Nuclear resonance fluorescence in94Mo,95Mo and96Mo

Using gaseous sources of Tc₂O₇ containing the radioactive isotopes⁹⁴Tc,⁹⁵Tc and⁹⁶Tc, levels at 871.0keV (⁹⁴Mo), 765.8, 820.6, 947.8, 1074.0keV (⁹⁵Mo) and 778.3keV (⁹⁶Mo) have been excited. From the effective cross sections for nuclear resonance scattering and from the lifetimes of the 947.8, 1074.0 and 778.3keV levels known from Coulomb excitation experiments the profiles of theγ-lines have been determined. A broadening of theγ-lines due to Coulomb explosion of the molecules has been observed. Making use of the line profiles, lifetimes ofΤ=(6.4±1.0) ps andΤ=(0.90 ± 0.20) ps have been determined for the 765.8 and 820.6keV levels, respectively. The angular distribution of the resonantly scattered radiation yields an amplitude ratioδ for the mixed M1 E2 765.8keV transition ofδ=0.14 _?0.009 ^+0.08 . TheB(E2) from a Coulomb excitation experiment and the lifetimeΤ from the present experiment yield ¦δ¦=0.07±0.01 for the 820.6keV transition.     

Study of the excited 0+ states through conversion electron spectroscopy of neutron rich Zr and Mo fission products

A windowless Si(Li) electron detector has been used in conjunction with the gas filled fission product separator JOSEF to study totally converted transitions in Zr and Mo isotopes. The existence of twoβ-decay modes in⁹⁶Y,⁹⁸Y and¹⁰⁰Nb is confirmed. The half-lives of theβ-decaying levels feeding O ₂ ⁺ states in⁹⁶Zr and⁹⁸Zr are 6.0 ± 0.4 sec and 0.60±0.05 sec respectively. A search for other first excited O ₂ ⁺ states shows that no such states are apparent in¹⁰⁰Zr and¹⁰⁴Mo.     

Magnetic moments of the 2 1 + states in102, 104Mo

Theg factors of the first excited 2⁺ levels in the neutron-rich nuclei¹⁰²Mo and¹⁰⁴Mo have been studied through the measurement of the perturbed angular correlations for theγ-γ cascades between the 0 ₂ ⁺ -2 ₁ ⁺ -0 ₁ ⁺ level sequences. The results of g=0.42±0.07 for¹⁰²Mo and ofg= _?0.11 ^+0.12 for¹⁰⁴Mo agree with the prediction of the vibrational-rotational model. In terms of IBA, with the assumption ofN _π=3 for the Mo isotopes which takes into consideration a two particle, two-hole excitation across the Z=40 subshell, the proton-bosong factor is deduced to beg _π=1.00±0.23. It is shown that this value provides evidence for subshell effects in¹⁰⁰Zr.     

Gamma decay of93Mo states from92Mo (d,pγ) and93Tc β-decay

The decay scheme of the fragmented single neutron states of93Mo up to 3.2 MeV excitation energy is obtained from a⁹²Mo(d,pγ)⁹³Mo coincidence experiment. The total γ-spectrum from⁹²Mo+d shows additional strong γ-decays following the β-decay of⁹³Tc produced by the (d, n) reaction. The decay scheme is discussed in the frame of the particle-core coupling model. The important role of 2⁺ core excited components inE2 andM1 transitions between states with different angular momentum of the single particle component is pointed out.     

States in95Mo and99Mo populated in the (3He, α) reaction

The (³He,α) reaction on⁹⁶Mo and¹⁰⁰Mo targets has been studied at a bombarding energy of 18 MeV. Thel _n transfer assignments have been made on the basis of angular distribution patterns and on an analysis of the ratios of the experimental and theoretical cross-sections of (³He,α) and (d, t) reactions data leading to the same final states. New states are observed in⁹⁵Mo at 3373 keV (9/2⁺); spin and parity assignments are made to levels in⁹⁹Mo at 1621 keV 7/2⁺ (9/2⁺), 1778 keV (5/2^?) and 2078 keV (11/2^?).     

