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本文测量了不同氘含量K(H1-xDx)2PO4晶体(DKDP晶体)在Z(XX)Y散射配置下的自发拉曼散射光谱, 并详细分析了氘含量对与横向受激拉曼散射(TSRS)增益系数有关的拉曼频移、半峰宽和散射强度的影响. 然后通过与去离子水拉曼散射对比得出了不同氘含量DKDP晶体的TSRS增益系数. 结果表明随着氘含量的增加DKDP晶体的TSRS增益系数先减小至KDP晶体的40.1%, 后增大至68.9%; 本文认为掺氘后拉曼半峰宽的变化是引起TSRS增益系数随氘含量变化的主要原因. 相似文献
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采用腔外单次通过方式,研究了一种新型晶体YbVO4的受激拉曼散射.当抽运激光为532 nm皮秒脉冲时获得了3级斯托克斯线(558.47 nm, 587.92 nm, 620.67 nm)和1级反斯托克斯线(507.58 nm),测得YbVO4晶体1级斯托克斯受激拉曼散射的稳态增益系数为17.8±0.2 cm/GW,受激拉曼散射的整体转换效率达到37%.实现了YbVO4晶体对355 nm皮秒激光的受激拉曼散射,观察到1级斯托克斯线(366.1
关键词:
受激拉曼散射
稳态增益系数
转换效率
4晶体')" href="#">YbVO4晶体 相似文献
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大口径氘化磷酸二氢钾(DKDP)晶体抗激光损伤性能偏低严重地制约着大型高功率激光装置输出水平.本研究利用离线亚纳秒激光预处理技术有效地提升了大口径DKDP晶体抗激光损伤性能.实际使用情况表明,采用离线亚纳秒激光预处理后,DKDP晶体在9 J/cm2激光通量辐照下的表面平均损伤密度得到大幅下降,由未处理前的5.02 pp/cm2(1pp表示1个百分点)降至0.55 pp/cm2,降幅为一个数量级.同时,激光预处理对晶体损伤尺寸具有一定的抑制作用,预处理后晶体损伤点尺寸分布曲线向尺寸减小的方向平移,尺寸分布峰值由预处理前的25μm降至预处理后的18—20μm. 相似文献
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采用腔外单次通过方式,研究了一种新型晶体YbVO4的受激拉曼散射.当抽运激光为532 nm皮秒脉冲时获得了3级斯托克斯线(558.47 nm,587.92 nm,620.67 nm)和1级反斯托克斯线(507.58 nm),测得YbVO4晶体1级斯托克斯受激拉曼散射的稳态增益系数为17.8 4±O.2 cm/Gw,受激拉曼散射的整体转换效率达到37%.实现了YbVO4晶体对355 nm皮秒激光的受激拉曼散射,观察到1级斯托克斯线(366.11 nm),根据抽运阈值得到相应的拉曼增益为29.0±0.3 cm/GW. 相似文献
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详细比较了磷酸二氢钾(KDP)晶体的自发拉曼散射和受激拉曼散射光谱,在受激拉曼散射(SRS)中观察到了自发拉曼散射中最强的振动模的三阶Stokes光(559.43,589.74,623.50nm),由于其他振动模的受激拉曼散射增益系数较小,其SRS光谱未观察到。另外,比较了传统生长的未退火和退火后的KDP晶体及快速生长的锥区和柱区KDP晶体的受激拉曼散射增益系数,结果表明生长方法和热退火对KDP晶体的受激拉曼散射增益系数无明显影响。 相似文献
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报道了0.53μm高功率激光辐照金盘靶产生的受激拉曼散射光光谱和散射光谱能量角分布,由散射光角分布计算的散射光能量与实验通过打靶透镜测得的受激拉曼散射能量不符,而且角的分布的实验结果与受激布里渊散射理论也不符。 相似文献
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Transient stimulated Raman scattering (TSRS) of picosecond dye laser pulses in ethanol has been investigated experimentally. In particular some temporal features of TSRS from the C-H stretching mode (2928 cm-1) in ethanol have been studied with a Photochron II streak camera with subpicosecond time resolution. It is shown that the use of TSRS provides a simple method for producing picosecond pulses tunable over the spectral region ≈492–532 nm and 691–772 nm by tuning a passively mode-locked Rhodamine 6G dye laser from 575–630 nm. 相似文献
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Laser-induced modification at 355 nm of deuterated potassium dihydrogen phosphate(DKDP) crystals following exposure to nanosecond(ns) and sub-ns laser irradiation is investigated in order to probe the absorption mechanism in damage initiation. Laser damage resistance is greatly improved by sub-ns laser conditioning,whereas only a little improvement occurred after ns laser conditioning at the same laser fluence. Moreover, scattering and transmittance variations after the two types of laser conditioning indicate similar reduction of linear absorption. However, by contrast, large differences on nonlinear absorption modification are discovered using Z-scan measurement. This characteristic absorption modification by laser irradiation provides evidence that a nonlinear absorption mechanism plays a key role in damage initiation at 355 nm. 相似文献
