Double Electron–Electron Resonance Between Trapped Electron and Hole in a Semiconductor

We demonstrate the spin interactions between dispersedly trapped electrons and holes in a semiconductor using the double electron–electron resonance (DEER) method of the pulsed electron paramagnetic resonance (EPR) techniques. An aluminum-doped titanium dioxide crystal is adopted as a spin system, in which optically generated electrons and holes are trapped, to reveal EPR signals that appear close to each other at a selected crystal orientation under an external magnetic field. We used the four-pulse DEER method by applying two microwave frequencies to a microwave cavity for pumping electrons and probing holes at the optimum temperature of 32 K. The dipolar modulation in the probed signal by pumping interacting spins was successfully detected. The observed non-oscillating decay shape indicates that the detected interaction is caused by widely distributed trapped electron and hole spins over long distances. We were able to extract a spin-pair distribution function by the first derivative of a background-corrected curve, referring to a previously reported method.     

Features of the Coupled Nuclear–Electron Spin Precession in the Bose–Einstein Condensate of Magnons

JETP Letters - The experimental detection of the Bose-Einstein condensate of magnons in coupled nuclear-electron spin precession in antiferromagnets brings the prospect of its use for magnonics and...     

Electron Spin Resonance–Native Signal in Thermally Treated Dental Tissue

Although the dosimetric Electron Spin Resonance (ESR) signal of hard tissues, particularly enamel, has been extensively studied, little attention has been paid to the native signal. This signal is known to be affected by the health of the tissue, as well as by socio–economic factors. In dental applications several clinical procedures, including the use of laser irradiation, can heat the tissue locally with side effects that must be studied. The purpose of the present work is to study the ESR signals in enamel and dentin tissues after thermal treatment with temperatures in the range of 100°C–300°C. Non‐irradiated permanent bovine teeth were studied. ESR measurements were performed with a Varian E‐4 ESR spectrometer operating in the X band range. Progressively larger ESR signals were produced in dentin tissues previously heat treated at and above 100°C. No detectable signals were observed in similarly treated enamel. The signal shows partial decay at four and six months after thermal treatment. The experimental data for dentin show a correlation with the Arrhenius function with an activation energy of (41 ± 2)10³ J/mol. After six months, the ESR signal shows a higher activation energy (67 ± 3)10³ J/mol and the decay shows a activation energy of (38 ± 2)10³ J/mol. A possible assignment of the signal origin in dentin is difficult. The water lost during thermal treatment and reincorporated during the following six months correlates with the signal gain and subsequent decay. The water lost can produce point defects in the hydroxyapatite, or structural changes in the collagen structure. The results observed here are useful for understanding the thermal effects produced in dentin by infrared laser irradiation, and provides a cautionary warning that annealing conditions in ESR studies of biological tissues should be standardized.     

Fully Optical Detection of Hyperfine Electron–Nuclear Interactions in Spin Centers in 6H-SiC Crystals with a Modified 13C Isotope Content

JETP Letters - Optically induced alignment and polarization of electron and nuclear spins in color centers with electron spin $$S = 3{\text{/}}2$$ , which lead to giant changes in photoluminescence...     

Nonlinear Dynamics of Parametric Oscillations of Exciton–Polaritons in a Semiconductor Microcavity

Journal of Experimental and Theoretical Physics - The polariton dynamics in a microcavity in the parametric oscillator mode is studied when two pump polaritons turn into polaritons of signal and...     

Hamiltonian Dynamics and Spectral Theory for Spin–Oscillators

We study the Hamiltonian dynamics and spectral theory of spin-oscillators. Because of their rich structure, spin-oscillators display fairly general properties of integrable systems with two degrees of freedom. Spin-oscillators have infinitely many transversally elliptic singularities, exactly one elliptic-elliptic singularity and one focus-focus singularity. The most interesting dynamical features of integrable systems, and in particular of spin-oscillators, are encoded in their singularities. In the first part of the paper we study the symplectic dynamics around the focus-focus singularity. In the second part of the paper we quantize the coupled spin-oscillators systems and study their spectral theory. The paper combines techniques from semiclassical analysis with differential geometric methods.     

Dynamics of Genuine Three-Qubit Entanglement in Ising Spin Systems

We investigate the dynamics of genuine three-qubit entanglement in the Ising model of three spins. A scheme is presented for generating the genuine three-qubit entanglement by the nearest-neighbour couplings. The effect of magnetic fields on the dynamics of genuine three-qubit entanglement is also discussed.     

Optical Absorption Spectra and Intraband Dynamics in Terahertz-Driven Semiconductor Superlattice

We have theoretically investigated the optical absorption spectrum and intraband dynamics by subjecting a superlattice to both a terahertz (THz)-frequency driving field and an optical pulse by using an excitonic basis.In the presence of a THz dc field, the satellite structures in the absorption spectra are presented. The satellite structure is a result from the THz nonlinear dynamics of Wannier-Stark ladder excitons. On the other hand, the coherent intraband polarization is investigated. We find that the excitonic Bloch oscillation is driven by the THz field and yields an intraband polarization that continues to oscillate at times much longer than the intraband dephasing time. The temporal evolution of the slowly varying components of the intraband polarization is dependent on the THz frequency.     

