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We present the first measurement on the resonantly enhanced three-photon excitation spectra of natural lithium using a Nd:YAG laser pumped dye laser in conjunction with a thermionic diode ion detector. Exploiting the linear and circular polarizations, the n2P3/2(8 ? n ? 11) and nf  2F7/2 (8 ? n ? 38) series have been observed via three-photon excitation from the ground state. The measured level energies reveal a dynamic shift from calculated values, which increases with an increase of the principal quantum number n. The ac stark shift and line broadening mechanisms are studied as a function of laser intensity. It is noted that the width increases and the line center shifts towards the higher energy side as the laser intensity is increased. The maximum observed shift for the 12f 2F7/2 line is 0.33 cm−1 corresponding to the laser intensity variation from 1.34 × 1012 W/m2 to 1.03 × 1013 W/m2, whereas its width increases from 0.36 cm−1 to 0.82 cm−1.  相似文献   

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We report on measurements of resonantly enhanced tunneling of Bose-Einstein condensates loaded into an optical lattice. By controlling the initial conditions of our system we were able to observe resonant tunneling in the ground and the first two excited states of the lattice wells. We also investigated the effect of the intrinsic nonlinearity of the condensate on the tunneling resonances.  相似文献   

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The tunneling conductance between two parallel 2D electron systems has been measured in a regime of strong interlayer Coulomb correlations. At total Landau level filling nuT=1 the tunnel spectrum changes qualitatively when the boundary separating the compressible phase from the ferromagnetic quantized Hall state is crossed. A huge resonant enhancement replaces the strongly suppressed equilibrium tunneling characteristic of weakly coupled layers. The possible relationship of this enhancement to the Goldstone mode of the broken symmetry ground state is discussed.  相似文献   

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Using both analytical and numerical methods to study transmission of light through dielectric-filled subwavelength apertures in a real metal, we have found that a propagating mode can in principle exist inside a waveguide of arbitrary small size if a particular relationship between the dielectric constants of the cladding and filling materials at the incident frequency is satisfied. Practical transmission through a subwavelength aperture of finite depth can be enhanced when the depth is such that Fabry-Pérot-like resonances are excited. For 810 nm light incident on a silicon-filled 50-nm-diameter aperture in a 200-nm-thick gold film, we found that a normalized near-field intensity ratio of 1.6 at the exit can be achieved. This resonantly enhanced transmission phenomenon may be advantageously applicable to near-field scanning optical microscopy and single-molecule spectroscopy.  相似文献   

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The sensitivity of a reflective single-port strip-line technique is increased by 10-20 times by amplification of a measured reflectivity response at a set of resonance frequencies. The resonant behavior is organized by connecting the strip cell to a network analyzer through a capacitor with a long coaxial cable. The capacitance defines the amplification; the cable length defines the resonance frequencies. S-parameters of the coaxial-to-strip junction and the field inhomogeneity inside the cell are accounted for by a reference measurement of sample with known constitutive parameters. Two methods for permeability calculation are suggested. The fist method is based on the comparison of Lorentzian parameters of resonance reflectivity curves. The second method is based on numerical solution of Fresnel's equation. The enhancement is essential at low-frequency part of the band, where the cell reflectivity is close to unity and the sensitivity of non-resonant technique is poor. The technique sensitivity is estimated by permeability measurements of Al stripes with different cross-section.  相似文献   

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We report on a remarkable resonance in the differential conductance of long quantum point contacts (QPCs) that is observed as a precursor to regular quantized transport. This effect is increasingly pronounced in longer QPCs, in which the differential conductance may resonantly exceed 2e2/h. From a study of the experimental characteristics of this feature, we suggest that it may be associated with the formation of a well-resolved energy gap that opens dynamically as a result of enhanced many-body interactions in long QPCs.  相似文献   

