129Ce高自旋态的形状变化

通过116Sn(16O,3n)Ce9Ce反应,利用多普勒移动衰减法测量了129Ce高自旋态的寿命.得到的跃迁四极矩表明129Ce的集体性相对于核芯128Ce减弱.这个因增加一个h11/2中子而引起集体性的降低可以解释为由于形状驱动效应产生三轴形变所造成的.正、负宇称带的跃迁四极矩与角动量的关系呈现相似的变化趋势,推测一对h11/2准质子可能对核芯性质起主要作用.     

丰中子核125Sb的高自旋态

利用在束γ谱学方法,通过¹²⁴Sn(⁷Li,α2n)反应首次研究了丰中子核¹²⁵Sb的高自旋态.建立了自旋达23/2⁺、激发能至2637keV的能级纲图,其中包括21条新γ跃迁和14个新能级.在1970,2110和2471keV识别出了3个同质异能态,估计了它们的寿命范围,并建议分别具有πg_7/2ν(h_11/2s_1/2),πg_7/2ν(h_11/2d_3/2),πg_7/2ν(h²_11/2)三准粒子组态.根据价质子与¹²⁴Sn核芯激发态的耦合讨论了¹²⁵Sb的能级结构.     

131Ce和131Pr价核子对形状变化的影响

利用95MeV的¹⁹F束轰击¹¹⁶Sn靶,采用11台反康普顿BGO-HPGe探测器对蒸发剩余核退激发射的γ射线进行γ-γ符合测量.通过对多普勒展宽峰的形状分析测定了¹³¹Ce和¹³¹Pr高自旋态的寿命.根据寿命数据提取的跃迁四极矩显示,在带交叉区发生形状变化.通过与相邻偶-偶核芯¹³⁰Ce的比较表明,价中子对核芯形状变化的影响大于价质子的影响.     

A=147—153核的Gamow—Teller跃迁

在壳模型的基础上系统研究了¹⁴⁶Gd区A=147-153核的Gamow-Teller跃迁.这些相对¹⁴⁶Gd核心为粒子态的核唯一的β允许衰变道为π1h_11/2→v1h_9/2的Gamow-Teller跃迁.计算结果表明,实验的约化几率B(GT)与计算的B(GT)比较,存在一个阻塞因子γ²,即γ²=B_exp(GT)/B_cal(GT)=0.17±0.05.     

丰中子奇A核145,147Ce的集体带结构

通过对²⁵²Cf自发裂变产生的瞬发γ谱的测量,对丰中子奇A核^145,147Ce的高自旋态进行了研究,首次识别了¹⁴⁵Ce的集体带结构,扩展了¹⁴⁷Ce的集体带结构,扩展了¹⁴⁷Ce的能级,并新识别了3个边带,粒子–转子模型的计算指出,^145,147Ce的晕带可能来自于νi_13/2轨道的耦合,¹⁴⁵Ce基态起源于(νh_9/2νf_7/2)组态混合,而¹⁴⁷Ce基态则起源于νh_9/2轨道.在这两个核中未观测到明显的八极形变带,然而,在¹⁴⁷Ce中观测到的一个边带,可能显露出八极关联的迹象.     

弱形变双奇核158Tm中的旋称反转

通过融合蒸发反应¹⁴⁴Nd(¹⁹F,5n)布居了双奇核¹⁵⁸Tm的高自旋态. 扩展了原来已知的带结构, 并建立了一条新转动带. 通过与相邻核的比较, 讨论¹⁵⁸Tm核中两条四准粒子带的内禀组态, 并分别指定为πh_11/2\otimes νh_9/2(α=+1/2)\otimes (νi_13/2)²和πh_11/2\otimes νh_9/2(α=－1/2)\otimes (νi_13/2)² 组态. 建立在πh_11/2\otimes νi_13/2组态上的转动带被观测到呈现持续旋称反转现象, 而前述的两条高自旋区的 四准粒子转动带也呈旋称反转. 对这两种类型的旋称反转现象的可能机制进行了简单而定性的讨论.     

丰中子核145,147La的八极形变

通过对²⁵²Cf自发裂变产生的瞬发γ谱的实验研究,建立与扩展了丰中子核^145,147La的高自旋态能级图,最高自旋态达到(41/2⁺)与(43/2^－).测得的交叉相联的相反宇称带及带间的强化E1跃迁说明在^145,147La中形成强的八极形变.对¹⁴⁵La的研究表明,具有轴对称形状的四极形变与具有反演不对称形状的八极形变在同一核中产生共存与竞争.在πh_11/2带中观测到的带交叉位于ω≈0.26—0.30MeV附近,由推转壳模型计算表明,它是由一对i_13/2中子的顺排所引起的.     

