Nonlinear steady-state sized resonances in diatomic nanostuctural objects

A new solution to modified Bloch equations for a diatomic quantum system consisting of two identical interacting atoms in a field of high-intensity continuous radiation is obtained. On the basis of this solution, the existence of nonlinear sized resonances whose properties strongly depend on the atomic spacing, on the polarization of the external field of radiation, and on the initial inversions of atoms constituting a nanostructural object is shown. Dispersion dependences of induced dipole moments and inversions of atoms of the object are investigated theoretically in the region of sized resonances for various irradiation conditions.     

Excitation of Rydberg states of atoms and diatomic molecules by short laser impulses

Excitation of multilevel Rydberg states (atoms and diatomic molecules) is studied under an intense time-periodic perturbation that is instantaneously turned on and off. For a one-quantum excitation from a lower lying state, general expressions for the Laplace images of the population amplitudes of Rydberg states are obtained with regard to their decay characteristics. It is shown that the problem considered is reduced to the determination of the positions and widths of the energy levels of a quantum system in the field of monochromatic laser radiation of the same frequency and intensity as that in a pulse mode. To determine these quantities, an integral formulation is proposed for the eigenvalue problem for energies that is relatively simply solved with regard to the effect of the ionic core and its complex vibration-rotation structure on diatomic molecules. The specific features of the excitation of Rydberg states and the behavior of Rydberg wave packets are studied depending on the intensity and duration of laser radiation. A quantum phenomenon of rotational orientation of electron-excited diatomic molecules is considered.     

Linear nonstationary optical dimensional resonances in atomic nanostructures

The existence of linear nonstationary optical resonances in a diatomic nanostructural object with a dipole-dipole atomic interaction has been proved. A new solution to the joint system of modified Bloch optical equations and nonlocal field equations is obtained for time intervals much shorter than the times of phase and energy relaxation. Formulas for effective polarizabilities of the object’s atoms, which have a set of dimensional resonances, are derived. The frequencies of these resonances significantly differ from the eigenfrequencies of the object’s atoms, and their properties depend on the interatomic distance, light-pulse duration, initial atomic inversions, and the orientation of the object’s axis relative to the direction of incidence of the external light wave.     

Nonlinear resonances in the near-field interaction between atoms

It has been shown that nonlinear near-field optical resonances occur in diatomic nanostructures consisting of identical or different two-level atoms in the presence of a radiation field when the dipole-dipole interaction is taken into account. The frequencies of these resonances depend strongly on the intensity of the external optical radiation, on the initial conditions, on the polarization of the external field with respect to the axis of the nanostructure, and on the interatomic distance. The interatomic interaction is taken into account beyond perturbation theory. For this reason, the effective polarizabilities of the atoms of the nanostructure are expressed in terms of the polynomials of both the interatomic distance and the electric field strength of the external optical wave. A “falling tower” effect that is caused by the nonlinear behavior of the local dipole moments of atoms in the nanostructure is predicted.     

Calculation of the fluorescence spectrum of two interacting atoms in external field

The radiation line profile for two identical dipole-dipole interacting two-level atoms in an external laser field is calculated. The stochastic component of the laser radiation is explicitly taken into account simulating it by the optical white noise. An explicit analytical expression for the radiation line profile is found for the case where the regular field component can be neglected.     

Collision of atoms under action of external magnetic and laser radiation fields with formation of Fano-Feshbach resonances

We investigate collision of two atoms in an external magnetic field and in the field of laser radiation with formation of Fano-Feshbach resonances. At one-photon resonance of laser radiation with two discrete vibrational states of molecule the dressed states are formed (Autler-Townes effect) which form Fano-Feshbach resonances in interaction with the external magnetic field. In addition, the lower molecular vibrational state is coupled with the continuum of the elastic channel via also LICS (laser-induced continuum structure) forming laser-induced resonance. We obtain cross-sections of elastic and inelastic resonant scattering and expression for the scattering length depending on the external magnetic and laser radiation fields.     

Modulation resonance in a laser

The response of the active atoms of an operating laser to the modulation of their energy intervals by an external field is theoretically investigated. On the condition that the active atoms are strongly saturated by off-resonant laser radiation, the resonant peculiarities take place in response to the modulating field.     

