In-beam study of 102Sn

Excited states in ¹⁰²Sn have been identified for the first time, in an in-beam γ-ray spectroscopic experiment. Two γ-ray transitions with energies 1472 and 497 keV following the decay of the seniority 6⁺ isomer with t_1/2 = 1.0(5) μs were unambiguously assigned to ¹⁰²Sn. Due to the very low cross section of about 2 μb for producing ¹⁰²Sn in the reaction ⁵⁰Cr(⁵⁸Ni,1α2n), a highly selective detector setup utilizing NORDBALL ancillary detectors and a recoil catcher device was used. High γ-ray detection efficiency was achieved with two EUROBALL Ge cluster detectors.     

E2 polarization charge in Sn

The nucleus ¹⁰²Sn, which is the lightest Sn isotope with known excited states, was investigated with the ⁵⁰Cr(⁵⁸Ni,α2n) reaction using delayed in-beam γ-ray and conversion-electron spectroscopy. The experimental setup was designed to study the decay of μs-long isomeric states by placing γ-ray and electron detectors behind the focal plane of the Fragment Mass Analyzer at the Argonne National Laboratory. A 44 keV conversion-electron line corresponding to the (6⁺)→(4⁺) transition in ¹⁰²Sn was identified and a half-life of 0.62^+0.43_−0.19 μs was measured for the (6⁺) state. From the available experimental information neutron effective charges from 1.6 to 2.3 e were deduced, based on the comparison with different shell-model calculations.     

The decay of115 mIn

The decay of^115m In has been investigated using accurate counting methods. The emission rate of conversion electrons plusβ ^?-particles was determined with a 4π proportional flow counter. The total andK-shell internal conversion coefficients of the 336 keVγ-ray in¹¹⁵In were measured by the electron X-ray coincidence method using combinations of a Si surface barrier with a NaI(Tl) detector and of a magneticβ-spectrometer with a high energy resolution Si(Li) detector, respectively. The conversion ratioR=K/(L+M+...) was deduced from electron spectra recorded with the magneticβ-spectrometer. The 336 keVγ-ray emission rate of all used sources was determined with a calibrated NaI(Tl)γ-ray spectrometer. A Ge(Li) detector has been used to determine the relative intensity of the 497 keVγ-ray in¹¹⁵Sn. As results have been deduced the 336 keVγ-ray emission per decay (N _γ1/N ₀=(45.9 ± 0.1)%), the total internal conversion coefficient (α=1.073 ± 0.014), theK-shell internal conversion coefficient (α _K=0.843±0.012), the conversion ratioR=3.63±0.07, theβ ^?-transition per decay going to the ground state (N _β1/N ₀=(5.0 ± 0.7)%) and to the first excited level in¹¹⁵Sn¹¹⁵Sn(N _β2/N ₀=(0.047 ± 0.002)%), and the 497 keVγ-ray emission (N _γ2/N _γ1=(0.103 ± 0.004)%). From the obtained internal conversion data it follows that the 336 keVγ-ray transition is ofM4 character with anE5 admixture of less than (3.5±1.5)%. The half-life of the isomeric state¹¹⁵ mIn has been determined with four different methods. The result isT _1/2=(4.486±0.004) h.     

Particle × phonon multiplets in 65 147 Tb82

High-spin states of¹¹⁵Sb were studied by inbeamγ-ray spectroscopy using the⁸⁹Y (²⁹Si, 2pn) fusionevaporation reaction at a beam energy of 108 MeV. The experiments includedγ-γ coincidence and directional correlation of oriented nuclei (DCO) ratio measurements using six BGO Compton suppressed Ge detectors. An intruderΔJ=2 rotational band has been identified for the first time and it is interpreted as the h_11/2 proton coupled to a two particle-two hole (2p ? 2h) deformed state of the¹¹⁴Sn core. A ΔJ=1 rotational band based on the 2p ? 1h, π{g ₇ ^2/2 ?g ₉ ^2/?1 }, configuration has been extended to the 29/2⁺ state at an excitation energy of 5241 keV.     

