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1.
We present an experimental study of the nonlinear optical absorption of the eutectic mixture E7 at the nematic?Cisotropic phase transition by the Z-scan technique, under continuous-wave excitation at 532?nm. In the nematic region, the effective nonlinear optical coefficient ??, which vanishes in the isotropic phase, is negative for the extraordinary beam and positive for an ordinary beam. The parameter $S_\textrm{NL}$ , whose definition in terms of the nonlinear absorption coefficient follows the definition of the optical-order parameter in terms of the linear dichroic ratio, behaves like an order parameter with critical exponent 0.22 ±0.05, in good agreement with the tricritical hypothesis for the nematic?Cisotropic transition.  相似文献   

2.
The dependences of the work function of ytterbium nanofilms on their thickness are studied. The films are evaporated at room temperature on the Si(111)7 × 7 surface of silicon samples doped to different levels and having different types of conduction (n and p). It is shown that these dependences exhibit a pronounced nonmonotonic behavior, which does not depend on the type of silicon used. It is established that the amplitude of the nonmonotonic variations in the work function is governed by the surface microroughness of the deposited layers, so that larger amplitudes correspond to smoother films. The variations in the work function of the films due to the deposition of electrically negative Si atoms on their surface are investigated. It is revealed that the sign of the variation depends on the film thickness. This result strange at first glance is associated with the fact that the electron density distribution at the metal-film-vacuum interface depends nonmonotonically on the amount of deposited ytterbium. This nonmonotonic behavior is a manifestation of electron density standing waves (Friedel oscillations) generated in the films by the ytterbium-silicon interface.  相似文献   

3.
《Physics letters. A》1998,244(6):561-564
The results of a computer simulation of the atomic structure of interfaces in YBa2Cu3O7−δ (twin boundary and large-angle symmetrical tilt grain boundary) are presented. These results allow us to determine the lattice displacements and distortions in the vicinity of analyzed interfaces. Basing on the strain level ≈ 0.01 as a phenomenological criterion for the suppression of superconductivity, estimates of the thickness of the nonsuperconducting regions enveloping interfaces are made.  相似文献   

4.
5.
《Surface science》1986,167(1):167-176
We have studied the initial stages of oxidation, the temperature dependence of the surface electronic structure, and the effect of phosphorus on oxidation of the Si(111)-(7 × 7) surface using optical second-harmonic generation. We have also observed a (√3 × √3)R30° LEED pattern due to surface reconstruction induced by < 0.5% P on Si(111).  相似文献   

6.
This paper reports on a study of the adsorption of CO molecules on the surface of ytterbium nanofilms of different thicknesses, which were sublimed on Si(111)7 × 7 at room temperature. Dependences of two types were investigated: the surface concentration of adsorbed molecules vs. CO dose expressed in langmuirs and the work function of films vs. CO dose. It was shown that the behavior of these dependences is mediated by size effects and Friedel oscillations generated by the ytterbium-silicon interface. Both effects exert an influence on the binding of CO molecules to the surface. At low molecule concentrations, this binding is effected through lone electron pairs localized at the carbon ends of the molecules. These electrons form a donor-acceptor bond to the vacant 5d level of the metal, with the level dropping below the Fermi level. At high CO molecule concentrations, the pattern becomes more complex; indeed, the enhanced Coulomb interaction gives rise to a partial transfer of electrons from the 5d level to the vacant 2π* orbital of CO molecules.  相似文献   

7.
The statistical properties of plasma fluctuations are characterized in the boundary region of HT-7 tokamak. A non-Gaussian feature is observed in fluctuations of ion saturation current and floating potential in most of the scrape-off layer regions. The statistical properties of fluctuations have a clear radial dependence, showing a near-Gaussian character in the proximity of the velocity shear layer location and another region where the poloidal velocity has a trend to zero. Fluctuations show a bursty character with pulses asymmetric in time and the time asymmetry reaches the minimum around the shear layer. From the results, we can see an obvious coupling of the pulses and the poloidal flow.  相似文献   

