Multipole mixing ratios of transitions in Te

Gamma-gamma directional correlation measurements were made on nine transitions in ¹²⁴Te with a NaI(Tl)-Ge(Li) detector arrangement and multichannel analysis. The multipole mixing ratios obtained were δ(646) = 0.000±0.001, δ(714) = 1.5_−0.3^+0.6, δ(723) = −3.3±0.2, δ(1437) = 3.7_−2.0^+2.7, δ(1489) = −3.4_−1.5^+0.9, δ(968) = −0.03_−0.05^+0.06, δ(1368) = −0.045±0.090, δ(1045) = 0.041_−0.041^+0.047, δ(1691) = −0.02±0.01, and δ(2091) = 0.00_−0.03^+0.02. The first δ is M3/E2, the next three are E2/M1, and the last five are M2/E1. The retardation (a factor of approximately 50) of the crossover to cascade transitions from the 2039 keV, third 2⁺ level to the second and first 2⁺ levels is essentially the same for both the M1 and E2 components. In addition, spin and parity assignments of 2⁺ were made for the 2039 and 2092 keV levels.     

Multipole mixing ratios of electromagnetic transitions in Gd

Using γ-γ(θ), γ(θ) (nuclear orientation) and e_k-γ(θ) directional correlation techniques, we have determined the multipole character of some transitions connecting the quadrupole and octupole quasi-vibrational bands to the ground state quasi-rotational band in ¹⁵²Gd following the decay of ¹⁵²Tb. For the γ-γ directional correlation measurements a high-energy resolution system employing a Ge(Li) and a NaI(Tl) detector was used while for the e_k-γ correlation we used a NaI(Tl) and magnetic lens spectrometer system. The nuclear orientation measurements were carried out at low temperatures obtained with a ³He-⁴He dilution refrigerator. The results show that the 2⁺ → 2⁺ transition between the β-vibrational and the ground state bands contains ≈ 10% Ml admixture, δ = − 3.05 ± 0.14, and a large E0 contribution while the similar transition from the γ-vibrational band has δ = 4.3 ± 0.7. These results are compared with Kumar's predictions for similar transitions in ¹⁵²Sm. Three other mixing ratios were also determined.     

Multipole mixing ratios of transitions in168Er

Time-integral and time-differentialγ-γ directional correlation measurements were performed for cascades in¹⁶⁸Er populated from the electron-capture decay of¹⁶⁸Tm(87d). The¹⁶⁸Tm source was dissolved in HF acid to minimize extranuclear perturbations. The results of the time-differential experiment for the 448-99.3 keV and 448-198 keV cascades showed agreement with time dependent interaction and gaveλ ₂(1094)=(0.79±0.09) ×10⁷ sec^?1. The attenuation factors for the 80 keV level were determined asG ₂₂ (80)=0.90±0.01 and G₄₄(80)=0.94±0.01. OnlyI=4 spin value for the 1094 keV level is consistent with our measurements. The 632, 731, 741, and 816 keV transitions connecting theK=2⁺ andK = 0⁺ rotational bands were found to be of almost pureE2 character. The 99.3, 198, 547, 720, 830, and 1277 keV transitions are of practically pureE1 multipolarity. The 448 keVMl transition has (0.8 _?0.4 ^+2.0 )%E2 admixture. The results for the 1014?80keV cascade give (23±4)%E3 component in the 1014 keV transition.     

Multipole mixing ratios of γ-transltions in 182W

γ-γ directional correlation experiments were performed on 14 cascades in ¹⁸²W populated from the β^? decay of ¹⁸²Ta(115 d). Two Ge(Li) detectors were used in a coincidence arrangement, and the ¹⁸²Ta sources were dissolved in HF acid to minimize extranuclear perturbations. For the 1189keV, 2^? → 2⁺ transition, the measured directional correlation coefficients are consistent only with multipole mixing ratios $\text{δ}\text{(}\text{M}\text{2}\text{E}\text{1)}\text{= 0.45 ± 0.03}\text{and}\text{δ}\text{(E3}\text{E1)}\text{= ?0.67 ± 0.07}$. These mixing ratios are discussed and compared with the known conversion coefficients for the 1189keV transition. The E2/M1 multipole mixing ratios determined are (energy in keV): δ(66) = 0.15 ± 0.15, δ(85) = 0.31 ± 0.05, δ(114) = 0.31 ± 0.05, 0.56 ≦ δ(179) ≦ 1.36, δ(1121) = 12⁺²_?1, and δ(1231) = ?(32⁺¹⁴²_?15). The measured M2/E1 mixing ratios are: δ(68) = 0.03 ± 0.02, δ(152) = 0.014 ± 0.013 and δ(156) = ?0.13 ± 0.19.     

