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1.
We present the results a study of structure by neutron diffraction and data on the magnetic properties (linear and nonlinear
(second and third order) susceptibilities) of polycrystalline La0.88MnO2.95. This compound exhibits an insulator-metal (IM) phase transition at T
IM
≈ 253 K (above the Curie temperature, T
C
≈ 244 K) and reveals colossal magnetoresistance. The crystal structure is found to be rhombohedral, and the space group is
R3c. Analysis of magnetic properties shows that at T* ≈ 258 K > T
C
, isolated paramagnetic clusters occur in the paramagnetic matrix; their concentration increases upon cooling. We observed
no noticeable differences between the temperature evolution of the clustered state of this manganite with its insulator-metal
transition and in the insulator La0.88MnO2.91. Possible scenarios of the paramagnet-ferromagnet and I-M transitions in a self-organized clustered structure are discussed. 相似文献
2.
D. P. Kozlenko T. A. Chan S. E. Kichanov A. V. Trukhanov S. V. Trukhanov B. N. Savenko 《Physics of Particles and Nuclei Letters》2011,8(10):1063-1065
The crystal and magnetic structures of manganite Pr0.7Ba0.3MnO3 have been studied at high pressures of up to 5.1 GPa and temperatures from 10 to 300 K by means of the neutron diffraction.
At normal pressure and a temperature T
C = 200 K, a ferromagnetic state forms in Pr0.7Ba0.3MnO3. At high pressures P ≥ 1.9 GPa and T < T
N ≈ 153 K, a new antiferromagnetic state of A-type have been observed. Under high pressure, the Curie temperature T
C increases with the characteristic quantity dT
C/dP ≈ 2.4 K/GPa. A possible reason for the appearance of an A-type antiferromagnetic phase in Pr0.7Ba0.3MnO3 at high pressures may be anisotropic uniaxial compression of oxygen octahedra along the b axis of the orthorhombic structure. 相似文献
3.
Karen B. Paul 《Central European Journal of Physics》2005,3(1):115-126
A monocrystal ofFe
3
O
4 is characterized by resistance, magnetoresistance and magnetic measurements in a temperature range from 4.2 K to 350 K and
magnetic field-cycling from −9 T to 9 T. The resistance measurements revealed a metal-insulator Verwey transition (VT) atT
v
=123.76 K with activation energy E=92.5 meV at T >T
v
and temperature-substitute for the activation energy below the VT,T
0=E/k
B
≈3800 K within 70 K–110K. The magnetotransport results independently verified the VT at 123.70 K, with discontinuous change
in the magnetic moment ΔM≈0.21 ΔM≈0.21μ
B
and resistance hysteresis, dependent on the magnetic field in a narrow temperature range of 0.4° around theT
v
. The magnetic characterization established self consistentlyT
v
as ≈123.67 K, the jump in the magnetization at the VT≈0.25μ
B
and confirmed, that the magnetocrystalline anisotropy is the main microscopic mechanism responsible for the magnetization
of the monocrystal (88%) with additional natural and imposed defects contributing as 12%. 相似文献
4.
N. E. Sluchanko A. V. Bogach V. V. Glushkov S. V. Demishev S. Yu. Gavrilkin N. Yu. Shitsevalova V. B. Filipov S. Gabani K. Flachbart 《JETP Letters》2010,91(2):75-78
The behavior of the specific heat near the quantum critical point x ∼ 0.3 in the Tm1 − x
Yb
x
B12 system has been studied. Detailed measurements have been performed on high-quality single-crystalline Tm0.74Yb0.26B12 samples within a wide temperature range of 1.9–300 K in a magnetic field up to 9 T. The temperature dependence of the magnetic
contribution to the specific heat has a logarithmic divergence of the form C/T ∼ lnT at T < 4 K, which can be attributed to the quantum critical behavior regime suppressed by the external magnetic field. The Schottky
anomaly of the magnetic contribution to the specific heat in Tm0.74Yb0.26B12 has been analyzed. 相似文献
5.
