相对论无规位相近似

讨论了建立在相对论平均场基态的相对论无规位相近似研究中的一致性问题. 研究表明考虑费米海和Dirac海的粒子 空穴激发对核的同位旋标量巨共振的能量有很大的影响. The fully consistent relativistic random phase approximation (RRPA) built on the relativist mean field (RMF) ground state is presented. The fully consistent RRPA requires that the nuclear RMF wave function and the RRPA renormalization are calculated in a same effective Lagrangian. A theoretically complete treatment of the RRPA at the mean field level with no sea approximation must include not only the usual particle hole states, but also the pairs formed from the occupied Fermi states and Dirac states. Effects of inclusion of Dirac sea states in various multipole excitations are investigated. Considerable effects on the isoscalar giant multipole resonances are observed.     

核的巨单极激发的求和规则和核物质的不可压缩性系数

采用近来在研究核基态中极为成功的相对论模型研究有限核的同位旋巨单极共振 ,从而给出核物质的不可压缩性系数 .讨论了建立在相对论平均场基态上的相对论无规位相近似的自洽处理 .自洽要求基态和巨共振激发态的研究从同一个有效拉氏量出发 .与相对论平均场的无海近似自洽 ,相对论无规位相近似不仅要包含正能态的粒子 -空穴激发 ,还必须考虑 Fermi海核子态和 Dirac海核子态激发的贡献 .用约束的相对论平均场方法得到核的巨单极共振的能量逆权重的求和规则 ,验证 Dirac海核子态的贡献 .比较理论计算和实验测量的巨单极共振的能量得到核物质的不可压缩性系数为 2 5 0 - 2 70 MeV. The isoscalar giant monopole resonance for finite nuclei and the nuclear matter incompressibility are studied in a consistent relativistic approach, which achieves a great success in describing the properties of nuclear ground states. The consistency in the relativistic random phase approximation (RRPA) built on the relativistic mean field (RMF) ground states are investigated. The RMF wave function of nucleus and the particle-hole residual interactions in RRPA are calculated from...     

Sum Rule in a Consistent Relativistic Random-Phase Approximation

A fully consistent relativistic random-phase approximation (RRPA) is studied in the sense that the relativistic mean-field (RMF) wavefunction of nucleus and the particlehole residual interactions in the RRPA are calculated from the same effective Lagrangian. A consistent treatment of RRPA within the RMF approximation, i.e., no sea approximation, has to include also the pairs formed from the Dirac states and occupied Fermi states, which is essential for satisfying the current conservation. The inverse energy-weighted sum rule for the isoscalar giant monopole mode is investigated in the constrained RMF. It is found that the sum rule is fulfilled only in the case where the Dirac state contributions are included.     

2s1/2—1d3/2壳层原子核能谱的壳模型分析

本文对2s_1/2-1d_3/2壳层原子核(A=30—40)能谱作了系统分析,计算仅限于由2s_1/2和1d_3/2支壳层产生的情态,但考虑了它们之间的全部组态混合效应。计算是采用多粒子壳模型的Talmi方法,将二体矩阵元当作参数,其值由实验确定。文中详细分析了Si³⁰,Si³¹,P³⁰,P³¹,P³²,S³²,Ar³⁷,Ar³⁸,K³⁸等原子核能谱,理论与实验符合颇好。     

Photoionization of some closed shell atoms and ions

Dipole-allowed single photoionization of some closed shell atoms and ions has been investigated in the relativistic random-phase approximation (RRPA). Application of relativisticmultichannel quantum defect theory (RMQDT) is made together with RRPA to analyse autoionizing resonances. Analysis points to the importance of interchannel coupling in high energy photoionization and reveals various degeneracies in relativistic atomic spectra to influence the low energy dynamics. Interesting threshold behavior in photoelectron spin polarization has been seen. Prospective future studies have been indicated.     

X-ray photoelectron spectra of nickel halides: multiplet structure and multi-electron excitations in Ni2+ 3p and 2p shells

The satellite structure in the X-ray photoelectron spectra of nickel halides has been measured. The satellites found in the photoelectron spectra of Ni²⁺ 3p and 2p subshells have two common sources: multiples splitting and multi-electron excitations. The experimental spectra are compared with theoretical results on multiples splitting and with calculations of band structure.     

Application of the second—order ground—state correlation and random—phase approximation on photoionization cross section of manganese

Using the many-body perturbation theory,we have calculated the photoionization cross section of 3p and 3d subshells of the neutral manganese,and discussed the second-order ground-state correlation and random-phase approx-imation correlations in detail.This is the first theoretical calculation for manganese as far as we know .our calculated results are more consistent with the experimental results than those given by other methods in the literature.     

