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1.
Using Stark-pulse-modulated photon echoes, we observe a novel type of rephasing phenomenon in a Eu(3+) - and Pr(3+) -codoped Y(2)SiO(5) crystal. By adjusting the Stark pulse during the rephasing and dephasing periods one can observe a full recovery of the photon echo, corresponding to perfect dephasing-rephasing balancing of the perturbations. We propose to use this effect as a spectroscopic technique to distinguish between reversible and irreversible Stark interactions.  相似文献   

2.
Awad ES  Cho PS  Goldhar J 《Optics letters》2007,32(4):352-354
We report a novel implementation of an all-optical rephasing, reshaping, and reamplification differential phase shift keying (DPSK) regenerator. The rephasing is based on converting phase noise into amplitude noise by using an interferometric configuration and then eliminating the amplitude noise by using a semiconductor optical amplifier (SOA). The reshaping is performed using gain competition and gain compression in a saturated SOA. The scheme was tested using 10Gbit/s, 2(23)-1 pseudorandom bit sequence return-to-zero DPSK data. The measurement shows removal of the degraded data error floor with a 6 order-of-magnitude improvement in bit-error rate. The measured negative power penalty is about 4dB. Mathematical analysis shows a reduction in DPSK phase-noise power by half.  相似文献   

3.
The third-order polarization emitted from groups of individual localized excitonic transitions after pulsed optical excitation is measured. We observe the evolution of the nonlinear response from the case of a free polarization decay for a single transition, to that of a photon echo for many transitions. The echo is shown to arise from the mutual rephasing of the emission from individual transitions.  相似文献   

4.
We report the first observation of echoes in the electric dipole moment of an ensemble of Rydberg atoms precessing in an external electric field F. Rapid reversal of the field direction is shown to play a role similar to that of a pi pulse in NMR in rephasing a dephased ensemble of electric dipoles resulting in the buildup of an echo. The mechanisms responsible for this are discussed with the aid of classical trajectory Monte Carlo simulations.  相似文献   

5.
We analyze the storage and retrieval of a weak light pulse, having two orthogonally (circularly) polarized components, onto an atomic ensemble of four-level atoms of the tripod type driven by a far detuned coupling field. The atoms are subject to a longitudinal magnetic field which produces a spatially varying Zeeman splitting of the lower levels along the medium and allows for a spatial encoding of the different angular frequencies of the input pulse during the storage phase. A single reversion of the external magnetic field results in a rephasing of the dipoles and leads to the release of the stored signals. The shape of the recovered pulse is a time-reversal copy of the input pulse. The application of an additional reversion of the magnetic field during the storage phase allows the release of a copy of the input pulse without time reversal. We also show that the system may operate like an all-optical multiplexer when considering two impinging optical fields which have orthogonal components. The proposal has potential applications in quantum information processing.  相似文献   

6.
We propose an efficient quantum memory scheme with natural inhomogeneous broadening in an asymmetric optical cavity. The scheme uses the strong rephasing pulses like traditional photon echo techniques rather than spectral holeburning, which enables us to have the potential implementation in a much broader range of material systems. In the condition of impedance matching to an optical cavity, we find that the input light pulse can be completely absorbed by an atomic ensemble. We also show that the quantum memory efficiency can be equal to unity even for a small optical depth of the atomic system.  相似文献   

7.
Laboratory vapor phase condensation experiments systematically yield amorphous, homogeneous, nanoparticles with unique deep metastable eutectic compositions. They formed during the nucleation stage in rapidly cooling vapor systems. These nanoparticles evidence the complexity of the nucleation stage. Similar complex behavior may occur during the nucleation stage in quenched-melt laboratory experiments. Because of the bulk size of the quenched system many of such deep metastable eutectic nanodomains will anneal and adjust to local equilibrium but some will persist metastably depending on the time–temperature regime and melt/glass transformation.  相似文献   

