Effect of the Radiation Power Density on the Sensitivity of a Diamond Detector

This paper presents the results of an experimental study of the sensitivity of a detector made of natural diamond of the IIa type as a function of the power density of the radiation of a pulsed xenon lamp. It has been shown that the sensitivity of the detector depends on the power density of the xenon lamp radiation and equals about (1–6)·10^–4 A/W. A monotonic decrease in sensitivity of the detector during a radiation pulse has been detected. The minimum resistance of the diamond crystal with an irradiated face of area 3 mm², placed 7 mm away from the axis of the xenon lamp, was 300 , which corresponds to a specific conductivity of 2.2 ^–1·m^–1.     

Generation of laser-polarized xenon using fiber-coupled laser-diode arrays narrowed with integrated volume holographic gratings

Volume holographic gratings (VHGs) can be exploited to narrow the spectral output of high-power laser-diode arrays (LDAs) by nearly an order of magnitude, permitting more efficient generation of laser-polarized noble gases for various applications. A 3-fold improvement in ¹²⁹Xe nuclear spin polarization, P_Xe, (compared to a conventional LDA) was achieved with the VHG-LDA’s center wavelength tuned to a wing of the Rb D₁ line. Additionally, an anomalous dependence of P_Xe on the xenon density within the OP cell is reported—including high P_Xe values (>10%) at high xenon partial pressures (1000 torr).     

Thermoluminescence glow curves of CaF2: Dy crystals irradiated by soft X-rays

Applying a deconvolution of the thermoluminescence glow curves, parameters of single glow peaks of CaF₂: Dy TLD 200 dosemeters irradiated by soft X-rays were determined. A dependence of the height ratio of low temperature (T393, 413 and 473 K) single peaks on energy of absorbed photons was measured in a region of 1–22.2 keV. Standard radionuclides¹⁰⁹Cd,²³⁸Pu,⁵⁵Fe and iodine laser produced aluminium plasma (T _e 500 eV) were used as soft X-ray sources. The ratios of the heights of different single peaks are discussed with respect to high local doses. The decreasing ratio of the heights of the first and third and/or second and third peak with increasing photon energy allows to determine reversely a mean photon energy of absorbed soft X-ray radiation.     

Investigations on the excited states of Eu2+ in CaF2-and SrF2-crystals by two-photon absorption spectroscopy

The two-photon-excitation spectra of Eu²⁺:CaF₂ and Eu²⁺:SrF₂ have been studied at 4.2 K in the region between 24,100cm^–1 and 28,100cm^–1. Besides a broad two-photon absorption region two groups of sharp lines at 27,600cm^–1 and 28,000cm^–1 in Eu²⁺:CaF₂ (27,670cm^–1 and 28,080cm^–1 in Eu²⁺:SrF₂) are identified with the transitions 4f ⁷:⁸ S _7/24f ⁷:⁶ P _7/2,⁶ P _5/2. It is shown that the 4f-states of Eu²⁺ in this host lattice differ significantly in their physical properties from the same states of the isoelectronic Gd³⁺. For these transitions, however, the calculated two-photon absorption rates are in good agreement with the experiments.A project of the Sonderforschungsbereich 65 Festkörperspektroskopie, Darmstadt-Frankfurt, supported by the Deutsche Forschungsgemeinschaft     

Rates of change in high temperature electrical resistivity and oxygen diffusion coefficient in Ba2YCu3Ox

The change in electrical resistance with time for bulk, thick-film, and thin-film Ba₂YCu₃O_x at atmospheric pressure is described as a function of the oxygen partial pressure (100 to 0.001%) and temperature (320°–750°C). The potential usefulness of these materials as oxygen sensors is demonstrated. The rate of equilibration is faster during oxygen uptake than during its loss. Time constants to reach equilibration (1/e remaining), qualitatively scale with sample dimensions. For a 1m film at 600° C, <1 s for the range of P_O2 (O2 being a shorthand for O₂) from 100% to 0.001%. The rate increases markedly with increasing P_O2. The actual resistance decreases with P_O2 at a rate of log/log P_O2 = 0.4 at 700° C showing adequate sensitivity for sensor purposes. Times for the transient resistance change in the sample where used to estimate the oxygen diffusion coefficient in the ceramic. The diffusivities obtained are 4·10^–11–1·10^–12 cm²/s in the 435°–320° C range, with an activation energy of 27 kcal/mole.     

