Magnetic field effects on coherent backscattering of light

We have studied the influence of magneto-optical Faraday rotation on coherent backscattering of light experimentally, theoretically and by computer simulations of Monte-Carlo type. The consistency of these three approaches reveals new aspects of the propagation of vector waves in turbid media with and without Faraday rotation. Experimentally, we have demonstrated that the Faraday rotation may almost completely destroy the reciprocity of light paths. However, as shown by the simulations, the cone of coherent backscattering may not only be destroyed but also shifted off the exact backscattering direction, parallel to the magnetic field, as long as the amount of circular polarization is not completely destroyed by the multiple scattering. The relationship between coherent backscattering, depolarization and Faraday rotation are explained by a simple path model of vector waves. This leads to a new characteristic correlation length required to properly describe the influence of Faraday rotation on multiple light scattering. Received 28 January 2000     

Estimation of light transport parameters in biological media using coherent backscattering

The suitability of using the angular peak shape of the coherent backscattered light for estimating the light transport parameters of biological media has been investigated. Milk and methylene blue doped milk were used as tissue phantoms for the measurements carried out with a He-Ne laser (632.8 nm). Results indicate that while the technique accurately estimates the transport length, it can determine the absorption coefficient only when the absorption is moderately high (α>1 cm⁻¹) for the long transport lengths typical of tissues. Further, the possibility of determining the anisotropy factor by estimating the single scattering contribution to the diffuse background is examined.     

Focusing coherent light through opaque strongly scattering media

We report focusing of coherent light through opaque scattering materials by control of the incident wavefront. The multiply scattered light forms a focus with a brightness that is up to a factor of 1000 higher than the brightness of the normal diffuse transmission.     

Nature of coherent enhancement of inelastic electron scattering from disordered media

The mechanism of weak localization of relatively fast electrons scattered with a fixed energy loss from disordered media is examined. The main focus of this paper is to put forward an explanation for why coherent enhancement of electron scattering in the inelastic-scattering channel takes place at angles which differ from π. A simplified kinematic model is proposed to determine the basic properties of the weak localization of electrons in the inelastic scattering channel. The model easily reproduces the range of scattering angles typical for the weak localization of electrons with fixed energy loss. The procedure does not require calculation of the contribution from the crossed diagrams. The results agree with those based on the dynamical theory associated with the calculation of the crossed and ladder diagrams. It is possible to follow the transition from the weak localization of the new type to the ordinary weak localization with decreasing energy loss. The weak localization of the new type is in accord with the weak localization of regular type if the energy loss is about the energy of an optical phonon.     

Visualization of scattering media upon backscattering of a linearly polarized nonmonochromatic light

The method of polarization visualization of multiply scattering macroinhomogeneous media, based on analysis of the spatial distributions of polarization characteristics of a linearly polarized radiation backscattered from a medium, is discussed. The effect of optical characteristics of the medium and the scattering geometry on the quality of the images obtained in the case of visualization of an absorbing heterogeneity immersed into a multiply scattering medium is considered. The comparative analysis of the quality of formed images was performed with the use of different polarization characteristics of the backscattered radiation as a visualization parameter. The theoretical interpretation of the obtained experimental results is given within the framework of the phenomenological approach based on the concept of the distribution of the effective optical paths of partial components of the scattered optical field. To calculate the probability density of the effective optical paths, the statistical simulation method was used.     

Rotation of the polarization ellipse under multiple light scattering in disordered media

A study is performed of the multiple small-angle scattering of circularly polarized waves in random media with large-size transparent inhomogeneities that are less dense than the surrounding medium. In these conditions, a new effect is observed—rotation of the polarization ellipse of the multiply scattered light.     

Spectral changes of light produced by scattering from disordered anisotropic media

We investigate theoretically changes in the spectrum of polychromatic light scattered by a disordered, birefringent medium. We derive an expression for the spectrum of scattered light for ordinary and extraordinary incident waves within the accuracy of the first Born approximation. Using this result, we analyze the changes in the spectrum of light due to the combined action of disorder and anisotropy in the scattering process.     

