Efficient and widely step-tunable terahertz generation with a dual-wavelength CO<Subscript>2</Subscript> laser

Coherent terahertz radiation in a widely step-tunable range of 72.3–2706 μm (0.11–4.15 THz) has been generated in GaAs crystal by difference-frequency generation using one CO₂ laser with dual-wavelength output. The peak power of THz pulse reaches 35 W at the wavelength of 236.3 μm, which corresponds to a pulse energy of 2.1 μJ. An average power of 10 μW has been achieved when working repetitively. This efficient terahertz radiation source is more compact and widely tunable than other THz sources pumped by CO₂ laser.     

Femtosecond laser plasma in CaF<Subscript>2</Subscript> crystal microchannel and effective generation of characteristic X-ray radiation

The dependence of the characteristic X-ray radiation yield from CaF₂ crystal on the formed microchannel depth under highly intensive (I ∼ 3 × 10¹⁵ W/cm²) laser pulses with different contrast was obtained. The maximum of the characteristic X-ray radiation yield at these experimental conditions corresponded to the microchannel depth of 30–50 μm. The efficiency of the laser radiation conversion to the characteristic X-ray radiation increased from 6 × 10⁻⁸ for the surface up to 10⁻⁷ in the microchannel. The dependence of the characteristic X-ray radiation yield on the viewing angle showed that the source of X-ray radiation was located near the surface inside the microchannel.     

Intracavity parametric conversion of radiation from a pulsed Nd:YVO<Subscript>4</Subscript> laser with high-power diode pumping

We have achieved intracavity parametric conversion of the radiation from a laser based on Nd:YVO₄ with high-power diode pumping. An LiF^2- crystal was used as the passive Q-switch for the Nd:YVO₄ laser. We have shown that by using an active element in the master laser with a passive region, we can form pulsed laser beams at a wavelength of 1.57 μm with peak power 3.2 kW and repetition rates up to 80 kHz, with beam quality parameter 1.4–1.8. __________ Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 73, No. 1, pp. 5–8, January–February, 2006.     

Fabrication of polaritonic structures in LiNbO<Subscript>3</Subscript> and LiTaO<Subscript>3</Subscript> using femtosecond laser machining

Fabrication of patterned materials in ferroelectric LiNbO₃ and LiTaO₃ crystals using femtosecond laser micromachining is presented and discussed. Damage feature sizes in the 10–100 μm range were achieved using 800-nm, 50-fs (FWHM) ultra-fast laser pulses with energies ranging from 10 μJ up to 350 μJ. Fabrication of polaritonic devices such as waveguides, resonators, focusing reflectors, diffractive and dispersive elements, photonic band gap materials, and other microstructures is demonstrated. PACS 77.84.Dy; 42.62.Cf; 71.36.+c     

Luminescence and selective heat radiation of Yb<Subscript>2</Subscript>O<Subscript>3</Subscript> upon the resonant and thermal laser excitation

Yb₂O₃ polycrystals with a size of up to 10 mm are synthesized using the sintering and melting of the ultrapure Yb₂O₃ powders by the CO₂-laser radiation with the power P _L ≤ 100 W at the wavelength λ = 10.6 μm at the melting point T _m = 2703 K, forming due to surface tension in melt, and crystallization in air. The analysis of the polycrystal microstructure using the methods of optical and electron microscopy and X- ray diffractometry shows that perfect oxide crystallites are formed in the course of crystallization after melting-through. The transformation of the luminescence and selective heat radiation (SHR) spectra of the Yb₂O₃ polycrystals is studied under the resonant excitation at λ ≈ 975 nm using a laser diode and the laser heating at the wavelength λ = 10.6 μm. When the resonant excitation power of the Yb³⁺ ions increases from 0.15 to 4.5 W, the Stokes luminescence of the Yb₂O₃ polycrystals is sequentially transformed into SHR and the thermal radiation of the crystal lattice. The transformation of the emission spectra of the Yb₂O₃ polycrystals with an increase in the laser heating intensity by about four orders of magnitude can be represented as the low-temperature heat radiation, spectral burst of the thermodynamically nonequilibrium SHR of the Yb³⁺ ions, and the high-temperature radiation of the crystal lattice. The temperature dependence of the luminescence spectra and SHR of the Yb₂O₃ polycrystals on the intensity of the laser and laser-thermal excitation and the concentration quenching of the Yb³⁺ luminescence in oxides indicate the key role of the interaction of the f-electron shell of the Yb³⁺ ions with the natural oscillations of the crystal lattice in the processes of the multiphonon excitation and nonradiative (multiphonon) and radiative (vibronic) relaxation.     

