Rapid roughening in thin film growth of an organic semiconductor (diindenoperylene)

The scaling exponents alpha, beta, and 1/z in thin films of the organic molecule diindenoperylene deposited on SiO2 under UHV conditions are determined. Atomic-force microscopy, x-ray reflectivity, and diffuse x-ray scattering were employed. The surface width displays power law scaling over more than 2 orders of magnitude in film thickness. We obtained alpha = 0.684+/-0.06, beta = 0.748+/-0.05, and 1/zeta = 0.92+/-0.20. The derived exponents point to an unusually rapid growth of vertical roughness and lateral correlations. We suggest that they could be related to lateral inhomogeneities arising from the formation of grain boundaries between tilt domains in the early stages of growth.     

Kinetic roughening in polymer film growth by vapor deposition

The growth front roughness of linear poly( p-xylylene) films grown by vapor deposition polymerization has been investigated using atomic force microscopy. The interface width w increases as a power law of film thickness d, w approximately d(beta), with beta = 0. 25+/-0.03, and the lateral correlation length xi grows as xi approximately d(1/z), with 1/z = 0.31+/-0.02. This novel scaling behavior is interpreted as the result of monomer bulk diffusion, and belongs to a new universality class that has not been discussed previously.     

Random walks on a ( 2+1)-dimensional deformable medium

A model of random walks on a deformable medium is proposed in 2+1 dimensions. The behavior of the walk is characterized by the stability parameter beta and the stiffness exponent alpha. The average square end-to-end distance l approximately equals (2nu) and the average number of visited sites approximately equals (k) are calculated. As beta increases, for each alpha there exists a critical transition point beta(c) from purely random walks ( nu = 1/2 and k approximate to 1) to compact growth ( nu = 1/3 and k = 2/3). The relationship between beta(c) and alpha can be expressed as beta(c) = e(alpha). The landscape generated by a walk is also investigated by means of the visit-number distribution N(n)(beta). There exists a scaling relationship of the form N(n)(beta)approximately n(-2)f(n/beta(z)).     

Neutron polarizabilities investigated by quasifree Compton scattering from the deuteron

Measuring Compton scattered photons and recoil neutrons in coincidence, quasifree Compton scattering by the neutron has been investigated at MAMI (Mainz) at theta(lab)(gamma) = 136 degrees in an energy range from 200 to 400 MeV. From the data a polarizability difference of alpha(n)-beta(n) = 9.8+/-3.6(stat)+2.1-1.1(syst)+/-2.2(model) in units of 10(-4) fm(3) has been determined. In combination with the polarizability sum alpha(n)+beta(n) = 15.2+/-0.5 deduced from photoabsorption data, the first precise results for the neutron electric and magnetic polarizabilities, alpha(n) = 12.5+/-1.8(stat)+1.1-0.6(syst)+/-1.1(model) and beta(n) = 2.7-/+1.8(stat)+0.6-1.1(syst)-/+1.1(model), are obtained.     

Maximal height scaling of kinetically growing surfaces

The scaling properties of the maximal height of a growing self-affine surface with a lateral extent L are considered. In the late-time regime its value measured relative to the evolving average height scales like the roughness: h*(L) approximately L alpha. For large values its distribution obeys logP(h*(L)) approximately (-)A(h*(L)/L(alpha))(a). In the early-time regime where the roughness grows as t(beta), we find h*(L) approximately t(beta)[lnL-(beta/alpha)lnt+C](1/b), where either b = a or b is the corresponding exponent of the velocity distribution. These properties are derived from scaling and extreme-value arguments. They are corroborated by numerical simulations and supported by exact results for surfaces in 1D with the asymptotic behavior of a Brownian path.     

What controls the thickness of wetting layers near bulk criticality?

