Zero bias anomaly in the density of states of low-dimensional metals

We consider the effect of Coulomb interactions on the average density of states (DOS) of disordered low-dimensional metals for temperatures T and frequencies ω smaller than the inverse elastic life-time 1/τ. Using the fact that long-range Coulomb interactions in two dimensions (2d) generate ln²-singularities in the DOS ν(ω) but only ln-singularities in the conductivity σ(ω), we can re-sum the most singular contributions to the average DOS via a simple gauge-transformation. If σ(ω) > 0, then a metallic Coulomb gapν(ω) ∝ |ω|/e ⁴ appears in the DOS at T = 0 for frequencies below a certain crossover frequency Ω ₂ which depends on the value of the DC conductivity σ(0). Here, - e is the charge of the electron. Naively adopting the same procedure to calculate the DOS in quasi 1d metals, we find ν(ω) ∝ (|ω|/Ω ₁)^1/2exp(- Ω ₁/|ω|) at T = 0, where Ω ₁ is some interaction-dependent frequency scale. However, we argue that in quasi 1d the above gauge-transformation method is on less firm grounds than in 2d. We also discuss the behavior of the DOS at finite temperatures and give numerical results for the expected tunneling conductance that can be compared with experiments. Received 28 August 2001 / Received in final form 28 January 2002 Published online 9 July 2002     

Mechanism of giant magnetoresistance in intermetallic compounds of rare-earth ions and actinides

Giant positive or negative magnetoresistance is calculated in a band model. The spectra of the band electrons in a two-sublattice antiferromagnetic intermetallic compound depend on the antiferromagnetism vector L(T,H). The metamagnetic transition to the ferromagnetic phase is accompanied by splitting with respect to the spin σ, displacement of the energy bands, and a decrease in the effective masses of the band electrons. This mechanism of giant negative magnetoresistance is also accompanied by an increase in the relaxation time τ_jσ. Scattering by chemical-bond fluctuations is considered as the main relaxation mechanism. Giant positive magnetoresistance results from a four-subband model of 4f and 5f intermetallic compounds. The electron effective masses m _jσ(J _jT ) of the (j,σ) bands increase with the mean angular momentum J _1T (T,H) of an ion in the jth sublattice of 4(5)f ions. The thermodynamics of such a four-sublattice model, the nonlinear magnetization and magnetoresistance curves, and the nonmonotonic dependence of the specific heat C _m(T,H) on the field H are calculated. Fiz. Tverd. Tela (St. Petersburg) 39, 1806–1814 (October 1997)     

The multiphoton ionization rate and the energy shift of atoms interacting with weak dichromatic fields with commensurate frequencies are simple functions of the phase difference

By implementing a time-independent, nonperturbative many-electron, many-photon theory (MEMPT), cycle-averaged complex eigenvalues were obtained for the He atom, whose real part gives the field-induced energy shift, Δ(ω ₁, F ₁;ω ₂, F ₂,ϕ), and the imaginary part is the multiphoton ionization rate, Γ(ω ₁, F ₁;ω ₂, F ₂,ϕ), where ω is the frequency, F is the field strength and ϕ is the phase difference. Through analysis and computation we show that, provided the intensities are weak, the dependence of Γ(ω ₁, F ₁;ω ₂, F ₂,ϕ) on ϕ is simple. Specifically, for odd harmonics, Γ varies linearly with cos(ϕ) whilst for even harmonics it varies linearly with cos(2ϕ). In addition, this dependence on ϕ holds for Δ(ω ₁, F ₁;ω ₂, F ₂,ϕ) as well. These relations may turn out to be applicable to other atomic systems as well, and to provide a definition of the weak field regime in the dichromatic case. When the combination of (ω ₁, F ₁) and (ω ₂, F ₂) is such that higher powers of cos(ϕ) and cos(2ϕ) become important, these rules break down and we reach the strong field regime. The herein reported results refer to Γ(ω ₁, F ₁;ω ₂, F ₂,ϕ) and Δ(ω ₁, F ₁;ω ₂, F ₂,ϕ) for He irradiated by a dichromatic ac-field consisting of the fundamental wavelength λ = 248 nm and its 2nd, 3rd and 4th higher harmonics. The intensities are in the range 1.0×10¹²-3.5×10¹⁴ W/cm², with the intensity of the harmonics being 1-2 orders of magnitude smaller. The calculations incorporated systematically electronic structure and electron correlation effects in the discrete and in the continuous spectrum, for ¹S, ¹P, ¹D, ¹F, ¹G, and ¹H two-electron states of even and odd parity. Received 9 July 2000 and Received in final form 2 November 2000     

Phonon scattering by paraelastic defects

The relaxation timeτ(ω) for the scattering of the lattice waves of frequencyω by the paraelastic defects has been calculated by using the Feynman graph method, applied to a previous theoretical model [8]. A simple expression for the resonance component ofτ(ω)⁻¹ has been derived.