C原子、离子光电离过程的规律研究

 基于Dirac-Slater自洽场方法,计算了C原子及各价离子从低能到高能的光电离截面。通过各种理论计算结果的比较,分析了Kramers公式的适用性。定量地考察了多极效应和相对论效应在不同能区对光电离截面的影响,并研究了光电离截面随光子能量、壳层、电离度变化的规律。     

类Li硼离子内壳层三重激发态2s2p~2的结构和俄歇过程

采用基于全相对论框架的多组态Dirac-Fock方法,研究了类Li硼离子内壳层三重激发态2s2p~2的结构和俄歇退激发过程.为了充分考虑电子关联效应,将活动空间扩展到n=8壳层.详细讨论了电子关联效应对类Li硼离子内壳层三重激发态2s2p~2结构和俄歇退激发过程的影响.结果表明,在对类Li硼离子内壳层三重激发态2s2p~2进行理论研究时,有必要考虑来自n=8壳层的电子关联效应.本文模拟的类Li硼离子内壳层三重激发态2s2p~2的俄歇电子谱与实验符合好.     

类Li硼离子内壳层三重激发态2s2p2的结构和俄歇过程

采用基于全相对论框架的多组态Dirac-Fock方法,研究了类Li硼离子内壳层三重激发态2s2p2的结构和俄歇退激发过程。为了充分考虑电子关联效应,将活动空间扩展到n=8壳层。详细讨论了电子关联效应对类Li硼离子内壳层三重激发态2s2p2结构和俄歇退激发过程的影响。结果表明,在对类Li硼离子内壳层三重激发态2s2p2进行理论研究时,有必要考虑来自n=8壳层的电子关联效应。本文模拟的类Li硼离子内壳层三重激发态2s2p2的俄歇电子谱与实验符合好。     

Selective excitation,coherent control,and attosecond spectrochronography of electron subshells in atomic systems

Optical field waveforms with an ultrabroad spectrum and a tailored phase are shown to enable selective excitation, coherent control, and attosecond spectrochronography of electron subshells in many-electron atomic systems. Analysis of the evolution of the density matrix of electron subshells in an atomic system driven by an ultrashort light pulse shows that the interference of different quantum pathways of electron dynamics plays a key role in the buildup of the nonlinear-optical response of such a system. Our analysis suggests a method whereby the attosecond dynamics of individual electron subshells in atoms can be coherently controlled with ultrashort laser pulses.     

X-ray photoionization cross sections for quantitative analysis

The relative photoemission intensities from subshells of 51 elements and simple compounds have been measured using X-ray photoelectron spectroscopy. The chemical composition of each specimen surface was monitored by Auger electron spectroscopy and contamination was minimized by Ar⁺ ion bombardment. Experimental photoelectron cross sections derived for MgKα (1254 eV) radiation were compared with theoretical Hartree-Slater subshell photoionization cross sections calculated by Scofield. Good correlation (r = 0.96) between theory and experiment was observed over two orders of magnitude for most of the elements studied. Relative cross sections for subshells of a given element are also consistent with theoretical values, with several notable exceptions. The results indicate that quantitative analysis of ESCA spectra is possible using the Scofield cross sections.     

Photoionization calculations for 5d, 5p,and 4f subshells of mercury

Photoionization cross section, branching ratio, and photoelectron angular distribution for intermediate 5d, 5p, and 4f subshells of mercury are calculated in the relativistic random-phase approximation. Comparison of the present results with the earlier results in the Hartree-Fock approximation shows the importance of correlations and relativistic effects.     

Parameters of the <Superscript>64,66,68,70</Superscript>Zn single-particle structure

Populations and energies of neutron subshells in ^{64, 66, 68, 70}Zn and proton subshells in ^{64, 66, 68}Zn are found from the joint evaluation of the data on stripping and pickup reactions and data on spins and parities of nuclear states. The analysis of the thus obtained parameters made it possible to find population features of the nucleon subshells in the nuclei mentioned. A relation between these features and the available data on the first excited 2⁺ states and deformations in this region of nuclei is shown.     

Atom-solid 3p level binding energy shift of transition metals Cr,Mn, Fe,Co, and Ni

Binding energy shifts between atomic and solid phases for transition metals Cr, Mn, Fe, Co, and Ni have been obtained for 3p subshells from simultaneously recorded atomic vapor and solid state spectra. This experimental technique provides higher accuracy in comparison to separate measurements and allows direct determination of the shifts. The observed shift values are compared to values obtained using the semiempirical Born–Haber cycle method and the peak structures of the solid state photoelectron spectra are compared to atomic 3p spectra. The binding energy shift of Cr is found to be much smaller than that of the other studied elements.     

Average 2p subshells fluorescence yield values of some elements in the atomic number range 60 ≤ Z ≤ 90

The average 2p (L_2,3) subshells fluorescence yield (?_2,3) in 11 elements with Z ranging from 60 to 90 were measured with corporation of total L_2,3 X-ray production cross-sections. Measurements were carried out exciting L₂ and L₃ subshells of relevant elements that were exposed to beam of selected K X-rays from secondary sources. The measured values were compared with theoretical and semi-empirical values. It is clear that the present values of experimental ?_2,3 are generally smaller than the calculated and semi-empirical values for some elements in the atomic number range 60–90.