We study the thickness of wetting layers in the binary-liquid mixture cyclohexane methanol. Far from the bulk critical point, the wetting layer thickness is independent of temperature, resulting from the competition between van der Waals and gravitational forces. Upon approaching the bulk critical temperature [t=(T(c)-T)/T(c)-->0], we observe that the wetting layer thickness diverges as t(-beta) with effective critical exponent beta=0.23+/-0.06. This is characteristic of a broad, intermediate scaling regime for the crossover from van der Waals wetting to critical scaling. We predict beta=beta/3 approximately 0.11, with beta the usual bulk-order parameter critical exponent, showing a small but significant difference with experiment.     

Critical scaling properties at the superfluid transition of 4He in aerogel

We study the superfluid transition of 4He in aerogel by Monte Carlo simulations and finite size scaling analysis. Aerogel is a highly porous silica glass, which we model by a diffusion limited cluster aggregation model. The superfluid is modeled by a three dimensional XY model, with excluded bonds to sites on the aerogel cluster. We obtain the correlation length exponent nu=0.73+/-0.02, in reasonable agreement with experiments and with previous simulations. For the heat capacity exponent alpha, both experiments and previous simulations suggest deviations from the Josephson hyperscaling relation alpha=2-dnu. In contrast, our Monte Carlo results support hyperscaling with alpha=-0.2+/-0.05. We suggest a reinterpretation of the experiments, which avoids scaling violations and is consistent with our simulation results.     

Tricritical point and the doping dependence of the order of the ferromagnetic phase transition of La1-xCaxMnO3

We report on the doping dependence of the order of the ferromagnetic metal to paramagnetic insulator phase transition in La1-xCaxMnO3. At x=0.33, magnetization and specific heat data show a first order transition, with an entropy change (2.3 J/mol K) accounted for by both volume expansion and the discontinuity of M approximately 1.7mu(B) via the Clausius-Clapeyron equation. At x=0.4, the data show a continuous transition with tricritical point exponents alpha=0.48+/-0.06, beta=0.25+/-0.03, gamma=1.03+/-0.05, and delta=5.0+/-0.8. This tricritical point separates first- (x<0.4) from second-order (x>0.4) transitions.     

Anisotropic scaling and generalized conformal invariance at Lifshitz points

The behaviour of the 3D axial next-nearest-neighbor Ising model at the uniaxial Lifshitz point is studied using Monte Carlo techniques. A new variant of the Wolff cluster algorithm permits the analysis of systems far larger than in previous studies. The Lifshitz point critical exponents are alpha = 0.18(2), beta = 0.238(5), and gamma = 1.36(3). Data for the spin-spin correlation function are shown to be consistent with the explicit scaling function derived from the assumption of local scale invariance, which is a generalization of conformal invariance to the anisotropic scaling at the Lifshitz point.     

Muon decay: measurement of the transverse polarization of the decay positrons and its implications for the fermi coupling constant and time reversal invariance

The two transverse polarization components P(T1) and P(T2) of the e(+) from the decay of polarized mu(+) have been measured as a function of the e(+) energy. Their energy averaged values are P(T1)=(6.3+/-7.7+/-3.4) x 10(-3) and P(T2)=(-3.7+/-7.7+/-3.4) x 10(-3). From the energy dependence of P(T1) and P(T2) the decay parameters eta,eta(') and alpha(')/A,beta(')/A are derived, respectively. Assuming only one additional coupling besides the dominant V-A interaction one gets improved limits on eta, beta(')/A, and the scalar coupling constant g(S)(RR): eta=(-2.1+/-7.0+/-1.0) x 10(-3), beta(')/A=(-1.3+/-3.5+/-0.6) x 10(-3), Re{g(S)(RR)}=(-4.2+/-14.0+/-2.0) x 10(-3), and Im{g(S)(RR)}=(5.2+/-14.0+/-2.4) x 10(-3).     

New scaling law for the decay exponent of bimolecular reactions in unbounded transitional flows

We propose a new scaling law for global kinetics of the stoichiometric reaction A+B-->P in unsteady, transitional flows. We find in the nonlinear flow regime the decay as approximately t(-alpha) where alpha is related to a space-time scaling parameter psi as alpha proportional, variant psi(m), for the considered parameter range m=0.067. In the linear flow regime, we find that the maximum is alpha approximately 2/3 for psi approximately 1. The proposed scaling law should be useful for linking dynamical subgrid processes with reaction kinetics in a variety of transitional flow systems.     

