利用微扰法分析两个相互耦合的参量四波混频过程

利用微扰法在旋转波近似下分析了铷原子中两个独立的参量四波混频过程和一个耦合的参量四波混频过程.当用超短激光脉冲相干激发这两个参量四波混频过程时,两个过程就会同时出现并且存在相互耦合作用.微扰分析表明,耦合的参量四波混频信号中可以观察到量子拍,量子拍幅度的大小不仅取决于超短脉冲的特性,而且依赖于两个耦合的参量四波混频过程中的相位匹配.     

倒V形四能级亚飞秒极化拍的三光子吸收和色散

基于孪生色锁噪声场的互相关效应，从理论上研究了倒V形(RV)四能级飞秒量级差频极化拍与极化拍中五阶非线性极化率，并提出了用一种相位敏感的方法来研究多能级原子相干造成的三光子六波混频过程.在抽泵光束为窄带末端情况下，场关联对信号和极化率的影响都很弱，在非窄带情况下，场关联会使极化强度自相干信号和极化拍信号产生关于零延时的不对称性和时域扫描上的辐射与物质失谐阻尼振荡(RDO)，而极化率会产生频域扫描上的RDO振荡.参考光信号是一路传播方向和六波混频信号稍有区别的双光于非简并四波混频信号.五阶非线性响应则由享生     

倒V形四能级亚飞秒极化拍的三光子吸收和色散

基于孪生色锁噪声场的互相关效应,从理论上研究了倒V形(RV)四能级飞秒量级差频极化拍与极化拍中五阶非线性极化率,并提出了用一种相位敏感的方法来研究多能级原子相干造成的三光子六波混频过程.在抽泵光束为窄带末端情况下,场关联对信号和极化率的影响都很弱,在非窄带情况下,场关联会使极化强度自相干信号和极化拍信号产生关于零延时的不对称性和时域扫描上的辐射与物质失谐阻尼振荡(RDO),而极化率会产生频域扫描上的RDO振荡.参考光信号是一路传播方向和六波混频信号稍有区别的双光于非简并四波混频信号.五阶非线性响应则由享生 关键词： 外差法 吸收 色散 非线性极化     

五能级原子开放系统中的多波混频共存特性

研究了受强缀饰场作用的五能级原子系统所产生的多波混频共存特性.研究发现,通过调节激光束方向,沿同一方向出射的八波混频、双缀饰四波混频和单缀饰六波混频信号因共用能级的原子相干产生而出现竞争现象,通过控制缀饰场减弱四波混频和六波混频信号强度,可以达到增强八波混频信号的目的.还对级联和并联两种不同缀饰方式下双缀饰四波混频过程的差别进行了详细分析. 关键词： 双缀饰四波混频 单缀饰六波混频 八波混频 抑制增强     

受限系统中电磁诱导吸收条件下的光子带隙

在超薄样室原子介质的受限系统中,观察了处于电磁诱导吸收条件下四波混频信号增强现象.实验结果表明增强效应与量子调控所产生的光子带隙有关,而光子带隙结构的变化会对四波混频信号起到增强或抑制的作用.     

光学外差法测量Ba原子的自电离态

提出了把三光子共振非简并六波混频(NSWM)和双光子共振非简并四波混频(NFWM)应用于研究Ba原子自电离态的光学外差探测方法。采用该方法测量了Ba原子的6P_３／２19d自电离态,并观察到了三光子共振 NSWM和双光子共振NFWM信号干涉引起的信号增强。该方法是一种纯非线性光学方法,具有优秀的空间分辨率和简单的光路。其中双光子共振非简并四波混频信号作为本地振荡光束,三光子共振非简并六波混频信号作为信号光束,通过 改变信号光束的频率来达到用光学外差探测法研究Ba原子自电离态的目的。该方法中,实现相位匹配所要求的条件不是很严格,可以在很宽的频率范围内实现相位匹配,而一般的六波混频很难做到相位匹配, 并且所测量的信号是相干光, 当用窄带宽的激光时,可以获得消多普勒的分辨率。     

四波混频与瑞利散射场的干涉现象

介绍在半导体量子阱的飞秒激光四波混频实验中观测到的新的干涉现象.分析表明,实验曲线中的相干振荡来自样品的瑞利散射与四波混频信号的干涉.运用此干涉模型进行了理论模拟,所得结果与实验符合得很好,并由此较准确地得到了介质的退相时间为44 fs. 关键词： 量子阱 四波混频 瑞利散射     

非相干光时延四波混频中V型三能级原子的布居弛豫量子拍的理论研究

对简并非相干光时延四波混频中布居弛豫量子拍的物理机制及产生过程进行了理论研究,并根据真空与原子耦合观点,具体分析讨论了两种情形的三宽带光脉冲作用于V型三能级原子布居弛豫量子拍的形成过程和讯号特征.经比较发现,理论与实验结果相当吻合.     

原子介质中的多波混频相干控制

多波混频是一种重要的非线性光学过程,其在非线性光学和量子信息科学中有重要的应用.本文详细讲述了该领域的进展.在频域中,首先通过电磁诱导透明在实验上得到了共存的四六波混频信号,继而观察到了它们之间伴随着能量交换和时空干涉的相互竞争.此外,两个竞争的四六波混频之间的抑制增强以及相应的AT分裂也被实验证实了.在空间域中,研究了因为两束泵浦光之间干涉导致的电磁诱导光栅,对多波混频信号的空间移动和分裂也进行了讨论,并且得到了带隙孤子,涡旋孤子,有荷偶极孤子,以及二维表面孤子.这些概念可以扩展到量子领域,并且与之相关的一些效应具有研究价值.本文同时也讨论了多波混频在腔量子电动力学中,里德堡态中,以及全固态量子计算中的发展前景以及潜在应用.     

