强激光场中氢负离子双光子电离能量谱的研究

利用强场近似(Strong field approximation,SFA)方法研究氢负离子(H-)在强激光场中双光子电离的能量谱,所得到的电离谱随角度的变化规律与实验结果符合得很好.进一步的研究表明,H-离子在强激光场中双光子电离的能量谱与有质动力能有关.激光场强度越大,光电子的有质动力能也越大,能量谱向左移动越明显...     

强激光场下的双光子自电离理论

本文研究了包括二阶离化过程的强激光场下的双光子自电离。导出了光电子谱的解析表达式,并对一些特殊情况下的光电子谱进行了分析。     

强激光场中的原子电离

按照激光场的强度，原子与强激光场的相互作用可以大致分成几个典型区域，文章概述了不同区域内民离的基本特征和相应的理论模型，重点介绍了描述强场电离程的准静态理论，并讨论了各种理论的适用范围。     

用强场近似方法研究强激光场中H原子的电离

利用传统的强场近似方法和考虑Coulomb修正的强场近似方法,计算了H原子在激光场中的总电离几率及H原子在不同波长激光场中电离的能量谱,并将得到的能量谱与直接数值求解含时Schrödinger方程的结果进行了比较,结果发现：当激光波长较长时,考虑Coulomb 修正的强场近似方法得到的结果与数值求解含时Schrödinger方程的结果符合得较好。     

理论研究强激光场中2pz态氢原子的电离

运用强场近似速度规范理论研究了激发态氢原子的电离情况,当 a.u. 时（ω是激光场的频率,γ是Keldysh绝热参数）,在线性极化激光场中推导了2pz态氢原子电离率的简单表达式,从公式中可以看出在低频极限的情况下,电离率和激光场频率ω成正比,这一公式对激发态氢原子电离机制的研究提供了重要的理论参考。     

理论研究强激光场中2pz态氢原子的电离

运用强场近似速度规范理论研究了激发态氢原子的电离情况,当ω1a.u.,γ1时(ω是激光场的频率,γ是Keldysh绝热参数),在线性极化激光场中推导了2pz态氢原子电离率的简单表达式,从公式中可以看出在低频极限的情况下,电离率和激光场频率ω成正比,这一公式对激发态氢原子电离机制的研究提供了重要的理论参考.     

高阶离化对强激光场诱导自电离的影响

本文讨论了以往强激光诱导自电离理论所忽略的二阶以上的高阶离化效应,得到了自电离谱的解析表达式,详细研究了高阶离化的影响。结果表明,当激光场足够强时,高阶离化使自电离谱和自电离态的缀饰态产生显著变化。 关键词：     

超强激光场中氘原子电离几率的研究

研究了在相对论领域内,超强激光场的不同条件（频率、强度、脉冲波形磁场分量）对氘原子电离几率的影响,研究表明：电离几率随激光强度的增加而增加,随激光频率的增加而减少。而激光脉冲波形对电离几率的影响仅在激光无磁场分量时比较显著。激光场的磁场分量对原子的电离有一定的影响。     

强激光场中模型氢原子和真实氢原子的高次谐波与电离特性研究

利用数值方法求解含时薛定谔方程，研究了一维、二维模型氢原子和真实的三维氢原子在强激光场中产生的高次谐波和电离特性.结果表明，在多光子电离区域和过垒电离区域，模型氢原子与真实的氢原子产生的高次谐波和电离概率差别很小；在隧道电离区域，它们产生的高次谐波的平台特征和截止位置相似，电离概率随时间变化的趋势相近，但其数值有明显的差异.对产生这种差异的原因进行了分析. 关键词： 强激光场 高次谐波 电离概率     

碘原子共振多光子电离光谱研究

用可调谐的染料激光(4600～5000(?)),共振(3+2)和(4+1)多光子电离探测了I(5p~2P_(3/2)~0)和1~#(5p~2P_(1/2)~0).碘原子是由碘分子(I_2)经激光解离而产生的.在上述激光波段中共观察到12个原子跃迁,其中,(4+1)多光子电离跃迁是首次观察到的.     

Plasmon energy gain and double ionization satellites in the Be Auger spectrum

Two relatively weak, higher energy satellites are observed at 18 and 38 eV above the Be KVV Auger spectrum. The lower energy satellite is assigned to coupling of energy from bulk plasmon de-excitations $\text{(}\text{h}\text{?}\text{ω ～ 18 eV)}$ with Auger electrons and the higher energy event to Auger electrons ejected from Be atoms with doubly ionized K levels.     