Hydrodynamic coarsening of binary fluids

By suitable interpretation of results from the linear analysis of interface dynamics, it is found that the hydrodynamic growth of the size L of domains that follow spinodal decomposition in fluid mixtures scales with time as L approximately t(alpha), with alpha = 4/7 in the inertial regime. The previously proposed exponent alpha = 2/3 is shown to indicate only the scaling of the oscillatory frequency omega(-2/3) approximately L of the largest structures of the system. The viscous dissipation in the system occurs within a layer of thickness L(d) that also follows a power law of the form L(d) approximately L3/4 in the inertial regime. In the viscous regime the growth is linear in time L approximately t and the dissipative region remains constant L(d) approximately L0.     

Temporal variability of the telluric sodium layer

The temporal variability of the telluric sodium layer is investigated by analyzing 28 nights of data obtained with the Colorado State University LIDAR experiment. The mean height power spectrum of the sodium layer was found to be well fitted by a power law over the observed range of frequencies, 10 microHz to 4 mHz. The best-fitting power law was found be be 10(beta)nu(alpha), with alpha=-1.79+/-0.02 and beta=1.12+/-0.40. Applications to wavefront sensing require knowledge of the behavior of the sodium layer at kilohertz frequencies. Direct measurements at these frequencies do not exist. Extrapolation from low-frequency behavior to high frequencies suggests that this variability may be a significant source of error for laser guide star adaptive optics in large-aperture telescopes.     

Determination of the 17O NMR tensors in potassium hydrogen dibenzoate: a salt containing a short O...H...O hydrogen bond

Solid-state 17O NMR spectra were obtained at 4.70, 11.75 and 19.60T for potassium hydrogen [17O(4)]dibenzoate (PHB) under both magic-angle spinning and stationary conditions. Spectral analyses yielded both the magnitude and orientation of the 17O chemical shift (CS) tensor and the electric field gradient (EFG) tensor for each of the two chemically distinct oxygen sites in PHB. For the oxygen site that is not involved in hydrogen bonding, the experimental 17O NMR tensors are: delta(iso)=287+/-2 ppm, delta(11)=470+/-5 ppm, delta(22)=380+/-5 ppm, delta(33)=10+/-5 ppm, C(Q)=8.30+/-0.02 MHz, eta(Q)=0.23+/-0.05, alpha=0+/-5 degrees, beta=90+/-5 degrees, and gamma=30+/-5 degrees. For the oxygen site in the short O...H...O hydrogen bond, the experimental 17O NMR tensors are: delta(iso)=213+/-2 ppm, delta(11)=370+/-5 ppm, delta(22)=190+/-5 ppm, delta(33)=80+/-5 ppm, C(Q)=5.90+/-0.02 MHz, eta(Q)=0.55+/-0.05, alpha=5+/-5 degrees, beta=90+/-5 degrees, and gamma=90+/-5 degrees. Extensive quantum mechanical calculations at both restricted Hartree-Fock and density functional theory levels were performed to investigate the effects of an effectively symmetrical O...H...O hydrogen bond on 17O CS and EFG tensors.     

Precise measurements of bulk-wave ultrasonic velocity dispersion and attenuation in solid materials in the VHF range

A general method was established for precisely measuring velocity dispersion and attenuation in solid specimens with acoustic losses in the very high frequency (VHF) range, using the complex-mode measurement method and the diffraction correction method. Experimental procedures were presented for implementing such a method and demonstrated this measurement method in the frequency range of 50-230 MHz, using borosilicate glass (C-7740) as a dispersive specimen and synthetic silica glass (C-7980) as a nondispersive standard specimen. C-7980 exhibited no velocity dispersion; velocity was constant at 5929.14 +/- 0.03 m/s. C-7740 exhibited velocity dispersion, from 5542.27 m/s at 50 MHz to 5544.47 m/s at 230 MHz with an increase of about 2 m/s in the measured frequency range. When frequency dependence of attenuation was expressed as alpha = alpha(0)f(beta), the results were as follows: alpha0 = 1.07 x 10(-16) s2/m and beta = 2 for C-7980 and alpha0 = 5.16 x 10(-9) s(1.25)/m and beta = 1.25 for C-7740.     