Dynamics of moving interacting atoms in a laser radiation field and optical size resonances

The forces acting on interacting moving atoms exposed to resonant laser radiation are calculated. It is shown that the forces acting on the atoms include the radiation pressure forces as well as the external and internal bias forces. The dependences of the forces on the atomic spacing, polarization, and laser radiation frequency are given. It is found that the internal bias force associated with the interaction of atomic dipoles via the reemitted field may play an important role in the dynamics of dense atomic ensembles in a light field. It is shown that optical size resonances appear in the system of interacting atoms at frequencies differing substantially from transition frequencies in the spectrum of atoms. It is noted that optical size resonances as well as the Doppler frequency shift in the spectrum of interacting atoms play a significant role in the processes of laser-radiation-controlled motion of the atoms.     

Untersuchung der Eigenschaften der Strahlung eines Lasers ohne äußere Rückkopplung

The following article describes the realization of a laser without any external resonance structure and the behaviour of the emitted radiation. The experimental setup consits of a discharge tube closed with Brewster windows and the excitation electronics. The excitation process which brings the atoms to the upper laser level (2 p₆ Neon) will not establish any coherence between the atoms. Space coherence of the radiation has its origin in the correlated behaviour of the radiating atoms. Theoretical and experimental values of the fringe visibility are in close agreement for a path difference till to 440 cm, if temporal coherence is measured in an MICHELSON experiment. Interference fringes result if the radiation emerging from both sides of the tube is superimposed. The contrast decreases rapidly with the number of radiation pulses producing the interference pattern.     

Spectroscopic temperature determination of aluminum monoxide in laser ablation with 266-nm radiation

We report time-resolved measurements of diatomic aluminum monoxide spectra in the study of laser ablation by the use of frequency-quadrupled 266 nm Nd:YAG laser radiation. Spectroscopic temperatures of 3432(35) K and 3329(13) K are obtained at a delay time of 20mu, respectively, by the use of the modified diatomic Boltzmann plot and by the use of the Nelder-Mead algorithm in the fitting of the recorded spectrum.     

Few-cycle attosecond pulses via periodic resonance interaction with hydrogenlike atoms

We show that it is possible to produce nearly bandwidth-limited few-cycle attosecond pulses based on periodic resonance interaction of a quasi-monochromatic radiation with the bound states of hydrogenlike atoms. A periodic resonance is provided by a far-off-resonant laser field with intensity much below the atomic ionization threshold via periodic tunnel ionization from the excited states and adiabatic Stark splitting of the excited energy levels. Without external synchronization of the spectral components, it is possible to produce 135 as pulses at 13.5 nm in Li2?-plasma controlled by radiation of a mode-locked Nd:YAG laser, as well as 1.25 fs pulses at 122 nm in atomic hydrogen controlled by radiation of a CO? laser.     

Spontaneous emission by two atoms with different resonance frequencies near a metal surface. II

The quantum-mechanical image method is extended to consider the interaction between the electromagnetic radiation and two different atoms with their electronic transition dipoles oriented in arbitrary directions near a perfectly conducting metal surface. The atom-atom and atom-surface separations are assumed to be smaller than the corresponding mean resonance wavelength. A general form of atom-image correlation state is constructed for the arbitrarily oriented atomic dipole and its physical interpretation is given. Based on this generalized formulation, the total emission rate is calculated for the diatomic system in several experimentally preparable initial states, whose initial emission rates are found to be dependent on the orientation of the emitting dipoles. These peculiar emission pattern can be accounted for by the dependence of the phase relations between the constituent terms of the diatomic states on the dipole orientation. Detailed examination in this regard is addressed, as an example, to the antisymmetric diatomic state.     

Near-field effect in two-atom system

The self-consistent problem is solved for the interaction of two dipole atoms situated at arbitrary distance from one another with the field of quasiresonant light wave. Atoms are considered to be linear Lorenz oscillators. Polarizing fields inside the system include both Coulomb and retarding parts. The solutions obtained are investigated for the case when atoms have the same polarizabilities and interatomic distance is much less than external light wavelength. Formulas for electric fields inside and outside of small object are obtained. It is shown that longitudinal and transverse optical oscillations are possible to exist inside small two-atom object. Dispersion laws of these oscillations depend upon interatomic distance and upon angle between axis of the system and the direction of propagation of external wave. The field outside the small object in wave zone is linearly polarized with the choice of linear polarization of external field. However, the directions of polarization of these waves are different and depend essentially upon frequency. The amplitude of field outside small object in wave zone is shown to depend essentially on the frequency of external field and interatomic distance. The results obtained are treated as near-field effect in the optics of small objects making it possible to investigate the structure of small objects with optical radiation. Received 26 October 1998 and Received in final form 26 January 2000     