Level structure of106Mo

The level scheme of the very neutron rich nucleus ₁₀₆ ⁴² Mo₆₄ has been studied for the first time through theβ decay of¹⁰⁶Nb. Six new excited states were observed inγ singles andγ-γ coincidence experiments in addition to the 2⁺, 4⁺ and 6⁺ members of the ground state band. The excitation energies and the deexcitation pattern suggest the interpretation of the levels at 710, 885 and 956 keV as the 2 ₂ ⁺ , 3 ₁ ⁺ and 0 ₂ ⁺ states, respectively. The data support the assumption of a non-axial deformation of¹⁰⁶Mo. A half-life of (1.02±0.05) s has been determined for theβ decay of¹⁰⁶Nb.     

Untersuchung von 0+−0+-Übergängen in12C,24Mg,28Si,32S und40Ca durch unelastische Elektronenstreuung

Transitions from the 0⁺ ground states to 0⁺ excited states at 7.65 (¹²C), 6.44 (²⁴Mg), 4.98 and 6.69 (²⁸Si), 3.78 (³²S) and 3.35 (⁴⁰Ca) MeV have been studied with 28 to 60 MeV electrons at scattering angles from 105 to 165°. Matrix elements and transition radii have been deduced, using DWBA-calculations. The monopole excitations can be uniquely distinguished from electric quadrupole excitations by the angular dependence of the cross sections. Some results forE2- andE3-transitions in¹²C,²⁸Si,³²S and⁴⁰Ca are given, too.     

Identification and structure of high spin particle-hole states in89Mo

Particle-γ andγ-coincidences of the reaction⁵⁸Ni(³⁶Ar, 4pn)⁸⁹Mo have been used to gain more information about high spin states in⁸⁹Mo and to establish the yrast sequence up to 7.6 MeV excitation energy and probable spin 37/2 ?. Spins and parities were assigned on the basis of DCO-ratios measured with the OSIRIS spectrometer and a large volume Ge detector placed at 162° to the beam. Furthermore, aγ-ray angular distribution experiment was carried out using the reaction⁵⁸Ni(³⁵Cl, 3pn)⁸⁹Mo. As in the neighboring isotopes⁸⁸Mo and⁹⁰Mo, the positive-parity high-spin states can be grouped into shell model multiplets characterized by increasing seniorities of proton particles and neutron holes in the 1g_9/2 shell. The negative-parity states can be explained with one nucleon moving in thep _1/2 orbit. The energies and wave functions of these states have been deduced by means of the shell model code RITSSCHIL. The 2584 keV (21/2⁺) is an isomeric state the mean life of which has been estimated from delayedγγ-coincidences.     

The level structures of the nuclei232Th and238U

Time-of-flight gating techniques have been used to study the decay γ-rays from states excited by inelastic scattering of neutrons from²³²Th and²³⁸U. Neutron energies up to 1900 MeV have been used. From accurate determinations of the γ-ray energies, intensities and thresholds, detailed level and decay schemes have been obtained for²³²Th and²³⁸U. New levels in both nuclei are observed at larger excitations than before and the present work is incompatible with some previously accepted spin and collective band assignments derived from Coulomb excitation studies.     

Structure of the Triplet of low-lying states in101Mo

The properties of the triplet of low-lying states in¹⁰¹Mo have been studied through spectroscopy of theγ radiation following thermal neutron capture in¹⁰⁰Mo and β^? decay of¹⁰¹Nb and through a measurement of the proton angular distributions in the¹⁰⁰Mo(d,p) reaction with 14 MeV deuteron energy. The half-lives of the 13.5 keV state and the 57.0 keV 5/2⁺ state have been measured as 226(7) and 133(7)ns, respectively. These values and the quadrupole/dipole mixing ratios of the 13.5 keV and 43.5 keV transitions yield spin and parity 3/2⁺ for the 13.5 keV level. The E2 components in the 13.5 (3/2⁺ →1/2⁺) and 43.5 keV (5/2⁺→3/2⁺) transitions are ≦ 8·10^?4 and 54(9)%, respectively. The possibility of an additional state near to the 57.0 keV level is discussed. IBFM/PTQM calculations, taking into consideration the transitional character of the¹⁰⁰Mo boson core, account for the electromagnetic-transition and transfer-reaction pattern of the triplet of states.     

