving multipass cavity, which provided an additional effective optical path length of 59.4 m. The duration of the chirped pulses was around 5.5 ps with a spectral width of 21 nm. The pulses were externally compressed to 607 fs by using a diffraction grating pair. To our knowledge, this is the highest reported pulse energy directly generated from a room-temperature mode-locked Cr??:forsterite laser.     

Diode-pumped 10-fs Cr3+:LiCAF laser

We demonstrate 10-fs pulses from a diode-pumped, soft-aperture Kerr lens mode-locked Cr3+:LiCAF laser with a spectral bandwidth of 150 nm and 40 mW of output power at a repetition rate of 110 MHz. For dispersion compensation, double-chirped mirrors and prisms are used. The pulses are characterized by use of spectral shearing interferometry.     

All-optically tunable waveform synthesis by a silicon nanowaveguide ring resonator coupled with a photonic-crystal fiber frequency shifter

A silicon nanowaveguide ring resonator is combined with a photonic-crystal fiber (PCF) frequency shifter to demonstrate an all-optically tunable synthesis of ultrashort pulse trains, modulated by ultrafast photoinduced free-carrier generation in the silicon resonator. Pump-probe measurements performed with a 50-fs, 625-nm second-harmonic output of a Cr:forsterite laser, used as a carrier-injecting pump, and a 1.50-1.56-μm frequency-tunable 100-fs soliton output of a photonic-crystal fiber, serving as a probe, resolve tunable ultrafast oscillatory features in the silicon nanowaveguide resonator response.     

0.2-TW laser system at 1kHz

We have developed a 1-kHz repetition-rate Ti:sapphire laser system that can simultaneously generate high peak and average powers of 0.2TW and 4W, respectively. The laser system generates 4-mJ energy pulses with a 20-fs pulse width. We eliminated thermal lensing in the system by cooling the Ti:sapphire crystal to 125K. The output 20-fs pulses were fully characterized by use of the new technique of transient-grating frequency-resolved optical gating. We demonstrate experimentally that the pulse duration at the output is limited only by fifth-order dispersion.     

14-fs pulse generation in Kerr-lens mode-locked prismless Cr:LiSGaF and Cr:LiSAF lasers: observation of pulse self-frequency shift

Kerr-lens mode-locked Kr-laser-pumped Cr:LiSGaF and Cr:LiSAF lasers containing only two newly developed low-loss chirped mirrors instead of conventional dielectric resonator mirrors and generating pulses of widths as small as 14-fs with as much as 100 mW of average output power are reported. We report what is to our knowledge the first experimental observation of a pulse self-frequency shift in crystalline active media that are characteristic of such short pulses at megawatt intracavity peak powers. We also believe this phenomenon to be one of the significant limiting factors for pulse duration in femtosecond Cr:LiSAF-type lasers.     

420-MHz Cr:forsterite femtosecond ring laser and continuum generation in the 1-2-micrometre range

We demonstrate a chromium-doped forsterite femtosecond ring laser that generates 30-fs pulses at a 420-MHz repetition rate with nearly 500 mW of average power. The compact solid-state design and broad spectral output make this laser attractive for telecommunications applications in the 1.3-1.5-micrometre region. Additional spectral broadening of the laser output in highly nonlinear optical fiber leads to octave-spanning spectra ranging from 1.06 to 2.17 micrometre. The octave is reached at a level of 18 dB below the peak. The underlying optical frequency comb can be linked to existing optical frequency standards.     

Quantum-dot-based saturable absorber for femtosecond mode-locked operation of a solid-state laser

A quantum-dot-based saturable absorber has been demonstrated to initiate the generation of femtosecond pulses from a passively mode-locked solid-state laser. Control and tuning of the pulse duration from 58 ps to 158 fs was achieved. The 158 fs transform-limited pulses at 1280 nm are the shortest pulses that were produced from the Cr:forsterite laser passively mode locked by an InAs/InGaAs quantum-dot semiconductor saturable absorber mirror.     

Attosecond active synchronization of passively mode-locked lasers by balanced cross correlation

A balanced cross correlator, the optical equivalent of a balanced microwave phase detector, is demonstrated. Its use in synchronizing an octave-spanning Ti:sapphire laser and a 30-fs Cr:forsterite laser yields 300-attosecond timing jitter measured from 10 mHz to 2.3 MHz. The spectral overlap between the two lasers is strong enough to permit direct detection of the difference in carrier-envelope offset frequency between the two lasers.     

High-average-power, 1-MW peak-power self-mode-locked Ti:sapphire oscillator

We describe a novel self-mode-locked Ti:sapphire ring laser that produces 13-fs pulses with peak powers exceeding 1 MW, pulse energies of 13 nJ, and average mode-locked output powers of 1.5 W at a cavity repetition frequency of 110 MHz. A complete resonator analysis describing the optimum mode-locking configuration is presented, together with fringe-resolved autocorrelation and sonogram measurements of the output pulses.