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1.
丁晓彬  董晨钟 《物理学报》2004,53(8):2490-2496
在相对论多组态Dirac-Fock理论方法基础上,通过系统考 虑电子关联效应和由于内壳层电子激发而导致的电子自旋-轨道波函数的弛豫效应,详细研究了Cs Ⅳ离子的4d内壳层电子激发组态4d95s25p5、辐射末态4d105s25p4及Auger末态4d105s25p3和4d105s15p4的能级结构及各种可能的辐射和Auger衰变过程.获得了与已有的实验结果和相关的半经 验准相对论组态相互作用计算结果相符的辐射跃迁能、振子强度以及线宽,预言了4d95s25p5态的以Auger衰变为主的 Auger电子谱的特 关键词: 内壳层激发态 辐射衰变 Auger衰变  相似文献   

2.
利用基于多组态Dirac-Fock方法的程序包GRASP92和RATIP以及最新发展的RERR06程序,详细计算了高离化态金离子(类镍Au51+、类铜Au50+和类锌Au49+)俘获一个自由电子到nl(n=4—8,l=0—3)壳层的辐射复合谱以及相应的辐射退激发谱.理论计算的辐射复合谱很好地重现了实验谱.研究结果表明:对类镍Au51+、类铜Au50+和类锌Au49+而言,将一个自由电子俘获到n=4壳层的概率最大;在辐射复合过程之后,处在n=4壳层的俘获电子的辐射退激发谱线最强,并且体现了整个辐射退激发谱的主要特征.  相似文献   

3.
朱志艳  朱正和  高涛  蒋刚 《物理学报》2004,53(10):3330-3335
基于全相对论多组态Dirac-Fock理论,采用“多功能相对论原子结构程序(GRASP2)”,考虑量子电动力学(QED)效应和Breit修正,涉及实验谱中Au等离子体M带的几类重要跃迁,计算了Au48+—Au52+离子的能级结构和能级简并度.用统计热力学方法计算 各离子的配分函数,由配分函数计算等离子体内这五种离子的电离与复合平衡常数,根据同 时反应的平衡理论研究电离与复合达到平衡时等离子体内各离子的相对分布. 关键词: 金等离子体 配分函数 平衡常数 离子丰度  相似文献   

4.
电子离子碰撞激发强度在超组态碰撞辐射模型中真实模拟非局域热动平衡金激光等离子体M带谱跃迁中离子的平均电离度、电荷态分布和能级布居数等离子的电离态特性是必不可少的.基于全相对论扭曲波电子碰撞激发计算程序REIE06,系统计算了高离化态金离子(Au51+、Au50+、Au49+)精细结构能级3d→4f和3d→5f的碰撞强度,计算中详细考虑了电子关联效应和Breit相互作用对碰撞强度的影响.计算结果与可获得的其它理论及实验结果进行了比较,取得了好的一致性.  相似文献   

5.
用超组态碰撞辐射模型模拟非局域热动力学平衡中Au的M带谱5f-3d跃迁的离子电离态特性,激光等离子体的光谱跃迂参数是必不可少的。利用多组态Dirac-Fock广义扩展平均能级方法,用GRASP^2系统地计算了激光Au等离子体中类铁金离子-类锗金离子的M带谱5f-3d的光谱跃迁波长.跃迁几率和振子强度,计算中考虑了重要的核的有限体积效应、Breit修正和QED修正,所得结果和最近的实验数据及理论计算值进行了比较。此结果可应用于对激光等离子体的模拟和诊断。  相似文献   

6.
基于全相对论多组态Dirac Fock理论 ,采用“多功能相对论原子结构程序 (GRASP2 )” ,考虑量子电动力学 (QED)效应和Breit修正 ,涉及实验谱中Au等离子体M带的几类重要跃迁 ,计算了Au4 8 —Au52 离子的能级结构和能级简并度 .用统计热力学方法计算各离子的配分函数 ,由配分函数计算等离子体内这五种离子的电离与复合平衡常数 ,根据同时反应的平衡理论研究电离与复合达到平衡时等离子体内各离子的相对分布基于全相对论多组态Dirac Fock理论 ,采用“多功能相对论原子结构程序 (GRASP2 )” ,考虑量子电动力学 (QED)效应和Breit修正 ,涉及实验谱中Au等离子体M带的几类重要跃迁 ,计算了Au4 8 —Au52 离子的能级结构和能级简并度 .用统计热力学方法计算各离子的配分函数 ,由配分函数计算等离子体内这五种离子的电离与复合平衡常数 ,根据同时反应的平衡理论研究电离与复合达到平衡时等离子体内各离子的相对分布  相似文献   

