Cluster ion emission from LiF induced by MeV N<Superscript>q+</Superscript> projectiles and <Superscript>252</Superscript>Cf fission fragments

Ion cluster desorption yields from LiF were measured at PUC-Rio with ≈0.1 MeV/u N ^q+ (q = 2,4,5,6) ion beams by means of a time-of-fight (TOF) mass spectrometer. A ²⁵²Cf source mounted in the irradiation chamber allows immediate comparison of cluster emissions induced by ≈65 MeV fission fragments (FF). Emission of (LiF) _n Li⁺ clusters are observed for both the N beams and the ²⁵²Cf fission fragments. The observed cluster size n varies from 1 to 6 for N ^q+ projectiles and from 1 to ≈40 for the ²⁵²Cf-FF. The size dependence of the Y(n) distributions suggests two cluster formation regimes: (i) recombination process in the outgoing gas phase after impact and (ii) emission of pre-formed clusters from the periphery of the impact site. The corresponding distribution of ejected negative cluster ions (LiF) _n F⁻ closely resembles that of the positive secondary (LiF) _n Li⁺ ions. The desorption yields of positive ions scale as Y(n) ∼ q ⁵. A calculation with the CASP code shows that this corresponds to a cubic scaling ∼S _e ³ with the electronic stopping power S _e , as predicted by collective shock wave models for sputtering and models involving multiple excitons (Frenkel pair sputtering). We discuss possible interpretations of the functional dependence of the evolution of the cluster emission yield Y(n) with cluster size n, fitted by a number of statistical distributions.     

Improved (1s)<Superscript>2</Superscript> variational model for helium

The ground-state energy of neutral helium is estimated variationally with a trial wavefunction of the form ϕ≈e ^−γ(rA/a _o)ⁿe^−γ(rB/a _o)ⁿ. This model represents a modification of traditional textbook examinations of this problem via inclusion of the power “n” as a second nonlinear variational parameter in addition to the usual effective nuclear charge γ and leads to an upper-limit on the ground state energy of −2.86107 E _h (E _h =1 hartree) in comparison with the traditional (n=1) result of −2.84766 E _h . This result represents a reduction of the percentage overestimate from the true ground-state energy (−2.90373 E _h ) of from 1.93 to 1.47. In comparison with the maximum accuracy obtainable from an uncorrelated trial wavefunction, −2.86168 E _h , the present trial wavefunction reduces the percentage overestimate from 0.49 (n=1) to 0.021. The optimum values of (n, γ) are determined to be ≈(0.897, 1.825).     

Fine and hyperfine structure of the muonic <Superscript>3</Superscript>He ion

On the basis of quasipotential approach to the bound state problem in QED we calculate the vacuum polarization, relativistic, recoil, structure corrections of orders α ⁵ and α ⁶ to the fine structure interval ΔE ^fs = E(2P _3/2) − E(2P _1/2) and to the hyperfine structure of the energy levels 2P _1/2 and 2P _3/2 in muonic ₂³He ion. The resulting values ΔE ^fs = 144 803.15 μeV, Δ$ \tilde E $ \tilde E ^hfs(2P _1/2) = −58 712.90 μeV, Δ$ \tilde E $ \tilde E ^hfs(2P _3/2) = −24 290.69 μeV provide reliable guidelines in performing a comparison with the relevant experimental data.     

Fine structure of the muonic <Superscript>4</Superscript>He ion

On the basis of quasi-potential approach to the bound state problem in QED we calculate the vacuum polarization, recoil and structure corrections of orders α⁵ and α⁶ to the fine splitting interval ΔE ^fs = E(2P _3/2) − E(2P _1/2) in muonic ₂⁴He ion. The resulting value ΔE ^fs = 146180.68 μeV provides reliable guideline in performing a comparison with the relevant experimental data.     

Search for solar axions generated by the Primakoff effect with resonance absorption by <Superscript>169</Superscript>Tm

We searched for resonant excitation of the first excited state of the ¹⁶⁹Tm nucleus by axions formed inside the Sun by the Primakoff effect, A + ¹⁶⁹Tm → ¹⁶⁹Tm* → ¹⁶⁹Tm + γ (8.41keV). Gamma quanta with an energy of 8.41keV were registered by a sectionalized Si(Li) detector installed in a low-background setup. As a result, we set a new upper limit for the photon to axion coupling constant, g _Aγ (GeV⁻¹)m _A (eV) ≤ 1.06 × 10⁻⁵, which for a hadronic axion model corresponds to a mass limit of m _A ≤ 169 eV at a 90% confidence level.     

