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《工程热物理学报》2015,(9)
本文研制了一套基于自发布里渊散射法的流体音速测量实验系统,分析得到该实验系统温度、压力测量的不确定度分别为0.02 K,10 kPa,音速测量的扩展不确定度为0.5%。测量了标准物质正戊烷310 K到470 K饱和液体和350 K到470 K饱和气体的音速,与文献值比较得到,该实验测量值的测量偏差为2.5%左右,验证了本实验系统的可靠性与稳定性。在温度为303.15 K~453.15 K,压力达5.5 MPa范围内,对燃料添加剂异丙醚的饱和液体和过冷液体的音速进行了测量,并依据实验数据给出了异丙醚音速的经验关联式,关联式的计算偏差为0.51%(饱和液体)和0.54%(过冷液体)。 相似文献
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分段自相关动态光散射法测量亚微米粒度 总被引:5,自引:0,他引:5
介绍了动态光散射法测量微粒尺度的原理,通过对相关函数相对的分析,提出了分段自相关的方法,该方法解决了高速,大数据量采集的困难,又不显著影响相关函数的精度,给出了实验装置及实验结果,测量结果与标准样品的标称值相符。 相似文献
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利用金刚石对顶砧技术,采用180°背向散射和60°前向对称散射两种几何配置,对水、氨、二水合氨和甲烷等含氢小分子液体进行了高温高压布里渊散射研究,计算了在室温(296K)和高温(410K)下的声速,比较了不同小分子液体中的声速及绝热体弹模量随压力的变化关系。在等温条件下,各体系中声速随着压力的增加逐渐增加;在相同温度下,甲烷液体的声速随着压力增加的速率明显高于水、氨及二水合氨液体;在相同的温度和压力条件下,水、氨及二水合氨液体的体弹模量明显高于甲烷液体的体弹模量,表明氢键的存在对于小分子液体弹性具有较大影响。二水合氨的体弹模量斜率在1.5GPa左右发生改变,表明液体结构可能发生了改变,并分析了氢键对该体系弹性性质的影响。研究有助于理解其他含氢小分子液体中压力和温度诱导的分子结构变化。 相似文献
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设计并搭建了超声光栅,观察了激光经过光栅形成的衍射斑纹,测量了声速;并利用超声光栅测定了不同温度、不同浓度的NaCl溶液中的声速,给出了声速-水温和声速-溶液浓度的依赖关系.水的温度每升高1℃,3.974 MHz的超声波的声速增加2.09 m/s,16.574 MHz的超声波的波速增加2.04m/s;声速随着NaCl溶液浓度的增大线性增加,NaCl溶液浓度每升高1%,3.974 MHz的超声波声速增加13.637 m/s,16.574 MHz的声波声速增加11.757 m/s.在此基础上,分析了不同频率的超声波对实验规律的影响,认为不同频率的超声波在相同条件下测量的溶液中声速大小的不同源于测量的随机误差. 相似文献
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利用两部智能手机,借助手机软件phyphox在家进行了多普勒效应实验.两部手机分别作为接收器和声源,让接收器和声源分别做自由落体运动,测得了接收频率和运动速度随时间的变化曲线,通过对数据的处理得到了声速和重力加速度值,并和理论值进行了对比,验证了用手机进行多普勒效应实验的可靠性,为以后实验的进行以及数据处理提供了参考. 相似文献
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Abstract The pressure dependence of the refractive index n(P) and of the longitudinal acoustic velocities of 4.1 methanol-ethanol solution have been measured in a diamond anvil cell up to 8.1 GPa. We utilize Brillouin scattering methods for this determination and detect, in the same back scattering configuration, acoustic wave propagation parallel to the faces of the diamond anvils as well as along the incident laser radiation direction. We also deduce that the polarizability of the fluid is reduced by about 15% over the pressure range studied. 相似文献
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Brillouin light spectra in water was experimentally investigated by a scanning Fabry-Perot interferometer. The optical properties of the scattering media were modulated by a plane ultrasound wave. An enhancement up to 10 times of the Brillouin signal by modulation with the ultrasound wave has been seen clearly. The dependence of the Brillouin signal amplitude on the ultrasound frequency, amplitude and the position of the ultrasound field based to the light beam was investigated experimentally. Very strong dependence of the enhancement with experimental conditions was obtained. 相似文献
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Valeri I. Kovalev 《Physics letters. A》2019,383(12):1378-1380
It is shown that the pump-probe technique in Brillouin scattering spectroscopy is accompanied by two specific distortions to a registered spectrum. The first appears due to an acoustic wave that unavoidably accompanies in a continuous medium the density wave driven by the pump and probe signals. The registered spectrum then splits to two spectral components, one corresponding to the propagation velocity of the driven density wave, and the other to the acoustic velocity. The other distortion is asymmetry of the spectrum which is shown to occur when the velocity of the driven density wave is greater than the acoustic velocity in the medium. 相似文献
