YbRh(2)Si(2): pronounced non-fermi-liquid effects above a low-lyingmagnetic phase transition

We report the first observation of non-Fermi-liquid (NFL) effects in a clean Yb compound at ambient pressure and zero magnetic field. The electrical resistivity and the specific-heat coefficient of high-quality single crystals of YbRh(2)Si(2) present a linear and a logarithmic temperature dependence, respectively, in more than a decade in temperature. We ascribe this NFL behavior to the presence of (presumably) quasi-2D antiferromagnetic spin fluctuations related to a very weak magnetic phase transition at T(N) approximately 65 mK. Application of hydrostatic pressure induces anomalies in the electrical resistivity, indicating the stabilization of magnetic order.     

Thermal conductivity in the vicinity of the quantum critical end point in Sr3Ru2O7

Thermal conductivity of Sr3Ru2O7 was measured down to 40 mK and at magnetic fields through the quantum critical end point at Hc=7.85 T. A peak in the electrical resistivity as a function of the field was mimicked by the thermal resistivity. In the limit as T-->0 K, we find that the Wiedemann-Franz law is satisfied to within 5% at all fields, implying that there is no breakdown of the electron despite the destruction of the Fermi liquid state at quantum criticality. A significant change in disorder [from rho0(H=0 T)=2.1 to 0.5 microOmega cm] does not influence our conclusions. At finite temperatures, the temperature dependence of the Lorenz number is consistent with ferromagnetic fluctuations causing the non-Fermi liquid behavior as one would expect at a metamagnetic quantum critical end point.     

Magnetism and superconductivity in Eu0.2Sr0.8(Fe0.86Co0.14)2As2 probed by 75As NMR

We report bulk superconductivity (SC) in Eu(0.2)Sr(0.8)(Fe(0.86)Co(0.14))(2)As(2) single crystals by means of electrical resistivity, magnetic susceptibility and specific heat measurements with T(c) is approximately equal to 20 K and an antiferromagnetic (AFM) ordering of Eu(2+) moments at T(N) is approximately equal to 2.0 K in zero field. (75)As NMR experiments have been performed in the two external field directions (H is parallel to ab) and (H is parallel to c). (75)As-NMR spectra are analysed in terms of first-order quadrupolar interaction. Spin-lattice relaxation rates (1/T(1)) follow a T(3) law in the temperature range 4.2-15 K. There is no signature of a Hebel-Slichter coherence peak just below the SC transition, indicating a non-s-wave or s(±) type of superconductivity. In the temperature range 160-18 K 1/T(1)T follows the C/(T+θ) law reflecting 2D AFM spin fluctuations.     

Magnetic behavior of Eu(3)Ni(4)Ga(4): antiferromagnetic order and large magnetoresistance

The results of the magnetic susceptibility, isothermal magnetization, heat capacity, electrical resistivity and magnetoresistance measurements on polycrystalline Eu(3)Ni(4)Ga(4) are presented. Eu(3)Ni(4)Ga(4) forms in Na(3)Pt(4)Ge(4)-type cubic crystal structure (space group [Formula: see text]). The temperature dependence of the magnetic susceptibility of Eu(3)Ni(4)Ga(4) confirms the divalent state (Eu(2+)) of Eu ions with an effective magnetic moment μ(eff)?=?7.98?μ(B). At low fields, e.g.?at 0.01?T, a magnetic phase transition to an antiferromagnetically ordered state occurs at T(N)?=?10.9?K, which is further confirmed by the temperature dependence of the heat capacity and electrical resistivity. The field dependence of isothermal magnetization at 2?K reveals the presence of two field induced metamagnetic transitions at H(c1) and H(c2)?=?0.55 and 1.2?T, respectively and a polarized phase above H(PO)?=?1.7?T. The reduced jump in the heat capacity at the transition temperature, ΔC|(T(N))?=?13.48?J/mol-Eu?K would indicate an amplitude modulated (AM) antiferromagnetic structure. An interesting feature is that a large negative magnetoresistance, MR?=?[ρ(H)?-?ρ(0)]/ρ(0), is observed in the vicinity of magnetic transition even up to 2T(N). Similar large magnetoresistance has been observed in the paramagnetic state in some Gd and Eu based alloys and has been attributed to the magneto-polaronic effect.     

