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A major focus on graphene‐based two‐dimensional (2D) materials is highlighted in recent days owing to their fascinating properties with widespread applications in electronic devices, catalysis, photonics and medicine. Here, we critically evaluate 2D materials based quantum dots (QDs) to understand the significant ways of fabrication adopted to meet their challenging demands in par with other 2D nanostructures to be in parallel with the current photonic technology with emphasis on future research scope to make use of these materials. We also discuss the different applications of 2D QDs emphasizing the realization of fluorescent probes which are in great demand to well‐establish these materials in the healthcare sector for the betterment of mankind. This study is a key priority and will bring a great impact in the advancement of simple yet challenging 2D QDs by bringing them towards the next level of applications point‐of‐view similar to that of graphene.  相似文献   

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吴元军  申超  谭青海  张俊  谭平恒  郑厚植 《物理学报》2018,67(14):147801-147801
以二硫化钼(MoS_2)为代表的过渡金属硫属化物属于二维层状材料,样品可以薄至单层.单层MoS_2是一种直接带隙半导体,在纳米逻辑器件、高速光电探测、纳米激光等领域具有广阔的应用前景.在实际应用中,温度是影响半导体材料能带结构和性质的主要因素之一.因此研究单层二维材料能带的温度依赖特性对理解其物理机理以及开展器件应用具有重要的意义.目前,在广泛采用的测量单层MoS_2反射谱的研究中,激子峰往往叠加在一个很强的光谱背底上,难以准确分辨激子的峰位和线宽.基于自行搭建的显微磁圆二向色谱系统,研究了单层MoS_2在65—300 K温度范围内的反射谱和磁圆二向色谱,结果表明磁圆二向色谱在研究单层材料激子能量和线宽方面具有明显的优势.通过分析变温的磁圆二向色谱,得到了不同温度下的A,B激子的跃迁能量和线宽.通过对激子能量和线宽的温度依赖关系进行拟合,进一步讨论了声子散射对激子线宽的影响.  相似文献   

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Cite this article: Tengdong Zhang(张腾东), Rui Fan(樊睿), Yan Gao(高炎), Yanling Wu(吴艳玲), Xiaodan Xu(徐晓丹), Dao-Xin Yao(姚道新), and Jun Li(李军) Possible coexistence of superconductivity and topological electronic states in 1T-RhSeTe 2025 Chin. Phys. B 34 027403  相似文献   

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Cite this article: Tengdong Zhang(张腾东), Rui Fan(樊睿), Yan Gao(高炎), Yanling Wu(吴艳玲), Xiaodan Xu(徐晓丹), Dao-Xin Yao(姚道新), and Jun Li(李军) Possible coexistence of superconductivity and topological electronic states in 1T-RhSeTe 2025 Chin. Phys. B 34 027403  相似文献   

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Cite this article: Tengdong Zhang(张腾东), Rui Fan(樊睿), Yan Gao(高炎), Yanling Wu(吴艳玲), Xiaodan Xu(徐晓丹), Dao-Xin Yao(姚道新), and Jun Li(李军) Possible coexistence of superconductivity and topological electronic states in 1T-RhSeTe 2025 Chin. Phys. B 34 027403  相似文献   

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Cite this article: Tengdong Zhang(张腾东), Rui Fan(樊睿), Yan Gao(高炎), Yanling Wu(吴艳玲), Xiaodan Xu(徐晓丹), Dao-Xin Yao(姚道新), and Jun Li(李军) Possible coexistence of superconductivity and topological electronic states in 1T-RhSeTe 2025 Chin. Phys. B 34 027403  相似文献   

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         下载免费PDF全文
Cite this article: Tengdong Zhang(张腾东), Rui Fan(樊睿), Yan Gao(高炎), Yanling Wu(吴艳玲), Xiaodan Xu(徐晓丹), Dao-Xin Yao(姚道新), and Jun Li(李军) Possible coexistence of superconductivity and topological electronic states in 1T-RhSeTe 2025 Chin. Phys. B 34 027403  相似文献   

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         下载免费PDF全文
Cite this article: Tengdong Zhang(张腾东), Rui Fan(樊睿), Yan Gao(高炎), Yanling Wu(吴艳玲), Xiaodan Xu(徐晓丹), Dao-Xin Yao(姚道新), and Jun Li(李军) Possible coexistence of superconductivity and topological electronic states in 1T-RhSeTe 2025 Chin. Phys. B 34 027403  相似文献   

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         下载免费PDF全文
Cite this article: Tengdong Zhang(张腾东), Rui Fan(樊睿), Yan Gao(高炎), Yanling Wu(吴艳玲), Xiaodan Xu(徐晓丹), Dao-Xin Yao(姚道新), and Jun Li(李军) Possible coexistence of superconductivity and topological electronic states in 1T-RhSeTe 2025 Chin. Phys. B 34 027403  相似文献   