Energies and mixing ratios of transitions in 72Ge

The lower energy γ-rays of ⁷²Ge from the decay of 14 h ⁷²Ga have been studied using a 2 m curved-crystal spectrometer. Mixing ratios for the 601, 630, 894 and 1051 keV transitions were determined from the γ-γ directional correlations. The E0 content of the 630 keV, 2⁺' → 2⁺ transition was found to be less than 2%. A spin of 3 for the 2065 keV level has been uniquely determined.     

The spin of the 2,198 keV level in74Ge and multipole mixing ratios of gamma transitions in the decay of74As

Directional-correlation measurements of several cascades in the⁷⁴As decay have been made with a NaI — Ge(Li) detectors system. In the⁷⁴Ge the following cascades were measured: 608–596 keV, 994–1,204 keV, 994-(608)-596 keV and 887-596 keV. The corresponding results give a unique spin assignment of 2 for the 2,198 keV level and determine theE2/M 1 mixing ratios ofδ(608)=3.4±0.4 andδ(994)=?(2.8 ± 0.2). In the⁷⁴Se it was measured the 635-635 keV cascade. The result obtained assigned the spin of the 1,270 keV level as 2 and fixed the E2/M1 mixing ratio of δ(635)=?(2.6 ± 0.2). Also aγ-intensity study has been made to determine the branching ratios of the transitions that deexcite the 1,270 keV level in⁷⁴Se. From these data aI(635)/I(1,270)=12.5 ± 5.0 is obtained.     

Energy levels of175Hf

The reaction¹⁷⁵Hf(d, t)¹⁷⁵Hf was studied using 12 MeV deuterons from the Florida State University super FN tandem Van de Graaff accelerator. The outgoing tritons were analyzed by means of a Browne-Buechner type broad range magnetic spectrograph. Twenty-four states in¹⁷⁵Hf have been identified and fifteen states have been given wave function assignments on the basis of the spectroscopy associated with rotational band structure in deformed odd-A nuclei. TheQ-value for the reaction was measured to be ?1925±8 keV.     

175Hf原子核的三轴超形变的探寻

通过采用TRS方法对实验上新发现的¹⁷⁵Hf原子核的两条高自旋转动带进行了研究, 以证明是否具有三轴超形变, 并且为了使结果能够更准确可靠, 选取了最靠近费米面的5个准粒子的组态进行了计算, 但是在这个组态上最后得出的总位能面上并没有发现能表明三轴超形变的明显的第二极小点的存在.     

Levels in159Ho as populated from decay of159Er

The level scheme of the odd proton nucleus¹⁵⁹Ho has been investigated using Ge(Li) and Si(Li) detectors. Results ofγ-ray singles, conversion electron spectra and coincidence experiments are reported. Assignments are made for several energy levels.     

Seven and nine quasi-particleK-isomers in175Hf

NewK-isomers with very high spin (up to 57/2) have been found in¹⁷⁵Hf. This is the highest spin isomer seen in deformed nuclei and involves 9 quasi-particles. The predominant decay to the I=55/2 state in aK ^π=35/2^?, 5 quasi-particle rotational band further demonstrates the surprising breakdown of theK-selection rules, reported previously in neighbouring nuclei.     