Bulk properties of the UCoGe Kondo-like system

We report on extensive experimental investigations of a single crystal of the orthorhombic uranium compound UCoGe. Bulk measurements on as-grown and annealed single crystals, recording magnetization, magnetic susceptibility, electrical resistivity, magnetoresistivity, thermopower, thermal conductivity and heat capacity data do not reproduce the previously reported coexistence of ferromagnetism with superconductivity. The latter phenomenon was only observed for the annealed sample at T _SC = 0.65 K. New observations show a crossover at around 13 K, visible in thermal and transport measurements as well as the coherent state around 50 K, signaled by a wide knee in ρ(T). Above this temperature, UCoGe exhibits a single-ion Kondo-like effect. The magnetoresistivity of the annealed single crystal increases negatively down to 4.2 K, reaching as a large value about ?27% at a field of 8 T. The latter may be interpreted in terms of fairly strong magnetic fluctuations existing in UCoGe at low temperatures.     

Ferromagnetic quantum critical fluctuations in YbRh2(Si0.95Ge0.05)2

The bulk magnetic susceptibility chi(T,B) of YbRh(2)(Si(0.95)Ge(0.05))(2) has been investigated close to the field-induced quantum critical point at B(c) = 0.027 T. For B < or= 0.05 T a Curie-Weiss law with a negative Weiss temperature is observed at temperatures below 0.3 K. Outside this region, the susceptibility indicates ferromagnetic quantum critical fluctuations, chi(T) proportional, variantT-0.6 above 0.3 K. At low temperatures the Pauli susceptibility follows chi(0) proportional, variant(B-B(c))(-0.6) and scales with the coefficient of the T(2) term in the electrical resistivity. The Sommerfeld-Wilson ratio is highly enhanced and increases up to 30 close to the critical field.     

Nonvanishing energy scales at the quantum critical point of CeCoIn5

Heat and charge transport were used to probe the magnetic field-tuned quantum critical point in the heavy-fermion metal CeCoIn5. A comparison of electrical and thermal resistivities reveals three characteristic energy scales. A Fermi-liquid regime is observed below T(FL), with both transport coefficients diverging in parallel and T(FL) -->0 as H --> Hc, the critical field. The characteristic temperature of antiferromagnetic spin fluctuations, T(SF), is tuned to a minimum but finite value at Hc, which coincides with the end of the T-linear regime in the electrical resistivity. A third temperature scale, T(QP), signals the formation of quasiparticles, as fermions of charge e obeying the Wiedemann-Franz law. Unlike T(FL), it remains finite at Hc, so that the integrity of quasiparticles is preserved, even though the standard signature of Fermi-liquid theory fails.     

Observation of bulk superconductivity in NaxCoO2.yH(2)O and NaxCoO2.yD(2)O powder and single crystals

Poly- and single-crystalline NaxCoO2 has been successfully intercalated with H2O and D2O as confirmed by x-ray diffraction and thermogravimetric analysis. Resistivity, magnetic susceptibility, and specific heat measurements show bulk superconductivity with T(c) close to 5 K in both cases. The substitution of deuterium for hydrogen has an effect on T(c) of less than 0.2 K. Investigation of the resistivity anisotropy of NaxCoO2.yH(2)O single crystals shows (a). almost zero resistivity below T(c), and (b). an abrupt upturn at T(*) approximately 52 K in both the ab plane and the c direction. The implications of our results on the possible superconducting mechanism will be discussed.     

Evidence for Jahn-Teller distortions at the antiferromagnetic transition in LaTiO3

LaTiO3 is known as a Mott insulator which orders antiferromagnetically at T(N)=146 K. We report on results of thermal expansion and temperature dependent x-ray diffraction together with measurements of the heat capacity, electrical transport measurements, and optical spectroscopy in untwinned single crystals. At T(N) significant structural changes appear, which are volume conserving. Concomitant anomalies are also observed in the dc resistivity, in bulk modulus, and optical reflectivity spectra. We interpret these experimental observations as evidence of orbital order.     

Observation of multiferroic properties in pyroxene NaFeGe2O6

We report the observation of multiferroicity in a clinopyroxene NaFeGe(2)O(6) polycrystal from the investigation of its electrical and magnetic properties. Following the previously known first magnetic transition at T(N1) = 13 K, a second magnetic transition appears at T(N2) = 11.8 K in the temperature dependence of the magnetization. A ferroelectric polarization starts to develop clearly at T(N2) rather than T(N1) and its magnitude increases up to ~13 μC m(-2) at 5 K, supporting the idea that the ferroelectric state in NaFeGe(2)O(6) stems from a helical spin order stabilized below T(N2). When a magnetic field of 90 kOe is applied, the electric polarization decreases to 9 μC m(-2) and T(N2) slightly increases by 0.5 K. At intermediate magnetic fields, around 28 and 78 kOe, anomalies in the magnetoelectric current, magnetoelectric susceptibility, and field derivative of magnetization curves are found, indicating field-induced spin-state transitions. Based on these electrical and magnetic properties, we provide a detailed low temperature phase diagram up to 90 kOe, and discuss the nature of each phase of NaFeGe(2)O(6).     

