Spin-charge fluctuations in itinerant helical magnets

Using a generalized random phase approach quantum fluctuations beyond the helical mean-field states of the Hubbard model off half filling are discussed. The collective mode spectrum is shown to exhibit spin-charge mixing and is found to be strongly renormalized by coupling to low-energy incoherent particle-hole excitations. Results for the collective mode dispersion which displays a significant anisotropy are presented for selected helical phases. Moreover phase space regions of ‘missing’ modes are identified with a finite wave length instability of the helical states suggesting novel inhomogeneous phases of the doped Hubbard model. P.A.C.S. : 71.27.+a, 75.30.Fv, 75.40.Gb     

Elementary spin excitations in ultrathin itinerant magnets

Elementary spin excitations (magnons) play a fundamental role in condensed matter physics, since many phenomena e.g. magnetic ordering, electrical (as well as heat) transport properties, ultrafast magnetization processes, and most importantly electron/spin dynamics can only be understood when these quasi-particles are taken into consideration. In addition to their fundamental importance, magnons may also be used for information processing in modern spintronics.     

On structural instabilities in itinerant magnets and superconductors

The influence of a structural distortion on the itinerant antiferromagnetic (IAF) phase and on the superconducting (S) phase is investigated using a free electron band structure for the electron and hole pockets. For equal concentrations of electrons and holes a metastable phase is found in which the lattice distortion coexists with the IAF or S phase. For unequal concentrations of electrons and holes the critical temperature and the value of the order parameter for the IAF or S phase (in the coexistence region) will always be enhanced by the onset of the structural distortion. The theoretical predictions are compared in the IAF case with the occurrence of a spin flip transition in chromium accompanied by a tetragonal distortion, and in the S case with experimental results on A-15 compounds exhibiting a martensitic phase transition.     

Frustration-induced insulating chiral spin state in itinerant triangular-lattice magnets

We study the double-exchange model at half-filling with competing superexchange interactions on a triangular lattice, combining exact diagonalization and Monte?Carlo methods. We find that in between the expected itinerant ferromagnetic and 120° Yafet-Kittel phases a robust scalar-chiral, insulating spin state emerges. At finite temperatures the ferromagnet-scalar-chiral quantum critical point is characterized by anomalous bad-metal behavior in charge transport as observed in frustrated itinerant magnets R2Mo2O7.     

On the dynamics of itinerant electron magnets in the paramagnetic state

It is shown how disordered local-moment states, in a metal such as Fe, may be stabilized by constraining magnetic fields. Effective interaction parameters between moments are defined in terms of spin density functional theory. On removing the constraints the moments initially precess but then decay rapidly, the latter process leading to an energy width of S(q, ω) at large q of order $\text{(k}{}_{\mathrm{B}}\text{T}{}_{\mathrm{C}}\text{W)}{}^{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}$, where T_C is the Curie temperature and W is the width of the d-band. T he consequences for neutron scattering experiments are discussed and the rather different case of Ni is considered.     

Exchange interactions,spin waves,and transition temperatures in itinerant magnets

This contribution reviews an ab initio two-step procedure to determine exchange interactions, spin-wave spectra, and thermodynamic properties of itinerant magnets. In the first step, the self-consistent electronic structure of a system is calculated for a collinear spin structure at zero temperature. In the second step, parameters of an effective classical Heisenberg Hamiltonian are determined using the magnetic force theorem and the one-electron Green functions. The Heisenberg Hamiltonian and methods of statistical physics are employed in subsequent evaluation of magnon dispersion laws, spin-wave stiffness constants, and Curie/Néel temperatures. The applicability of the developed scheme is illustrated by selected properties of various systems such as transition and rare-earth metals, disordered alloys including diluted magnetic semiconductors, ultrathin films, and surfaces. A comparison to other ab initio approaches is presented as well.     

Non-linear spin fluctuations and phase transitions in itinerant electron magnets: CMR manganites

We present a review analyzing the effects of coupling of transverse magnons with longitudinal spin fluctuations in isotropic itinerant ferro- and antiferromagnets. It is shown that this coupling essentially changes the spectrum of longitudinal fluctuations. At low-temperatures their spectrum is dominated by the linear Landau relaxation, is purely quasielastic and described by a broad central peak of a paramagnon type. On approaching the critical temperature non-linear magnetic relaxation due to mode–mode couplings can dominate and lead to a rapid increase of the central peak and to a new mechanism of magnetic phase transitions governed by non-linear spin fluctuations. The formalism is applied to the CMR manganites where the observed quasielastic fluctuations can be viewed as non-linear spin-lattice fluctuations strongly affected by magnons.     