Hyperfine structure of <Emphasis Type="Italic">S</Emphasis>- and <Emphasis Type="Italic">P</Emphasis>-wave states in muonic-helium ion

Corrections of order α ⁵ and α ⁶ to the hyperfine structure of S- and P-wave energy levels of the muonic-helium ion are calculated. Electron-vacuum-polarization effects, corrections for the nuclear structure, and recoil effects are taken into account. The numerical values obtained for respective hyperfine splitting, −1334.73 meV (1S), −166.64 meV (2S), −58 712.90 μeV (2P _1/2), and −24 290.69 μeV (2P _3/2), can be viewed as a reliable estimate for a comparison with experimental data, and the hyperfine-structure interval of Δ₁₂ = 8ΔE ^hfs(2S) − ΔE ^hfs(1S) = 1.59 meV can be used to test QED predictions.     

X-ray spectra induced by <Superscript>129</Superscript>Xe<Superscript><Emphasis Type="Italic">q</Emphasis>+</Superscript> impacting the metal surface

Using the slow highly charged ions ¹²⁹Xe ^q+ (q = 25, 26, 27; initial kinetic T ₀⩽4.65 keV/a.u.) to impact Au surface, the Au atomic Mα characteristic X-ray spectrum is induced. The result shows that as long as the charge state of projectile is high enough, the heavy atomic characteristic X-ray can be effectively excited even though the incident beam is very weak (nA magnitude), and the X-ray yield per ion is in the order of 10⁻⁸ and increases with the kinetic energy and potential energy of projectile. By measuring the Au Mα-X-ray spectra, Au atomic N-level lifetime is estimated at about 1.33×10⁻¹⁸ s based on Heisenberg uncertainty relation. Supported by the National Natural Science Foundation of China (Grant Nos. 10574132, 10274088 and 10405025), the Talent Introduction Project of Xianyang Normal University (Grant No. 05XSYK103) and the Education Commission Foundation of Shaanxi Province (Grant No. 04JK300)     

ESR determination of the thermal stability of Mn<Superscript>2+</Superscript> ion binding sites in different legume lectins

The legume lectins are a large family of homologous carbohydrate-binding proteins. Their carbohydrate specificity and quaternary structure vary widely. The carbohydrate binding activity of legume lectins depends on the simultaneous presence of calcium and transition-metal ions, especially the Mn²⁺ ion. In the present work, thermal stabilities of Mn²⁺ binding sites in pea, lentil, soybean and kidney-bean lectins have been studied by electron spin resonance spectroscopy in the temperature range of 120–400 K in different atmospheres. The evolution of parameters, such as the line width, peak-to-peak intensity associated with the hyperfine transition [m _I (+5/2) → m′ _I (−5/2)] at the lowest magnetic field side of the central electron transition [m _S (+1/2) → m′ _S (−1/2)] of the Mn⁺² ion, g-factor and hyperfine splitting was evaluated. Annealing was also performed at high temperatures (353, 373, 383, 403 and 443 K) and the oxidation activation energy of Mn²⁺ ions in the indicated legumes was determined.     

On the unusual properties of the 282 keV state in <Superscript>135</Superscript>Sb

Recently the first excited state in ¹³⁵Sb has been observed at the unexpectedly low excitation energy of only 282keV and interpreted as mainly d _5/2 proton coupled to the ¹³⁴Sn core. Based on theoretical considerations it was suggested that its low excitation energy is related to a relative shift of the proton d _5/2 and g _7/2 orbits induced by the neutron excess. We have measured the lifetime of the 282keV state by the advanced time-delayed βγγ(t) method. The measured half-life, T _1/2 = 6.1(4)ns, yields exceptionally low limits of B(M1;5/2₁ ⁺→7/2₁ ⁺)≤3.0×10^-4 μ ² _N and B(E2;5/2₁ ⁺→7/2₁ ⁺)≤54e ² fm ⁴. These strongly hindered M1 and slow E2 transition rates are similar to those for the transition de-populating the first excited state at 405keV in ²¹¹Bi. Results of shell model calculations with realistic interactions are presented. The M1 decay rate was found to be extremely sensistive both to the wave function and to the M1 effective operator.     