Transport properties of SmO

The electrical resistivity and thermoelectric power of SmO are measured between 4.2 and 300 K. The existence of a low temperature T² law in the resistivity and the large and roughly constant magnetic susceptibility suggest that SmO presents large spin fluctuations.     

Field-dependent diamagnetic transition in magnetic superconductor Sm1.85Ce0.15CuO4-y

The magnetic penetration depth of single crystal Sm(1.85)Ce(0.15)CuO(4-y) was measured down to 0.4 K in dc fields up to 7 kOe. For insulating Sm2CuO4, Sm3+ spins order at the Ne el temperature, T(N)=6 K, independent of the applied field. Superconducting Sm(1.85)Ce(0.15)CuO(4-y) (T(c) approximately 23 K) shows a sharp increase in diamagnetic screening below T(*)(H) which varied from 4.0 K (H=0) to 0.5 K (H=7 kOe) for a field along the c axis. If the field was aligned parallel to the conducting planes, T(*) remained unchanged. The unusual field dependence of T(*) indicates a spin-freezing transition that dramatically increases the superfluid density.     

Spin, charge and lattice couplings in Cu-deficient oxysulphide BiOCu0.94S

The electrical and magnetic properties of slightly Cu-deficient BiOCu(0.94)S are investigated using neutron diffraction, ac magnetic susceptibility, magnetization and electrical resistivity measurements. The Cu spins order in a ferromagnetic arrangement below T(C) = 250 K. An antiferromagnetic component develops below 180 K when the crystalline unit cell experiences a sharp thermal contraction upon cooling, resulting in a canted ferromagnetic spin arrangement at low temperatures. In the magnetically ordered state the electrical transport can be described using three-dimensional variable range hopping conduction. An applied magnetic field can effectively reduce the hopping barrier. Spin-charge couplings are clearly revealed when the resistivity departs from the hopping conduction and begins to increase with increasing temperatures above 250 K where the Cu spins become disordered.     

Large variations in the magnetic ordering behavior of EuCu(2)As(2) with the application of external pressure and magnetic field

The influence of external pressure on the electrical transport and magnetic properties of EuCu(2)As(2), crystallizing in a ThCr(2)Si(2)-type structure, is reported. The system is known to be an antiferromagnet below T(N) ≈ 15 K in the absence of external magnetic fields. We find that there is a gradual reduction of T(N) with the application of a magnetic field with an extrapolated value of the critical field of around 18 kOe which can drive T(N) to zero. Electrical resistivity under pressure (<11 GPa) reveals that the magnetic ordering temperature is pushed up dramatically to higher temperatures which is quite interesting if compared with the behavior in isostructural FeAs-based systems containing Eu. Above 7 GPa, the pressure-induced state appears to be ferromagnetic. The results thus reveal interesting changes in the magnetic ordering behavior of this compound with increasing pressure and magnetic fields.     

非晶态TbFe2薄膜的磁性和电性

本文研究了TbFe₂非晶态薄膜的磁性和电性,测量了M_s(T)(77—800K),ρ(T)(4.2—400K)和穆斯堡尔谱(18K,400K),得到居里温度T_c～400K,电阻极小值温度T_min～360K,在T<360K范围内观察到温度系数为负的类Kondo效应,用Hesse和Window两种不同方法解出了室温穆斯堡尔谱的超精细场,得到了H=210kOe和H=25kOe两种分布,其中前一组给出了铁磁性,后一组可能与类Ko 关键词：     

Interplay between disorder and quantum and thermal fluctuations in ferromagnetic alloys: the case of UCu2Si2-xGex

We consider, theoretically and experimentally, the effects of structural disorder, quantum fluctuations, and thermal fluctuations in the magnetic and transport properties of certain ferromagnetic alloys. We study the particular case of UCu2Si2-xGex. The low temperature resistivity, rho(T,x), exhibits Fermi liquid behavior as a function of temperature T for all values of x, which can be interpreted as a result of the magnetic scattering of the conduction electrons from the localized U spins. The residual resistivity, rho(0,x), follows the behavior of a disordered binary alloy. The observed nonmonotonic dependence of the Curie temperature, T(c)(x), with x can be explained within a model of localized spins interacting with an electronic bath. Our results clearly show that the Curie temperature of certain alloys can be enhanced due to the interplay between quantum and thermal fluctuations with disorder.     