8.
The structures of zigzag-zigzag, armchair-zigzag, zigzag-chiral, armchair-armchair, armchair-chiral, and chiral-chiral pair connections produced by single-walled carbon nanotubes 1.5–5.0 diameter with the use of the combined 5–7 and 4–8 topological defects have been calculated by molecular mechanics methods. It has been established that the use of the combined 5–7 topological defect makes it possible to produce connections between pairs of single-walled carbon nanotubes with any conductivities, chiralities, and diameters, whereas the use of the combined 4–8 topological defect provides a means for forming connections between nanotubes only with the same type of conductivity. The angles between the axes of nanotubes connected by the combined 5–7 and 4–8 topological defects lie in the ranges 145°–180° and 112°–178°, respectively. It has been revealed that there are correlations between structural parameters of the connections and the relative arrangement of the simple topological defects in the combined topological defects.  相似文献   

9.
The initial stages of the formation of iron silicides in the Fe/Si(111)7 × 7 system in the course of solid-phase epitaxy are investigated using high-resolution photoelectron spectroscopy (~100 meV) with synchrotron radiation. The spectra of the Si 2p core and valence-band electrons obtained after deposition of iron coverages of up to 28 monolayers on the surface of the sample and subsequent isochronous annealings at 650°C are measured and analyzed. It is shown that the first to form under Fe deposition is an ultrathin film of the metastable silicide FeSi with a CsCl-type structure, on which a layer of the Fe-Si solid solution with segregated silicon grows. At coverages in excess of 10 monolayers, an iron film grows on the surface of the sample. Annealing of a silicon crystal coated with a Fe layer leads to the sequential formation of two stable silicide phases, namely, the ?-FeSi and β-FeSi2 phases, in the near-surface region of the sample. It is found that the process of solid-phase synthesis of the ?-FeSi phase passes through the stage of transformation of the iron film into the Fe-Si solid solution.  相似文献   

10.
The phase composition, electronic structure, and magnetic properties of ultrathin cobalt films (no thicker than 20 ?) applied on a Si(111)7 × 7 surface at room temperature are studied by high-resolution photoelectron spectroscopy using synchrotron radiation and magnetic linear dichroism. It is shown that, as the cobalt thickness increases, first interface cobalt silicide and then an island (discontinuous) film of silicon-in-cobalt solid solution form on the silicon surface. A metal cobalt film starts growing after the deposition of a ∼7-?-thick Co layer. It is found that the ferromagnetic ordering of the system, which is characterized by surface magnetization, sets in after the deposition of a ∼6-?-Co layer at the stage of Co-Si solid solution formation.  相似文献   

11.
The radiative capture reaction t + α → 7Li + γ is investigated in the framework of the algebraic version of the resonating group method at low energies. The Hasegawa-Nagata nucleon-nucleon potential is used in calculations. The lowest compatible with the Pauli exclusion principle wave functions of a translationally invariant shell model are adopted as the internal wave functions for α and t clusters. The obtained results are in reasonable agreement with the experimental data.  相似文献   

12.
The elastic scattering properties for collisions between two ^7Li atoms are investigated in the cold and ultracold regimes separately. Based on recent theoretical and experimental results, we present the improved hybrid potentials for the singlet X^1 ∑g^+ and triplet a^3 ∑u^+ ground states of the Li2, Our calculated values for the scattering lengths α and the effective ranges re are compared with previous ones, and found them to be in good agreement. The scattering lengths are 34.6α0 for the singlet state and -27.6α0 for the triplet state. Shape resonances occur in the collisions at low energies. We also calculate the total cross sections and the energy positions of shape resonances for both X^1 ∑g^+ and a^3 ∑u^+ states.  相似文献   

13.
The two 3H+4He and 3He+4He fusion reactions at low energies are usually viewed as an approximate external capture process. We study the 4He(3H,γ)rLi and 4He(SHe,γ)7Be reactions in a cluster model, which can take into account two- and three-body electromagnetic currents, using minimal substitution in the explicit momentum dependence of the two- and three-cluster interactions. Our main goal is to explore how the cross section of the low-energy 3H+4He or 3He+4He capture reactions depends on energy. The astrophysical S-factors for these reactions are calculated at very low energies. We construct the conserved realistic Argonne v18 for two nucleons and Urbana IX or Tucson-Melbourne three-cluster interactions, which are considered for calculation. We also calculate the binding energies and the structural properties of a Hq-4He or 3He+4 He systems. The binding energies are found to be -37.72 (-36.32) MeV and -39.35 (-37.43) MeV, with (without) three-body interactions for 7Be and 7 Li, in satisfactory agreement with other theoretical results and experimental data, respectively.  相似文献   

