Synthesis and decay properties of superheavy atoms in nuclear reactions induced by stable and radioactive ion beams

This talk consists of two parts. The first one presents the results of investigations performed in 1998-2000 in Dubna on the synthesis of superheavy nuclei in reactions induced by ⁴⁸Ca ions. The radioactive decay properties of the nuclei, indicating a considerable increase in the α-decay and spontaneous fission half-lives of the isotopes of elements 110-116 when approaching the closed neutron shell at N = 184, are given. In the second part the possible ways of advancing into the region of more neutron-rich nuclei, using stable and radioactive ion beams, are discussed. Since so far no intense radioactive ion beams are available, some experiments with stable beams are considered as a test for the suggested ideas. Received: 1 May 2001 / Accepted: 4 December 2001     

High-spin states in neutron-rich nuclei explored with deep-inelastic HI reactions

The use of deep-inelastic heavy-ion reactions for the spectroscopy of neutron-rich nuclei is discussed. Conclusions from the N/Z equilibration process studies are outlined and examples of spectroscopic results obtained for the neutron-rich spdf shell nuclei, N = 82 isotones and nuclei from the ²⁰⁸Pb region are reviewed. Received: 1 May 2001 / Accepted: 4 December 2001     

Modeling a neutron-rich nuclei source

The deuteron break-up process in a suitable converter gives rise to intense neutron beams. A source of neutron-rich nuclei based on the neutron-induced fission can be realised using these beams. A theoretical optimization of such a facility as a function of the incident deuteron energy is reported. The model used to determine the fission products takes into account the excitation energy of the target nucleus and the evaporation of prompt neutrons. Results are presented in connection with a converter-target specific geometry. Received: 1 December 2000 / Accepted: 12 May 2001     

Gamma-ray spectroscopy of the neutron-rich Ni region through heavy-ion deep-inelastic collisions

Nuclei in the neutron-rich Ni region have been studied by γ-ray spectroscopy. Gamma-rays emitted from isomers, with T _1/2 > 1 ns, produced in heavy-ion deep-inelastic collisions were measured with an isomer-scope. The nuclear structure of the doubly magic ⁶⁸Ni and its neighbor ^69,71Cu is discussed on the basis of the shell model. Future experiments for more neutron-rich Ni nuclei are also viewed. Received: 1 May 2001 / Accepted: 4 December 2001     

Photofission for the production of radioactive beams: Experimental data from an on-line measurement

A PARRNe 1 experiment (Production d'Atomes Radioactifs Riches en Neutrons) aimed at the production of neutron-rich radioactive noble gases produced by photofission has been performed at CERN. The LEP Pre-Injector (LPI) has been used to deliver a 50 MeV electron beam. The results obtained show clearly that the use of an electron beam to produce neutron-rich fission fragments for futur RNB facilities is an option that should not be neglected. Received: 20 July 2001 / Accepted: 5 June 2002 / Published online: 19 November 2002 RID="a" ID="a"e-mail: ibrahim@ipno.in2p3.fr Communicated by D. Guerreau     

Model calculations of a two-step reaction scheme for the production of neutron-rich secondary beams

A two-step reaction scheme for the production of extremely neutron-rich radioactive beams, fission followed by cold fragmentation, is considered. The cross-sections of the second step, the cold fragmentation of neutron-rich fission fragments, are estimated with different computer codes. Discrepancies between an empirical systematics and nuclear-reaction codes are found. Received: 27 January 2003 / Accepted: 6 March 2003 / Published online: 27 May 2003     

Spectroscopy of nuclei far from stability at GANIL: Recent experiments

The structure of neutron-rich light nuclei around N = 20, 28 has been investigated at GANIL by means of in-beam gamma spectroscopy using fragmentation reactions of ³⁶S and ⁴⁸Ca beams on a Be target. Gamma decay of relatively high-lying excited states have been measured for the first time in nuclei around ³²Mg and ⁴⁴S. Level schemes are proposed and discussed for a large number of these neutron-rich nuclei around N = 20 and N = 28. Received: 1 May 2001 / Accepted: 4 December 2001     