166Er levels populated in the166Tm decay

The decay of¹⁶⁶Tm has been investigated with samples obtained by chemical extraction and mass-separation from spallation products of tantalum irradiated with 660 MeV protons. Measurements of gamma rays, - bi-dimensional coincidences, CE- coincidences and internal conversion electrons have been performed. About 300 -transitions have been observed; most of them are placed in a level scheme of¹⁶⁶Er. The properties of some rotational and vibrational bands and of some other levels are discussed.The authors express their thanks to A. V.Zolotavin for his extended discussions on different aspects of the¹⁶⁶Tm decay, N. A.Lebedev, I. I.Gromova for the preparation of the targets and to co-workers of refs. [4, 5, 14, 15 and 16], who participated in this work at different stages.     

Niederenergetische Gammalinien vom Neutroneneinfang in Lu 175 und Lu 176

The low energy gamma-rays from neutron-capture in Lu 175 and Lu 176 have been investigated by means of the bent crystal-spectrometer at the DR-3-reactor at Risø. From the transitions in Lu 177 3 rotational bands have been determined. The levels of the (404)K=7/2⁺ groundstate rotational band are: 121,62 keV (I=9/2), 268,79keV (I=11/2), 440,66 keV (I=13/2), 636,22 keV (I=15/2), 854,34 keV (I=17/2). The level-sequence of the (514)K=9/2^?-band is: 150,39 keV (I=9/2), 288,99 keV (I=11/2), 451,49 keV (I=13/2), 637,05 keV (I=15/2) and 844,88 keV (I=17/2). At 457,92 keV is the basis for the (402)K=5/2⁺-band the higher levels of which are 552,05 keV (I=7/2), 671,89 keV (I=9/2), 816,63 keV (I=11/2), 985,23 keV (I=13/2), 1176,73keV (I=15/2) and probably 1389,5 keV (I=17/2). The energies of the levels apart from the 1389 keV-level have an accuracy of 7×10^?5. The energy differences between the 3 bands agree very well with the values expected from the Bohr-Mottelson-formulaE=A·I(I+1)+B·I ²(I+1)². The calculated branching-ratios within the 3 bands are in fairly good agreement with the experimental values. Theg _K -factors have been determined for 2 bands: It was found that for the (514)-bandg _K =1,16±0,04 and for the (402)-bandg _K =1,33±0,07.     

Levels in189Os populated in the decay of189Re

The excited level scheme of¹⁸⁹Os as populated by the decay of 23.4-h¹⁸⁹Re has been studied by use of Ge(Li) and Si(Li) detectors in the γ-ray singles and coincidence mode. The data confirm the presence of excited levels in¹⁸⁹Os at 30.8 (J ^π=9/2^?), 36.2 (1/2^?), 69.5 (5/2^?), 95.2 (3/2^?), 216.7 (7/2^?), 219.4 (7/2^?), 233.6 (3/2^?), 275.8 (5/2^?), 496.8 (1/2^?, 3/2⁺) and 599.8 (1/2^?, 3/2⁺) keV. The spin and parity assignments are based on multipolarities determined by internal conversion coefficient measurements and decay systematics. A decay scheme is established for¹⁸⁹Re which accommodates 98% of the electromagnetic transition intensity. No evidence for the 150-d¹⁸⁹Re isomer was found in this study.     

Electric quadrupole moments and strong interaction effects in pionic atoms of 165Ho, 175Lu, 176Lu, 179Hf and 181Ta

The effective quadrupole moments Q_eff of the nuclei of ¹⁶⁵Ho, ¹⁷⁵Lu, ¹⁷⁶Lu, ¹⁷⁹Hf and ¹⁸¹Ta were accurately measured by detecting the pionic atom 5g-4f X-rays of the elements. The spectroscopic quadropole moments, Q_spec, were obtained by correcting Q_eff for nuclear finite size effect, distortion of the pion wave function by the pion-nucleus strong interaction, and contribution to the energy level splittings by the strong interaction. The intrinsic quadrupole moments, Q₀, were obtained by projecting Q_spec into the frame of reference fixed on the nucleus. The shift, ε₀, and broadening, Γ₀, of the 4f energy level due to the strong interaction between the pion and the nucleons for all the elements were also measured. Theoretical values of ε₀ and Γ₀ were calculated and compared to the experimental values. The measured values of Q₀ were compared with existing results in muonic and pionic atoms. The measured values of ε₀ and Γ₀ were also compared with existing values.     