High-spin states in108Sn

High spin states in¹⁰⁸Sn have been investigated using the⁹²Mo(¹⁹F,p2nγ)¹⁰⁸Sn reaction. In-beam measurements ofγ-γ-coincidences,γ-ray excitation functions andγ-ray angular distributions were performed with Ge(Li)-detectors, one of which had a Nal Compton suppression shield. A level scheme for¹⁰⁸Sn has been constructed up to anI ^π=(14^?) state.     

High-spin states in106Cd

Levels of¹⁰⁶Cd, populated by¹⁰⁴Pd(α, 2nγ)¹⁰⁶Cd have been studied measuring direct and delayedγ-ray spectra,γ-γ coincidences andγ-ray angular distributions. A decay level scheme is proposed including states up to 4659.8 keV. IntenseE2 transition cascades have been observed. The half-life of an isomeric level located at 4659.8 keV has been measured:T _1/2= 62±6ns. Nuclear Reactions ¹⁰⁴Pd(α, 2nγ),E _α=31MeV; measuredE _γ,I _γ,γ-γ coinc, σ(θ)T _1/2.¹⁰⁶Cd deduced levels,J, π, Enriched targets. Ge(Li) detectors.     

Thermal neutron captureγ-ray spectroscopy of59Ni and61Ni

Theγ-radiation emitted after thermal neutron capture in isotopically enriched⁵⁸Ni and⁶⁰Ni was measured at the ILL high flux reactor by means of Ge/NaI detectors operated in Compton suppression and pair spectrometer mode. The neutron binding energies were determined asB _n (⁵⁹Ni)=8999.15(23) keV and B_n(⁶¹Ni)=7820.07(20) keV; some 95% of the totalγ-ray fluxes through^59,61Ni were assigned. Theγ-ray strength functions of the primary transitions and the level densities are discussed.     

High spin level structure in127Ba produced by the118Sn(12C, 3n) reaction

High-spin states in¹²⁷Ba have been produced by the reaction¹²⁸Sn(¹²C,3n)¹²⁷Ba and studied by in-beamγ-ray spectroscopic techniques. The odd-parity states form a level system based upon a 9/2^? state and generated by an odd neutron in theh _11/2 shell coupled to a triaxial core. Theg _7/2 shell is responsible for theΔ I=1, even-parity band.     

High-spin states in107Sn

High-spin states in¹⁰⁷Sn were studied using the reaction⁵⁴Fe(⁵⁶Fe, 2pn)¹⁰⁷Sn. An odd-parity band was identified as based on thevh _11/2 orbit by measuring theγ-ray linear polarization. Also were confirmed the excited states based on thevd _5/2 andvg _7/2 orbits. The halflives of the 17/2⁺ and 11/2^? states were measured to be 0.25(4) ns and 28(11) ps, respectively. The experimental level structure and its interpretation were in good agreement with a shell model calculation.     

Collective excitations in145Ba

High-spin levels in¹²⁵Ba have been produced in the¹¹⁶Sn(¹² C, 3n) reaction and studied by in-beam spectroscopic methods. Two strongly populated band structures are observed. The odd-parity one is based on a 7/2^? state and can be explained as the result of the coupling between anh _11/2 neutron-hole and a prolate type triaxial core. The even-parity band, built on a 7/2⁺ state, corresponds to collective excitations associated with a neutron-hole in theg _7/2 shell. Comparisons with heavier odd-A Ba isotopes and discussions are made in the frame work of the triaxial core model. Nuclear Reactions¹¹⁶Sn(¹²C, 3nγ), E=45–55 MeV; measuredσ(E;E _γ,θ),γγ-coinc,γ-γ delay. Enriched target, Ge(Li) detectors.¹²⁵Ba deduced levels,J,π,γ-mixing.     

Band structure on the low-j orbitals in the nucleus125Xe

In¹²⁵Xe eight lowlying band structures of positive parity were established via the¹²²Te(α, n) reaction by means of in-beamγ-ray spectroscopy using a setup of 6 compton suppressed germanium detectors. The systematics of the related quasi- ′s′_1/2, ′d′_3/2, and ′g′_7/2 bands with the variation of the fermi level in the triaxially deformed region from¹²⁵Xe to¹²⁹Xe is discussed.     