Behavior of the excitation cross sections of the perturbed series of the xenon atom

Behavior of the excitation cross sections of the perturbed 6s[3/2]_n°?np[1/2]₀ spectral series of the xenon atom is experimentally studied. By using the methods of extended electron beam and optical spectroscopy, the cross sections are measured and the optical excitation functions are recorded for the transitions of this series with n=6–13. A deviation of the dependence Q=f(n) from a power-law function is revealed, as well as changes in the form of optical excitation functions and in the nature of the branching caused by perturbation of the 7p[1/2]₀ level by levels of the 5p ⁵(² P _1/2°)6p configuration.     

The Debye-Waller factor and the diffusion process for hydrogen in Nb,Ta, and V single crystals investigated by neutron spectroscopy

Quasielastic scattering of slow neutrons on hydrogen diffusing in the-phase of NbH_0.02, TaH_0.13 and VH_0.07 single crystals was investigated in a wide range of temperatures and scattering vectorsQ (0.5Q2.5 Å^–1). The incoherent scattering lawS _d (Q,) for four different diffusion models was consistently compared with the measured lineshapes. At elevated temperatures one had to introduce correlated jumps to describe the experimental data, whereas at room temperature a model with jumps between adjacent sites is sufficient. The integrated quasielastic intensityI(Q) obtained from the fit ofS _d (Q,) with the measured spectra follows an isotropic Debye-Waller factor with mean square amplitudes u ²=0.02–0.04 Ų for H in Ta (20°C–500°C), and u ²=0.03–0.04 Ų for H in Nb (20°C–300°C). For H in V,I(Q) obtained from the analysis of the quasielastic scattering deviates from a normal Debye-Waller factor behaviour. This effect is assumed to be due to the flight process between the interstitial sites. On the other hand, a normal Debye-Waller factor was obtained from theQ-dependence of the inelastic scattering of the band modes, with values of u ²=0.02–0.04 Ų (135°C–500°C). The observed values of u ² were compared with theoretical calculations.     

Determination of the effective cross sections for the excitation of the mercury metastable level 63P2

The deexcitation of the metastable mercury level 6³P₂ by electron impact was investigated by the method of impact of the second kind in a Hanle-type tube. These data and the relations of Klein and Rosseland were then used to reconstruct the excitation functiori for the 6S₀ 6³P₂ transition in mercury. A single maximum located 0.3 eV to the right of the excitation threshold was observed on the excitation function of the 6³P₂ level. A formula is also presented for the effective cross sections for the excitation of the mercury metastable 6³P₂ level. The effective cross section at the maximum of the excitation function of the 6³P₂ level is 2.9 · 10^–16 cm² ±30%.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 12, pp. 85–91, December, 1970.The authors are deeply grateful to V. A. Fabrikant and the participants of the seminar under his direction for a discussion of the present results.     

Collisional broadening of Ba I line (553.5 nm) by He or Ar

The Doppler-free line shape of the 6s ^{2 1} S ₀ – 6s ¹6p ^{1 1} P ₁ transition at 553.5 nm in natural Ba in the presence of an argon or helium buffer gas has been measured at 744 K for gas pressures from 0.2 to 100 Torr. Using the measured data for pressures above 5 Torr, the broadening rate coefficients for the half width at half maximum (HWHM) are determined to be (4.9±0.5)10^–9 and (5.0±0.5)10^–9 s^–1 cm^–3 for helium and argon respectively.     