Torus Equivariant Spectral Triples for Odd-Dimensional Quantum Spheres Coming from <Emphasis Type="Italic">C</Emphasis><Superscript>*</Superscript>-Extensions

The torus group (S ¹)^ℓ+1 has a canonical action on the odd-dimensional sphere S _q ^2ℓ+1. We take the natural Hilbert space representation where this action is implemented and characterize all odd spectral triples acting on that space and equivariant with respect to that action. This characterization gives a construction of an optimum family of equivariant spectral triples having nontrivial K-homology class thus generalizing our earlier results for SU _q (2). We also relate the triple we construct with the C ^*-extension      

Partial-wave analysis for elastic <Emphasis Type="Italic">p</Emphasis><Superscript>13</Superscript>C scattering at astrophysical energies

A standard partial-wave analysis was performed on the basis of known measurements of differential cross sections for elastic p ¹³C scattering at energies in the range 250–750 keV. This analysis revealed that, in the energy range being considered, it is sufficient to take into account the ³ S ₁ wave alone. A potential for the triplet ³ S ₁-wave state of the p ¹³C system in the region of the J ^p T = 1⁻¹ resonance at 0.55 MeV was constructed on the basis of the phase shifts obtained from the aforementioned partial-wave analysis.     

High-spin states of<Superscript>125</Superscript>Sb: Particle-core excitation coupling

Excited states of¹²⁵Sb have been studied using in-beam γ spectroscopy techniques via the¹²⁴Sn(⁷Li, α2n) reaction at a beam energy of 32 MeV. A high-spin level scheme including 21 new γ-transitions and 14 new excited states have been established. Three isomers have been identified at 1970, 2110 and 2471 keV and the ranges of their half-lives have been estimated from the delayed coincidence data. The level structure of¹²⁵Sb is discussed in terms of particle-core excitation coupling. With the help of empirical shell model calculations the three isomers are proposed to have three-quasiparticle πg_7/2⊗v(h _11/2 s _1/2)₅₋, πg_7/2⊗v(h _11/2 d _3/2)₇₋ and πg_7/2⊗v(h ₁₁^2/2)₁₀ ⁺ configurations, respectively.     

<Superscript>4</Superscript>He<Superscript>3</Superscript>H<Superscript>2</Superscript>H three-body model of the <Superscript>9</Superscript>Be nucleus

Within the framework of the single-channel approximation, an {αtd} model of the ⁹ Be nucleus is presented. A comparative analysis of the t ⁶ Li wave functions describing relative motion of bound states constructed in {ααn} and {αtd} cluster representations is carried out on the example of calculations of the ⁹ Be(γ,t₀)⁶ Li process characteristics. __________ Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 1, pp. 85–89, January, 2008.     

Direct calculation of transition intensities in LiYF<Subscript>4</Subscript>: Nd<Superscript>3+</Superscript>

Duan’s simple model is extended to analyze the mixing of the 4f ^{N − 1}5d configuration with the 4f ^N states. The explicit static coupling and traditional dynamic coupling are considered, and the parameters are fitted according to the absorption spectrum in LiYF₄: Nd³⁺. The parameter values obtained are as follows: T ₃₂ = −28i × 10⁻⁷, T ₅₂ = −1151i × 10⁻⁷, A ₃₂² = 192i × 10⁻¹² cm, A ₅₂⁴ = i × 10⁻¹² cm, A ₇₂⁶ = 54i × 10⁻¹² cm, and A ₇₆⁶ = −680i × 10⁻¹² cm. Compared to the experimental measurements, the present model yields better results than those obtained from the Judd-Ofelt theory. The text was submitted by the authors in English.     

Deuteron scattering on <Superscript>6</Superscript>Li at an energy of 25 MeV

At an energy of 25 MeV and in the angular range 7°−175° in the laboratory frame, angular distributions were measured for elastic deuteron scattering on ⁶Li nuclei and for the respective inelastic-scattering processes accompanied by the transitions to the ground state (1+) of the ⁶Li nucleus and to its excited state at E _x = 2.186 MeV (J ^π = 3⁺). The resulting data were analyzed on the basis of the optical model of the nucleus and the coupled-reaction-channel method with allowance for the mechanism of alpha-particle-cluster exchange. It is shown that only upon including, in the analysis, channel coupling and the exchange mechanism can the experimental cross sections for elastic and inelastic scattering be reproduced over the entire range of angles.     

Cluster radioactivity leading to doubly magic <Superscript>100</Superscript>Sn and <Superscript>132</Superscript>Sn daughters

Decay of neutron-deficient ^{128 − 137}Gd parents emitting ⁴He to ³²S clusters are studied within the Coulomb and proximity potential model. The predicted half-lives are compared with other models and most of the values are well within the present experimental limit for measurements (T _1/2 < 10³⁰ s). The lowest T _1/2 value for ²⁸Si emission from ¹²⁸Gd indicates the role of doubly magic ¹⁰⁰Sn daughter in cluster decay process. It is also found that neutron excess in the parent nuclei slows down the cluster decay process. Geiger–Nuttal plots for all clusters are found to be linear with different slopes and intercepts. The α-decay half-lives of ^{148 − 152}Gd parents are computed and are in agreement with experimental data. The role of doubly magic ¹³²Sn daughter in cluster decay process is also examined for various neutron-rich Ba, Ce, Nd, Sm and Gd parents emitting clusters ranging from ⁴He to ³²Si. Alpha-like structures are most probable in the decays leading to ¹⁰⁰Sn, while non-α-like structures are probable in the decays leading to ¹³²Sn. The neutron–proton asymmetry in parent and daughter nuclei is responsible for the reduced decay rate in the decay leading to ¹³²Sn.     

