Processing of metals by double pulses with short laser pulses

Experimental results related to the influence of time delayed pulses for ablation efficiency with short multi pulses (pulse duration of 5 ps) are reported. A significant improvement of the micro structuring quality at relatively high fluence regime in metals is obtained. Less removed or recast matter is observed and the processed surface appears to be smoother with better roughness. Ablation depths and burr heights are compared for single pulses and double pulses in steel, Al and Cu as a function of scans number. Best results are obtained for weak time delays, typically less than 1 ps. PACS 79.20.Ds; 42.62.Cf; 81.65.Cf     

Theory of the interaction of high-power short laser pulses with plasmas

A theory of the interaction of short laser pulses with plasmas is constructed based on the previously developed kinetic theory of a tenuous plasma. The generation of fast electrons by a relativistically strong femtosecond laser pulse in a plasma with a nearly critical density is investigated. The results obtained agree with the results from particle-in-cell simulations and with the experimental data.     

Molecular alignment by trains of short laser pulses

We show that a dramatic field-free molecular alignment can be achieved after exciting molecules with proper trains of strong ultrashort laser pulses. Optimal two- and three-pulse excitation schemes are defined, providing an efficient and robust molecular alignment. This opens new prospects for various applications requiring macroscopic ensembles of highly aligned molecules.     

Photonuclear reactions induced by intense short laser pulses

A measurement of the decay in time of nuclei excited by an intense short laser pulse of energy E₀$E_0$ yields the Fourier transform of the autocorrelation function of the associated scattering matrix. We determine the optimal length (in time) of the pulse and evaluate the time-decay function using random-matrix theory. That function is shown to contain information not otherwise available. We approximate that function in a manner that is useful for the analysis of data. For E₀$E_0$ below the threshold energy En$E_n$ of the first neutron channel, the time-decay function is exponential in time t while it is the product of an exponential and a power in t   for E₀>En$E_0>E_n$. The comparison of the measured decay functions in both energy domains yields an unambiguous and novel test of random-matrix theory in nuclei.     

Nuclear quantum optics with x-ray laser pulses

The direct interaction of nuclei with superintense laser fields is studied. We show that present and upcoming high-frequency laser facilities, especially together with a moderate acceleration of the target nuclei to match photon and transition frequency, do allow for resonant laser-nucleus interaction. These direct interactions may be utilized for the model-independent optical measurement of nuclear properties such as the transition frequency and the dipole moment, thus opening the field of nuclear quantum optics. As an ultimate goal, one may hope that direct laser-nucleus interactions could become a versatile tool to enhance preparation, control, and detection in nuclear physics.     

Floquet theory for short laser pulses

We develop adiabatic perturbation theory for quantum systems responding to short laser pulses, with or without a frequency chirp. Our approach rests on lifting the time-dependent Schr?dinger equation to an extended Hilbert space, then applying standard perturbational techniques to Floquet states in this extended space, and finally projecting back to the physical Hilbert space. The same strategy also allows us to construct superadiabatic bases for monitoring the quantum evolution in the course of a pulse. These bases provide a diagnostic tool for improving the efficiency of pulse-induced population transfer. The formalism is applied to the selective excitation of molecular vibrational states by chirped laser pulses, which exploit either successive single-photon resonances or a multiphoton resonance, and by a STIRAP-like process. Received: 23 June 1998 / Revised: 18 August 1998 / Accepted: 25 August 1998     

Ionization of clusters in strong x-ray laser pulses

The effect of intense x-ray laser interaction on argon clusters is studied theoretically with a mixed quantum/classical approach. In comparison to a single atom we find that ionization of the cluster is suppressed, which is in striking contrast to the observed behavior of rare-gas clusters in intense optical laser pulses. We have identified two effects responsible for this phenomenon: A high space charge of the cluster in combination with a small quiver amplitude and delocalization of electrons in the cluster. We elucidate their impact for different field strengths and cluster sizes.     