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Cite this article: Tengdong Zhang(张腾东), Rui Fan(樊睿), Yan Gao(高炎), Yanling Wu(吴艳玲), Xiaodan Xu(徐晓丹), Dao-Xin Yao(姚道新), and Jun Li(李军) Possible coexistence of superconductivity and topological electronic states in 1T-RhSeTe 2025 Chin. Phys. B 34 027403  相似文献   

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王枫秋 《中国物理 B》2017,26(3):34202-034202
As the fundamental optical properties and novel photophysics of graphene and related two-dimensional(2D) crystals are being extensively investigated and revealed, a range of potential applications in optical and optoelectronic devices have been proposed and demonstrated. Of the many possibilities, the use of 2D materials as broadband, cost-effective and versatile ultrafast optical switches(or saturable absorbers) for short-pulsed lasers constitutes a rapidly developing field with not only a good number of publications, but also a promising prospect for commercial exploitation. This review primarily focuses on the recent development of pulsed lasers based on several representative 2D materials. The comparative advantages of these materials are discussed, and challenges to practical exploitation, which represent good future directions of research, are laid out.  相似文献   

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Layered growth of molybdenum disulphide (MoS2) was successfully achieved by pulsed laser deposition (PLD) method on c ‐plane sapphire substrate. Growth of monolayer to a few monolayer MoS2, dependent on the pulsed number of excimer laser in PLD is demonstrated, indicating the promising controllability of layer growth. Among the samples with various pulse number deposition, the frequency difference (A1g–E12g) in Raman analysis of the 70 pulse sample is estimated as 20.11 cm–1, suggesting a monolayer MoS2 was obtained. Two‐dimensional (2D) layer growth of MoS2 is confirmed by the streaky reflection high energy electron diffraction (RHEED) patterns during growth and the cross‐sectional view of transmission electron microscopy (TEM). The in‐plane relationship, (0006) sapphire//(0002)MoS2and sapphire//MoS2 is determined. The results imply that PLD is suitable for layered MoS2 growth. Additionally, the oxide states of Mo 3d core level spectra of PLD grown MoS2, analysed by X‐ray photoelectron spectroscopy (XPS), can be effectively reduced by adopting a post sulfurization process. (© 2015 WILEY‐VCH Verlag GmbH &Co. KGaA, Weinheim)  相似文献   

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We found that non‐magnetic defects in two‐dimensional topological insulators induce bound states of two kinds for each spin orientation: electron‐ and hole‐like states. Depending on the sign of the defect potential these states can be also of two kinds with different distribution of the electron density. The density has a maximum or minimum in the center. A surprising effect caused by the topological order is a singular dependence of the bound‐state energy on the defect potential.

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Monolayer transition‐metal dichalcogenides have inspired worldwide efforts in optoelectronic devices but real applications are hindered with their reduced optical absorption due to their atomically ultrathin signature. In this study, by utilizing their biradical nature such as excellent absorption coefficient, broad bandwidth from the ultraviolet to near‐infrared region, and small triplet–singlet energy gap, a series of helicene 5,14‐diaryldiindeno[2,1‐f:1′,2′‐j]picene (DDP) derivatives ( 1ab , 1ac , and 1bb ) are integrated with monolayer MoS2 for extraordinary photodetector performance and outstanding stability. Via comprehensive time‐resolved studies, the interfacial charge‐transfer process from the DDPs to the MoS2 layer is evidenced by the stabilized exciton property of the organics ( 1ac )/MoS2 heterostructure. Significantly, the 1ac /MoS2 photodetector exhibits an ultrahigh photoresponsivity of 5 × 107 A W−1 and a fast response speed of 45 ms due to the highly efficient photoexcited carrier separation and the matched type‐II energy band alignment. The biradical 1ac /MoS2 hybrid photodetector shows no sign of degradation after one‐month operation. The results pave a new avenue for biradical based high‐performance and super‐broadband optoelectronic devices.  相似文献   

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Strong two‐photon absorption (TPA) in monolayer MoS2 is demonstrated in contrast to saturable absorption (SA) in multilayer MoS2 under the excitation of femtosecond laser pulses in the near‐infrared region. MoS2 in the forms of monolayer single crystal and multilayer triangular islands are grown on either quartz or SiO2/Si by employing the seeding method through chemical vapor deposition. The nonlinear transmission measurements reveal that monolayer MoS2 possesses a nonsaturation TPA coefficient as high as ∼(7.62 ±0.15) ×103 cm/GW, larger than that of conventional semiconductors by a factor of 103. As a result of TPA, two‐photon pumped frequency upconverted luminescence is observed directly in the monolayer MoS2. For the multilayer MoS2, the SA response is demonstrated with the ratio of the excited‐state absorption cross section to ground‐state cross section of ∼0.18. In addition, the laser damage threshold of the monolayer MoS2 is ∼97 GW/cm2, larger than that of the multilayer MoS2 of ∼78 GW/cm2.

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