Complex dynamics of correlated electrons in molecular double ionization by an ultrashort intense laser pulse

With a semiclassical quasistatic model we achieve insight into the complex dynamics of two correlated electrons under the combined influence of a two-center Coulomb potential and an intense laser field. The model calculation is able to reproduce experimental data of nitrogen molecules for a wide range of laser intensities from the tunneling to the over-the-barrier regime, and predicts a significant alignment effect on the ratio of double over single ion yield. The classical trajectory analysis allows us to unveil subcycle molecular double ionization dynamics.     

超短强激光脉冲激励甲烷团簇的内电离机理

采用三维粒子动力学模拟方法研究了甲烷团簇在超短强激光脉冲激励下的爆炸动力学行为,重点讨论了几种典型的内电离机理对团簇爆炸过程中离子的价态和动能的影响.研究表明,在激光脉冲强度比较小的情况下,团簇中的原子主要是在光场作用下通过隧道电离的方式发生电离.当激光场进一步增强时,势垒压低电离是电离的主要方式.在相同的较高激光强度下,团簇更容易通过势垒压低电离达到高的电离价态.团簇发生电离后,其内部库仑电场的点火电离效应和内部滞留自由电子的碰撞电离效应也将增强团簇的再次电离过程. 关键词： 超短强激光脉冲 甲烷团簇 内电离     

Momentum distributions of ne(n+) ions created by an intense ultrashort laser pulse

Vector momentum distributions of Ne(n+) (n = 1,2,3) ions created by 30 fs, approximately 1 PW/cm(2) laser pulses at 795 nm have been measured using recoil-ion momentum spectroscopy. Distinct maxima along the light polarization axis are observed at 4.0 and 7.5 a.u. for Ne2+ and Ne3+ production, respectively. Hence, mechanisms based on an instantaneous release of two (or more) electrons can be ruled out as a dominant contribution to nonsequential strong-field multiple ionization. The positions of the maxima are in accord with kinematical constraints set by the classical "rescattering model."     

Single and double ionization of the hydrogen molecule in an intense few-cycle laser pulse

In this paper, we present ab initio two-electron model calculations of laser-induced single and double ionization of the hydrogen molecule in a linearly polarized laser field with static nuclei located along the polarization axis. Within the model, the center-of-mass motion of the two electrons is restricted along the polarization axis of the field, while the relative electron motion is unrestricted. The results of numerical simulations allow us to identify and characterize the mechanisms leading to single and double ionization in an intense few-cycle laser pulse. The role of the rescattering mechanism on the ionization processes is analyzed in particular.     

Coulomb expansion of deuterated methane clusters irradiated by an ultrashort intense laser pulse

The simulations of three-dimensional particle dynamics show that when irradiated by an ultrashort intense laser pulse, the deuterated methane cluster expands and the majority of deuterons overrun the more slowly expanding carbon ions, resulting in the creation of two separated subelusters. The enhanced deuteron kinetic energy and a narrow peak around the energy maximum in the deuteron energy distribution make a considerable contribution to the efficiency of nuclear fusion compared with the ease of homonuelear deuterium clusters. With the intense laser irradiation, the nuclear fusion yield increases with the increase of the cluster size, so that deuterated heteronuelear clusters with larger sizes are required to achieve a greater neutron yield.     

近共振区超短强激光脉冲激发的等离子体尾波场

用一维相对论粒子模拟研究了相对论超短强激光脉冲在等离子体中传播时激发的尾波场,初步获得了近共振区尾波场的峰值幅度随激光脉冲宽度变化的特点,发现在近共振区等离子体波激发出现增强。通过准静态近似下尾波激发的一维非线性方程数值求解,并与粒子模拟结果比较,得到了该非线性方程的适用范围：当激光脉冲宽度小于等离子体波波长的4倍时,该方程所得结果与粒子模拟结果一致;而当激光脉冲宽度大于该数值时,该方程不再适用。     

近共振区超短强激光脉冲激发的等离子体尾波场

 用一维相对论粒子模拟研究了相对论超短强激光脉冲在等离子体中传播时激发的尾波场,初步获得了近共振区尾波场的峰值幅度随激光脉冲宽度变化的特点,发现在近共振区等离子体波激发出现增强。通过准静态近似下尾波激发的一维非线性方程数值求解,并与粒子模拟结果比较,得到了该非线性方程的适用范围：当激光脉冲宽度小于等离子体波波长的4倍时,该方程所得结果与粒子模拟结果一致;而当激光脉冲宽度大于该数值时,该方程不再适用。     

On self-focusing of an ultrashort intense relativistic laser pulse in a plasma

The development of the spatiotemporal (filamentation) instability of a laser pulse upon excitation of a plasma wave is studied numerically and analytically. It is shown that first, as in a medium with inertialless cubic nonlinearity, the filamentation of radiation occurs and then filaments are attracted to each other. The following evolution differs weakly from the evolution of a smoothed wave beam in a medium with inertial nonlinear response.     

