Ionization of a single hydrogen-like atom by laser pulse of near-atomic strength

The dynamics of high-harmonic generation and atom ionization by a strong and superstrong laser field are studied. In contrast to many earlier works, the present theory does not impose limitations on the laser field’s strength. We solve the nonrelativistic problem of a single hydrogen-like atom’s ionization from the ground state by a short laser pulse of subatomic, atomic, and superatomic field strength. Within the framework of the proposed method, we investigated the matrix elements of the ionization transition and revealed its substantially nonlinear dependence on the laser field strength. Both ionization and recombination processes are taken into account. The proposed method enables us to take into account the arbitrary order multiphoton ionization processes.     

Spreading of atomic wave packets and semiclassical chaos

The correspondence between the statistical properties of the evolution of a quantum system and Lyapunov instability and the chaos of its semiclassical analog has been demonstrated. The results of the analyses of atomic motion in a laser field in the semiclassical approximation (dynamics is described by several nonlinear equations) and without this approximation (dynamics is described by an infinite system of linear equations) are compared. In the ranges of the parameters for which the semiclassical dynamics of point-like atoms is unstable, the fast “spreading” of quantized wave packets in the momentum space is observed. Thus, deterministic chaos “imitates” the statistics of the quantum nondeterministic effects, although the semiclassical and quantum solutions are fundamentally different.     

Atom as a “dressed” nucleus

We show that the electrostatic potential of an atomic nucleus “seen” by a fast charged projectile at short distances is quantum mechanically smeared due to nucleus motion around the atomic center of inertia. For example, the size of the “positive charge cloud” in the Hydrogen ground state is much larger than the proper proton size. For target atoms in excited initial states, the effect is even larger. The elastic scattering at large angles is generally weaker than the Rutherford scattering since the effective potential at short distances is softer than the Colombian one due to a natural “cutoff”. In addition, the large-angle scattering leads to target atom excitations due to pushing the nucleus (⇒ inelastic processes). The Rutherford cross section is in fact inclusive rather than elastic. These results are analogous to those from QED. Non-relativistic atomic calculations are presented. The difference and the value of these calculations arise from nonperturbatively (exact) nucleus “dressing” that immediately leads to correct physical results and to significant technical simplifications. In these respects a nucleus bound in an atom is a simple but rather realistic model of a “dressed” charge in the QFT. This idea is briefly demonstrated on a real electron model (electronium) which is free from infinities.      

Helium atom in intense and superintense laser fields: A new theoretical approach

A quantum hydrodynamical study is made of the dynamical changes of a helium atom interacting with lasers of two different intensities, but having the same frequency. Under the intense laser field, electron density oozes out of the helium atom by absorbing laser photons and getting promoted to higher excited states including the continuum. Under the superintense field, electron density partly moves away from the helium nucleus but remains in the “quasi-bound” dressed states along with the laser field, thus suppressing ionization.     

Response of an atom interacting with an arbitrarily polarized electromagnetic field

We develop the theory of interaction of the electromagnetic field and a single atom being in an arbitrary state and having an arbitrary direction of the angular momentum of the atomic electron with respect to the direction of the field polarization vector. It is shown that the atom response current has a tensor structure and depends on both the direction of the angular momentum of the atom, and the polarization vector of the external field. The tensor character of the response is determined by the externally induced anisotropic distribution of the probability density of spatial localization of the atomic electron. It is shown that the induced-anisotropy effects clarify the harmonic generation mechanism at play during the non-resonance interaction of laser radiation with atomic media. The developed theory is applied to the analysis of the problem about the generation of terahertz waves in a two-color laser field. It is shown that the change in the mutual orientation of wave polarization vectors leads to a significant increase in the efficiency of conversion of high-frequency fields to low-frequency ones. It is shown for the first time that the generation of terahertz waves is possible in the preionization regime, when the generation mechanism is related to atomic nonlinearity.     