质量数在160-180核区形变双奇核高自旋态实验研究

基于在160-180核区形变双奇核高自旋态研究中所取得的研究结果和最近几年陆续发表的双奇核高自旋态核谱学数据,系统地考察和研究了πh_11/2⊙νi_13/2强耦合带和πh_9/2⊙νi_13/2半退耦带旋称反转的特征和规律.指出^182,184Au核素的πh_13/2⊙νi_13/2半退耦带也可能出现旋称反转;有限的实验数据似乎支持这一观点.首次在双奇核^178,180Ir的πh_11/2⊙νi_13/2强耦合带中发现了低转频下的逐渐顺排现象;在¹⁷⁸Ir核中发现了回弯频率反常超前.这些反常现象可能与核形变(或中子对力)的组态依赖性有关.     

一个可能的117Cs核πh11/2带的观测

在对²⁸Si轰击⁹²Mo靶反应进行的在束γ测量中,观测到一个全新的转动带,通过对其跃迁强度、结构特性的分析,认定它可能是建立在¹¹⁷Cs核的h_11/2质子能级上的转动带.     

135La高自旋态的实验研究

利用在束γ谱实验技术,通过¹²⁸Te(¹⁰B,3n)¹³⁵La反应研究了¹³⁵La的高自旋态.基于γγ符合关系、γ射线的相对强度和各向异性度的测量结果,建立了¹³⁵La的能级纲图.在hω≈0.40MeV附近,观测到基于πh_11/2质子轨道上的负宇称带的带交叉.比较N=78同中子素链能级结构的系统性,认为该带交叉是由一对h_11/2准质子发生转动顺排造成的.在高自旋态处,观测到具有很强M1跃迁、Signature劈裂很小的ΔI=1负宇称带,根据系统性认为该带是建立在πh_11/2(νh_11/2)²组态上的γ≈–60°的扁椭球形变带.     

Signature splitting in 129Ce

The high spin states of 129Ce have been populated via heavy-ion fusion evaporation reaction 96Mo (37C1, 1p3n) 129Ce. The γ-γ coincidence and intensity balance used to measure the B(M1; I→I-1)/B(E2; I→I-2) (the probability ratio of the dipole and quadrupole transition) in v7/2[523] rotational band of 129Ce. And the energy splitting (Δe') has been got through the experimental Routhians. The lifetimes and quadrupole moments Qt have been extracted from the lineshape analyses using DSAM. The deformation of the v7/2[523] rotational band of 129Ce was extracted from the Qt and moment of inertia JRR.     

Lifetime measurements of the high spin yrast states in 128Ce

Lifetime measurements of the high spin states in the yrast band of ¹²⁸Ce were performed using the Doppler shift attenuation method in connection with the reaction ¹⁰⁰Ru(³²S, 2p2n) ¹²⁸Ce at incident energy of 141 MeV. In the vicinity of the band crossing, the previously reported anomalously high B(E2) value was not observed. The gross behavior of the normalized transition strength is approximate to symmetric rotor. It is confirmed that the trend of increase in collectivity with decreasing neutron number, which was indicated in the previous studies on ^{130, 132, 134}Ce, continues in ¹²⁸Ce. The value of quadrupole deformation parameter β₂ deduced from the measured lifetimes is in good agreement with the theoretical calculation using a cranking model based on a non-axially deformed Woods-Saxon potential.     

Lifetime measurements of the high spin yrast states in128Ce

Lifetime measurements of the high spin states in the yrast band of¹²⁸Ce were performed using the Doppler shift attenuation method in connection with the reaction¹⁰⁰Ru(³²S, 2p2n)¹²⁸Ce at incident energy of 141 MeV. In the vicinity of the band crossing, the previously reported anomalously highB(E2) value was not observed. The gross behavior of the normalized transition strength is approximate to symmetric rotor. It is confirmed that the trend of increase in collectivity with decreasing neutron number, which was indicated in the previous studies on^130,132,134Ce, continues in¹²⁸Ce. The value of quadrupole deformation parameterβ ₂ deduced from the measured lifetimes is in good agreement with the theoretical calculation using a cranking model based on a non-axially deformed Woods-Saxon potential.     

Effect of a triaxial nuclear shape on proton tunneling: the decay and structure of 145Tm

Gamma rays deexciting states in the proton emitter 145Tm were observed using the recoil-decay tagging method. The 145Tm ground-state rotational band was found to exhibit the properties expected for an h{11/2} proton decoupled band. In addition, coincidences between protons feeding the 2{+} state in 144Er and the 2{+}-->0{+} gamma-ray transition were detected, the first measurement of this kind, leading to a more precise value for the 2{+} excitation energy of 329(1) keV. Calculations with the particle-rotor model and the core quasiparticle coupling model indicate that the properties of the pi{11/2} band and the proton-decay rates in 145Tm are consistent with the presence of triaxiality with an asymmetry parameter gamma approximately 20 degrees .     