Collapse of 5 f -Electron Ferromagnetism in UPtAl Under High Pressures

UPtAl exhibits a ferromagnetic ordering of U magnetic moments at temperatures below T C =42.5 K. The magnetic-ordering transition is accompanied by an anomaly in the temperature dependence of electrical resistivity. This allows us to determine the value of Curie temperature from 𝜌 vs. T data that can be measured at very high pressures, at which reliable magnetization measurements are difficult. We report on resistivity measurements performed on an UPtAl single crystal under hydrostatic pressures p h 8 GPa. It was observed that the initial increase of T C with p becomes gradually reduced for p >2 GPa until the maximum T C value of , 48 K is reached between 4 and 6 GPa that is followed by a progressively developing downturn of the T C ( p ) curve. The latter result is attributed to the approaching collapse of the U 5 f -moment ferromagnetism. Low-temperature resistivity data point to a rapidly reduced magnetic anisotropy at highest pressures.     

Correlation between electron state density change and the electrical resistivity and magnetic permeability changes in the nanostructured powder of the NiMo alloy

The nanostructured powders of the Ni_95.4Mo_4.6 and Ni₉₉Mo₁ alloys (average crystallite dimensions of 14 and 21 nm) were obtained by the electrochemical deposition from ammonium solutions of nickel and molybdenum salts. The method of differential scanning calorimetry (DSC) and measurement of temperature dependence of the powder's electrical resistivity, magnetic permeability and the thermoelectromotive force were employed to examine structural changes of the powders. The nanocrystalline alloys Ni_95.4Mo_4.6 and Ni₉₉Mo₁ were stable up to about 460 K. The thermal stabilization of the alloys takes place within the temperature interval of 460–570 K. As a result of this process, a decrease in the electrical resistivity and increases in magnetic permeability as well as electron state density in the proximity of the Fermi level are observed. The crystallization temperature depends upon the current density of powder formation. The nanocrystalline alloy Ni_95.4Mo_4.6 obtained at j=70 mA cm⁻² becomes crystallized in the temperature range between 650 and 840 K, while the Ni₉₉Mo₁ alloy obtained at j=180 mA cm⁻² crystallizes in the 580–950 K temperature interval. The electrical resistivity and magnetic permeability of the nanocrystalline alloy decreased while the alloy's electron state density near the Fermi level increased after the process of crystallization took place. The electrical resistivity decrease recorded during the structural changes was due to an increase in the electron state density in the proximity of the Fermi level, as well as to an increase in the mean free path of the conducting electrons.     

The pressure induced insulator to metal transition in FeSb2

The evolution of the ground state properties of FeSb(2) has been investigated via temperature (4.2-300 K), magnetic field (0-12 T) and pressure (0-8.8 GPa) dependent electrical resistivity studies. The temperature dependence of the resistivity follows activated behavior in the high temperature (HT) regime (T > 60 K), while variable range hopping (VRH) dictates the transport in the intermediate temperature (IT) regime (10 K > T > 45 K) and power law behavior is observed in the low temperature (LT) regime (T < 10 K). The pressure profoundly affects the resistivity in all the temperature regimes. The energy gap (Δ) extracted in the HT regime initially increases with pressure and then decreases, while the VRH parameter T(0) deduced in the IT regime is seen to decrease monotonically and vanish beyond 5 GPa leading to an insulator to metal transition (MIT) on account of delocalization of the electronic states in the gap. The analysis of the logarithmic derivative of the conductivity indicates the MIT to occur at ~6 GPa. The magnetoresistivity is found to be positive. The analysis of the resistivity behavior under pressure and magnetic field indicates that the former induces delocalization, while the latter tends to assist localization of the defect states inside the gap of FeSb(2).     

Temperature dependence of thermal and electrical conductivity of Bi-based high-Tc (2 2 2 3) superconductor

Superconducting samples with nominal composition Bi_1.6Pb_0.4Sr₂Ca₂Cu₃O_δ were prepared by the conventional solid-state reaction technique. The samples have been characterized by X-ray diffraction, dc electrical resistivity, ac magnetic susceptibility and thermal conductivity. The X-ray diffraction studies were done at room temperature and the lattice constants of the material were determined by indexing all the peaks. All the above measurements show that, there exists two phases i.e. high-T_c (2 2 2 3) and low-T_c (2 2 1 2). The information obtained from dc electrical resistivity data agrees with ac magnetic susceptibility measurements. The onset temperature T_c (onset) and zero resistivity temperature T_c (R = 0) of the samples remains within the temperature 120 ± 1 K and 103 ± 1 K. Thermal conductivity has been measured with a transient plane source (TPS) technique in the temperature range 77–300 K. The estimation of the electrical resistivity change due to scattering by phonons and impurities has been discussed. An increase in thermal conductivity is observed above and below T_c (R = 0). The electron–phonon scattering time, phonon-limited mobility and the size of the electron–phonon constant are also calculated. Wiedemann–Franz law is applied to gain prediction about the magnitude of electronic and phonon contribution to the total thermal conductivity of the samples. It is observed that heat is mainly conducted by the phonons in this system.