N. B. Ivanova N. V. Kazak Yu. V. Knyazev D. A. Velikanov L. N. Bezmaternykh S. G. Ovchinnikov A. D. Vasiliev M. S. Platunov J. Bartolomé G. S. Patrin 《Journal of Experimental and Theoretical Physics》2011,113(6):1015-1024
Co3O2BO3 and Co2FeO2BO3 single crystals with a ludwigite structure are fabricated, and their crystal structure and magnetic properties are studied
in detail. Substituted ludwigite Co2FeO2BO3 undergoes two-stage magnetic ordering at the temperatures characteristic of Fe3O2BO3 (T
N1 ≈ 110 K, T
N2 ≈ 70 K) rather than Co3O2BO3 (T
N
= 42 K). This effect is explained in terms of preferred occupation of nonequivalent crystallographic positions by iron, which
was detected by X-ray diffraction. Both materials exhibit a pronounced uniaxial magnetic anisotropy. Crystallographic direction
b is an easy magnetization axis. Upon iron substitution, the cobalt ludwigite acquires a very high magnetic hardness. 相似文献
6.
D. P. Kozlenko N. T. Dang Z. Jirák S. E. Kichanov E. V. Lukin B. N. Savenko L. S. Dubrovinsky C. Lathe C. Martin 《The European Physical Journal B - Condensed Matter and Complex Systems》2010,77(3):407-411
The crystal and magnetic structures of Pr0.15Sr0.85MnO3
manganite have been studied by means of powder X-ray and neutron diffraction
in the temperature range 10–400 K at high external pressures up to 55 and 4 GPa, respectively. A structural phase transition
from cubic to tetragonal
phase upon compression was observed, with large positive pressure
coefficient of transition temperature dT
ct
/dP = 28(2) K/GPa. The C-type
antiferromagnetic (AFM) ground state is formed below T
N
≈ 260 K
at ambient pressure. While at ambient pressure the structural and magnetic
transition temperatures are close, T
ct
~ T
N
, upon compression
they become decoupled with T
N
≪ T
ct
due to much weaker
T
N
pressure dependence with coefficient dT
N
/dP = 3.8(1) K/GPa. 相似文献
7.
Influence of an external magnetic field on the reluctance of the YBa
2
Cu
3
O
x ceramics is investigated. A significant reluctance of the oxygen-deficient ceramics (with critical temperature Tc < 77 K) is established for a sample in the normal state at T < 160 K. It is demonstrated that after ceramics annealing that
restores the oxygen content to a nearly optimum value, the magnetic field has essentially no effect on the sample reluctance
at temperatures exceeding Tc. To explain the revealed mechanisms, a model involving ferromagnetic clusters effectively decreasing the free carrier density
is used.
__________
Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 4, pp. 68–71, April, 2007. 相似文献
8.
B. I. Belevtsev N. V. Dalakova M. G. Osmolovsky E. Yu. Belyaev A. A. Selyutin 《Bulletin of the Russian Academy of Sciences: Physics》2009,73(8):1130-1133
The resistive, magnetoresistive and magnetic properties of cold-pressed CrO2, powder prepared by hydrothermal synthesis from chromic anhydride have been studied. The powder particles (with a mean diameter
of about 120 nm) were nearly spherical. The particles stabilized with a β-CrOOH surface layer. The powder compact (with a
Curie temperature of about 385 K) revealed nonmetallic temperature behavior of the resistance (with an R(T) dependence close to exponential at T < 20 K). A giant negative magnetoresistance (MR) (∼20% at T ≈ 5K) is found. MR decreased rapidly with an increase in temperature (to 0.3% at T > 200 K). Such MR behavior is shown to
be typical of a system of magnetic grains with magnetic (spin-dependent) tunneling. 相似文献
9.