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《中国物理 B》2015,(4)
In this paper, the Raman gain coefficients of ammonium dihydrogen phosphate(ADP) and potassium dihydrogen phosphate(KDP) crystals are measured. By using a pump source of a 30-ps, 532-nm laser, the gain coefficients of ADP and KDP are 1.22 cm/GW, and 0.91 cm/GW, respectively. While for a 20-ps, 355-nm pump laser, the gain coefficients of these two crystals are similar, which are 1.95 cm/GW for ADP and 1.86 for KDP. The present results indicate that for ultra-violet frequency conversion, the problem of stimulated Raman scattering for ADP crystal will not be more serious than that for KDP crystal. Considering other advantages such the larger nonlinear optical coefficient, higher laser damage threshold,and lower noncritical phase-matching temperature, it can be anticipated that ADP will be a powerful competitor to KDP in large aperture, high energy third-harmonic generation or fourth-harmonic generation applications. 相似文献
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Da-he Liu Jin-wei Shi Xu-dong Chen Min Ouyang Wen-ping Gong 《Frontiers of Physics in China》2010,5(1):82-106
The principle of a lidar based on Brillouin scattering is introduced. The basic physics of the Brillouin lidar is discussed.
The applications of the Brillouin lidar in remote sensing of the ocean, such as measurement of the sound speed and the bulk
viscosity of water and detecting submerged objects are investigated. An actual Brillouin lidar system is developed. Also,
several basic problems related to Brillouin lidar are studied in detail. The attenuation coefficient of a pulsed laser beam
with high pulsed energy in water is investigated; it is helpful to reveal the propagation property of a laser beam in water.
The investigations on the threshold value of SBS are made theoretically and experimentally. Finally, a novel phenomena is
investigated experimentally, in which Stimulated Raman scattering can be enhanced by stimulated Brillouin scattering. 相似文献
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The temperature dependence of the static dielectric susceptibility obtained from the experiment on Raman scattering in a deuterated
KDP (DKDP) crystal has been described using the cluster approximation in terms of the microscopic mean-field theory. The optimum
values obtained for parameters of the cluster approximation are in good agreement with experimental data over a wide temperature
range. These values are found to be comparable to the estimates previously obtained in describing experimental data on the
DKDP crystal. 相似文献
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采用传统降温法,利用高纯原料从氘化程度为80%的溶液生长了四方相磷酸二氘钾(DKDP)晶体,并按Ⅱ类三倍频方式切割晶体。三倍频用DKDP晶体的最大问题在于其抗光伤阈值低于KDP晶体,严重限制了激光输出的能量密度和晶体使用寿命。考察了不同波长下三倍频DKDP晶体的损伤阈值,以及激光退火效应。实验表明,激光退火对于DKDP晶体的损伤阈值有显著的提升作用,基频、倍频、三倍频的提升效果分别达到1.4,1.9,2.7倍,是改善DKDP晶体抗光伤能力的有效途径。 相似文献