Discrete photodetection of quantum jumps on the V configuration of atomic levels

A theory of the discrete photodetection of quantum jumps on the V configuration of atomic levels has been developed. A three-level source atom is placed in a cavity excited by a resonance fluorescence field. The cavity is tuned to exact resonance with an atomic transition. The cavity mode state is tested by a flux of unexcited (at the entrance) probe atoms passing through the cavity. The energy states of the outgoing probe atoms are detected by ionization chambers, which are assumed ideal. This a posteriori statistical information is indirectly related to the numerical characteristics of a measured quantum system consisting of the source atom and cavity mode. The “tuning” conditions for a discrete photodetector, i.e., the rules for choosing the parameters and durations of the interactions of the cavity mode with the probe and source atoms, intensities of the pump and probe fields that are necessary for observing quantum jumps from the “bright” state to the “dark” one and vice versa, have been determined. A two-state model that describes the dynamics of a quantum jump has been analyzed. The formulas have been obtained for the observable characteristics of quantum jumps: the mean residence time of the quantum system in quasistationary states (durations of the bright and dark periods), probabilities of quantum jumps, mean excitation levels of the quantized cavity mode, etc.     

Ionization of a hydrogen atom from its ground state by a coherent bichromatic laser field

We study the “coherent phase control” between the three-photon ionization by a fundamental laser field and the one-photon ionization by its third harmonic for a hydrogen atom in its ground state. The relative phase δ of the harmonic field with respect to the fundamental laser radiation “modulates” the interference between the two ionization channels, which is important near the crossing points between the ionization rates of the two individual processes. Numerical results for the total ionization rate and for the angular distribution of the photoelectrons as a function of the phase δ are presented for frequencies located in the vicinity of the atomic resonances corresponding to the absorption of two laser photons. Received 31 August 2000 and Received in final form 6 February 2001     

Kinetics and Optical Properties of the Strongly Driven Gas Medium of Interacting Atoms

This paper investigates stimulated emission and absorption near resonance for a driven system of interacting two-level atoms. Microscopic kinetic equations for the density matrix elements of N-atom states including atomic motion are built, taking into account atom-field and atom-atom interactions. Analytical solutions are given for the resulting macroscopic equations in different limits, for a system composed of a strong coherent “pump” field and a weak counter-propagating “probe” field. It was shown that the existence of a dipole-dipole (long-range) interaction between atoms separated by distance less than the pump wave-length can cause the formation of periodic polarization and population structures (gratings in time and space) in the pumped medium without a probe field. The magnitude of pump induced population grating can have a strong dependence on the relation between the pump field detuning and the polarization decay rate. The “interaction” between pump and probe induced polarization/population gratings through a dipole-dipole interaction mechanism causes the absorption line shape asymmetry. Under certain conditions, this asymmetry is revealed in increasing probe gain for the “red”-shifted (relative to pump) probe and suppressing the gain for the “blue”-shifted probe field when pump is “red”-shifted relative to the ensemble averaged resonant frequency. The theoretical results are consistent with experimental data for the probe gain or absorption as the function of frequency and the dependance of the gain on atomic density for sodium vapor when the pump laser is tuned near the D ₂ line. Here the dependance of gain on particle density was explained in the terms of the long-range interaction between the atoms.     

Hindered decay of an unstable system: A quantum zeno effect

A direct test of the so-called “quantum Zeno effect” is proposed for a truly decaying system. It is suggested that the lifetime of an unstable atom can be extended by illuminating it with an intense laser beam at the frequency of another of its transitions. The “Zeno” time is also compared to the lifetime     

Nonlinear terahertz response of -type GaAs

Excitation of an n-type GaAs layer by intense ultrashort terahertz pulses causes coherent emission at 2 THz. Phase-resolved nonlinear propagation experiments show a picosecond decay of the emitted field, despite the ultrafast carrier-carrier scattering at a sample temperature of 300 K. While the linear THz response is in agreement with the Drude response of free electrons, the nonlinear response is dominated by the super-radiant decay of optically inverted impurity transitions. A quantum mechanical discrete state model using the potential of the disordered impurities accounts for all experimental observations.     

Lateral field instability and six-wave mixing in a diode laser with broad active area