A. Kh. Matiev A. N. Georgobiani V. V. Kodin M. A. Matiev 《Bulletin of the Russian Academy of Sciences: Physics》2010,74(9):1326-1328
The electrical conductivity and magnetoresistance effect of n and p types of CuInSe2 single crystals were studied within the temperature range of 4.2–300 K and within magnetic fields of up to 6 T. It was found
that the hopping mechanism of conductivity dominates in the temperature range of 4.2–100 K. A peculiarity of electrical conductivity
behavior, accompanied by a change in the magnetoresistance sign in the vicinity of T ≈ 60 K, was revealed. 相似文献
10.
K. A. Shaykhutdinov S. I. Popkov A. N. Lavrov L. P. Kozeeva M. Yu. Kameneva V. V. Val’kov D. M. Dzebisashvili A. D. Fedoseev 《JETP Letters》2010,92(5):332-337
The behavior of the low-temperature specific heat C(T) for YBa2Cu3O6 + x
single crystals with the doping level corresponding to the normal phase has been studied by the relaxation technique at different
values of the applied magnetic field. It has been found that the C(T)/T plot exhibits such an anomaly as a steep increase with decreasing temperature from T about 4 K down to T ≤ 2 K (the minimum temperature value accessible in the experiment). The applied magnetic field as high as 9 T inverts this
anomaly and leads to a sharp drop in C(T)/T during cooling within the same temperature range. A model involving the Schottky-type centers formulated in this work and
the data on spin correlation functions has allowed us to calculate the temperature dependence of the specific heat, which
fits the experimental curves quite well. 相似文献
11.
Charge density wave (CDW) depinning and sliding regimes have been studied in NbSe3 at low temperatures down to 1.5 K under magnetic field of 19 T oriented along the c-axis. We found that the threshold field for CDW depinning becomes temperature independent below T
0 ≈ 15 K. Also CDW current to frequency ratio characterizing CDW sliding regime increases by factor 1.7 below this temperature.
The results are discussed as a crossover from thermal fluctuation to tunneling CDW depinning at T < T
0. Besides, we found that CDW sliding strongly suppresses the amplitude of Shubnikov-de Haas oscillations of magnetoresistance. 相似文献
12.
Ruiting Sun Xiaoli Wang Jing Shi Le Wang 《Applied Physics A: Materials Science & Processing》2011,104(1):129-133
New perovskite solid solution ceramics of (1−x)BaTiO3-xBi(Mg1/2Ti1/2)O3 ((1−x)BT-xBMT, x≤0.09) were synthesized by the solid-state reaction technique. X-ray diffraction studies have revealed a stable single perovskite
structure for all samples. Dielectric measurements were carried out at different frequencies and temperatures. The polarization
evolutions with temperatures were measured to investigate the ferroelectric properties. All the compositions show features
of ferroelectrics with diffuse phase transition, though the temperature T
m
of their dielectric constant maximum ε
m
is frequency dependent. The dielectric constant peak ε(T) of (1−x)BT-xBMT ceramics become broad with increasing BMT content. During the temperature range of ε(T) peak summit, (1−x)BT-xBMT ceramics present quasi-linear dielectric phenomenon under high electric field with very high dielectric constant. 相似文献
13.
A. M. Balagurov I. A. Bobrikov V. Yu. Pomjakushin E. V. Pomjakushina D. V. Sheptyakov I. O. Troyanchuk 《JETP Letters》2011,93(5):263-268
The magnetic and crystal structures of the Pr0.5Sr0.5CoO3 metallic ferromagnet have been studied by the neutron diffraction technique. It is demonstrated that below 150 K, the compound
is mesoscopically separated into two crystalline phases with different spatial symmetries and with different directions of
the magnetic anisotropy. The phase separation exists down to 1.5 K, and at temperatures below 90 K, the low-symmetry phase
occupies about 80% of the sample volume. The main structural difference between the phases is the configuration of oxygen
atoms around praseodymium and, to a certain extent, around cobalt. The ferromagnetic structure with the magnetic moment lying
in the basal plane of the structure (μCo ≈ 1.7 μ
B
at 1.5 K) arises at 234 K, whereas the component directed along the long axis of the unit cell appears at 130 K. The formation
of the new structural phase and change in the orientation of the magnetic moment give rise to the anomalies of the physical
and magnetic characteristics of this compound observed earlier at temperatures about 120 K. 相似文献
14.