Ultrafast structural dynamics using time-resolved x-ray diffraction driven by relativistic laser pulses

Based on a femtosecond laser plasma-induced hard x-ray source with a high laser pulse energy( 100 mJ) at 10 Hz repetition rate,we present a time-resolved x-ray diffraction system on an ultrafast time scale.The laser intensity is at relativistic regime(2 × 10~(19) W/cm~2),which is essential for effectively generating K_α source in high-Z metal material.The produced copper K_α radiation yield reaches to 2.5 × 10~8 photons/sr/shot.The multilayer mirrors are optimized for monochromatizating and two-dimensional beam shaping of K_α emission.Our experiment exhibits its ability of monitoring the transient structural changes in a thin film SrCoO_(2.5) crystal.It is demonstrated that this facility is a powerful tool to perform dynamic studies on samples and adaptable to the specific needs for different particular applications with high flexibility.     

Fully coherent x-ray pulses from a regenerative-amplifier free-electron laser

We propose and analyze a regenerative-amplifier free-electron laser (FEL) to produce fully coherent, hard x-ray pulses. The method makes use of narrow-bandwidth Bragg crystals to form an x-ray feedback loop around a relatively short undulator. Self-amplified spontaneous emission (SASE) from the leading electron bunch in a bunch train is spectrally filtered by the Bragg reflectors and is brought back to the beginning of the undulator to interact repeatedly with subsequent bunches in the bunch train. The FEL interaction with these short bunches regeneratively amplifies the radiation intensity and broadens its spectrum, allowing for effective transmission of the x rays outside the crystal bandwidth. The spectral brightness of these x-ray pulses is about 2 to 3 orders of magnitude higher than that from a single-pass SASE FEL.     

Excitation of multiple wakefields by short laser pulses in quantum plasmas

We present a theoretical investigation of the excitation of multiple electrostatic wakefields by the ponderomotive force of a short electromagnetic pulse propagating through a dense plasma. It is found that the inclusion of the quantum statistical pressure and quantum electron tunneling effects can qualitatively change the classical behavior of the wakefield. In addition to the well-known plasma oscillation wakefield, with a wavelength of the order of the electron skin depth (λe=c/ωpe, which in a dense plasma is of the order of several nanometers, where c is the speed of light in vacuum and ωpe is the electron plasma frequency), wakefields in dense plasmas with a shorter wavelength (in comparison with λe) are also excited. The wakefields can trap electrons and accelerate them to extremely high energies over nanoscales.     

Investigation of ultrafast nuclear spin polarization induced by short laser pulses

We theoretically investigate the dynamics of nuclear spin induced by short laser pulses and show that ultrafast nuclear spin polarization can take place. Combined use of the hyperfine interaction together with the static electric field is the key for that. Specifically we apply the idea to unstable isotopes, (27)Mg and (37)Ca, with nuclear spin of 1/2 and 3/2, respectively, and show that 88% and 62% of nuclear spin polarization can be achieved within a few to tens of ns, which is 2-3 orders of magnitude shorter than the time needed for any known optical methods. Because of its ultrafast nature, our scheme would be very effective not only for stable nuclei but also unstable nuclei with a lifetime as short as mus.     

Spectroscopic investigation of sparks produced by short laser pulses in He

The spatial and temporal development of the temperature and the electron density of a spark produced in He at 10 atm in the focus of a lens by a mode-locked laser pulse having only 1.5 mJ energy have been investigated. Measuring the absolute intensity of the continuum radiation emitted by the spark and the broadening of a Heii-line it can be concluded that local thermodynamic equilibrium has established 15 ns after the initiation of the plasma. At this time a temperature of 65000 K and a maximum electron density of 1.4·10¹⁹ cm⁻³ was found with a pressure of 20 times the initial gas pressure. These values are in agreement with the values required for an expansion model given in an earlier work basing on a radiation mechanism which explains the stepwise growth of a laser spark under the influence of a train of mode-locked pulses.     

Amplification of short laser pulses by Raman backscattering in capillary plasmas

Short laser pulses can be significantly amplified in the process of Raman backscattering in plasma inside an oversized dielectric capillary. A dielectric capillary allows obtaining high intensities of the output radiation by sustaining efficient amplification at large distances compared to the diffraction length. The efficiency of the interaction between the pump wave and the amplified pulse is shown not to be critically sensitive to the transverse structure of the wave fields. For a quasi-single-mode initial seed pulse and a low pump intensity, the amplified pulse tends to preserve its transverse structure due to nonlinear competition of the capillary eigen-modes. At a high power of the pump wave, multimode amplification always takes place but the growth of the front peak of the pulse still follows the one-dimensional model. The Raman backscattering instability of the pump wave resulting in the noise amplification can be suppressed in detuned interaction by chirping the pump wave or arranging an inhomogeneous plasma density profile along the trace of amplification. The efficiency of the desired pulse amplification does not significantly depend on detuning in the case of a smooth detuning profile. Density inhomogeneities are shown to exert less influence on the amplification within a capillary than in the one-dimensional problem. Parameters of a future experiment on the Raman amplification of a short laser pulse inside a capillary are proposed.     