Modified crossed-beam PLD method for the control of ion energy spectrum

The modified crossed-beam pulsed laser deposition method, which allows wide-range variations in the energy of deposited particles, is presented for the first time. Time-of-flight curves (TFCs) of silicon ions that are formed by the crossed plumes from two silicon targets and the erosion plume from one silicon target are measured using the Langmuir probe technique. It is demonstrated that the TFCs of ions from the erosion plume are approximated by sums of the one-dimensional Maxwell velocity distributions. Variations in the ion concentrations that result from the interaction are measured. Transformations of the energy spectrum of the plasma beam formed by crossed plumes are determined using variations in the angle between the plumes.     

Laser-produced copper ion energy spectrum employing Thomson scattering technique

Investigations were performed on laser-assisted ion emission when a copper target was irradiated with a Nd:YAG laser (1.064 μm 10 mJ and 1.1 MW). Charge states present in the ion core emitted from plasma were determined employing Faraday cup arrangement using a four-channel 500 MHz Digital Storage Oscilloscope YOKOGAWA DL 1740. The Thomson parabola scattering (TPS) technique was used to measure the energy of ions emitted from plasma. Singly charged positive ions were found to be in excessive amount. For the energy analysis, the ion beam was collimated using a pinhole arrangement. The collimated beam was then made to pass through a uniform magnetic field of 0.4 T. A solid-state nuclear track detector PM-355 was used to register the ion tracks. The energy of ions, found to be in the range of 9–50 keV. The ion energy spectra d ² N/dEdΩ show a decreasing trend with increasing ion energy. The empirical relation dN/dE ∞ E ^?n fits well with the experimental data at higher values of energy, i.e., greater than 20 keV.     

355 nm激光作用下苯甲醚的多光子电离质谱研究

在355 nm激光作用下,利用多光子电离技术结合飞行时间质谱(TOF-MS)对苯甲醚分子进行了研究。实验结果表明苯甲醚分子的多光子电离机制属于母体分子电离-解离模型。通过对主要碎片离子的可能形成过程的讨论,得出该波长下母体分子离子解离的主要有两种通道,但是随激光能量的增强,甲基移除通道逐步占据优势成为主要通道。应用高斯软件采用HF/6-31G(d) 方法对苯甲醚分子和苯甲醚阳离子基态的几何构型进行优化得到其稳定构型,并计算了苯甲醚分子离子及其初级解离产物的能量。比较两条通道的碎片离子能量的变化,理论验证了实验中苯甲醚分子主要解离通道的合理性。     

Nitrogen ion spectrum from a low energy plasma focus device

The nitrogen ion spectrum generated from a low energy Mather-type Plasma Focus device is reported. The main species of ions present are N ⁺¹, N⁺², and N⁺³. It is found that its relative concentrations at a distance of several cm from the ion source are in agreement with those predicted for an equilibrium charge-state of the beam, and hence the spectrum of the neutral nitrogen is also derived. By taking into account the lateral spread of the beam due to multiple elastic scattering with the background gas, the derivation of absolute values for the total ion spectrum within the investigated energy range (>170 keV), the total number and total energy of the fast particles has been obtained     

Parameterization of the energy spectrum of an impurity ion in a perturbing field

The method of parameterizing the energy spectrum for systems with symmetries of the simplest point groups (SR groups) in an external stationary perturbing field has been generalized to the third approximation. The sums over intermediate states are partially convolved in 3n coefficients. We retain sums of derivatives of the given matrix elements which refer to states of all possible energy levels which enter into the external parameters which represent the minimal set of parameters describing the corrections to the energy. We give formulas for calculating the external parameters and establish the connection with the internal parameters in the usual version of the stationary theory of perturbations. In determining the parameters from experimental data the advantage of our method is found in those cases where the number of external parameters is less than the number of internal ones, which is the usual case. The method is illustrated using the Zeeman and Stark effects for energy levels of the T_2g type for an impurity ion having O_h site symmetry, as an example.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 3, pp. 61–67, March, 1995.     

The theoretical and experimental study of the ionization processes during the low energy ion sputtering

The process by which atoms are ionized as they are sputtered from a metal surface has been analyzed both theoretically and experimentally. In the theoretical part the expressions for ionization coefficient R⁺ of atoms having the ionization energy much larger than the metal work function have been derived using a molecular orbital method. The effect of the level crossing was estimated in an approximate way. In the experimental part the SIMS experiments on clean Ni and Al surfaces and on Ni surface covered with a submonolayer of adsorbed K, Na and Al are reported. It has been found and it is for the first time reported that the energy distribution of ions sputtered from a submonolayer of adatoms is independent of energy (200–2500 eV) and mass (Ar⁺ Xe⁺ of incident ions and depends only upon the adsorption energy of the adatom. The energy distribution of ions sputtered from bulk samples has been found dependent on the primary ion energy. The measurement of the absolute value of R⁺ has shown that there is a strong correlation between the number of the adatom valence d-electrons and the value of R⁺, the value of R⁺ being smaller for atoms with more d-electrons. These experimental data have been compared with the theoretical expressions and the important role of the mechanism which takes into account the bending of the adatom energy level has been assessed.