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Zusammenfassung Die Relaxationszeitτ(ω) für die Streuung der Gitterwellen der Frequenzω an den paraelastischen Defekten wurde nach der Methode der Feynmanschen Graphen berechnet, wobei ein früheres theoretisches Modell [8] angewendet wurde. Ein einfacher Ausdruck für den Resonanzteil vonτ(ω)⁻¹ wurde hergeleitet.

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Résumé Nous avons calculé le temps de relaxationτ(ω) des ondes du réseau de fréquenceω, qui sont diffusées par des défauts para-élastiques, en appliquant la méthode des graphes de Feynman à un modèle théorique antérieur [8]. Une simple expression pour la partie résonante deτ(ω)⁻¹ a été dérivée.

     

Reciprocity relations for the effective electrical conductivity of randomly inhomogeneous media in the fractal regime

An exact relation for the realization-averaged effective conductivities in the fractal region is found for two-dimensional randomly inhomogeneous media. It has the form {σ _e (τ,L)~× {1/σ _e (−τ,L)~⁻¹=σ _e ² (τ=0, L≫ξ), where ξ is the correlation length (the self-averaging scale), L is the size of the system, τ=(p-p _c )/p _c , and p _c is the percolation threshold. For L≫ ξ, the system is self-averaged, and the relation transforms into the Dykhne reciprocity relation, A. M. Dykhne, Zh. éksp. Teor. Fiz. 59, 110 (1970) [Sov. Phys. JETP 32, 63 (1971)] σ _e (τ)σ _e (−τ])=σ _e ² (τ=0)= σ ₁ σ ₂. A similar relation is obtained for media with an exponentially broad distribution of local conductivities, as well as for individual realizations of some deterministic structures. Zh. éksp. Teor. Fiz. 113, 1484–1490 (April 1998)     

Remarks on positive semigroups

Let ℳ be a von Neumann algebra with a cyclic and separating vector Ω and let ω(·) denote the corresponding vector state, i.e., ω(A)=(Ω, AΩ) A ∈ ℳ. We have proved that a positive semigroup τ on ℳ can induce the dynamical semigroup in the GNS representation associated with ω if the state ω is a τ-invariant one. Some applications are given.     

ωN final state interactions and ω-meson production from heavy-ion collisions

We calculate the elastic and inelastic ωN→ωN, →πN, →ρN, →ρπN, →ππN, →σN reactions within a boson exchange approximation where the ωρπ coupling constant and form factor are fixed by the reaction πN→ωN in comparison to the experimental data. We find rather large ωN cross sections at low relative momenta of the ω-meson which leads to a substantial broadening of the ω-meson width in nuclear matter. The implications of the ωN final state interactions are studied for ω production in ¹²C +¹²C, ⁴⁰Ca +⁴⁰Ca and ⁵⁸Ni +⁵⁸Ni reactions at about 2 · A GeV within the HSD transport approach; the drastic changes of the transverse mass spectra relative to a general m _T-scaling (for π⁰ and η mesons) might be controlled experimentally by the TAPS Collaboration. Received: 28 April 1999 / Revised version: 7 June 1999     

Stereodynamics of the reaction He+H<Stack><Subscript>2</Subscript><Superscript>+</Superscript></Stack> → HeH<Superscript>+</Superscript> + H: a theoretical study

Quasiclassical trajectory method for the title reaction He +H₂⁺ → HeH⁺ + H was carried out on the potential energy surface which was revised by Aquilanti et al. [Chem. Phys. Lett. 469, 26 (2009)]. The initial vibrational quantum number of reactant was set as v=1, v=2 and v=3. Stereodynamics information of the reaction was obtained, such as the distributions of product angular momentum P(θ _r ), P(ϕ _r ),p(ϕ _r , θ _r ) and the two commonly used polarization-dependent differential cross sections (PDDCSs) (2π/σ)(dσ ₀₀/dω _t ) and (2π/σ)(dσ ₂₀/dω _t ), to get the alignment and orientation of product molecules. The results show that the influence of both the collision energy and vibrational quantum number (v) to the reaction are highly sensitive.     