Levels in182W populated in the decay of182Ta

Theγ-rays emitted in theβ-decay of¹⁸²Ta have been reinvestigated with improved statistics in attempting to clarify the reported new levels at 1460.41, 1592.98, 1620.36, 1712.29 and 1762.91 keV in¹⁸²W observed in theβ-decay of¹⁸²Ta. The present study demonstrated that the fifteen newγ-rays, which were used to support the existence of the five new levels, are not relevant to theγ-decay of¹⁸²Ta. Therefore the five new levels are not populated in this decay. Additionally, theγ-ray with an energy of 1035.6 keV (0 ₂ ⁺ →2 ₁ ⁺ ) deexciting theβ-band head in¹⁸²W is observed for the first time in the present decay study and the previous tentative placement of the 351.0 keVγ-ray in the level scheme is confirmed by the present coincidence measurements.     

Levels in124Te populated in the decay of124Sb

The levels in¹²⁴Te have been investigated by studying the gamma rays emitted following the decay of 60d¹²⁴Sb. Gamma-gamma coincidence spectra have been taken with gates set at 603, 646, 709, 714 and 723 keV gamma rays by using 105 cm³ Ge(Li)-110 cm³ HPGe coincidence system. 69 gamma rays have been observed and nine of them are reported for the first time. Four new levels in¹²⁴Te at 2512, 2550.2, 2808 and 2814.5 keV are proposed. Levels reported in literatures at 2412 and 2733 keV are excluded from the level scheme of¹²⁴Te based on the present study. The experimentally determined energy spectrum of low-lying positive parity states, B(E2) ratios and electric quadrupole moment of the first excited state are compared with the IBM-1 predictions.     

Levels in160Yb from the radioactive decay of160Lu

Theγ-rays following the radioactive decay of¹⁶⁰Lu into¹⁶⁰Yb have been studied. The Lu source was produced in the¹⁴⁴Sm(¹⁹F, 3n) reaction at 85 MeV. Excitation functions, half-lives,γ-γ andγ-X-ray coincidences and conversion electrons were measured. Twoβ ⁺ decaying states in¹⁶⁰Lu were found with half-lives of 36.2(3) s and 40(1) s.¹⁶⁰Yb levels deduced from the decay of¹⁶⁰Lu are presented.     

Nuclear magnetic resonance of175Hf oriented in iron

Nuclear magnetic resonance of¹⁷⁵Hf oriented at low temperature in iron has been observed with a sample prepared by ion implantation. The centre frequency of the broad resonance line isv _L (B _ext = 0)=138.53(36)MHz. Possible origins of the large inhomogeneous line width of FWHM=11.0(1.1) MHz are discussed. A comparison with model calculations for combined magnetic and electric hyperfine interaction indicates that the centre frequency may be interpreted as the magnetic interaction frequency for¹⁷⁵Hf in unperturbed substitutional sites of the host iron. With theg-factor of¹⁷⁵Hf from literature the magnetic hyperfine field of Hf in Fe is derived asB _hf=?64.9(9.3) T fitting well into systematics.     

Energy levels of Kr populated by Br decay

The γ-rays following the β-decay of ⁸²Br have been investigated using a 220 mm³ Ge(Li) detector, an anti-Compton NaI(Tl) spectrometer and a two-dimensional coincidence arrangement. The ⁸²Br was produced by thermal neutron activation of ammonium bromide. The presence of eight, well-known and 11 weak γ-rays has been established. It has been shown through half-life measurements that the newly identified γ-rays belong to ⁸²Br decay and that the high-energy peaks are not to summing effects. All the reported transitions have been incorporated in a level scheme of ⁸²Kr by introducing levels at 0, 776, 1474, 1820, 1953, 2093, 2426, 2554, 2647 and 2828 keV. Limits on probable spin and parity values for the newly-introduced levels have been established. The level introduced at 2828 keV on the basis of a 1008–1043 keV γγ-coincidence must be fed by a weak β-branch of ⁸²Br with an end-point energy of 263 keV and log ft of approximately 6.1.