H.-F. Li Y. Su Tapan Chatterji A. Nefedov J. Persson P. Meuffels Y. Xiao D. Vaknin Th. Brückel 《The European Physical Journal B - Condensed Matter and Complex Systems》2010,74(4):457-461
Soft X-ray resonant scattering studies at the Mn LII, III- and the La MIV, V- edges of single-crystal LaSr2Mn2O7 are
reported. At low temperatures, below TN ≈ 160 K, energy scans with a fixed momentum transfer at the A-type antiferromagnetic (0 0
1) reflection around the Mn LII, III-edges with incident linear σ and π polarizations show strong resonant enhancements. The
splitting of the energy spectra around the Mn LII, III-edges may indicate the presence of a mixed valence state, e.g., Mn3+/Mn4+.
The relative intensities of the resonance and the clear shoulder-feature as well as the strong incident σ and π polarization
dependences
strongly indicate its complex electronic origin. Unexpected enhancement of the charge Bragg (0 0 2) reflection at the La MIV, V-edges with
σ polarization has been observed up to 300 K, with an anomaly appearing around the orbital-ordering transition temperature,
TOO ≈
220 K, suggesting a strong coupling (competition) between them. 相似文献
15.
The heavy-fermion metal CePd1−x
Rh
x
can be tuned from ferromagnetism at x = 0 to the nonmagnetic state at some critical concentration x
c
. The non-Fermi liquid behavior (NFL) at x ≃ x
c
is recognized by the power-law dependence of the specific heat C(T) given by the electronic contribution susceptibility X(T) and volume expansion coefficient α(T) at low temperatures: C/T ∝ X(T) ∝ α(T)/T∝ 1/ √T. We also demonstrate that the behavior of the normalized effective mass M
N
*
observed in CePd1−x
Rh
x
at x ≃ 0.8 agrees with that of M
N
*
observed in paramagnetic CeRu2Si2 and conclude that these alloys exhibit the universal NFL thermodynamic behavior at their quantum critical points. We show
that the NFL behavior of CePd1−x
Rh
x
can be accounted for within the frameworks of the quasiparticle picture and fermion condensation quantum phase transition,
while this alloy exhibits a universal thermodynamic NFL behavior that is independent of the characteristic features of the
given alloy such as its lattice structure, magnetic ground state, dimension, etc.
The text was submitted by the authors in English. 相似文献
16.
D. P. Kozlenko Z. Jirák N. O. Golosova B. N. Savenko 《The European Physical Journal B - Condensed Matter and Complex Systems》2009,70(3):327-334
The crystal and magnetic structure of the perovskite-like, oxygen deficient
cobalt oxide YBaCo2O5.5 has been studied by means of neutron and
X-ray diffraction in the 10–300 K temperature range. The magnetic ground
state is characterized by a coexistence of two distinct antiferromagnetic
phases. In the first one, the ionic moments of high-spin Co3+ ions in
the pyramidal sites are ordered in a spiral arrangement, while octahedral
sites are non-magnetic due to presence of low-spin Co3+ ions. The
arrangement in the second phase is collinear of the G-type, with non-zero
moments both in pyramidal (high-spin Co3+ ions) and octahedral sites
(presumably a mixture of the low- and high-spin states). With increasing
temperature, at 260–300 K, the system develops a gradual structural
transformation, which is associated with appearance of spontaneous magnetic moment.
This process is related to a thermally induced reversion of low- and
high-spin states at the octahedral sites to the intermediate-spin Co3+
states, resulting in an insulator-metal transition at TC ≈
TIM ≈ 295 K. 相似文献
17.