Evidence of non-statistical structures in the elastic and inelastic scattering of58Ni+58Ni and58Ni+62Ni and intermediate dinuclear states

Excitation functions and angular distributions of⁵⁸Ni+⁵⁸Ni and⁵⁸Ni+⁶²Ni scattering at energies just above the Coulomb barrier have been measured aroundθ _cm=90° in energy stepsΔE _cm=0.25 MeV fromE _cm ? 110 MeV toE _cm ? 120 MeV for⁵⁸Ni+⁵⁸Ni and fromE _cm ? 110 MeV toE _cm ? 118 MeV for⁵⁸Ni+⁶²Ni. Evidence for structure of non-statistical character has been found in the angle-summed excitation functions; this evidence is corroborated by the analysis of the angular distributions. This is the first time that non-statistical structure in elastic and inelastic scattering is reported with high confidence level for this mass and excitation energy ranges. Attempts are presented to understand the nature of this structure, including the presence of intermediate dinuclear states and virtual states in a potential well.     

The decay of the 11.80 MeV isobaric analog resonance in93Tc to negative parity states in92Mo

The 2,524 keV 5^? state and 2,848 keV3^? state in⁹²Mo were excited by inelastic proton scattering going through the 11.80 MeV isobaric analog resonance in⁹³Tc. Angular distributions of the 3^?→ 2⁺ and 5^?→ 4⁺ γ-rays were measured and analyzed in order to obtain the partial waves of the outgoing protons.     

The nilsson-potential parameters for neutrons at A≃-100 and new deformation values for103Mo and105Mo

The half-lives of the first excited levels in odd-neutron nuclei¹⁰³Mo and¹⁰⁵Mo have been measured. From these data, values of the deformation parameter of?=0.31±0.05 and 0.29±0.06 for¹⁰³Mo and¹⁰⁵Mo, respectively, have been deduced assuming prolate spheroidal shapes. The present results in combination with previously determined properties of the ground-state bands of these nuclei are used to determineμ, the magnitude of the coefficient of the 1² term, in the Nilsson Hamiltonian, for the new region of deformation atA～-100.     

Nucleon transfer reactions to rotational states induced by206, 208Pb projectiles

In a systematic study of nucleon transfer reactions accompanied by Coulomb excitation we have bombarded¹⁵²Sm,¹⁶⁰Gd and²³²Th with^{206, 208}pb beams at incident energies close to the Coulomb barrier. Particle-gamma coincidence techniques were used to identify excited states of reaction products populated through inelastic scattering and in nucleon transfer reactions. One-neutron stripping and pick-up reactions on¹⁵²Sm were observed leading to known states of the rotation alignedi _13/2-bands in¹⁵³Sm and¹⁵¹Sm. In the¹⁶⁰Gd+^{206, 208}Pb systems no significant population of low lying states of product nuclei was found in the nucleon-transfer channels. Large cross sections were observed for one- and two-neutron pick-up from²³²Th at an incident energy of 6.4 MeV/u. Around the grazing angle they are of the same order of magnitude as the cross section measured for inelastic scattering. The results are analyzed in the framework of semiclassical models.     

On the coexistence of oblate and prolate deformed bands in83Zr

Deformation parameters of the positive parity yrast band and negative parity bands in⁸³Zr are deduced from lifetimes andE2/M1 mixing ratios. Lifetimes of high spin states have been determined from recoil distance Doppler shift and Doppler shift attenuation measurements using the⁵⁴Fe(³²S,2pnγ) ⁸³Zr reaction. Ten lifetimes and five lifetimes limits were determined. The positive parity band, built on theg _9/2 K=5/2 orbital has an average deformation ¦β ₂¦=0.28(2), and shows a reduction ofE2 transition strengths in the observed backbend region at I^π≈21/2⁺. In contrast, theE2 strengths in the negative parity states show a steady increase up to I^π≈=15/2^?. These states are more strongly deformed than the positive parity states (¦β ₂¦=0.33(3)). TheE2/M1 mixing ratios show that the negative parity band hasK=3/2 and is prolate, and favour oblate deformation for the positive parity yrast band. In theK=1/2^? band theE2 strength of the 7/2^?→3/2^? transition yields a deformation ¦β ₂¦=0.26(5). The band structure is compared with calculations within the Hartree-Fock Bogoliubov cranking model.     