Photoacoustic spectroscopy of thin films of As<Subscript>2</Subscript>S<Subscript>3</Subscript>, As<Subscript>2</Subscript>Se<Subscript>3</Subscript> and GeSe<Subscript>2</Subscript>

Photoacoustic spectroscopy (PAS) is one of the important branches of spectroscopy, which enables one to detect light-induced heat production following the absorption of pulsed radiation by the sample. As₂S₃, As₂Se₃ and GeSe₂ exhibit a wide variety of photo-induced phenomena that enable them to be used as optical imaging or storage medium and various electronic devices, including electro-optic information storage devices and optical mass memories. Therefore, accurate measurement of thermal properties of semiconducting films is necessary to study the memory density. The thermal conductivity of thin films of As₂S₃ (thickness 100 μm and 80 μm), As₂Se₃ (thickness 100 μm and 80 μm) and GeSe₂ (thickness 120 μm and 100 μm) has been measured using PAS technique. Our result shows that the thermal conductivity of thicker films is larger than the thinner films. This can be explained by the thermal resistance effect between the film and the surface of the substrate.      

CH<Subscript>3</Subscript>OH optically pumped by a <Superscript>13</Superscript>CO<Subscript>2</Subscript> laser: new laser lines and assignments

We report 12 new THz (far-infrared) laser lines from methanol (CH₃OH), ranging from 58.1 μm (5.2 THz) to 624.6 μm (0.5 THz). A ¹³CO₂ laser of wide tunability (110 MHz) has been used for optical pumping, allowing access to previously unexplored spectral regions. Optoacoustic absorption spectra were used as a guide to search for new THz laser lines, which have been characterized in wavelength, polarization, offset, relative intensity, and optimum operation pressure. For 20 laser lines previously observed, we have measured the absorption offset with respect to the ¹³CO₂ laser line center. PACS 33.20.Ea; 33.20.Vq; 33.80.-b     

Sub-wavelength micromachining of silica glass by irradiation of CO<Subscript>2</Subscript> laser with Fresnel diffraction

We investigated a simple and productive micromachining method of silica glass by ablation using a TEA CO₂ laser (10.6 μm) with a spatial resolution down to sub-wavelength scale. The silica glass was irradiated by the TEA CO₂ laser light through a copper grid mask with square apertures of 20×20 μm² attached to the silica glass surface. After the irradiation, circular holes with a diameter of several μm were formed on the silica glass surface at the centers of the apertures due to the Fresnel diffraction effect. The minimum diameter of the holes was 3.4 μm. The characteristics of the micromachining are discussed based on the electric field distributions of the CO₂ laser light under the mask using a three-dimensional full-wave electromagnetic field simulation.     

Discovery and frequency measurement of short-wavelength far-infrared laser emissions from optically pumped <Superscript>13</Superscript>CD<Subscript>3</Subscript>OH and CHD<Subscript>2</Subscript>OH

A three-laser heterodyne system was used to measure the frequencies of twelve previously observed far-infrared laser emissions from the partially deuterated methanol isotopologues ¹³CD₃OH and CHD₂OH. Two laser emissions, a 53.773 μm line from ¹³CD₃OH and a 74.939 μm line from CHD₂OH, have also been discovered and frequency measured. The CO₂ pump laser offset frequency was measured with respect to its center frequency for twenty-four FIR laser emissions from CH₃OH, ¹³CD₃OH and CHD₂OH. PACS 07.57.Hm; 42.55.Lt; 42.62.Eh     

Effect of resonator length on ZnGeP<Subscript>2</Subscript> doubly resonant optical parametric oscillator pumped by a Tm,Ho:GdVO<Subscript>4</Subscript> laser

The effect of resonator length on ZnGeP₂ doubly resonant optical parametric oscillator was reported in this letter. With the employment of a Tm,Ho:GdVO₄ laser as the pump source at 2.05 μm, we have found that there are obvious peaks of the output power when the resonator lengths are matched to the length of the pump source. The ZGP OPO can generate a maximum output power of 4.27 W at 3.80 μm signal and 4.45 μm idler when the resonator length matches that of the pump source.     