缀饰原子系统中双光子共振非简并四波混频

本文研究了缀饰原子系统中的双光子共振非简并四波混频.理论上我们研究了多普勒增宽的四能级系统中耦合光场对双光子共振非简并四波混频的影响,发现加入强耦合场后,非简并四波混频频谱出现Autler-Townes分裂;在不同双光子共振失谐时,由于量子干涉双光子共振非简并四波混频的信号能够被抑制或增强.实验上我们在Ba原子蒸汽中,通过引入基态6s2和自电离里德堡态6pnd之间的原子相干证实了该现象.本方法提供了一种不仅可以测得共振频率和横向弛豫,而且可以测得两个高激发原子态之间的跃迁的偶极矩阵元的新的光谱学工具.     

Observation of Quantum Beating from Two Coupled Parametric Six-Wave Mixing Signals in Rb

Two processes of coupled difference-frequency axially phase-matched parametric six-wave mixing are carried out in Rb vapour by two-photon excitation using fs laser pulses, and parametric six-wave mixing signals in the infrared and near infrared regime are detected. The infrared parametric six-wave mixing signals are up-converted into the visible spectral range by sum-frequency mixing with the pump laser in a LiIO₃ crystal. Moreover, quantum beating at 608cm^-1, corresponding to the 7s-5d energy difference in Rb, is observed from the sum-frequency signal at 495nm. As a result, we obtain modulated light signals in the visible, near infrared and infrared spectral ranges, and study the interference between 7s and 5d states of Rb.     

Fully Quantized Theory of Six-Wave Mixing with Matter Waves

We show that Wu-Yang theory of fully quantized four-wave mixing can be generalized to the six-wave mixing and derive the analytical solution of the coupled equations describing the quantum dynamics of six-wave mixing.     

中间态引入量子干涉的三光子共振非简并六波混频

理论研究了五能级系统中三光子共振非简并六波混频(NSWM) 由于中间能级加入耦合光场而产生的量子干涉效应. 分析了耦合光场对三光子共振NSWM信号以及频谱的影响. 研究发现, 在强耦合场作用下, NSWM的频谱出现了Autler-Townes分裂, 它反映的是两个缀饰态的能级, 量子干涉可以使NSWM信号被抑制或增强. 提出利用量子干涉对NSWM信号产生增强作用, 可以由耦合场产生的缀饰态代替原子固有能级, 成为三光子共振的中间态, 从而控制耦合场来选择三光子共振的中间态的位置.     

Electromagnetically induced transparency based six-wave mixing in a Doppler-broadened folded four-level system

We study phase-conjugate six-wave mixing spectroscopy based on electromagnetically-induced-transparency in a Doppler-broadened folded four-level system.It is found that the six-wave mixing spectrum can be either Doppler-free or very broad,depending on whether the interference between the polarisations of atoms with different velocities is constructive or destructive.To obtain the Doppler-free six-wave mixing spectrum in the folded four-level system,the conditions are more stringent in comparison with those in the cascade and N-type four-level systems.This polarisation interference can be controlled in the presence of a strong coupling field.     

低维半导体异质结中的量子相干红外发射机理理论研究

给出了一种在非粒子反转条件下量子阱和量子点激光器的红外发射机理.此种红外发射是基于在同一作用区产生并作为红外场相干源的两种带间跃迁激光场的共振非线性混合.这种频率下转换机理并不依赖于在半导体激活媒质中的长时相干假定条件,在室温和泵注入电流条件下仍然有效.频率下转换的固有效率可以达到相当于每个可见光子产生一个红外光子的量子极限值.根据红外发射的可参变特性,这种非粒子反转的方法尤其适用于长波红外工作范围.     

Noise characteristic of sum-frequency mixing orange solid-state laser

A laser-diode-pumped Nd:YVO₄ orange solid-state laser is described in this paper. The fundamental wavelengths at 1064 and 1342 nm oscillate simultaneously and generate the 593.5 nm wavelength by intracavity sum-frequency mixing in a KTP crystal using type II phase matching. The noise characteristic of laser output has been measured and analyzed at different pumping powers. The relationship between the amplitude noise of sum-frequency mixing output and the longitudinal modes of fundamental frequency has been investigated. The results show that the sum-frequency mixing output has low noise if one of the fundamental wavelengths is single longitudinal mode. The experiment shows that amplitude noise of the intracavity sum-frequency mixing laser is lower than that of intracavity frequency doubled laser with the same structure.     

Enhanced or suppressed six-wave mixing in a five-level atomic system

We show the enhancement and suppression of a six-wave mixing (SWM) signal in the electromagnetically induced transparency in a five-level ⁸⁵Rb atomic system. The results show the Autler—Townes splitting and the enhancement or suppression of SWM, which are caused respectively by a self-dressing effect and by an external dressing effect in the presence of mutual dressing between two SWM signals. In addition, we observe the polarization dependence of the enhancement and suppression of the SWM signals.     

Tunable Sum Frequency Mixing of a Ti∶sapphire Laser and a Nd∶YAG Laser

In this paper the theoretical and experimental results of sum-frequency mixing of a Ti∶sapphire laser and a 1.064 μm Nd∶YAG laser are presented. By using two KTP crystals cut at θ=76° and 85° (φ=90° in both crystals), respectively, the sum-frequency mixing tuning range from 459.3 to 509.6 nm in one Ti∶sapphire laser setup is experimentally achieved. The maximum output energy was 14.6 mJ and the energy conversion efficiency was up to 15.2%.