Interaction of short laser pulses with biological structures

Focusing of light pulses emitted by a Q-switched laser, which have a duration of some nanoseconds, into a medium leads to laser-induced breakdown. The shockwaves produced by this propagate through the medium and can interact with inhomogeneities situated within the medium and consequently cause destruction. Because of the increasing interest in these short light pulses in the medical field the interaction of the shockwaves with biological tissue has been investigated. The observed results indicate the influence of two physical quantities of the shockwave: the peak pressure and the duration.     

High-average-power 2-kHz laser for generation of ultrashort x-ray pulses

We describe a Ti:sapphire-based laser-x-ray system specifically designed for generation of ultrafast x-ray pulses in the tenths-of-nanometers spectral range at a 2-kHz repetition rate. To obtain high-contrast laser pulses we divide the laser system into a section for generation of microjoule, high-contrast pulses with pulse cleaning and a subsequent section for chirped-pulse amplification and pulse compression. This laser section operates in conjunction with an x-ray-generation section based on a moving copper wire in a He atmosphere. The high reliability of the entire system permits maintenance-free production of x-ray pulses over tens of hours. Average x-ray fluxes of 10(13) photons/(s 4pi sr 1 keV) at 3 keV and 10(9) photons/(s 4pi sr) above 5 keV of photon energy are produced.     

Ultrafast x-ray pulses emitted from a liquid mercury laser target

We report the generation of ultrashort, hard-x-ray pulses from a liquid mercury target irradiated by 5 kHz laser pulses. The new x-ray source is designed for time-resolved x-ray absorption spectroscopy as well as imaging applications. This marks the first laser-driven plasma x-ray source that continuously recycles the target material, facilitating maintenance-free operation. Theoretical calculations show mercury targets emit shorter x-ray pulses than targets of lighter elements under identical illumination and x-ray detection conditions.     

Nanostructuring of thin Au films by means of short UV laser pulses

The particle size distribution, morphology and optical properties of the Au nanoparticle (NP) structures for surface enhanced Raman signal (SERS) application are investigated in dependence on their preparation conditions. The structures are produced from relatively thin Au films (10–20 nm) sputtered on fused silica glass substrate and irradiated with several pulses (6 ns) of laser radiation at 266 nm and at fluencies in the range of 160–412 mJ/cm². The SEM inspection reveals nearly homogeneously distributed, spherical gold particles. Their initial size distribution of the range of 20–60 nm broadens towards larger particle diameters with prolonged irradiation. This is accompanied by an increase in the uncovered surface of the glass substrate and no particle removal is observed. In the absorption profiles of the nanostructures, the broad peak centred at 546 nm is ascribed to resonant absorption of surface plasmons (SPR). The peak position, halfwidth and intensity depend on the shape, size and size distribution of the nanostructured particles in agreement with literature. From peak intensities of the Raman spectra recorded for Rhodamine 6G in the range of 300–1800 cm⁻¹, the relative signal enhancement by factor between 20 and 603 for individual peaks is estimated. The results confirm that the obtained structures can be applied for SERS measurements and sensing.     

Femtosecond X-ray line emission from multilayer targets irradiated by short laser pulses

The invention of high-power, ultra-short-pulse lasers has opened the way to investigations aimed at the creation of a new type of bright X-ray source for various uses including material science applications and time-resolved X-ray diffraction for biology. The efficiency with which laser energy incident on a solid target is converted into an X-ray emission depends on many factors, including the temporal profile of the laser pulse. Here we report the results of our theoretical and experimental investigations of the line X-ray emission from layered solid targets irradiated by ultra-short laser pulses. The laser prepulse parameters and target thickness are optimized to convert the maximum laser energy into an emission in the selected X-ray line. Multilayer foils are proposed to increase the energy of the K-line emission from laser plasma while simultaneously keeping the X-ray pulse duration at a hundred femtoseconds. The emission is studied both experimentally and theoretically by means of an analytical model and numerical simulations. PACS 52.38.Ph; 52.38.Dx; 52.50.Jm