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Using Schroedinger-Maxwell formalism, we propose and analyse a continuous-wave four-wave mixing (FWM) scheme for the generation of coherent light in a five-state double-A atomic system with or without spontaneously generated coherence (SGC) based on electromagnetically induced transparency (EIT). We derive the corresponding explicit analytical expressions for the generated FWM field under the steady-state condition. The influence of hyperfine sublevel and SGC effect on the amplitude of the generated FWM field is predicted in detail via the derived analytical expressions. We also give a brief discussion on the experimental realization of the proposed scheme.  相似文献   

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The dynamics of spatiotemporal patterns in oscillatory reaction-diffusion systems subject to periodic forcing with a spatially random forcing amplitude field are investigated. Quenched disorder is studied using the resonantly forced complex Ginzburg-Landau equation in the 3:1 resonance regime. Front roughening and spontaneous nucleation of target patterns are observed and characterized. Time dependent spatially varying forcing fields are studied in the 3:1 forced FitzHugh-Nagumo system. The periodic variation of the spatially random forcing amplitude breaks the symmetry among the three quasi-homogeneous states of the system, making the three types of fronts separating phases inequivalent. The resulting inequality in the front velocities leads to the formation of "compound fronts" with velocities lying between those of the individual component fronts, and "pulses" which are analogous structures arising from the combination of three fronts. Spiral wave dynamics is studied in systems with compound fronts. (c) 2000 American Institute of Physics.  相似文献   

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王传奎   总被引:2,自引:4,他引:2  
在杂化密度泛函理论的水平上研究了硝基苯氨(para—nitroaniline—pNA)分子的几何结构,并采用含时密度泛函理论(Time Dependent Density Functional Theory-TDDFT)研究了pNA分子的非线性光学性质。利用两态模型计算了pNA分子的一阶非线性光学超极化率β,并讨论了基矢效应和βz的色散关系。研究结果表明,对于该类分子,利用6—31 G基函数组可以得到收敛的结果。对于处于汽相的pNA分子,计算得到的结果和最近的实验结果符合得很好。对于在较低的频率范围内,两态模型给出的βz的色散关系和实验结果符合得较好;在较高的频率范围内,还应考虑其它态的贡献。  相似文献   

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A resonantly photo-pumped soft x-ray laser process is studied for neon-like iron ions with an automatic line match scheme. The special advantages of this scheme are shown. The temporal characteristics of lasing gains and their dependences on the pump strength and electron density are investigated. Unlike the electron-collisional excitation and some other photo-pumped excitation schemes, it is demonstrated that main photopumped gains come from 2p-4d-3p-3s transition channels. Using the experimental data of pump strengths from a non-LTE plasma produced in our experiment as input data, our model yields a peak gain of 5.6 cm–1, 2.8 cm–1 and 1.9 cm–1 on the dominant lasing transitions at 38.74 nm, 25.47 nm and 20.46 nm.  相似文献   

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A multiwavelength Er:YAP laser pumped by MgO:PPLN locked at 1535 nm with etalon was reported. 170 mW of 1609 nm, 120 mW of 1623 nm output were achieved under total incident pump power of 7 W at 77 K. The slope efficiency were 5.5, 7.2% of the two wavelength.  相似文献   

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Zhou J  Kuzyk MG  Watkins DS 《Optics letters》2006,31(19):2891-2893
We use numerical optimization to find a one-dimensional potential energy function that yields the largest hyperpolarizability, which we find is within 30% of the fundamental limit. Our results reveal insights into the character of the potential energy functions and wave functions that lead to the largest hyperpolarizability. We suggest that donor-acceptor molecules with a conjugated bridge with many sites of reduced conjugation to impart conjugation modulation may be the best paradigm for making materials with huge hyperpolarizabilities that approach the fundamental limit.  相似文献   

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A continuous wave Er:YAP laser pumped by Mgo:PPLN laser locked at 1535 nm was reported. 170 mW of 1609 nm output was achieved under total incident pump power of 7 W at 77 K. The slope efficiency were 5.0 and 3.1% with the cavity length 75 and 140 mm.  相似文献   

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