Switching of vortex polarization in 2D easy-plane magnets by magnetic fields

We investigate the dynamics of out-of-plane (OP) vortices, in a 2-dimensional (2D) classical Heisenberg magnet with a weak anisotropy in the coupling of z-components of spins (easy plane anisotropy), on square lattices, under the influence of a rotating in-plane (IP) magnetic field. Switching of the z-component of magnetization of the vortex is studied in computer simulations as a function of the magnetic field's amplitude and frequency. The effects of the size and the anisotropy of the system on the switching process are shown. An approximate dynamical equivalence of the system, in the bulk limit, to another system with both IP and OP static fields in the rotating reference frame is demonstrated, and qualitatively the same switching and critical behavior is obtained in computer simulations for both systems. We briefly discuss the interplay between finite size effects (image vortices) and the applied field in the dynamics of OP vortices. In the framework of a discrete reduced model of the vortex core we propose a mechanism for switching the vortex polarization, which can account qualitatively for all our results. A coupling between the IP movement (trajectories) of the vortex center and the OP core structure oscillations, due to the discreteness of the underlying lattice, is shown. A connection between this coupling and our reduced model is made clear, through an analogy with a generalized Thiele equation. Received 6 June 2002 / Received in final form 4 November 2002 Published online 6 March 2003 RID="a" ID="a"e-mail: juan.zagorodny@uni-bayreuth.de     

Method of analysis of neutron polarization using noncentrosymmetric cubic helicoidal magnets

A new way of analyzing the polarization of thermal and cold neutron beams, based on the dependence of the neutron-scattering cross section on the neutron polarization upon diffraction from a magnetic spiral, is proposed. In this method, the working element of the neutron-polarization analyzer is a single-crystal noncentrosymmetric cubic helicoidal MnSi magnet, the spin spiral in which is formed at T < T _c (T _c = 29 K) in the magnetic-field range H < H _C2 ～ 500 mT. Since the spiral period d in MnSi is 180 Å, thermal and cold neutrons with wavelengths λ ≤ 2d diffract from this structure. It is established that the efficiency of neutron-polarization analysis is as high as 100% with the experimental geometry when the polarization vector P is parallel to the scattering vector Q.     

Magnetic disorder in itinerant systems

We present an averaging procedure to study the behaviour of a magnetically disordered electron system. A model with stochastic localized magnetic fields at the atomic sites is introduced and a CPA-like method, which has regard to the vector character of the stochastic fields, is employed. The resulting new effects for the density of states are demonstrated for two examples.     

ModifiedT-matrix approximation in itinerant ferromagnets

In this paper we investigate the effect of spin wave excitations on the one-particle energy spectrum of an itinerant ferromagnet. A modifiedT-matrix approximation is developed which takes into account also the effect of other collective modes. In the case of a completely polarized system we obtain a new type of quasi-particle at low excitation energy, and a large damping of the usual one-particle excitations.     

Magnetic domain formation in itinerant metamagnets

We examine the effects of long-range dipolar forces on metamagnetic transitions and generalize the theory of Condon domains to the case of an itinerant electron system undergoing a first-order metamagnetic transition. We demonstrate that, within a finite range of the applied field, dipolar interactions induce a spatial modulation of the magnetization in the form of stripes or bubbles. Our findings are consistent with recent observations in the bilayer ruthenate Sr(3)Ru(2)O(7).     

Universal spin-flip transition in itinerant antiferromagnets

We reveal a universal spin-flip (SF) transition as a function of temperature in spin-density-wave (SDW) systems. At low temperatures the antiferromagnetic (AFM) polarization is parallel to the applied field and above a critical temperature the AFM polarization flips perpendicular to the field. This transition occurs in any SDW system and may be considered as a qualitative probe of the itinerant character of AFM in a given material. Our SF transition may provide an explanation to the long-standing puzzle of the SF transition observed in chromium and may be at the origin of the equally puzzling SDW-I to SDW-II transition in Bechgaard salts for which we make experimental predictions.     

Detecting itinerant single microwave photons

Single-photon detectors are fundamental tools of investigation in quantum optics and play a central role in measurement theory and quantum informatics. Photodetectors based on different technologies exist at optical frequencies and much effort is currently being spent on pushing their efficiencies to meet the demands coming from the quantum computing and quantum communication proposals. In the microwave regime, however, a single-photon detector has remained elusive, although several theoretical proposals have been put forth. In this article, we review these recent proposals, especially focusing on non-destructive detectors of propagating microwave photons. These detection schemes using superconducting artificial atoms can reach detection efficiencies of 90% with the existing technologies and are ripe for experimental investigations.     

Local moment stability in itinerant electron magnetism

We derive a generalized Stoner criterion for the stability of local magnetic moments with various orientations for the case of the Alexander-Anderson-Moriya band structure model. The calculation of the variation of the local moment with magnetic order for both strong ferromagnets and weak antiferromagnets allows us to conclude that the more the Stoner criterion is fulfilled in the ground state, the less the local moments are sensitive to disorder.     

Disorder induced ferromagnetism in itinerant electron system

The possibility of the appearance of the ferromagnetism in the case of itinerant electrons in an amorphous system, is discussed by using the Hubbard model within the Hartree-Fock approximation. The corresponding system in its crystalline state is regarded to be paramagnetic.