The low temperature electric quadrupole orientation of184Ir and185Ir in rhenium

The half-lives of¹⁸⁴Ir,¹⁸⁵Ir and¹⁸⁶Ir have been determined to be 3.14(2) h, 14.4(1) h and 16.64(3) h, respectively. The quadrupole frequenciesv _Q = e²qQ_s/h of¹⁸⁴Ir and¹⁸⁵Ir in rhenium single crystal have been determined to be Q_s(¹⁸⁴Ir) = + 2.0(3) b MHz and Q_s(¹⁸⁵Ir) = +2.0(3) b MHz. Adopting the value of –3.6(2)×10¹⁷ V·cm^–2 for the electric field gradient eq at T=0 K, the values of the ground-state spectroscopic quadrupole moments of these isotopes are determined to be Q_s(¹⁸⁴Ir)=+2.0(3) b and Q_s(¹⁸⁵Ir)=–2.5(3) b. The¹⁸⁵Ir moment is only consistent with the ground state Nilsson configuration , the¹⁸⁴Ir moment is consistent with K4 with a predominant K=4 component, in disagreement with K=0,1 found for¹⁸⁶Ir. Our analysis differs in detail from the recent nuclear orientation study by Hagn et al.[1].     

Large-scale collisional energy transfer in laser-pumped metastable Ca atoms: Excitation of resonance states of Ca II

We report the first experimental observation of the excitation of the 4p ² P _{3/2, 1/2} resonance states of Ca II (located at 74 720.4 and 74 497.5 cm^–1 above the ground state of Ca I) following pulsed-laser pumping of the 4s ^{2 1} S _O–4s4p ³P₁ intercombination transition of Ca I (E _ex = 15 210 cm^–1). Large scale collisional transfer of energy between the laser-excited atoms is believed to be responsible for this. This is possibly because sufficient time is available (_rad of the 4s4p ³ P ₁ state is approximately 350 µs) for collisions to build such a high level of excitation. Some interesting additional features of the fluorescence spectra of the laser-pumped Ca vapor, such as temperature dependence of the fluorescence intensities and evolution in time of some selected states, are also presented.     

Submillimeter laser action of CW optically pumped CF2Cl2 (Fluorocarbon 12)

Eleven new CW far infrared (FIR) laser lines have been observed in the 600 m–1200 m range from the CF₂Cl₂ (Fluorocarbon 12) molecule optically pumped by a CO₂ laser. A 510^–4–10^–3 accuracy is achieved in the measurement of the FIR wavelengths.The frequency offset between the CO₂ pump center and the absorption line centers are measured using the transferred Lamb dip technique. Owing to a recent spectroscopic study of the CF₂ ³⁵Cl₂ molecule three lines may be assigned with great confidence as rotational transitions in thev ₆ vibrational band 923 cm^–1 of this main isotope.     

A new sequence of high-spin states built on the 17/2+ isomer in85Kr

High-spin states in⁸⁵Kr have been studied via in-beam spectroscopy by bombarding a⁸²Se target with 32 MeV⁷Li ions. Since⁸⁵Kr is only formed with a small relative cross section proton-— coincidence techniques have been applied to enhance the rays of⁸⁵Kr, even with respect to those of⁸⁶Kr, in the measurements. A new sequence of high-spin states with excitation energies up to 4.8 MeV and tentative spins up to (23/2) has been established on top of the 17/2⁺ s isomer. A tentative assignment of the configurationvg ₉ ^2/–1 (g _9/2 p ₃ ^2/–1 orf ₅ ^2/–1 ) to the new levels is proposed.Supported by Deutsche Forschungsgemeinschaft     

Population of the higher-lying vibrational levels of the nitrogen B3π state in a glow discharge

The absolute populations of the higher-lying vibrational levels of the B³ state of the nitrogen molecule in a glow discharge have been determined for pressures from 0.1 to 1.0 torr and current densities from 80 to 200 mA/cm². The absolute concentrations of molecules at levels v = 5, 6, ..., 12 under these conditions are of the order of 10⁹–10¹¹ cm^–3. The most probable processes leading to a population of the B³ state are thought to be direct electronic impact, cascade transitions, and collisions of normal molecules with molecules in the singlet state.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii Fizika, No. 2, pp. 57–63, February, 1971.     