Relaxation phenomena of polar non-polar liquid mixtures under low and high frequency electric field

Simultaneous calculation of the dipole moment μ_j and the relaxation time τ_j of a certain number of non-spherical rigid aliphatic polar liquid molecules (j) in non-polar solvents (i) under 9.8 GHz electric field is possible from real ε′_ij and imaginary ε″_ij parts of the complex relative permittivity ε*_ij. The low frequency and infinite frequency permittivities ε_0ij and ε_∞ij measured by Purohitet al [1,2] and Srivastava and Srivastava [3] at 25, 35 and 30°C respectively are used to obtain static μ_s. The ratio of the individual slopes of imaginary σ″_ij and real σ′_ij parts of high frequency (hf) complex conductivity σ*_ij with weight fractionsw _jatw _j → 0 and the slopes of σ″_ij— σ′_ij curves for differentw _js [4] are employed to obtain τ_js. The former method is better in comparison to the existing one as it eliminates polar-polar interaction. The hf μ_js in Coulomb metre (C m) when compared with static and reported μs indicate that μ_s s favour the monomer formations which combine to form dimers in the hf electric field. The comparison among μs shows that a part of the molecule is rotating under X-band electric field [5]. The theoretical μ_theos from available bond angles and bond moments of the substituent polar groups attached to the parent molecules differ from the measured μ_js and μs to establish the possible existence of mesomeric, inductive and electromeric effects in polar liquid molecules.     

Relaxation phenomena of binary polar liquid mixture in C6H6 from conductivity of solution measured at 10 GHz electric field

The dielectric relaxation times τ _jk ’s and dipole moments μ _jk ’s of the binary (jk) polar mixtures of N,N-dimethyl formamide (DMF) and pyridine dissolved in benzene (i) are estimated using linear slope of σ _jk ″ − σ _ijk ′ curves as well as ratio of slopes of σ _ijk ″ − w _jk and σ _ijk ″ − w _jk curves at w _jk → 0 for different mole fractions τ _jk ’s of pyridine and experimental temperatures under 9.875 GHz electric field. The measured μ _jk ’s and τ _jk ’s agree well with the reported values validating the proposed methods. The solute-solute (dimer) molecular associations are inferred from the plot of τ _jk − x _j and μ _jk − x _j curves for x _j = 0.0 to 0.5 of pyridine and thereafter solute-solvent (monomer) molecular association occurs. The theoretical μ_theo’s are calculated to predict solute-solute and solute-solvent molecular association. The μ _jk − T curves are drawn to show elongation of bond angles and bond moments with temperatures. The thermodynamic energy parameters are calculated from Eyring’s rate theory equations to know the molecular dynamics as well as to ascertain Debye-Smyth relaxation mechanism of the systems.     

Dielectric losses in statistical mixtures

The specific features of the dielectric spectra of statistical mixtures in the form of heterogeneous systems with spherical particles chaotically arranged in the space have been investigated. The distribution function of relaxation times f(τ) has been restored. It has been established that the relaxation times are continuously distributed within a wide interval [τ₁, τ₂]. Different methods for broadening the relaxation time distribution interval and approximating the relaxation time distribution function f(τ) have been analyzed. It has been demonstrated that f(τ) is a nonmonotonic function with two maxima at the boundaries and a minimum in the vicinity of the midpoint of the interval [τ₁, τ₂]. These features of the relaxation time distribution function are responsible for the large difference between the average relaxation frequencies of the permittivity and the dielectric loss (electrical conductivity).     