Production of neutron-rich isotopes in fission of uranium induced by neutrons of 20 MeV average energy

In the context of a parameter study conducted by several laboratories for future European radioactive beam facilities based on fast-neutron induced fission, in particular for the SPIRAL-II project at GANIL, we have measured the yields of neutron-rich isotopes in the mass range of 88 to 144. These nuclei were obtained as fission products of natural uranium bombarded by neutrons of 20 MeV average energy emitted by a thick carbon target irradiated by 50 MeV deuterons. Yields have been measured using on-line mass separation with the ion-guide method. Compared with proton-induced fission at 25 MeV the magnitude of cross-sections, except for the symmetric region, is similar. Z-distributions of isobars have the same width, 0.7 charge units, but their maxima are shifted by about 0.8 charge units, favouring production of the neutron-richer isobars. Our data allow calculations of absolute cross-sections for fission of natural uranium induced by neutrons of about 20 MeV. Received: 10 July 2000 / Accepted: 27 October 2000     

Shell effects and pairing correlations in fission investigated with radioactive beams

The secondary-beam facility at GSI allows to produce a large variety of exotic nuclei at relativistic energies. This technique offers a unique oportunity to investigate systematically fission in inverse kinematics. In the present experiment, the fission properties of more than 70 different actinides and preactinides were investigated at low excitation energy. The elemental yields and kinetic energies of the fission residues present new signatures of shell structure and pairing correlations. Received: 1 May 2001 / Accepted: 4 December 2001     

Measurement of the interaction cross-section and related topics

Recent experimental results concerning interaction cross-sections ( σ_I) are reviewed. The σ_I values were measured by a transmission method using the fragment separator at GSI. The σ_I values for B, C, N, O and F isotopes and the recently measured σ_I for Ar are presented. As related topics, an analysis by the recently developed Glauber model for a few-body system is introduced. By using this analysis, the effective density distributions for light neutron-rich nuclei can be deduced. The recently shown magic number N = 16 near to the neutron drip line is also discussed. Received: 1 May 2001 / Accepted: 4 December 2001     

Muon capture on neutron-rich nuclei

Future facilities will allow the exploration of extremely neutron-rich nuclei far from the valley of stability. It is discussed that the strong-neutron excess results in changes in the collective excitations of such nuclei compared to conventional stable nuclei. We propose muon capture as an experimental tool to explore such changes. We will quantify our discussion by the calculation of the total and differential muon capture rates on selected calcium isotopes between ⁴⁰Ca and ⁶⁰Ca. Our calculations are based on the random phase approximation and agree nicely with the measured rates for ⁴⁰Ca and ⁴⁴Ca. Received: 6 April 2001 / Accepted: 14 May 2001     

High-spin states following multi-nucleon transfer

High-spin states in neutron-rich nuclei, populated following deep-inelastic multi-nucleon transfer, have been studied using the GAMMASPHERE array at the LBNL, USA. A ⁶⁴Ni beam at an energy ∼ 15% above the Coulomb barrier was incident upon a thick ²⁰⁸Pb target, leading to the population of more than 130 different nuclei. The strongest channels correspond to nuclei close to the projectile and target, although transfer of up to 50 nucleons has been observed. New high-spin states in neutron-rich ^60,62Fe and ^68,70,72Zn nuclei have been observed. Some limitations of this method of high-spin spectroscopy are discussed, including the apparent difficulty of populating odd-odd and odd-even isotopes via this type of reaction. The data have been searched for superdeformed (SD) states in the A = 190-200 region, but no evidence for their presence has been found. Received: 14 April 2000 / Accepted: 12 September 2000     