Study of the isobar configurations in the <Superscript>12</Superscript>C and <Superscript>16</Superscript>O ground states

Experimental research on positive-pion photoproduction on the oxygen nucleus in the ¹⁶O(γ, π⁺p) reaction at high recoil momenta of the residual nuclear system was performed. The yield for the ¹⁶O(γ, π⁺p) reaction was analyzed using a model that takes Δ-isobar configurations in nuclei ground states into account, together with the earlier-measured yield of the¹²C(γ, π⁺p) reaction. The estimated number of isobars per nucleon N _Δ = 0.012 ± 0.005 was obtained for the ¹²C nucleus, and ¹⁶O N _Δ = 0.018 ± 0.004 was obtained for the ¹⁶O nucleus.     

Effect of Sr<Superscript>2+</Superscript> ion substitution with trivalent ions (Sc<Superscript>3+</Superscript>, In<Superscript>3+</Superscript>, La<Superscript>3+</Superscript>, Bi<Superscript>3+</Superscript>) on its ferroelectric instability in SrTiO<Subscript>3</Subscript>

The vibration frequencies of unstable ferroelectric and antiferrodistortion modes and the dependences of the energy on the ion displacement amplitude have been calculated within the generalized Gordon-Kim model for distortions along eigenvectors of these modes in the mixed compounds Sr_{1 − x} A _x Ti_{1 − x} /₄□ _x/4O₃ and Sr_{1 − y} A _2y /₃□ _y/3TiO₃ (A = Sc³⁺, In³⁺, La³⁺, Bi³⁺; □ is the vacancy). To compensate an excess positive charge, vacancies are introduced into the Ti⁴⁺ or Sr²⁺ site. Calculations have been performed in the “daverage” crystal approximation for impurity concentrations of 0.25 and 0.50. To this end, a set of 40 atomic superlattices with various orderings of heterovalent ions Sr²⁺ and impurity A ³⁺ has been considered. It has been found that each impurity type, independently of charge balance, induces ferroelectric instabilities in doped compounds. In the case of doping with In³⁺ and La³⁺ for concentration x = 0.25, the possibility of rotating the polarization vector has been shown.     

Associated single photons and doubly-charged scalars at linear <Emphasis Type="Italic">e</Emphasis><Superscript>−</Superscript><Emphasis Type="Italic">e</Emphasis><Superscript>−</Superscript> colliders

Doubly-charged scalars, predicted in many models having exotic Higgs rep-resentations, can in general have lepton-number violating (LFV) couplings. We show that by using an associated monoenergetic final state photon seen at a future linear e ⁻ e ⁻ collider, we can have a clear and distinct signature for a doubly-charged resonance. The strength of the ΔL = 2 coupling can also be probed quite effectively as a function of the recoil mass of the doubly-charged scalar.      

The hyperfine splittings in heavy-light mesons and quarkonia

Hyperfine splittings (HFS) are calculated within the Field Correlator Method, taking into account relativistic corrections. The HFS in bottomonium and the B _q (q = n, s) mesons are shown to be in full agreement with experiment if a universal coupling α _HF = 0.310 is taken in perturbative spinspin potential. It gives M(B*) −M(B) = 45.7(3) MeV, M(B _s ^* ) − M(B _s ) = 46.7(3) MeV (n _f = 4), while in bottomonium Δ_HF(b $ \bar b $ \bar b ) = M(Υ(9460)) − M(η _b (1S)) = 63.4 MeV for n _f = 4 and 71.1 MeV for n _f = 5 are obtained; just the latter agrees with recent BaBar data. For unobserved excited states we predict M(Υ(2S))−M(η _b (2S)) = 36(2)MeV,M(Υ(3S))−M(η _b (3S)) = 28(2)MeV, and also M(B _c ^*) = 6334(4) MeV, M(B _c (2S)) = 6868(4) MeV, M(B _c ^* (2S)) = 6905(4) MeV. The mass splittings between D(2³ S ₁) − D(2¹ S ₀), D _s (2³ S ₁) − D _s (2¹ S ₀) are predicted to be ∼75 MeV, which are significantly smaller than in several other studies but agree with the mass splitting between recently observed D(2533) and D*(2610).