Transition probabilities and energy levels in heavy odd-mass isotopes of Sn (A=119–125)

The de-excitation of levels in^119–125Sn populated in the decay of In isotopes has been studied using on-line isotope separators. Level half-lives have been measured in^119–123Sn. a near cancellation of the matrix element for B(E2; g_7/2→ d_3/2) is observed to occur in¹²¹Sn and is probably due to pairing effects. Very low lying 9/2^? levels have been observed in^121–125Sn and are suggested in^{127, 129}Sn. These levels have been interpreted as three quasi-particle states based on the unique parity h_11/2 level. A possible mixing of theg _7/2 level with a close lying 7/2⁺ three quasi-particle state in¹²³Sn is discussed. Radioactivity.^119–125In from²³⁵U(n, f) and²³⁸U(α, f), isotope separated sources; measuredE _γ ,I _γ , E_ce, I_ce,γγ-coin,Βγ-delay, deduced multipolarities.^119–123Sn deduced levels,I, π, B(λ). Ge(Li), Si(Li), NaI(Tl) and plastic detectors, Ge(Li)-Ge(Li) coin, plastic detector — NaI(Tl) delay.     

Tentative level diagram of146Pm below 1.1 MeV

The level scheme of the doubly odd nucleus¹⁴⁶Pm was investigated by means of in-beam spectroscopy. The¹⁴⁶Nd(p, n) reaction in the 3.5–8 MeV proton energy interval on enriched targets has been used to populate the exited states of¹⁴⁶Pm. High resolutionγ-ray spectra using Ge(Li) and hyperpure Ge detectors and conversion electrons with a mini-orange spectrometer were measured. Withγ-exitation functions andnγ-coincidences usingnγ-discriminated NE231 neutron detectors transitions in¹⁴⁶Pm were identified,γγ-coincidences gave information aboutγ-cascades. With these data a level scheme of 38 levels below 1.1 MeV exitation energy has been deduced including 73 transitions. For 12 transitions experimental conversion coefficients have been evaluated, which agree with the expected values forM1/E2-transitions.     

Electromagnetic decay of fragmented analogue states in 45Sc

The ⁴⁴Ca(p, γ) reaction was studied for 45 resonances for E_p = 1.6?2.2 MeV. The overall proton energy resolution was 300–350 eV; the γ-rays were detected with both NaI(T1) and Ge(Li) detectors. Partial and total γ-ray widths were measured for each of the fine structure states of the $\text{3}\text{2}{}^{\mathrm{?}}$ and $\text{1}\text{2}{}^{\mathrm{?}}$ analogue states at E_p = 1.65 and 2.04 MeV, respectively. The data are examined for correlations between the partial widths (Γ_p, Γ_p′, Γ_γi, Γ_γ^total) in different channels. The γ-ray intensities are compared with (τ, d) spectroscopic factors.     

Studies of γ-ray transitions in171Yb

The decay of¹⁷¹ Lu(t_1/2=8.2 day) to the levels of¹⁷¹Yb has been studied using large volume high resolution Ge(Li), x-ray Ge(Li) and NaI(Tl) detectors.γ-γ coincidence and directional correlation experiments have been performed. Spin-parity of 5/2^?, 7/2⁺, 5/2^?, 9/2⁺, 7/2^?, 7/2^?, 11/2⁺, 9/2^?, 9/2^? and 5/2^? have been assigned to the 75.87, 95.26, 122.37, 167.62, 208.00, 230.61, 259.02, 835.21, 948.37 and 1024.87 keV levels respectively. Several new coincidence relations have been observed in the present work. Two newγ-transitions at 141.45 and 821.30 keV observed and two levels at 766 and 944 keV been proposed. Multipolarity assignments have been made for most of theγ-transitions from theK-shell internal conversion coefficients obtained using the presentγ-ray intensities and the published conversion electron intensities. A revised level scheme for¹⁷¹Yb has been proposed and compared with published data. Radioactivity¹⁷¹Lu; measuredT _1/2,E _γ ,I _γ ,γγ coin,γγ (θ), I.C.C.,¹⁷¹Yb deduced levels,J, γ-mixing,π. Enriched targets, Ge(Li) detectors.     