Dynamics of two-photon picosecond absorption in ZnWO<Subscript>4</Subscript> and PbWO<Subscript>4</Subscript> crystals

A method has been proposed to analyze the dynamics of interband two-photon absorption in a nonlinear medium excited by a sequence of picosecond laser pulses of variable intensity and continuous probe radiation. Induced absorption leading both to hysteresis in the dependence of the absorption on the intensity of laser pump radiation and to the opacity of crystals at the pump wavelength has been revealed in initially transparent ZnWO₄ and PbWO₄ crystals irradiated by a train of 523.5-nm pulses with a duration of 20 ps at pump intensities of 5 to 140 GW/cm². The kinetics of an increase in absorption and its subsequent relaxation at a 523.5-nm picosecond excitation of the crystals have been measured with continuous 633-nm probe radiation. An exponential component of the increase in absorption with the time constant τ = 2−3.5 and 8–9.5 μs depending on the direction of the linear polarization of pump radiation has been revealed at 300 K in ZnWO₄ and PbWO₄ crystals, respectively. The absorption relaxation kinetics in the crystals are complicated and approach an exponential at a late stage with the constant τ = 40−130 and 12–80 ms for the ZnWO₄ and PbWO₄ crystals, respectively.     

Room-temperature diode-pumped Yb<Superscript>3+</Superscript>-doped LiYF<Subscript>4</Subscript> and KYF<Subscript>4</Subscript> lasers

We present a comparative analysis on the growth, the spectroscopic features, and the cw laser action of room-temperature Yb(5%):LiYF₄ (YLF) and Yb(10%):KYF₄ (KYF) crystals. Optical slope efficiencies of 33% and 52% have been demonstrated for Yb:YLF and Yb:KYF crystals, respectively. A remarkable wide wavelength tunability from 1.01 to 1.07 μm has been obtained for both laser crystals.     

Lasing from a solid-state Ca<Subscript>3</Subscript>Ga<Subscript>2</Subscript>Ge<Subscript>3</Subscript>O<Subscript>12</Subscript>:Nd<Superscript>3+</Superscript> laser at a high power of diode pumping

Experimental data for cw lasing from a compact solid-state laser based on a neodymium-doped calcium-gallium-germanium-garnet crystal (Ca₃Ga₂Ge₃O₁₂:Nd³⁺) at a wavelength of 1.06 μm in the case of intense diode pumping are reported. The laser output reaches 0.7 W for a cavity 15 mm long and an active element 1 mm thick. It is shown that the output power is limited by a thermal lens placed in the active element.     

Temperature-dependent Sellmeier equation in the MIR for the extraordinary refractive index of 5% MgO doped congruent LiNbO<Subscript>3</Subscript>

We present a temperature-dependent Sellmeier equation for the extraordinary refractive index of 5 mol % MgO doped congruent lithium niobate. This equation is adapted for wavelengths in the range of 1.3–5 μm and temperatures between 40 °C and 200 °C. The calculation of the appropriate Sellmeier coefficients is based on the wavelengths of the signal and idler radiation measured for quasi-phase-matched optical parametric generators excited by 10-ns-long, 1064-nm pulses of a Q-switched Nd:YVO₄ laser. PACS 42.65.Ky; 42.70.Mp; 42.65.Yj     

Research of Tm (5.5 at %), Ho (0.55 at %):GdVO<Subscript>4</Subscript> laser pumped by diode laser at 800 nm

In this paper, we report a Tm (5.5 at %), Ho (0.55 at %):GdVO₄ laser pumped by diode laser at 800 nm. To our best knowledge, it is the first time that the use of Tm (5.5 at %), Ho (0.55 at %):GdVO₄ crystal among the similar experiments. We observed the influences of LD working temperature i.e. pump wavelength to 2 μm laser conversion efficiency. In the conditions of the continuous wave and 10 kHz acousto-optic Q-switch, high efficiency output of 2.05 μm laser was obtained. With the maximum pump power of 34.6, 13.9, and 13.6 W at 2.05 μm laser output was achieved respectively. Single laser pulse width was 25.6 ns in 10 kHz acousto-optic Q-switched condition.     