Inverse problem for the Grad-Shafranov equation with affine right-hand side

For a given domain ω ⋐ ℝ² with boundary γ = ∂ω, we study the cardinality of the set $ \mathfrak{A}_\eta \left( \Phi \right) $ \mathfrak{A}_\eta \left( \Phi \right) of pairs of numbers (a, b) for which there is a function u = u _(a,b): ω → ℝ such that ∇² u(x) = au(x) + b ⩾ 0 for x ∈ ω, u| _γ = 0, and ||∇u(s)| − Φ(s) ⩽ η for s ∈ γ. Here η ⩾ 0 stands for a very small number, Φ(s) = |∇(s)| / ∫ _γ |∇v| d γ, and v is the solution of the problem ∇² v = a ₀ v + 1 ⩾ 0 on ω with v| _γ = 0, where a ₀ is a given number. The fundamental difference between the case η = 0 and the physically meaningful case η > 0 is proved. Namely, for η = 0, the set $ \mathfrak{A}_\eta \left( \Phi \right) $ \mathfrak{A}_\eta \left( \Phi \right) contains only one element (a, b) for a broad class of domains ω, and a = a ₀. On the contrary, for an arbitrarily small η > 0, there is a sequence of pairs (a _j , b _j ) ∈ $ \mathfrak{A}_\eta \left( \Phi \right) $ \mathfrak{A}_\eta \left( \Phi \right) and the corresponding functions u _j such that ‖f _u ^j+1‖ − ‖f _u ^j ‖ > 1, where ‖f _u ^j = max _x∈ω |f _u ^j (x)| and f _u ^j (x) = a _j u _j (x) + b _j . Here the mappings f _u ^j : ω → ℝ necessarily tend as j → ∞ to the δ-function concentrated on γ.     

ρ(ω) → π0π0γ, ρ(ω) → ηπ0γ decays in the local quark Nambu-Jona-Lasinio model

The branching ratios and photon spectra of the rare processes ρ(ω) → π ⁰ π ⁰ γ, ρ(ω) → ηπ ⁰ γ are calculated in the framework of the standard local quark Nambu-Jona-Lasinio model. Three types of diagrams are considered: the quark box and the pole diagrams with scalar (σ, α ₀(980)) and vector (ρ, ω) mesons. The obtained estimates for the widths of the processes ρ(ω) → π ⁰ π ⁰ γ are in satisfactory agreement with existing experimental data. Predictions are made for the widths of the processes ρ(ω) → ηπ ⁰ γ. The text was submitted by the authors in English.     

Transport and dielectric properties of thin polycrystalline CoO films

Transport and dielectric properties of polycrystalline CoO films were studied as functions of the applied field, frequency and temperature. TheI–V plots showed that the Poole-Frenkel field emission mechanism is responsible for conduction at fields>10⁵ V/cm. The ac conductivity σ(ω), the imaginary part of the dielectric constantε ₂, and tan δ plots as functions of frequency revealed three dispersion regions. The σ(ω) andε ₂ frequency dependence indicates a non-adiabatic hopping of charge carriers at low frequencies and adiabatic hopping at high frequencies. The activation energy of a dielectric oscillator is 0.15 eV. Work supported by the Office of Naval Research.     

Conductivity of ionic crystals when they are irradiated by picosecond electron beams

This paper discusses the pulsed electron conductivity σ of KCl, KBr, and NaCl crystals when they are excited by an electron beam (0.2 MeV, 50 ps) with current densities in the interval j=(30–10⁴) A/cm². It is shown that the lifetime of the electrons in the conduction band is τ≪100 ps. To explain the experimental σ(j) dependences, a model is proposed that includes electron capture by structural defects and stable radiation defects at low excitation densities and electron capture predominantly by unstable radiation defects generated by the excitation pulse at high excitation densities. Fiz. Tverd. Tela (St. Petersburg) 41, 1200–1203 (July 1999)     

New data for the 197Au(γ, nX) and 197Au(γ, 2nX) reaction cross sections

The results from experimental and theoretical studies of the total and partial cross sections of photoneutron reactions on the ¹⁹⁷Au isotope were analyzed. The cross sections for reactions σ(γ, nX) = σ(γ, n) + σ(γ, np) + … + σ(γ, 2nX) = σ(γ, 2n) + σ(γ, 2np) + … were evaluated in the energy range 7 ≤ E _γ ≤ 30 MeV using an approach free of the shortcomings of experimental photoneutron multiplicity sorting methods. The total photoneutron reaction cross sections σ^exp(γ, xn) = σ^exp(γ, nX) + 2σ^exp(γ, 2nX) + … = σ^exp(γ, n) + σ^exp(γ, np) + 2σ^exp(γ, 2n) + 2σ^exp(γ, 2np) + … were used as the initial experimental data. The contributions from the cross sections σ(γ, nX) and σ(γ, 2nX) to the cross sections σ^exp(γ, xn) were separated using the multiplicity transition functions F ₁ ^theor = σ^theor(γ, 1nX)/σ^theor(γ, xn) and F ₂ ^theor = σ^theor(γ, 2nX)/σ^theor(γ, xn), calculated within an updated version of the pre-equilibrium model of photonuclear reactions. New evaluated data for both partial reaction cross sections, i.e., σ^eval (γ, 1nX) = F ₁ ^theorσ^exp(γ, xn) and σ^eval(γ, 2nX) = F ₂ ^theorσ^exp(γ, xn), were obtained. The cross sections σeval(γ, nX) and σ^eval.(γ, 2nX) evaluated using the theoretically calculated functions F _1,2^theor are consistent with the Livermore data, but substantially contradict the Saclay data.     