Probing shell structure in neutron-rich nuclei with in-beam γ-spectroscopy

The structure of neutron-rich light nuclei around N = 20 and 28 has been investigated at GANIL by means of in-beam gamma-spectroscopy using fragmentation reactions of ³⁶S and ⁴⁸Ca beams on a Be target. Gamma-decay of relatively high-lying excited states have been measured for the first time in nuclei around ³²Mg and ⁴⁴S. Level schemes are proposed and discussed for a large number of these neutron-rich nuclei around N = 20 and N = 28. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: azaiez@ipno.in2p3.fr     

Spectroscopy on very neutron-rich nuclei beyond N = 20

Recent studies on nuclear structure by using radioactive isotope beams available at the RIKEN projectile-fragment separator (RIPS) are introduced. Special emphasis is given to two selected experiments from recent programs that highlight studies on the magicity loss observed for very neutron-rich nuclei beyond N = 20 in the “island-of-inversion” region; the particle stability of ³¹F, and the low-lying excited states of ³⁴Mg. Received: 1 May 2001 / Accepted: 4 December 2001     

First identification of rotational bands in 103Tc: Evolution of intrinsic proton states of the 97-105 43Tc isotopes

High-spin states of ¹⁰³ ₄₃Tc have been identified for the first time, this nucleus being produced as fission fragment following the fusion reaction ³⁷Cl + ¹⁷⁶Yb at 170 MeV bombarding energy. The high-spin level scheme has been built from the prompt gamma rays detected using the Euroball III array. It exhibits similarities with those of the neighbouring isotopes and isotones. All the band head configurations observed in the ^97-105Tc isotopes are identified from the behaviour of the rotational bands built on them. The single-proton states located around the Fermi level are discussed as a function of deformation of these nuclei. Received: 19 January 2001 / Accepted: 23 February 2001     

Production of neutron-rich nuclei in fission induced by neutrons generated by the p + <Superscript>13</Superscript>C reaction at 55 MeV

Cross-sections for the production of neutron-rich nuclei obtained by neutron-induced fission of natural uranium have been measured. The neutrons were generated by bombarding a ¹³C target with 55 MeV protons. The results, position of the maximum in the (Z, A)-plane, width and magnitude, are very comparable with those where the neutrons are generated by bombardment of natural ¹²C graphite with 50 MeV deuterons. Depending on the geometry of the converter/target assembly the isotope yields, however, are a factor of 2-3 lower due to less efficient production of neutrons per primary projectile, especially at small forward angles. Received: 8 November 2002 / Accepted: 20 December 2002 / Published online: 15 April 2003     

Haloes and clustering in light, neutron-rich nuclei

Clustering is a relatively widespread phenomenom which takes on many guises across the nuclear landscape. Selected topics concerning the study of halo systems and clustering in light, neutron-rich nuclei are discussed here through illustrative examples taken from the Be isotopic chain. The production and detection of multineutron clusters is also briefly presented. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: orr@caelav.in2p3.fr     

On the difference between proton and neutron spin-orbit splittings in nuclei

The latest experimental data on nuclei at ¹³²Sn permit us for the first time to determine the spin-orbit splittings of neutrons and protons in identical orbits in this neutron-rich doubly magic region and compare the case to that of ²⁰⁸Pb. Using the new results, which are now consistent for the two neutron-rich doubly magic regions, a theoretical analysis defines the isotopic dependence of the mean-field spin-orbit potential and leads to a simple explicit expression for the difference between the spin-orbit splittings of neutrons and protons. The isotopic dependence is explained in the framework of different theoretical approaches. Received: 13 February 2002 / Accepted: 20 February 2002     

Frontiers and challenges of the nuclear shell model

Two recent developments of the nuclear shell model are presented. One is a breakthrough in computational feasibility owing to the Monte Carlo Shell Model (MCSM). By the MCSM, the structure of low-lying states can be studied with realistic interactions for a wide, nearly unlimited basically, variety of nuclei. The magic numbers are the key concept of the shell model, and are shown to be different in exotic nuclei from those of stable nuclei. Its novel origin and robustness will be discussed. Received: 1 May 2001 / Accepted: 4 December 2001