8.
We consider a parametrization of the lepton mixing matrix in which the deviations from maximal atmospheric mixing and vanishing reactor mixing are obtained in terms of small corrections from the charged lepton sector. Relatively large deviations for the reactor mixing angle from zero as indicated by T2K experiment can be obtained in this parametrization. We are able to further reduce the number of complex phases, thus, simplifying the analysis. In addition, we have obtained the sides of unitarity triangles and the vacuum oscillation probabilities in this parametrization. The Jarlskog rephasing invariant measure of CP violation at the leading order has a single phase difference which can be identified as Dirac-type CP violating phase in this parametrization.  相似文献   

9.
We theoretically investigate the evolutions of two-dimensional, third-order, nonlinear pho-ton echo rephasing spectra with population time by using an exact numerical path integral method. It is shown that for the same system, the coherence time and relaxation time of excitonic states are short, however, if the couplings of electronic and intra-pigment vibra-tional modes are considered, the coherence time and relaxation time of this vibronic states are greatly extended. It means that the couplings between electronic and vibrational modes play important roles in keeping long-lived coherence in light-harvesting complexes. Particularly, by using the method we can fix the transition path of the energy transfer in bio-molecular systems.  相似文献   

10.
An Autler-Townes(AT) spectroscopy based on phase conjugate six-wave mixing(SWM) is proposed to detect AT doublet of high-lying state in a Doppler-broadened cascade four-level system.It is found that the SWM spectrum is dependent strongly on the ratios between the magnitudes of the wave vectors.We discuss how the Doppler broadening affects the SWM spectrum from a time-domain viewpoint and find that,due the atomic motion,the atomic polarizations acquire different phases for atoms with different velocities as time evolves.The Doppler free SWM spectrum can be obtained only when the atomic polarization can be rephasing again at certain time after the interactions of all the incident fields.  相似文献   

11.
Molecular wave-packet (WP) interferometry has been demonstrated in the A electronic state of the HgAr van der Waals complex with two time-delayed UV fs pulses at 254 nm. The interferograms of three vibrational levels in the WP's display almost 100% fringe contrast as a function of the interpulse delay tau, which is tuned with sub-10 as stability and resolution. It is clearly observed that the three interferograms show their dephasing and rephasing within a single vibrational period, allowing us to prepare arbitrary relative populations of the three levels by adjusting a single parameter tau.  相似文献   

12.
The vibrational dynamics of the first four antisymmetric stretch vibrational levels of azide in an ionic glass have been measured and correlated using a heterodyned fifth-order two-dimensional infrared pulse sequence. By rephasing a two-quantum coherence, a process not possible with third-order spectroscopy, solvent effects on the frequencies and anharmonicities of the potential energy surface are measured. Fifth-order pulse sequences are another step towards precisely controlling vibrational coherence in analogy to the manipulation of spins in NMR but with ultrafast time resolution.  相似文献   

13.
A two-dimensional (2D) infrared spectrum of Mn2(CO)10 is measured by using chirped-pulse upconversion (CPU) of the nonlinear signal field plus a reference local oscillator. By converting the spectrum to the visible, a silicon CCD camera can be used. The method offers an attractive alternative to direct IR detection due to the technological maturity of silicon and its greater intrinsic detectivity over HgCdTe. Using CPU, we acquired a rephasing 2D IR spectrum in a few seconds.  相似文献   

14.
The rephasing invariant formulation for the K0-K0 system is given and used to discuss the signs of the B parameter in M12 calculation andsin δ in the K-M matrix (both are positive). The meaning of the singularity appeared in the exact formula of the ε parameter, which does not appear in the popular formula in the literature, is also discussed.  相似文献   

15.
We describe a novel velocity-selection technique for measuring dispersive phase shifts in matter-wave interferometers. Where conventional velocity-selection techniques simply reduce the width of the initial velocity distribution, here, the velocity distribution is chopped into a series of narrow peaks such that the velocity dependence of the phase shifts will result in a rephasing of the interference for certain strengths of applied potential. This technique overcomes limitations due to wide and poorly known velocity distributions and thus allows a better determination of the applied interaction with complete independence from the initial velocity distribution of the beam.Dedicated to H. Walther on the occasion of his 60th birthday  相似文献   