β-band excitation in inelastic hadron scattering and the mixing of the breathing mode into the low-lying β-vibrations

The excitation of the ²⁴Mg β-band 0⁺ and 2⁺ states at 6.43 MeV and 7.35 MeV, respectively, in inelastic hadron scattering has been considered in the collective model where coupling of these states of the states of the ground state band is via a ß-vibration coupled to the static deformation. It is found that coupled channel effects on the 0⁺ state excitation are rather important and moreover the excitation of the 0⁺ state can be satisfactorily explained only if a monopole breathing mode form factor is included in addition to the monopole β-vibration form factor.     

Theβ + decay of the new isotope86Mo and the first observation of86m Nb

Theβ ⁺ decay of⁸⁶Mo has been firstly investigated by means ofβγ spectroscopy. The⁸⁶Mo nuclei were produced by fusion-evaporation reactions of⁵⁴ Fe (³⁵Cl, 1 p2n) and⁵⁸Ni (³²S,2p 2n) at beam energies of 103 and 120 MeV, respectively. Threeγ rays of 47.3, 49.8 and 187.0 keV were unambiguously identified to follow theβ ⁺ decay of⁸⁶Mo by results ofXγ andβγ coincidence and cross-bombardment. A half life and a maximumβ ⁺-ray energy of⁸⁶Mo were determined to be 19.6±1.1 s and 3.9±0.4 MeV, respectively. A decay scheme of⁸⁶Mo is proposed in this article. Furthermore, a decay of⁸⁶Nb has been studied using the same combinations of projectiles and targets, and a newβ-decaying isomer^86m Nb was observed with a half life of 56.3±8.3 s.     

The gamma-decay of34Ar

States in³⁴Ar up to 5.5 MeV excitation energy, populated by the³²S(³He,nγ) reaction at 8–12 MeV bombarding energy, have been investigated with the Doppler shift attenuation method,nγ angular correlation andnγγ triple coincidence measurements. For the states at 2.09, 3.29 and 4.52 MeV the lifetimes 200±60 fs, 130±60 fs and 260±80 fs have been found, respectively. Thenγ correlations yielded the spin assignmentsJ ^μ=(2⁺) for the level at 4.13 MeV andJ ^μ=3^? for the 4.52 MeV state, and the mixing ratiosδ(3.29→2.09)=?0.12±0.05 andδ(4.13→3.29)=?0.52±0.15. The results are compared with shell model calculations and predictions from the weak coupling unified model.     

Oblate shapes of200, 202, 204Hg

Measurements of the reorientation effect for the first excited 2⁺ states in^{200, 202, 204}Hg were performed by exploiting the dependence of theγ-ray yield on Q₂+ for different projectiles. For²⁰⁰Hg, a positive quadrupole moment of Q₂=0.96±0.11 eb (for negative interference) or Q₂=1.11±0.11 eb (for positive interference) was determined indicating an oblate shape. Small positive Q₂ values were also found for²⁰²Hg and²⁰⁴Hg. Nine B(E2) values for excitation of the 2⁺, 2⁺′ and 4⁺ states in^196–204Hg measured.     

Odd neutron nuclei near A=100: Rotational bands in103Mo and105Mo populated in theβ − decays of103Nb and105Nb

Theβ ^? decays of¹⁰³Nb and¹⁰⁵Nb have been studied at the fission product separators JOSEF and LOHENGRIN. Half-lives of (1.5±0.2) s and (2.95±0.06) s, respectively, have been determined for these decays. Fromγ singles andγ-γ coincidence measurements extended level schemes for¹⁰³Mo and¹⁰⁵Mo have been established for the first time. The lowest energy levels of these nuclei are consistent with the interpretation as members of rotational bands built on a 3/2⁺ [411] Nilsson state. Evidence is presented for the location of the 9/2⁺ [404] configuration.