Strong coupling constant from scaling violations in fragmentation functions

We present a new determination of the strong coupling constant alpha(s) through the scaling violations in the fragmentation functions for charged pions, charged kaons, and protons. In our fit we include the latest e+e- annihilation data from CERN LEP1 and SLAC SLC on the Z-boson resonance and older, yet very precise, data from SLAC PEP at center-of-mass energy sqaure root of s = 29 GeV. At next-to-leading order, we find alpha(s)(5)(M(Z)) = 0.1170+/-0.0073. A new world average of alpha(s) is given.     

Experimental observation of disorder-driven hysteresis-loop criticality

We have studied the effect of magnetic disorder on the magnetization reversal process in thin Co/CoO films. The antiferromagnetic CoO layer allows a reversible tuning of the magnetic disorder by simple temperature variation. For temperatures above a critical temperature T(c), we observe a discontinuous magnetization reversal, whereas smooth magnetization loops occur for T相似文献   

Pressure spectrum in homogeneous turbulence

The pressure spectrum in homogeneous steady turbulence is studied using direct numerical simulation with resolution up to 1024(3) and the Reynolds number R(lambda) between 38 and 478. The energy spectrum is found to have a finite inertial range with the Kolmogorov constant K = 1.65+/-0.05 followed by a bump at large wave numbers. The pressure spectrum in the inertial range is found to be approximately P(k) = B(p)epsilon;(4/3)k(-7/3) with B(p) = 8.0+/-0.5, and followed by a bump of nearly k(-5/3) at higher wave numbers. Universality and a new scaling of the pressure spectrum are discussed.     

Compton scattering from the deuteron and extracted neutron polarizabilities

Differential cross sections for Compton scattering from the deuteron were measured at MAX-Lab for incident photon energies of 55 and 66 MeV at nominal laboratory angles of 45 degrees, 125 degrees, and 135 degrees. Tagged photons were scattered from liquid deuterium and detected in three NaI spectrometers. By comparing the data with theoretical calculations in the framework of a one-boson-exchange potential model, the sum and the difference of the isospin-averaged nucleon polarizabilities, alpha(N)+beta(N)=17.4+/-3.7 and alpha(N)-beta(N)=6.4+/-2.4 (in units of 10(-4) fm(3)), have been determined. By combining the latter with the global-averaged value for alpha(p)-beta(p) and using the predictions of the Baldin sum rule for the sum of the nucleon polarizabilities, we have obtained values for the neutron electric and magnetic polarizabilities of alpha(n)=8.8+/-2.4(total)+/-3.0(model) and beta(n)=6.5-/+2.4(total)-/+3.0(model), respectively.     

Is a Griffiths phase a prerequisite for colossal magnetoresistance?

Detailed measurements of the magnetic and transport behavior of the two La(1-x)Ca(x)MnO(3) single crystals exhibiting colossal magnetoresistance are summarized. The x=0.21 sample exhibits unusual exponents (delta = 20+/-1, gamma = 1.71+/-0.1, beta = 0.09+/-0.01, T(C) = 182+/-1 K) and, more importantly, a Griffiths phase characterized by an exponent lambda = 0.70+/-0.2. By contrast, the x=0.20 specimen displays Heisenberg model behavior with no evidence of such a phase. Thus while a Griffiths phase accounts for the behavior of La(1-x)Ca(x)MnO(3) near optimal doping, it does not appear to be a prerequisite for colossal magnetoresistance in this system.