16.
Experimental evidence is presented showing that photocurrents in silicon can be used as highly sensitive readout probes for coherent spin states of localized electrons, the prime candidates for quantum bits in various semiconductor based quantum computer concepts. Conduction electrons are subjected to fast Rabi oscillation induced by means of pulsed electron spin resonance. The collective spin motion of the charge carrier ensemble is reflected by a spin-dependent recombination rate and therefore by the sample conductivity. Because of inhomogeneities, the Rabi oscillation dephases rapidly. However, a microwave induced rephasing is possible causing an echo effect whose intensity contains information about the charge carrier spin state and the coherence decay.  相似文献   

17.
To establish which technical variables influence the detection of deep vein thrombosis by magnetic resonance imaging, 2 dogs, 5 normal volunteers and 17 patients were studied using a 1.5 T whole-body system. A sequential slice gradient echo acquisition (TR 25, TE 13, 0 = 30 degrees, 2 NEX, flow compensation rephasing gradients) in the axial plane was found to be optimal for detecting venous thrombosis. Thus, when using appropriate technique, MRI may identify deep venous thrombosis accurately. It may also allow the diagnosis of conditions which may simulate venous thrombosis clinically since the most common of these, ruptured Baker's cyst, cellulitis, muscle tear, hematoma and external venous compression are all readily identified by MRI.  相似文献   

18.
The Motion Artifact Suppression Technique (MAST) is a method which uses a series of gradient echos that are computed to cancel velocity, acceleration and pulsatility components of involuntary motion in MR imaging. A total of 916 patient studies were performed over a nine month period using MAST sequences with a TE 40, 60, 80, 100, 120, and 26/112. There was considerable improvement in long TR, long TE images. Cerebrospinal fluid flow artifacts were reduced. Body and spine images had reduced flow and respiratory artifacts. Spin rephasing in blood vessels caused increase intraluminal signal. This might be useful for cardiovascular imaging.  相似文献   

19.
Two closely spaced 778 nm, 4-ps pulses, two-photon resonant with the 5S-5D transition in Rb vapor generate a ground state grating, which later is excited by a similar third pulse, producing conical yoked superfluorescence echo on the 5S-6P, 420-nm transition. The intensity of this emission as a function of the relative delay between the leading excitation pulses is governed by the dynamics of Doppler dephasing and rephasing. This is the first observation of an echo effect induced by a spontaneous relaxation process.  相似文献   

20.
Insomnia is a common sleep disorder that is closely associated with the occurrence and deterioration of cardiovascular disease, depression and other diseases. The evaluation of pharmacological treatments for insomnia brings significant clinical implications. In this study, a total of 20 patients with mild insomnia and 75 healthy subjects as controls (HC) were included to explore alterations of electroencephalogram (EEG) complexity associated with insomnia and its pharmacological treatment by using multi-scale permutation entropy (MPE). All participants were recorded for two nights of polysomnography (PSG). The patients with mild insomnia received a placebo on the first night (Placebo) and temazepam on the second night (Temazepam), while the HCs had no sleep-related medication intake for either night. EEG recordings from each night were extracted and analyzed using MPE. The results showed that MPE decreased significantly from pre-lights-off to the period during sleep transition and then to the period after sleep onset, and also during the deepening of sleep stage in the HC group. Furthermore, results from the insomnia subjects showed that MPE values were significantly lower for the Temazepam night compared to MPE values for the Placebo night. Moreover, MPE values for the Temazepam night showed no correlation with age or gender. Our results indicated that EEG complexity, measured by MPE, may be utilized as an alternative approach to measure the impact of sleep medication on brain dynamics.  相似文献   

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