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Single-crystal elasticity of the rhodochrosite at high pressure by Brillouin scattering spectroscopy
ABSTRACTThe sound velocity properties of single-crystal rhodochrosite (MnCO3) were determined up to 9.7?GPa at ambient temperature by Brillouin scattering spectroscopy. Six elastic constants were calculated by a genetic algorithm method using the Christoffel's equations at each pressure. The elastic constants increased linearly as a function of pressure and its pressure derivatives ?Cij/?P for C11, C33, C44, C12, C13, C14 were 5.86 (±0.36), 3.82 (±0.44), 2.06 (±0.39), 5.07 (±0.27), 5.34 (±0.44), 1.52 (±0.24), respectively. Based on the derived elastic constants of rhodochrosite, the aggregate adiabatic bulk and shear moduli (Ks and G) were calculated using the Voigt-Reuss-Hill averages and the linear fitting coefficients (?Ks/?P)T and (?G/?P)T were 5.05(±0.26) and 0.73(±0.05), respectively. The aggregate Vp of rhodochrosite increased clearly as a function of pressure and its pressure derivative ?Vp/?P was 7.99(±0.53)?×?10?2?km/(s?GPa), while the aggregate Vs increased slowly and ?Vs/?P was only 1.19(±0.12)?×?10?2?km/(s?GPa). The anisotropy factor for As of rhodochrosite increased from ~40% at 0.8?GPa to ~48% at 9.7?GPa, while Ap decreased from ~19% to ~16% at the corresponding pressure. 相似文献
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Summary We have performed Brillouin and depolarized Rayleigh light scattering on water-methanol solutions as a function of methanol
molar fraction and temperature. For this system, molecular-dynamics (MD) simulation predicts that a shell of water forms around
a methanol molecule, prediction which has been recently confirmed by neutron diffraction experiments. The results obtained
by light scattering and presented here confirm previous observations and show, in addition, an increase of the stability in
time of the water structure in the shells when temperature decreases and methanol concentration approaches a particular value.
Paper presented at the I International Conference on Scaling Concepts and Complex Fluids, Copanello, Italy, July 4–8, 1994. 相似文献
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Stimulated Brillouin scattering is studied by numerically solving the Vlasov-Maxwell system. A cascade of stimulated Brillouin scattering can occur when a linearly polarized laser pulse propagates in a plasma. It is found that a stimulated Brillouin scattering cascade can reduce the scattering and increase the transmission of light, as well as introduce a bursting behaviour in the evolution of the laser-plasma interaction. The bursting time in the reflectivity is found to be less than half the ion acoustic period. The ion temperature can affect the stimulated Brillouin scattering cascade, which can repeat several ×at low ion temperatures and can be completely eliminated at high ion temperatures. For stimulated Brillouin scattering saturation, higher-harmonic generation and wave-wave interaction of the excited ion acoustic waves can restrict the amplitude of the latter. In addition, stimulated Brillouin scattering cascade can restrict the amplitude of the scattered light. 相似文献