7.
师应龙  董晨钟 《物理学报》2009,58(4):2350-2357
在相对论多组态Dirac-Fock理论方法基础上,通过系统考虑电子关联效应、弛豫效应以及相对论高阶修正,详细研究了C Ⅱ离子1s-2p光激发形成的内壳层电子激发态(1s2s22p2和1s2s2p3)、辐射和Auger末态的能级结构以及各种可能的衰变过程.计算了C Ⅱ离子1s内壳层光激发能量、辐射和Auger衰变率及其线宽,进一步由不确定关系推出了这些激发态的能级寿命,并与最新的实验结果和已有的理论结果进行了比较. 关键词: 内壳层激发态 线宽 寿命 多组态Dirac-Fock方法  相似文献   

8.
根据扩展的全相对论多组态Dirac-Fock理论,采用"多功能相对论原子结构程序GRASP2(General-Purpose Relativistic Atomic Structure Program 2,1992),考虑量子电动力学(QED)效应和Breit修正,结合惯性约束聚变(ICF)实验室等离子体中已经观察到的激光照射Au元素所产生的一些多重电荷态离子的外壳层共振线跃迁光谱,选取重要的电子组态,计算激光金等离子体中类镓Au48+离子的光谱跃迁波长、能级寿命和能级宽度.计算所得波长值与实验值符合较好,能级寿命与能级宽度的大小关系符合海森堡的能量与时间测不准原理.计算结果对金等离子体中的离子平均寿命、电荷态分布和平均电离度的研究具有一定的参考价值.  相似文献   

9.
在全相对论理论框架下,研究了类In等电子序(Ba VIII-Nd XII)低激发态组态5s~24f和5s`25p间的光谱性质.系统地研究了Breit相互作用和量子电动力学(QED)效应对能级的影响.离子Pr~(~(10+))附近出现相对论轨道4f-5p能级交叉,窄的能级间隔可以使得跃迁波长在现代激光范围,这可能设计成原子钟.计算得到Pr~(10+)基态和激发态磁偶极和电四极超精细结构常数.目前的计算结果可以为实验测量提供理论依据.  相似文献   

10.
辐射复合过程在超组态碰撞辐射(SCROLL)模型中真实模拟非局域热动力学平衡(non-LTE)高Z材料Au激光等离子体M带谱5f-3d跃迁中各种复杂离子的电离态特性是一个主要过程.基于准相对论多组态Hartree-Fock理论和扭曲波近似,采用组态平均的方法,从头计算了金M带类铁金离子-类锗金离子的辐射复合速率系数,计算过程中包含了大量的单激发和双激发态,结果表明高Z元素由于自电离能级的广泛分布和复杂的级联效应,致使高Z元素的辐射复合系数不同于低Z元素的,其计算结果可用来模拟Au的激光等离子体M带5f-3d跃迁的平均电离度和电荷态分布及能级布居数.  相似文献   

11.
K. P. Santhosh  R. K. Biju 《Pramana》2009,72(4):689-707
Based on the concept of cold valley in fission and fusion, the radioactive decay of superheavy280–314116 nuclei was studied taking Coulomb and proximity potentials as the interacting barrier. It is found that the inclusion of proximity potential does not change the position of minima but minima become deeper which agrees with the earlier findings of Gupta and co-workers. In addition to alpha particle minima, the other deepest minima occur for 8Be, 12,14C clusters. In the fission region two deep regions are found each consisting of several comparable minima, the first region centred on 208Pb and the second is around 132Sn. The cluster decay half-lives and other characteristics are computed for various clusters ranging from alpha particle to 70Ni. The computed half-lives for alpha decay match with the experimental values and with the values calculated using Viola-Seaborg-Sobiczewski (VSS) systematic. The plots connecting computed Q values and half-lives against neutron number of daughter nuclei were studied for different clusters and it is found that the next neutron shell closures occur at N = 162, 172 and 184. Isotopic and isobaric mass parabolas are studied for various cluster emissions and minima of parabola indicate neutron shell closure at N = 162, 184 and proton shell closure at Z = 114. Our study shows that 162276114 is the deformed doubly magic and 184298114 is the spherical doubly magic nuclei.   相似文献   

12.
Half-life time and branching ratio for cluster decay from various xenon isotopes are studied taking Coulomb and proximity potentials as interacting barrier. Inclusion of proximity potential reduces the height of potential barrier, which closely agrees with the experiments. It is found that4He,8Be,12C and16O emissions are well within the present upper limit for measurements (T 1/2 1030 s). Our predicted half-life time values lie close to those values reported by Gupta and collaborators based on preformed cluster model (PCM) and also with those values reported by Poenaruet al based on ASAFM. The calculated half-life time shows that8Be from108Xe and110Xe are most favourable for emission (T 1/2 ≈ 108 s). LowestT 1/2 value for8Be emission from108Xe stress the role of doubly magic100Sn daughter in cluster decay process. The logarithm of half-life time calculated for4He emission from110Xe is −0.39 s which is in good agreement with experimental value which is −0.40 s. Geiger-Nuttall plots for all clusters are studied and are found to be linear. Nuclear structure effect and shell effect are evident from the observed variation in slope and intercept of Geiger—Nuttall plots. It is found that neutron excess in the parent will slow down the cluster decay process.  相似文献   