Power scaling of a continuous-wave and passively Q-switched Yb:KLu(WO<Subscript>4</Subscript>)<Subscript>2</Subscript> laser end-pumped by a high-power diode

The power scaling capacity of a diode end-pumped Yb:KLu(WO₄)₂ laser, operating in the continuous-wave (cw) and passively Q-switched regimes, has been investigated. A cw output power of 11.5 W was achieved with an optical-to-optical efficiency of 41% with respect to the incident pump power, while the slope efficiency amounts to 60%. The passively Q-switchedoperation yielded an average output power of 4.3 W at the fundamental wavelength of 1031.7 nm, and 1.15 W of Raman radiation at 1139.3 nm. The total slope efficiency for Q-switched operation was 40%. The highest pulse energy, duration, and peak power were 170 μJ, 2.2 ns, and 77.3 kW for the fundamental radiation, and 51 μJ, 2.3 ns, and 22.2 kW for the Raman radiation. PACS 42.55.Rz; 42.55.Xi; 42.55.Ye     

High-power,high-quality ZGP OPO pumped by a Tm,Ho:GdVO<Subscript>4</Subscript> laser

We report a ZGP OPO system capable of producing >6 W at a signal wavelength of 3.80 μm and an idler wavelength of 4.45 μm. The pumping source is the Tm,Ho:GdVO₄ laser operated at 2.049 μm with an M ² of 1.07. The ZGP OPO generated a total combined output power of 6.1 W at signal wavelength and idler wavelength under pumping power of 18.3 W, and an M ² of 1.7 for OPO output was obtained.     

Intracavity laser spectroscopy of CH<Subscript>4</Subscript> and NH<Subscript>3</Subscript> gases by using a pulse-periodic Cr<Superscript>2+</Superscript>:ZnSe laser

The results of studying the characteristics of an intracavity laser spectrometer based on a polycrystalline Cr²⁺:ZnSe laser operating in a pulse-periodic regime with the pulse-repetition rate of 3 kHz and pulse duration of ∼50 ns are presented. Intracavity spectra of absorption of NH₃ and CH₄ gases in the vicinity of 2.35 μm are measured. The estimate of the spectrometer sensitivity is provided.     

High-power,blue-light generation in a dual-structure,periodically poled,stoichiometric LiTaO<Subscript>3</Subscript> crystal

High-power blue light was generated from a diode-side-pumped Q-switched 1319 nm Nd:YAG laser with a periodically poled, stoichiometric LiTaO₃ (PPSLT) crystal. The PPSLT sample used in this experiment consists of two segments in series: the first segment has a period of 14.08 μm for the second harmonic generation (SHG) and the second segment has periods of around 4.6 μm for the generation of blue light by mixing fundamental and SH. An average power of 466 mW of a 440 nm blue light was obtained at the fundamental power of ∼5.4 W with a conversion efficiency of 8.6%. The output power fluctuated by 3% over a half-hour period. This result indicates that our scheme is a practical method to construct a reliable compact blue laser. PACS 42.70.Mp; 42.79.Nv; 42.55.Xi     

All fiber MOPA laser-pumped,continuous-wave,mid-infrared,singly-resonant optical parametric oscillator based on periodically poled MgO-Doped LiNbO<Subscript>3</Subscript>

We report a continuous-wave (CW) mid-infrared singly resonant optical parametric oscillator (SRO) based on periodically poled MgO-doped LiNbO₃ (PPMgLN) pumped by a high power, single frequency fiber laser in master oscillator-power amplifier (MOPA) configuration at 1.064 μm. Using four-mirror ring OPO cavities, at the PPMgLN’s grating period of 30.5 μm and the temperature of 23°C, we achieved the maximum idler output power of 7.2 W at 3.4 μm when the pump power was 52.8 W. The total power-conversion efficiency from the pump to the idler in this experiment is about 13.6%, and corresponds to ∼44% of quantum-limited performance.