Ce和O空位共掺杂TiO_2的电子结构与光学性质

采用基于密度泛函理论加U的计算方法,研究了Ce和O空位单(共)掺杂锐钛矿相TiO_2的电子结构和光吸收性质.计算结果表明,Ce和O空位共掺杂TiO_2的带隙中出现了杂质能级,且带隙窄化为2.67 eV,明显比纯TiO_2和Ce,O空位单掺杂TiO_2的要小,因而可提高TiO_2对可见光的响应能力,使TiO_2的光吸收范围增加.光吸收谱显示,掺杂后TiO_2的光吸收边发生了显著红移;在400.0—677.1 nm的可见光区,共掺杂体系的光吸收强度显著高于纯TiO_2和Ce单掺杂TiO_2,而略低于O空位单掺杂TiO_2.此外,Ce掺杂TiO_2中引入O空位后,TiO_2的导带边从-0.27 eV变化为-0.32 eV,这表明TiO_2的导带边的还原能力得到了加强.计算结果为Ce和O空位共掺杂TiO_2在可见光光解水方面的进一步研究提供了有力的理论依据.     

The h112 and g72 band structures in 131Ce and 129Ce

High-spin levels in ^{129, 131}Ce have been produced by the reactions ^{116, 118}Sn(¹⁶O, 3n) ^{129, 131}Ce and studied by in-beam γ-ray spectroscopic techniques. Two strongly populated band structures are observed. The odd-parity levels based on a $\text{9}\text{2}{}^{\mathrm{?}}$ state constitute a system explained in the triaxial-rotor-plus-particle model as the result of the coupling of an $\text{h}{}_{\mathrm{<mtext>11</mtext><mtext>2</mtext>}}$ neutron-hole to a prolate-type triaxial core. The even-parity band built on a $\text{7}\text{2}{}^{\mathrm{+}}$ state corresponds to collective excitations associated with a neutron-hole in the $\text{g}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}$ shell. Backbending effect observed in the yrast cascade is discussed.     

Sp(4, R) symmetry in light nuclei

A classification of nuclear states according to the non-compact Lie algebra Sp(4, R) is investigated. This model strikes a compromise between the Sp(6, R) and Sp(2, R) models and furnishes a practical, yet algebraically simple means for selecting those shell-model core excitations which are needed for the development of quadrupole collectivity in rotational bands of deformed nuclei. Applications to rotational bands in ²⁴Mg and ¹⁶O, including shell-model excitations with excitation energies up to 10?ω, show that the core excitations needed to fit observed E2 rates in these nuclei are too large to be treated by perturbation theory. Despite this, a definite symplectic band structure emerges. The nature of the core excitations is very simple, so that it may be feasible to incorporate such symplectic excitation structures into more detailed shell-model calculations.     

High-spin levels in137,139Ce and139,141Nd evidence for hole-core coupling

Excited states of the¹³⁷Ce,¹³⁹Ce,¹³⁹Nd and¹⁴¹Nd nuclei have been studied using the¹³⁸Ba(α, 5nγ)¹³⁷Ce,¹³⁸Ba(³He, 4nγ)¹³⁷Ce,¹³⁸Ba(α, 3nγ)¹³⁹Ce,¹⁴⁰Ce(α, 5nγ)¹³⁹Nd,¹⁴⁰Ce(³He,4nγ)¹³⁹Nd,¹⁴⁰Ce(α, 3nγ)¹⁴¹Nd and¹⁴²Ce(α, 5nγ)¹⁴¹Nd reactions. Singlesγ-ray spectra,γ —γ coincidence spectra, angular distributions and time distributions ofγ-rays with respect to beam pulses have been measured. Gamma transitions between excited states with spin values up to 21/2, 23/2 or 25/2 have been observed. Isomeric states with T_1/2=70 ns have been observed in¹³⁹Ce at 2631.5 keV (19/2) and in¹⁴¹Nd probably at 2952.0 keV (19/2). The level structure observed in the nuclei studied can be explained if the neutron-holes are coupled to the doubly even core excitations. The coupling of theh _11/2 neutron-hole with the 2⁺, 4⁺ and 3^? collective excitations are calculated in terms of the weak and intermediate coupling models. The intermediate coupling results seem to be in better agreement with the experimental data. The energies of theree-particle states, being the result of the coupling of theh _11/2 neutron-hole with the two-proton excitations in the core, are well reproduced in the calculations when empirical values of the two-body interaction matrix elements were used.     

Collective Band Structures in Neutron-Rich Odd-A 145,147Ce Nuclei

Through study of the prompt r-rays emitted in the spontaneous fission of ²⁵²Cf, high spin states of neutron-rich odd-A ^145,147Ce nuclei have been investigated. The levels in ¹⁴⁷Ce have been extended. A collective band in ¹⁴⁵Ce have been identified for the first time. The results from the particle rotor model calculations indicate that the yrast bands in ¹⁴⁵Ce and ¹⁴⁷Ce originate from vi_13/2 orbital coupling and the ground states of ¹⁴⁵Ce and ¹⁴⁷Ce originate from (vh_9/2,vf_7/2) and vh_9/2 configiration, respectively. No obvious octupole deformation was observed in these two isotopes, but a side band obtained in ¹⁴⁷Ce may show some octupole correlations.