强激光场中双原子分子多光子激发的李代数方法

用“模拟势－李代数”方法研究了双原子分子在强激光场中的多光子振动激发，计算了跃迁几率与外场频率、时间的关系，讨论了有两个激光场时跃迁儿率所受的影响． 关键词：     

Kinetic energy release of diatomic and linear triatomic molecules in intense femtosecond laser fields

The kinetic energy release of fragment ions produced by the interaction of femtosecond laser pulse radiation with diatomic and linear triatomic molecules N_2, CO, CO_2 and CS_2 is investigated. In the case of linear polarization, angles at which the kinetic energy release of ions has the maximum value are different from the alignment of molecules though the kinetic energy release of fragment atomic ions depends on the angle between the laser polarization vector and the detection axis of the time-of-flight. For the diatomic molecules, the critical internuclear distance in multielectron dissociative ionization with a circularly polarized light is larger than that with a linearly polarized light. For linear triatomic molecules, our data indicate that a concerted Coulomb explosion process is a universal phenomenon in the interaction of molecules with intense laser fields, even in the circularly polarized regime. During two C－O (or C－S) bonds breaking simultaneously, the C ion obtained larger energy in circular polarization than that in the linear polarization. Different variations of kinetic energy release between the diatomic and the linear triatomic molecules are discussed.     

Near-field effect in optics of small objects composed of dipole atoms

A self-consistent problem of interaction of two dipole atoms separated by an unrestricted distance with the field of a quasi-resonance light wave was solved on the assumption that the investigated atoms are Lorentz linear oscillators and the polarizing fields inside the system consist of the Coulomb and the retarded parts. The solution obtained was investigated for the case where the atoms have the same polarizability and the distance between them is much smaller than the length of the external light wave. Formulas for the electric fields inside a small object and outside it have been obtained. It is shown that inside a small two-atom object there can take place longitudinal and transverse optical vibrations accompanied by corresponding dispersion effects depending on the interatomic distance and the angle between the axis of the system and the direction of propagation of the external light wave. The field outside the small object in the wave zone is linearly polarized when the external wave has linear polarization. However, the direction of polarization of the corresponding waves is largely determined by their frequency. It is also shown that the amplitude of the field outside the small object in the wave zone depends greatly on the frequency of the external field and the interatomic distance. The effects observed are considered as a near-field effect in optics of small objects. This phenomena makes it possible to investigate the structure of small objects with the use of optical radiation. Ul'yanovsk Branch of the Institute of Radio Engineering and Electronics, Russian Academy of Sciences, 48 Goncharov Str., Ul'yanovsk, 432700, Russia; e-mail: gadomsky@quant.univ.simbirsk.su. Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 66, No. 6, pp. 765–770, November–December, 1999.     

Ground state of a Bose-Einstein condensate which scatters coherently laser radiation

We present a self-consistent method of taking into account back action of a laser radiation to a Bose-Einstein condensate of neutral atoms. The light is coherently scattered inside the degenerate atomic sample, thus its intensity and, consequently, the atomic ground level AC Stark shift are spatially varying. This leads to a small deformation of the atomic cloud and, if the external radiation is abruptly switched off, to generation of collective excitations. Received 8 May 1999 and Received in final form 11 October 1999     

Interference phenomena at the elastic collision of atoms with formation of the Feshbach resonance in the presence of laser radiation field

Resonant scattering of atoms with formation of the Feshbach resonance in the presence of a laser radiation coupling the levels of two bound atoms (a molecule) is considered. The laser field leads to a second resonance in scattering and broadening of resonances, which facilitates the possibility of experimental observation of asymmetry of the total scattering cross-section arising because of interference between resonant and potential scatterings. The effects associated with interference of the two channels of decay of a bound system of two atoms (a molecule) in the laser field are studied. An expression is obtained for the scattering length in collision of two cold atoms in the field of laser radiation.     

Micro-Raman scattering by laser-modified structures with Ge/Si quantum dots

Structures with self-assembled Ge/Si quantum dots grown by molecular-beam epitaxy are exposed to pulsed radiation of a picosecond laser. Changes in the vibrational spectrum of nanostructures under an external action are studied by Raman spectroscopy. An analysis of the Raman spectra measured with a micron spatial resolution along the exposed region indicates a mixing of Ge and Si atoms and a change in the induced mechanical stresses in quantum dots.