14.
We have studied the superconducting transitions of Y1Ba2Cu3D x O7–x samples where O has been replaced by D=F, S, or Cl andx=0.2-2. No single phase compounds were obtained forx>0.2. No dramatic increase inT c was registered. Generally the results can be interpreted as a dilution of the highT c 1 2 3 phase by other phases as the dopant concentration increases, ultimately suppressingT c completely. Possibly there is an increase ofT c for an intermediate dopant range,x, in the Cl series.  相似文献   

15.
The desorption kinetics of the chain oxygen atoms in the YBa2Cu3O7– (YBCO) superconductor were studied using isothermal vacuum annealing (VA). The number of the O(1) atoms per unit cell in the crystal was measured at three temperatures of 390, 415, and 450°C for various annealing times. From these measurements it was found that at high temperatures the loss of the O(1) atoms from the YBCO is very rapid, and so, low annealing temperatures must be used in order to see the fine details of the desorption phenomena. When the log of the instantaneous O(1) occupancy vs. time was plotted, three distinct linear segments were obtained for each temperature. This, I think is an indication of the existence of multiple desorption processes. From the slopes of these lines, I have evaluated three free energies of activation to be 1.14(6), 1.45(3), and 1.91(13) eV. These results are explained in terms of oxygen ordering in the chains.  相似文献   

16.
We extend a previous theoretical study, in which we have predicted that a solid–solid phase transition can be induced by a laser in arsenic under pressure, to higher fluences. In particular, we compute the fluence that is needed to induce an ultrafast structural transition from the A7 to the simple cubic phase as a function of the applied pressure. We further discuss the possibility of ultrafast, laser-induced melting.  相似文献   

17.
18.
Optical second harmonic generation spectra have been experimentally obtained from a clean Si(111) 7 × 7 in two different polarization configurations isolating the rotational anisotropic and isotropic contributions. The energy of the fundamental photon is varied from 0.8 eV to 2.5 eV. For comparison, we also use a microscopic formulation based on the semi-empirical tight binding method to evaluate the nonlinear surface susceptibility tensor χ(2ω). Good agreement between theory and experiment is obtained with respect to the number of resonances, their position in energy, and surface or bulk character.  相似文献   

19.
Measurements of boundary fluctuations and fluctuation driven electron fluxes have been performed in ohmic and lower hybrid current drive enhanced confinement plasma using a graphite Langmuir probe array on HT-7 tokamak. The fluctuations are significantly suppressed and the turbulent fluxes are remarkably depressed in the enhanced plasma. We characterized the statistical properties of fluctuations and the particle flux and found a non-Gaussian character in the whole scrape-off layer with minimum deviations from Gaussian in the proximity of the velocity shear layer in ohmic plasma. In the enhanced plasma the deviations in the boundary region are all reduces obviously. The fluctuations and induced electron fluxes show sporadic bursts asymmetric in time and the asymmetry is remarkably weakened in the lower hybrid current driving (LHCD) phase. The results suggest a coupling between the statistical behaviour of fluctuations and the turbulent flow.  相似文献   

20.
More than 70% of the total plasma current is sustained by the bootstrap current and current drive during the synergy of lower hybrid current driving (LHCD) and ion Berstein wave (IBW) heating on the HT-7 tokamak.The lower hybrid non-inductive current source is off-axis and well localized, and more than 35% bootstrap current plasma has been obtained. The IBW in controlling electron pressure profile can be integrated into the LHCD target plasma. The largest steep gradient of the electron pressure profile in the region ρ - 0.5-0.7 mostly comes from the electron temperature profile, which may induce the large fraction bootstrap current. The large off-axis bootstrap current can help to create negative magnetic shear, and the good plasma confinement is achieved.  相似文献   

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