Spin Chemistry Investigation of Peculiarities of Photoinduced Electron Transfer in Donor–Acceptor Linked System

Photoinduced intramolecular electron transfer in linked systems, (R,S)- and (S,S)-naproxen-N-methylpyrrolidine dyads, has been studied by means of spin chemistry methods [magnetic field effect and chemically induced dynamic nuclear polarization (CIDNP)]. The relative yield of the triplet state of the dyads in different magnetic field has been measured, and dependences of the high-field CIDNP of the N-methylpyrrolidine fragment on solvent polarity have been investigated. However, both (S,S)- and (R,S)-enantiomers demonstrate almost identical CIDNP effects for the entire range of polarity. It has been demonstrated that the main peculiarities of photoprocesses in this linked system are connected with the participation of singlet exciplex alongside with photoinduced intramolecular electron transfer in chromophore excited state quenching.     

Electron Spin Pairing and Excitations in High—Tc Superconductors

Effective spin coupling between conduction electrons mediated by local Cu moments in the doped CuO2 plane may induce the instability of the normal states of conduction electrons and pairing at Cu stes,where the superexchange interaction between local moments influenced by hole doping has been found to be Ising-like in recent experiments.By a mean field approach,we show that spin pairing and strong pair-pair interaction in the doped antiferromagnetic ordered Ising-like CuO2 plane gives rise to high-temperature superfluid condensation and the exceptional features of quasi-particle excitation in cuprates such as spin gap,pseudogap,and the linear temperature dependence of resistivity ρab in the normal states.     

Spin Dynamics of Supramolecular Dimer [Mn4]2 Interacting With a Spin-polarized Electron

A new family of the supramolecular antiferromagnetically exchange-coupled dimer of single-molecules magnets, [Mn4]2, really behave as a quantum mechanical coupled system and can be used for quantum computation [Tiron et al (2003) Phys. Rev. Lett. 91 227203]. We study the time evolution of [Mn4]2 dimer interacting     

Semiconductor–Metal Transition in Magnetic Semiconductor Compounds at High Pressure

Journal of Experimental and Theoretical Physics - The magnetic, transport, and magnetotransport properties of ferromagnetic Zn0.1Cd0.9GeAs2 + 10% MnAs and Zn0.1Cd0.9GeAs2 + 15% MnAs nanocomposites...     

Nonlinear Dynamics of Parametric Oscillations of Exciton–Polaritons in a Semiconductor Microcavity with Allowance for Decay

Optics and Spectroscopy - We have studied the dynamics of polaritons in a microcavity in the parametric oscillator regime, when the pump is carried out by two laser pulses with close frequencies....     

Enhanced Spin Injection into ZnO Semiconductor Measured by Magnetoresistance

We prepare 2× （NiFe/CoZnO）/ZnO/（CoZnO/Co）×2 spin valve structures used for spin injection by sputtering and photolithography. In the junctions, the free magnetic layer 2× （NiFe/CoZnO） and the fixed magnetic layer （CoZnO/Co） × 2 are used to realize the spin valve functions in the external switch magnetic field. Since the wide gap semiconductor ZnO layer is located between the two magnetic semiconductor layers CoZnO, the electrical ,spin injection from the magnetic semiconductor CoZnO into the non-magnetic semiconductor ZnO is realized. Based on the measured magnetoresistance and the Schmidt model, the spin polarization ratio in the ZnO semiconductor is deduced to be 11.7% at 90K and 7.0% at room temperature, respectively.     

Finite-Temperature Entanglement Dynamics in an Anisotropic Two-Qubit Heisenberg Spin Chain

This paper investigates the entanglement dynamics of an anisotropic two-qubit Heisenberg spin chain in the presence of decoherence at finite temperature. The time evolution of the concurrence is studied for different initial Werner states. The influences of initial purity, finite temperature, spontaneous decay and Hamiltonian on the entanglement evolution are analyzed in detail. Our calculations show that the finite temperature restricts the evolution of the entanglement all the time when the Hamiltonian improves it and the spontaneous decay to the reservoirs can produce quantum entanglement with the anisotropy of spin-spin interaction. Finally, the steady-state concurrence which may remain non-zero for low temperature is also given.     

Interference of γ Radiation in the Spin Space during Nuclear Resonance Scattering

Journal of Experimental and Theoretical Physics - In the multispace interference pattern appearing during nuclear resonance scattering of γ radiation in an iron borate crystal, along with the...     

Interactions between Surface Impurities and the Electron–Hole System of a Semiconductor Crystal

The effects of creation and annihilation of impurities on the surface of a highly doped semiconductor under changes in the surface concentration n of dopant atoms constituting impurities are predicted theoretically. The effects are determined by electrostatic interactions of charged surface impurity species with charge carriers and semiconductor ions. The effects are observed in a certain range of n, provided the surface impurities exhibit donor (acceptor) properties, and the semiconductor is doped with an acceptor (donor) impurity.