13.
Based on the concept of cold valley in cold fission and fusion, we have investigated the cluster decay process in 248–254Cf isotopes. In addition to alpha particle minima, other deep minima occur for S, Ar and Ca clusters. It is found that inclusion of proximity potential does not change the position of minima but minima become deeper. Taking Coulomb and proximity potential as interacting barrier for post-scission region, we computed half-lives and other characteristics for various clusters from these parents. Our study reveals that these parents are stable against light clusters and unstable against heavy clusters. Computed half-lives for alpha decay agree with experimental values within two orders of magnitude. The most probable clusters from these parents are predicted to be 46Ar, 48,50Ca which indicate the role of doubly or near doubly magic clusters in cluster radioactivity. Odd A clusters are found to be favorable for emission from odd A parents. Cluster decay model is extended to symmetric region and it is found that symmetric fission is also probable which stresses the role of doubly or near doubly magic 132Sn nuclei. Geiger-Nuttal plots were studied for various clusters and are found to be linear with varying slopes and intercepts.   相似文献   

14.
Cluster decay of superdeformed76, 78, 80Sr isotopes in their ground state are studied taking the Coulomb and proximity potential as the interacting barrier for the post-scission region. The predictedT 1/2 values are found to be in close agreement with those values reported by the preformed cluster model (PCM). Our calculation shows that these nuclei are stable against both light and heavy cluster emissions. We studied the decay of these nuclei produced as an excited compound system in heavy-ion reaction. It is found that inclusion of excitation energy increases the decay rate (decreasesT 1/2 value) considerably and these nuclei become unstable against decay. These findings support earlier observation of Guptaet al based on PCM.  相似文献   

15.
The mass spectrum ofcb meson is investigated with an effective quark-antiquark potential of the form -αc/r +Ar νwith ν varying from 0.5 to 2.0. TheS andP-wave masses, pseudoscalar decay constant, weak decay partial widths in spectator model and the lifetime ofB cmeson are computed. The properties calculated here are found to be in good agreement with other theoretical and experimental values at potential index,ν = 1  相似文献   

16.
The recent observations of the purely leptonic decay Ds+→μ+νμ and τ+ντ at CLEO-c and B factory may allow a possible contribution from a charged Higgs bosom One such measurement of the decay constant fDs differs from the most precise unquenched lattice QCD calculation by a level of 4σ.Meanwhile,the measured ratio,BR(D+s+→μ.+νμ)/BR(D+→μ+νμ),is larger than the standard model prediction at a 2.0σ level.We discuss that the precise measurement of the ratio BR(Ds+→μ+νμ)/BR(D+μ+νμ) at BES-Ⅲ will shed light on the presence of new intermediate particles by comparing the data with the theoretical predictions,especially,the predictions of high precise unquenched lattice QCD calculations.  相似文献   

17.
We report on the final analysis of a search for the decay μ+→e+γ performed at SIN. No evidence for the existence of the process has been found. An upper limit for the branching ratio of 1.0 × 10?9 (90% confidence) is presented. The measured positron-photon energy distributions are completely described by the decay μ+e+νeνμγ and accidental coincidences.  相似文献   

18.
利用32S轰击106Cd靶,通过3p4n反应产生了131Pm,反应产物经过毛细管及带收集传输系统传输到低本底区,测量了反应产物的X,γ单谱,并进行了X-γ,γ-γ符合测量,得到了131Pm的半衰期及衰变γ线,并建立了简单的衰变纲图.  相似文献   

19.
Considering Coulomb and proximity potentials as barriers, we have calculated the half lives for 12C emission from various Ba isotopes using different mass tables. The half life for 112Ba isotope calculated by us is 6.020×103 s which is comparable with the experimental value 5.620×103 s. From our study it is found that 114Ba is the good parent for 12C emission whose emission rate is favorable for measurement. The half lives predicted by us lie very close to those reported by Shanmugam et al using their cubic plus Yukawa plus exponential model. It is observed that inclusion of proximity potential does not produce significant deviation from the linear nature of the Geiger-Nuttall plots. Also it is found that the neutron excess in the parent nuclei slows down the exotic decay process.  相似文献   

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