New quasiparticles hystons and coherent photoinduced dynamics of molecules in polar disordered media

Using methods of statistical thermodynamics, it is shown that after pulse excitation the evolution of a “polar luminescent probe—polar disordered medium” system is described by an equation of damping vibrations. This allows the conclusion that in the solvate shell of the probe molecule synchronous rotational vibrations (librations) of the molecules of the medium occur, whose damping is caused by dielectric friction. Such a collective synchronous motion is considered as a motion of a quasiparticle called a hyston. The moment of inertia J_n and mass M_h of a hyston are defined as J_h=2m² ₁a^-3Ω₀ ^-2(ε-1)/(2ε+1), M_h=J_hM_s/J_s, where m₁ is the dipole moment of the probe molecule in the excited S₁-stute; a is the Onsager radius; Ω₀ is the cyclic frequency of harmonic vibrations of the hyston; ε is the dielectric constant; M_s and J_s are the mass and moment of inertia of a molecule of the medium, respectively. The correlation function of the motion of the molecules c(t) is a solution of the equation of hyston motion. The fluorescence response s(t) in measurements with time resolution coincides with the correlation function: s(t)=c(t). The concepts concerning hystons make it possible to describe macroscopic photoinduced coherent motion that is manifested against a background of thermal motion of the medium molecules. Institute of Molecular and Atomic Physics, National Academy of Sciences of Belarus, 70, F. Skorina Ave., Minsk, 220072, Belarus. Translated from Zhurnal Prikladnei Spektroskopii, Vol 65, No. 2, pp. 176–183, March–April, 1998.     

Light localization signatures in backscattering from periodic disordered media

The backscattering line shape is analytically predicted for thick disordered medium films where, remarkably, the medium configuration is periodic along the direction perpendicular to the incident light. A blunt triangular peak is found to emerge on the sharp top. The phenomenon roots in the coexistence of quasi-1D localization and 2D extended states.     

Light localization signatures in backscattering from periodic disordered media

The backscattering line shape is analytically predicted for thick disordered medium films where, remarkably, the medium configuration is periodic along the direction perpendicular to the incident light. A blunt triangular peak is found to emerge on the sharp top. The phenomenon roots in the coexistence of quasi-1D localization and 2D extended states. The text was submitted by the author in English.     

Nonlinear coherent transport of waves in disordered media

We present a diagrammatic theory for coherent backscattering from disordered dilute media in the nonlinear regime. We show that the coherent backscattering enhancement factor is strongly affected by the nonlinearity, and we corroborate these results by numerical simulations. Our theory can be applied to several physical scenarios such as scattering of light in a nonlinear Kerr medium or propagation of matter waves in disordered potentials.     

Self-organized transition to coherent activity in disordered media

Synchronized oscillations are of critical functional importance in many biological systems. We show that such oscillations can arise without centralized coordination in a disordered system of electrically coupled excitable and passive cells. Increasing the coupling strength results in waves that lead to coherent periodic activity, exhibiting cluster, local and global synchronization under different conditions. Our results may explain the self-organized transition in a pregnant uterus from transient, localized activity initially to system-wide coherent excitations just before delivery.     

Time-resolved optical backscattering model in highly scattering media

A time-resolved backscattering model, which combines a single large-angle scattering with multiple small-angle scatterings, is used to produce a scattered-light profile about a medium. Inhomogeneity of the medium is included in the model. Some multidimensional integrals can be evaluated analytically.     

Anomalous coherent backscattering of light from opal photonic crystals

We studied coherent backscattering (CBS) of light from opal photonic crystals with incomplete band gaps. We observed a dramatic broadening of the CBS cone for incident angles close to the Bragg condition in the crystals. We modify the conventional CBS theory to incorporate Bragg attenuation resulting from the photonic band structure. By fitting the CBS data with the modified theory, we extract both the disorder-induced light mean-free path and the Bragg attenuation length of the inherent opal photonic crystal.