The electromagnetic field inside a nonlinear active medium of a laser is considered as a system of counterpropagating waves. Such an approach changes radically an earlier studied behavior of the lateral field instability due to self-deformaion (or self-focusing). In our calculations we used an expression for a laser field in the form of two “strong” counterpropagating waves whose complex amplitudes have weak perturbations. Amplitude perturbations of each of the “strong” waves can be presented by two spatial harmonics corresponding to two weak perturbation waves with wave vectors making some tilted angle ±φ with the cavity axis. Thus six waves would participate in the interaction: two counterpropagating strong waves and two pairs of weak waves. Using this approach, we have developed a theory for the propagation of four “weak” perturbation waves in a nonlinear amplifying medium in the presence of two counterpropagating “strong” waves. It is shown that perturbation waves with tilted angle φ⋍0.5–1.2° inside the active region, and respecively, with the side lobes of the far-field pattern at ∼1.7–4°, have the greatest growth increment. These perturbation waves produce lateral intensity modulation with period 10–30 μm for the 0.85 μm lasing wavelength. The appearance of such waves corresponds to the instability threshold of a homogeneous lateral distribution of optical power in a diode laser. The present theory makes it possible to investigate the stability of the homogeneous lateral optical intensity distribution in a diode laser of any design. This allows one to choose a suitable design of a laser with a homogeneous lateral distribution at high radiation power. Translated from Preprint No. 43 (1992) of the Lebedev Physics Institute, Russian Academy of Sciences.     

New lasers based on c-cut vanadat crystals

Spectroscopic and lasing properties of c-cut Nd-doped Nd:Gd_0.7Y_0.3VO₄, Nd:YVO₄, and Nd:GdVO₄ crystals were investigated. Spectral tuning from 1062 to 1067 nm was demonstrated. CW, Q-switching and mode-locking regimes for two-color laser operations were realized. A novel THz source based on Q-switch two-color diode-pumped solid state c-cut Nd:GdVO₄ laser with Filter Lio as selective element and the GaSe nonlinear optical crystals as convertor was demonstrated. Terahertz radiation with wavelength 436 mm (0.56 THz) was detected. One picosecond laser pulses in mode-locking diode pumped c-cut vanadat lasers with a Kerr-lens and PbS-doped glasses as saturable absorbers are observed.     

<Emphasis Type="Italic">S</Emphasis>-matrix approach to the problem of high-harmonic generation in the field of intense laser wave

A method using expansion of the wave function in the basis of photonic and free atomic eigenstates is proposed for calculating the emission spectrum of an atom in a laser field. The wave function is constructed using the Kramers?Henneberger transformation so that the expression for the transition S matrix explicitly includes the nonlinear interaction with the laser field. The expansion coefficients are determined by the residual interaction, which depends on the coordinates of the classical free electron motion in the laser field. Resonances at the atomic transition frequencies explicitly arise in the emission spectrum when the residual interaction is considered in the first order. The numerical solution of the timedependent Schro¨ dinger equation for the hydrogen atom within the semiclassical approach is used to obtain emission spectra for laser pulses of different intensities and durations.     

Control for atom response in multicomponent laser fields

A theory of the nonlinear optical response of an atom interacting with a superposition of arbitrarily polarized fields is developed. The theory is based on the analytical solution of the boundary-value problem for an electron moving in a spherically symmetric intraatomic field and in the field of an external electromagnetic field. By means of the example of an argon atom interacting with a bichromatic field formed by the first and second harmonics of a Ti:sapphire laser, it is shown that, when an atom interacts with the field of two polarized pulses the polarization directions of which are not collinear, the response spectrum significantly depends on the laser radiation parameters—the duration and intensity of pulses, the time of delay between them, and the angle between the directions of polarization vectors. Generation of THz radiation is shown to be possible in the ionization-free regime due to intraatomic nonlinearity.     

Crossing of quasilevels in the open Jaynes-Cummings model

The nonlinear dynamics of an open quantum system consisting of a “dressed” atom, i.e., an atom coupled with an external multifrequency electromagnetic field, and a single quantized mode of an electromagnetic field is studied. At different crossing points of the quasilevels of the dressed atom, the average number of photons in the quantized mode may either increase without limit with the passage of time or oscillate within finite limits. In the latter case a decrease of the number of photons is accompanied by regularization of their statistics, which may become sub-Poissonian. Zh. éksp. Teor. Fiz. 114, 474–483 (August 1998)     

Effect of laser focus in two-color synthesized waveform on generation of soft x-ray high harmonics

Synthesis of multi-color laser pulses has been developed as a promising way to improve low conversion efficiency of high-order harmonic generation (HHG). Here we systematically study the effect of laser focus in a two-color waveform on generation of macroscopic HHG in soft x-rays. We find that the dependence of HHG yields on laser focus at low or high gas pressure is sensitive to the characteristics of single-atom harmonic response, in which "short"-or "long"-trajectory emissions can be selectively controlled by changing the waveform of two-color synthesized laser pulse. We uncover the phase-matching mechanism of HHG in the gas medium by examining the propagation of the two-color waveform and the evolution of time-frequency emissions of high-harmonic field. We further reveal that the nonlinear effects, such as geometric phase, atomic dispersion, and plasma defocusing, are responsible for modification of two-color waveform upon propagation. This work can be used to find better macroscopic conditions for generating soft x-ray HHG by employing two-color optimized waveforms.     