Interaction of intense ultrashort laser pulse with shell target

Based on numerical PIC modeling and an analytical model, we analyze the interaction of a short high-intensity laser pulse with homo- and heterogeneous (two-layer) shell targets. We show that the shell target is capable of focusing ions in a narrow region. In this case, the ion energy exceeds the ion energy for a flat infinite target of the same thickness. We propose to use the effect of focusing and cumulation of ions to implement the collision of ionic beams that counterpropagate from opposite sides of the sphere and to increase the yield of ion-ion reactions. The constructed model makes it possible to calculate the energy of the ion and the number of ions in the region of focusing.     

Nanospallation induced by an ultrashort laser pulse

A femtosecond laser pulse with power density of 10¹³ to 10¹⁴ W/cm² incident on a metal target causes ablation and ejection of the surface layer. The ejected laser plume has a complicated structure. At the leading front of the plume, there is a spall layer where the material is in a molten state. The spall layer is a remarkable part of the plume in that the liquid-phase density does not decrease with time elapsed. This paper reports theoretical and experimental studies of the formation, structure, and ejection of the laser plume. The results of molecular dynamics simulations and a theoretical survey of plume structure based on these results are presented. It is shown that the plume has no spall layer when the pulse fluence exceeds an evaporation threshold F _ev. As the fluence increases from the ablation threshold F _a to F _ev, the spall-layer thickness for gold decreases from 100 nm to a few lattice constants. Experimental results support theoretical calculations. Microinterferometry combined with a pump-probe technique is used to obtain new quantitative data on spallation dynamics for gold. The ablation threshold is evaluated, the characteristic crater shape and depth are determined, and the evaporation threshold is estimated.     

超短超强激光实验伴生电磁脉冲的模拟研究

靶室腔体谐振产生的电磁辐射是超短超强激光与靶相互作用实验中生成的电磁脉冲(EMP)来源之一。基于有限元分析方法,对靶室腔谐振产生电磁脉冲和电磁脉冲通过窗口向外传播这两个过程进行仿真模拟。前者模拟获得空腔和含结构模型谐振时特征磁场,结果显示内部结构对电磁场强度分布和谐振频率有显著影响;后者模拟结果显示,窗口外侧电场强度比窗口内侧高约40%,而且电磁脉冲传播到靶室外后呈球面波形式扩散并衰减。对电磁脉冲的强度衰减规律进行了分析,得到该衰减曲线的拟合函数。     

Gauge independent theory applied to a model of atomic ionization by an intense laser pulse

An explicitly gauge invariant strong field theory is introduced and tested using a model laser-atom interaction. The theory relies on a power series in the target potential. Transitions amplitudes are obtained by using a corresponding series in the momentum space wave function. We demonstrate that this approach is explicitly gauge invariant to all orders. A well know 1D delta function potential model is used to test the convergence of the series in the evaluation of total ionization probabilities and ionization spectra. Actually, the convergence is verified when both, the perturbation as well as the order of the expansion, are increased.     

Expansion of matter heated by an ultrashort laser pulse

Recent experiments have utilizied high-power subpicosecond laser pulses to effect the ultrafast heating of a condensed material to temperatures far above the critical temperature. Using optical diagnostics it was established that a complicated density profile with sharp gradients, differing substantially from an ordinary rarefaction wave, forms in the expanding heated matter. The present letter is devoted to the analysis of the expansion of matter under the conditions of the experiments reported by D. von der Linde, K. Sokolowski-Tinten, and J. Bialkowski, Appl. Surf. Science 109/110, 1 (1996); K. Sokolowski-Tinten, J. Bialkowski, A. Cavalleri et al., Proc. Soc. Photo-Opt. Instum. Eng. 3343, 46 (1998); and, K. Sokolowski-Tinten, J. Bialkowski, A. Cavalleri et al., Phys. Rev. Lett. 81, 224 (1998). It is shown that if the unloading adiabat passes through the two-phase region, a thin liquid shell filled with low-density two-phase matter forms in the expanding material. The shell moves with a constant velocity. The velocity in the two-phase material is a linear function of the coordinate (flow with uniform deformation), and the density is independent of the coordinate and decreases with time as t ⁻¹. Pis’ma Zh. éksp. Teor. Fiz. 69, No. 4, 284–289 (25 February 1999)     