S. V. Trukhanov A. V. Trukhanov A. N. Vasiliev H. Szymczak 《Journal of Experimental and Theoretical Physics》2010,111(2):209-214
The magnetic and thermal properties of the anion-deficient La0.70Sr0.30MnO2.85 manganite are investigated in wide temperature (4–350 K) range, including under hydrostatic pressure (0–1.1 GPa). Throughout
the pressure range investigated, the sample is spin glass with diffused phase transition into paramagnetic state. It is established,
that spin glass state is a consequence of exchange interaction frustration of the ferromagnetic clusters embeded into antiferromagnetic
clusters. The magnetic moment freezing temperature T
f
of ferromagnetic clusters increases under pressure, freezing temperature dependence on pressure is characterized by derivative
value ∼4.5 K/GPa, while the magnetic ordering T
MO temperature dependence is characterized by derivative value ∼13 K/GPa. The volume fraction of sample having ferromagnetic
state is V
fer ∼ 13% and it increases under a pressure of 1.1 GPa by ΔV
fer ≈ 6%. Intensification of ferromagnetic properties of the anion-deficient La0.70Sr0.30MnO2.85 manganite under hydrostatic pressure is a consequence of oxygen vacancies redistribution and unit cell parameters decrease.
The most likely mechanism of frustrated exchange interactions formation is discussed. 相似文献
18.
A. V. Malakhovskii E. V. Eremin D. A. Velikanov A. V. Kartashev A. D. Vasil’ev I. A. Gudim 《Physics of the Solid State》2011,53(10):2032-2037
The magnetic properties of the Nd0.5Gd0.5Fe3(BO3)4 single crystal have been studied in principal crystallographic directions in magnetic fields to 90 kG in the temperature
range 2–300 K; in addition, the heat capacity has been measured in the range 2–300 K. It has been found that, below the Néel
temperature T
N = 32 K down to 2 K, the single crystal exhibits an easy-plane antiferromagnetic structure. A hysteresis has been detected
during magnetization of the crystal in the easy plane in fields of 1.0–3.5 kG, and a singularity has been found in the temperature
dependence of the magnetic susceptibility in the easy plane at a temperature of 11 K in fields B < 1 kG. It has been shown that the singularity is due to appearance of the hysteresis. The origin of the magnetic properties
of the crystal near the hysteresis has been discussed. 相似文献
19.
We report measurements of the temperature dependence of the electrical resistivity, ρ(T), and magnetic pen-etration depth, λ(T), for polycrystalline samples of Eu0.5K0.5Fe2As2 with T
c
= 31 K. ρ(T) follows a linear temperature dependence above T
c
and bends over to a weaker temperature dependence around 150 K. The magnetic penetration depth, determined by radio frequency
technique displays an unusual minimum around 4 K which is associated with short-range ordering of localized Eu3+ moments.
The article is published in the original. 相似文献
20.
D. M. Zashchirinskii L. I. Koroleva A. S. Morozov Yu. V. Dolzhenkova 《Physics of the Solid State》2011,53(2):316-319
The magnetocaloric effect ΔT has been studied by a direct method in two samples of the manganite Sm0.55Sr0.45MnO3, namely, a single crystal (sample A) and a ceramic sample (sample C). The temperature dependences of the ΔT effect of both samples exhibit a maximum at T
max = 143.3 K for the sample A and T
max = 143 K for the sample C. In these maxima, the values of the ΔT effect are 0.8 and 0.4 K in the magnetic field H = 14.2 kOe for the samples A and C, respectively. In addition, the ΔT(T) curve of the sample A has a minimum at T
min = 120 K, in which ΔT = −0.1 K. The maximum value of the ΔT effect increases with an increase in the magnetic field H in the range of magnetic fields up to 14.2 kOe, and the rate of this increase at H > 8 kOe is higher than that at H < 8 kOe. These features of the ΔT effect are explained by the presence of ferromagnetic and antiferromagnetic A- and CE-type clusters in the samples. 相似文献