Longitudinal Current Induced by a Plane Electromagnetic Wave in a Single Atom

The change in the polarization state of the atomic response due to the appearence of the longitudinal component, which has been predicted in [A. Andreev, S. Stremoukhov, and O. Shoutova, Europhys. Lett. 120, 14003 (2017)], has been studied. The dependence of the vector properties of the atomic current induced in an atom with unit angular momentum in the ground state on the properties of a two-color laser field with orthogonally polarized components has been analyzed. It has been shown that the variation of the delay time between the frequency components of the laser field makes it possible to efficiently control the polarization of the components of the atomic response field. The effect of the mutual orientation of the electric component of the laser field and the angular momentum of the atom on the longitudinal component of the atomic current and on the polarization properties of the generated radiation has been demonstrated.     

Consistent Histories in Quantum Cosmology

We illustrate the crucial role played by decoherence (consistency of quantum histories) in extracting consistent quantum probabilities for alternative histories in quantum cosmology. Specifically, within a Wheeler-DeWitt quantization of a flat Friedmann-Robertson-Walker cosmological model sourced with a free massless scalar field, we calculate the probability that the universe is singular in the sense that it assumes zero volume. Classical solutions of this model are a disjoint set of expanding and contracting singular branches. A naive assessment of the behavior of quantum states which are superpositions of expanding and contracting universes suggests that a “quantum bounce” is possible i.e. that the wave function of the universe may remain peaked on a non-singular classical solution throughout its history. However, a more careful consistent histories analysis shows that for arbitrary states in the physical Hilbert space the probability of this Wheeler-DeWitt quantum universe encountering the big bang/crunch singularity is equal to unity. A quantum Wheeler-DeWitt universe is inevitably singular, and a “quantum bounce” is thus not possible in these models.     

Local Wick Polynomials and Time Ordered Products¶of Quantum Fields in Curved Spacetime

In order to have well defined rules for the perturbative calculation of quantities of interest in an interacting quantum field theory in curved spacetime, it is necessary to construct Wick polynomials and their time ordered products for the noninteracting theory. A construction of these quantities has recently been given by Brunetti, Fredenhagen, and K?hler, and by Brunetti and Fredenhagen, but they did not impose any “locality” or “covariance” condition in their constructions. As a consequence, their construction of time ordered products contained ambiguities involving arbitrary functions of spacetime point rather than arbitrary parameters. In this paper, we construct an “extended Wick polynomial algebra”– large enough to contain the Wick polynomials and their time ordered products – by generalizing a construction of Dütsch and Fredenhagen to curved spacetime. We then define the notion of a local, covariant quantum field, and seek a definition of local Wick polynomials and their time ordered products as local, covariant quantum fields. We introduce a new notion of the scaling behavior of a local, covariant quantum field, and impose scaling requirements on our local Wick polynomials and their time ordered products as well as certain additional requirements – such as commutation relations with the free field and appropriate continuity properties under variations of the spacetime metric. For a given polynomial order in powers of the field, we prove that these conditions uniquely determine the local Wick polynomials and their time ordered products up to a finite number of parameters. (These parameters correspond to the usual renormalization ambiguities occurring in Minkowski spacetime together with additional parameters corresponding to the coupling of the field to curvature.) We also prove existence of local Wick polynomials. However, the issue of existence of local time ordered products is deferred to a future investigation. Received: 27 March 2001 / Accepted: 6 June 2001     

Feynman diagram approach to atomic collisions

A quantum field theoretic formulation of atomic collision phenomena involving non-relativistic free and bound systems is developed and a calculational procedure in terms of Feynman diagrams is prescribed. Matrix elements of several atomic collision processes have been calculated. In most cases standard quantum mechanical results are reproduced. But in some cases new terms appear in the scattering matrix whose contribution though negligibly small in the low energy region, become important at higher energies. A large portion of this work formed material for an invited talk delivered by one of us (T.P.) at the Second National Workshop on Atomic and Molecular Physics at Visva-Bharati, Santiniketan (India) held from 18–23 November 1979.