Single attosecond burst generation during ionization of excited atoms by intense ultrashort laser pulses

We develop an analytical approach to describing the generation of a single attosecond burst during barrier-suppression ionization of a hydrogen atom by an intense laser pulse. We derive analytical expressions that describe the evolution of the electron wave packet in the time interval between the detachment from the atom and the collision with the parent ion for an arbitrary initial atomic state by assuming the atom to be fully ionized in one laser-field half-period. For various s-states, we derive expressions for the profile of the attosecond burst generated when the electron packet collides with the ion and analyze the dependence of its generation efficiency on the principal quantum number n of the initial atomic state. The results obtained are compared with the results of three-dimensional numerical calculations. We show that the attosecond pulse generation efficiency can be several orders of magnitude higher than that in the case of ionization from the ground state when pre-excited atomic states are used.     

Ponderomotive acceleration of electrons by an ultrashort laser pulse

By using the corrected solutions for an ultrashort laser pulse, we study the laser-driven electron violent acceleration in vacuum. Our simulations demonstrate that an ultrashort laser pulse with an intensity a₀≡eE₀/m_eωc=3 can accelerate electrons to an energy more than 0.5 GeV. The scaling laws for the net energy gain in different pulse length and laser radius at focus are also studied. Its acceleration mechanism is found to be ponderomotive acceleration.     

Effect of electron excitation in nonsequential double ionization by intense laser fields

We study the double ionization process of atoms in intense laser fields. The momentum distributions of the correlated electrons are calculated. Contrary to the general expectation, we show an increasing proportion of the electrons ionized via excitation with the increasing laser intensity. These electrons generally have small energy thus they concentratedly distribute on the central region of the momentum diagram. Consequently, the central part of the momentum diagram becomes more notable in higher intensity laser fields. Further study suggests that this phenomenon is general in double ionization.     

Evolution of a super-broadened spectrum in a filament generated by an ultrashort intense laser pulse in fused silica

We report experimental and theoretical investigations of the evolution of super-broadened spectrum generation by intense 50-fs pulses propagating in bulk fused silica. Based on good agreement between the experimental results and numerical simulations, a mechanism of supercontinuum generation (SCG) is proposed. At first, both self-phase modulation (SPM) and stimulated Raman scattering (SRS) contribute substantially but slowly to the broadening before filament formation takes place. After filamentation, a plasma grows rapidly and asymmetric spectral broadening results in a blue-shifted spectrum extending to about 400 nm. A time-resolved experiment of the SCG was also performed using a double-pump technique. The temporal behavior suggests that the vibrational mode excited by the stimulated Raman process by the first pulse contributes to the occurrence of self-focusing. PACS 42.65.Re; 42.25.Bs     

All optical electron injector using an intense ultrashort pulse laser and a solid wire target

Energetic electron bunches were generated by irradiating a solid tungsten wire 13 μm wide with 50 femtosecond pulses at an intensity of ∼3×10¹⁸ W/cm². The electron yield, energy spectrum and angular distribution were measured. These energetic electron bunches are suitable for injection into a laser driven plasma accelerator. An all-optical electron injector based on this approach could simplify timing and alignment in future laser-plasma accelerator experiments. PACS 41.75.Ht; 41.75.Lx; 52.38.Kd; 52.38.Ph     

Photoelectron angular distributions at the ionization of atoms by intense sub-one-cycle laser pulses

The phase sensitivity of the photoelectron angular distributions by intense sub-one-cycle linearly polarized laser pulses has been discussed within the analytic Landau-Dykhne approximation. In both cases of sine and cosine laser pulses most of the electrons are ejected along the polarization axis of the laser field. Nevertheless the electron yield and the electron kinetic energies are much larger for the cosine waveform pulse.