Collective bands in even mass Sn isotopes

Positive parity bands in ^{112, 114, 116, 118}Sn have been excited up to levels with spin and parity J^π = 12⁺ using Cd(α, 2nγ)Sn reactions. The experiments consisted of γ-ray excitation function, γ-γ coincidence, lifetime, γ-ray angular distribution, γ-ray linear polarization and conversion electron measurements. The observed bands show strong resemblances with ground-state bands of transitional nuclei in this mass region. It is pointed out that the J^π = 0⁺ band-heads originate from 2p-2h excitations in the Z = 50 proton shell. The excitation energies of the band-heads are calculated by means of the macroscopic-microscopic renormalization method. Pair correlations between the 2h and 2p configurations are included separately in a phenomenological way by taking into account the pairing energies of the Cd and Te ground states with respect to the Sn ground state.     

Constraints on the universe as a numerical simulation

The level scheme above the proton threshold in ²⁶Si is crucial for evaluating the ²⁵Al(p, γ)²⁶Si stellar reaction, which is important for understanding the astrophysical origin of the long-lived cosmic radioactivity ²⁶Al(T _1/2 = 7.17 × 10⁵ y) in the Galaxy. The excited states in ²⁶Si have been studied using an in-beam γ-ray spectroscopy technique with the ²⁴Mg(³He, nγ)²⁶Si reaction. γ-rays with energies up to 4.6 MeV emitted from excited states in ²⁶Si have been measured using large volume HPGe detectors. The spin-parity of one of the most important states reported recently at 5890.0keV has been assigned as 0⁺ by γ-γ angular correlation measurements in this work.     

Angular momentum transfer in 12C-, 20Ne- and 40Ar-induced fission

Angular momentum transfer in a variety of ¹²C-, ²⁰Ne- and ⁴⁰Ar-induced fission reactions has been investigated using γ-ray multiplicity techniques. Fission fragments were detected in coincidence using a pair of solid-state detectors. The fragment masses were deduced from the kinetic energies and emission angles using two-body kinematics. The γ-ray multiplicities (M_γ) of the fission fragments were measured utilizing an array of eight NaI detectors. For most of the systems studied, M_γ is nearly independent of the exit-channel mass asymmetry. The strongest dependence on mass is observed in the systems ¹⁵⁴sm + 240 MeV ⁴⁰Ar, where a minimum exists at symmetry, and ¹⁹⁷Au + 164 MeV ²⁰Ne, where nuclear structure effects are suggested by the data. For all the reactions the quantity M_γ tends to decrease gradually with increasing fragment kinetic energy. The magnitude of M_γ generally appears to be larger than expected on the basis of rigid rotation, suggesting a spin enhancement effect. The data are compared with a simple model which assumes the statistical excitation of a variety of angular momentum bearing collective modes. Reasonable agreement is obtained with the experimental results. The roles of other collective effects, such as shape fluctuations and angular momentum fractionation, are also considered.     

Search for an isomer in94Rb

Measurements of theβ-ray half-life,γ-ray and X-ray spectra andγ-ray half-lives have been done with a plastic scintillation detector, a high resolution Ge(HP) detector and a 142 cm³ Ge(Li) detector to search for an isomeric state in⁹⁴Rb. Mass-separated activities of⁹⁴Rb were obtained from the He-jet type on-line mass-separator at the Kyoto University reactor. No isomeric transition was found in theγ-ray and X-ray measurements with the upper limits of 3×10^?4 and 8×10^?5, respectively, as compared with the 836.9 keV transition. Half-lives obtained from theγ-ray decay measurements are discussed in the light of classification given byQ _β -value measurements.     

High-energy γ-rays in α-accompanied spontaneous fission of 252 C f

An experiment was performed on prompt γ-ray emission in binary and α-particle accompanied spontaneous fission of ²⁵² C f using the Darmstadt-Heidelberg 4π NaI Crystal Ball spectrometer. The enhancement in γ-ray yield, denoted as the “high-energy component”, which appears between 3.5 and 8 MeV and in the region of near-symmetric fragment mass splits, was observed to be equally pronounced in both fission modes. Analyzing the fragment mass dependence of the mean γ-ray multiplicity in both fission modes clearly identifies the disintegration of equilibrated fission fragments in a narrow mass range around the double-magic ¹³²Sn as the source of these γ-rays.