Breit–Wigner Approximation and the Distribution¶of Resonances

For operators with a discrete spectrum, {λ _j ²}, the counting function of λ _j 's, N (λ), trivially satisfies N ( λ+δ ) −N ( λ−δ ) =∑ _j δ_{λ j} ((λ−δ,λ+δ]). In scattering situations the natural analogue of the discrete spectrum is given by resonances, λ _j ∈ℂ₊, and of N (λ), by the scattering phase, s(λ). The relation between the two is now non-trivial and we prove that

Thermodynamical Limit for Correlated Gaussian Random Energy Models

 Let {E _Σ (N)} _ΣΣN be a family of |Σ _N |=2 ^N centered unit Gaussian random variables defined by the covariance matrix C _N of elements c _N (Σ,τ):=Av(E _Σ (N)E _τ (N)) and the corresponding random Hamiltonian. Then the quenched thermodynamical limit exists if, for every decomposition N=N ₁ +N ₂ , and all pairs (Σ,τ)Σ _N ×Σ _N :

Dielectric relaxation of binary polar liquid mixture measured in benzene at 10 GHz frequency

The dielectric relaxation times τ _jk ’s and dipole moments μ _jk ’s of the binary (jk) polar liquid mixture of N,N-dimethyl acetamide (DMA) and acetone (Ac) dissolved in benzene (i) are estimated from the measured real σ′ _ijk and imaginary σ″ _ijk parts of complex high frequency conductivity σ* _ijk of the solution for different weight fractions w _jk ’s of 0.0, 0.3, 0.5, 0.7 and 1.0 mole fractions x _j of Ac and temperatures (25, 30, 35 and 40°C) respectively under 9.88 GHz electric field. τ _jk ’s are obtained from the ratio of slopes of σ″ _ijk -w _jk and σ′ _ijk -w _jk curves at w _jk → 0 as well as linear slope of σ″ _ijk -σ′ _ijk curves of the existing method (Murthy et al, 1989) in order to eliminate polarpolar interaction in the latter case. The calculated τ’s are in excellent agreement with the reported τ’s due to Gopalakrishna’s method. μ _jk ’s are also estimated from slopes β’s of total conductivity σ _ijk -w _jk curves at w _jk → 0 and the values agree well with the reported μ’s from G.K. method. The variation of τ _jk ’s and μ _jk ’s with x _j of Ac reveals that solute-solute molecular association occurs within 0.0–0.3x _j of Ac beyond which solute-solvent molecular association is predicted. The theoretical dipole moments μ _theo’s are calculated from bond angles and bond moments to have exact μ’s only to show the presence of inductive, mesomeric and electromeric effects in the substituent polar groups. The thermodynamic energy parameters are estimated from ln(τ _jk T) against 1/T linear curve from Eyring’s rate theory to know the molecular dynamics of the system and to establish the fact that the mixture obeys the Debye-Smyth relaxation mechanism.      

Rotational excitations in muonic atom scattering by molecular hydrogen

A computational scheme based on the infinite order sudden approximation (IOS) is proposed for treating molecular and screening effects in muonic atom scattering at low energies. With this scheme the differential (dσ/dΩ(ɛj← 0|θ) and the total σ_tot(ɛ) cross-sections of muonic atom scattering on molecules of hydrogen isotopes are calculated at energies ɛ_rot=ℏω_I⩽ɛ⩽ɛ_vib= ℏω_03BD;. The IOS permits a quantitative analysis of the dependence of the differential cross-sections on the scattering angle and on the rotational excitations, particularly the rotational rainbow effects. An attractive feature of this approach is also to include the energy and the angular dependencies in the “input” cross-sections describing the muonic atom scattering on each bare nucleus of the molecule. The calculated total cross-sections ω_tot(ɛ) are in agreement with the data obtained earlier with the pseudopotential approach. This revised version was published online in August 2006 with corrections to the Cover Date.