Intensity distributions of spectral lines and elementary processes in a negative glow discharge column

The connection is established between the intensity distributions of the spectral lines along a negative glow discharge column and the individual elementary processes which take place in a low-temperature nonequilibrium plasma (direct electron excitation, step processes, recombination, collisions of the second kind, and charge exchange). The experiments were made in pure inert gases and mixtures of them at pressures 1–30 mm Hg and discharge current densities of 10^–2–10⁺¹ mA/cm². Knowledge of the intensity distributions together with some additional data (such as the electron density, the energy distribution function of the electrons, and the population of the levels) makes it possible to estimate more accurately the rates and cross sections of the reactions which lead to excitation of the glow discharge.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 7, pp. 41–49, July, 1980.     

Investigation of the excitation of nitrogen molecules in the positive column of a discharge in a mixture of CO2 and N2

The absolute populations of the electron states of the nitrogen molecule C³_u and B³_g in the positive column of a discharge in a mixture of CO₂ and N₂ at an overall pressure of 2.5 mm Hg, a ratio of the components of 11, and a current of 60 mA, are determined. An estimate is made of the possibility of exciting the electron state C³_u by direct electron collision and by multistage excitation from the electron state B³_g. It is suggested that the most probable process by which the electron state C³_u is excited is multistage excitation from vibrational levels of the electron state B³_g.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 10, pp. 49–52, October, 1972.     

A μSR study of spin density wave condensation in Cr85Mo15

Zero field SR spectra from Cr₈₅Mo₁₅ are well described by the sum of a lightly damped (0.02s^–1<₁<0.2s^–1) and a heavily damped (2s^–1<₂<15s^–1) exponential. The temperature dependence of these components is discussed in relation to the condensation of the incommensurate spin density wave and the onset of the antiferromagnetic state in this Cr-like alloy below T_N=120K. Evidence is presented for the nucleation of the spin density wave at temperatures greater than 1.5T_N.     

Relative populations of vibrational levels in nitrogen B3πg state in glow discharge

The relative populations of the first through sixth vibrational levels are determined for the nitrogen molecule B³_g state in a glow discharge. Deviation from Boltzmann's law is observed for distribution of the molecules over the vibrational levels for the B³_g state.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 2, pp. 64–68, February, 1972.     

Estimating gas temperature in the channel of a high-temperature jet discharge in air

Consideration is made of determining gas temperature in the channel of a high-frequency jet discharge in air over the intensity distribution of lines for the rotational spectrum band for the transition A² X²II (0-0) in the radiation of hydroxyl. It is shown that the branches R₂ and Q₁ of this band are the most useful for temperature measurements at atmospheric pressure. Within error limits, the temperature in the discharge channel as determined from the lines of the R₂-branch is T_gas = (3120 ± 70) and (3380 ± 90) K in the cross sections of the discharge at a distance of 3 and 30 mm, respectively.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 2, pp. 3–7, February, 1987.     

73Ge: a new high resolution PAC probe

Long lens electron spectrometers were used to make electron-gamma and electron-electron PAC measurements for the 5/2⁺ 13.3 keV state of⁷³Ge. Sources of⁷³As were produced in the decay of⁷³Se implanted at the CERN/ISOLDE facility. The magnetic interaction in nickel was determined as _L=74.2(7) Mrad s^–1 and the quadrupolar frequency in antimony asv _Q =19.7(2) MHz. The nuclear moments derived are =–1.08(3) _N and |Q|=0.70(8) b.