Measurements of γ-γ and γ-electron directional correlations in119Sb

The directional correlations ofγ-γ andγ-electron cascades in¹¹⁹Sb are measured, in the decay of^119mTe. Bothγ-γ andγ-electron directional correlation coefficients are determined for the cascades (energies in keV): 153.5-1212.7, 942.3-270.5, (976.2+979.3)-270.5, 1095.7-270.5 and 1136.8-270.5. For the cascades 912.6-1366.2, 2013.4-270.5 and 2089.9-270.5γ-γ directional correlations are measured. The mixing ratios evaluated are:δ(M2/E1, 153.5 keV)=0.0003±0.0023,δ(E2/M1, 270.5 keV)=-0.39±0.29,δ(E2/M1, 942.3 keV)= ?0.26±0.12,δ(E3/M2,1095.7 keV)=?0.01±0.07, andδ(M3/E2,1212.7 keV) =0.004±0.007. The result is compared with theoretical predictions.     

E2/M1 Mixing ratios of 2+-2+-transitions in58Fe,74Ge and186Os

E2/M1 mixing ratios of 2⁺-2⁺-transitions in⁵⁸Fe,⁷⁴Ge and¹⁸⁶Os were determined by measuring the angular correlation of the 2-2-0γγ-cascades in these nuclei. The following values were obtained:⁵⁸Fe(863 keV):δ=+1.10±0.20;⁷⁴Ge(609keV):δ=?2.9±0.8 and¹⁸⁶Os(630keV):δ=?13 _?3.5 ^+5.5 . These results are compared with theoretical predictions.     

Multipole mixing ratios of transitions in175Lu populated from the decay of175Hf

Electron capture decay of¹⁷⁵Hf(70 d) provides a possibility for unambiguous determination of the sign and magnitude of multipole mixing ratios for 89 keV and 114 keV transitions in¹⁷⁵Lu. This is because both gamma rays are in coincidence with the 230 keV transition which is of a pureE2 character. The results of theγ —γ directional correlation measurements, in terms ofE2/M1 mixing ratiosδ, areδ ₈₉ = 0.11±0.07 andδ ₁₁₄ = 0.465±0.005. In addition the directional correlation measurements of the 89γ- 343γ and 319γ-114γ cascades yieldδ ₃₄₃ = 0.08±0.07 andδ ₃₁₉ = ?0.152±0.015.Radioactivity ¹⁷⁵Hf from¹⁷⁴Hf(n, γ); measuredγ —γ(θ) deducedδ(E2/M1); Ge(Li) detectors.     

Spins of the levels and multipole mixing ratios of transitions in 125Sb determined from γ-γ directional correlation and polarization-directional correlation measurements

In order to resolve several discrepancies in spin assignments to levels in ¹²⁵Sb, directional correlations and polarization-directional correlations have been measured for several γ-γ cascades in ¹²⁵Sb populated from the decay of ¹²⁵Sn. Earlier results obtained from using NaI and Ge(Li) and NaI detectors were difficult to interpret due to the complex structure of the decay scheme. To improve the experimental situation, we have used two coaxial Ge(Li) detectors for the angular correlation measurements and a coaxial Ge(Li)-planar Ge(Li) combination for the polarization-directional correlations. Combination of the results of these measurements give unique spin assignments of $\text{11}\text{2}$^?, $\text{11}\text{2}$^?, $\text{9}\text{2}$⁺, $\text{11}\text{2}$⁺ and $\text{9}\text{2}$⁺ to the 1982 keV, 1890 keV, 1420 keV, 1089 keV and 1067 keV levels, respectively. The determined E2/M1 mixing ratios are : δ(470) = 0.010±0.027, δ(1067) = ?0.86±0.18, and δ(916) = ?0.02±0.01.     

Double-electron capture of Se and the search for neutrinoless decay

Experimental results on the measurement of the double-electron capture (εε) decay process of ⁷⁴Se are described. This decay is particularly interesting, because ⁷⁴Se is almost degenerate to the second excited state at 1204 keV in the daughter nucleus ⁷⁴Ge. Such a degeneracy favors a neutrinoless decay because of the large phase-space suppression for a decay with two neutrinos. Subsequent de-excitation would generate a 2γ-ray cascade of 608 and 596 keV, whose coincident detection provides a unique signature for this particular εε process. The 2γ-ray cascade has been searched for by a HPGe γ-ray detector in coincidence with a NaI detector using 3 kg of natural selenium.     

Spin values of the low lying nuclear levels of201Hg

Gamma-gamma directional correlations have been investigated for the cascades of 135-30 keV and 135-32 keV in²⁰¹Hg from the decay of²⁰¹Tl. A combination of NaI (Tl) and Si (Li) detectors was used for the experiments. Spin values ofI=1/2, 3/2 and 1/2 have been assigned to 1.58, 32.19 and 167.49 keV energy levels. In addition, the relative intensities of theγ rays have been measured with a Ge (Li) detector system. The results are 2.2±0.2, 2.2±0.2, 26.5±1.3, 1.6±0.1 and 100 for theγ rays of 30.60, 32.19, 135.34, 165.88 and 167.43 keV energies, respectively.     

Spin des 921 keV-Zustandes in99Tc

The angular correlation of the⁹⁹Tc 739-181 keV gamma-gamma cascade has been measured in a liquid molybdenium source. The result was:A ₂=0.0930 ± 0.0028,A ₄=?0.0095 ± 0.0042. The spin of the 921 keV level was determined to 3/2⁺. The mixing ratio of the 739 keV gamma-transition was measured to δ (E2/M1)=5.9 _?0.3 ^+0.4 .     

Multipole mixing ratios of γ-transltions in 182W

γ-γ directional correlation experiments were performed on 14 cascades in ¹⁸²W populated from the β^? decay of ¹⁸²Ta(115 d). Two Ge(Li) detectors were used in a coincidence arrangement, and the ¹⁸²Ta sources were dissolved in HF acid to minimize extranuclear perturbations. For the 1189keV, 2^? → 2⁺ transition, the measured directional correlation coefficients are consistent only with multipole mixing ratios $\text{δ}\text{(}\text{M}\text{2}\text{E}\text{1)}\text{= 0.45 ± 0.03}\text{and}\text{δ}\text{(E3}\text{E1)}\text{= ?0.67 ± 0.07}$. These mixing ratios are discussed and compared with the known conversion coefficients for the 1189keV transition. The E2/M1 multipole mixing ratios determined are (energy in keV): δ(66) = 0.15 ± 0.15, δ(85) = 0.31 ± 0.05, δ(114) = 0.31 ± 0.05, 0.56 ≦ δ(179) ≦ 1.36, δ(1121) = 12⁺²_?1, and δ(1231) = ?(32⁺¹⁴²_?15). The measured M2/E1 mixing ratios are: δ(68) = 0.03 ± 0.02, δ(152) = 0.014 ± 0.013 and δ(156) = ?0.13 ± 0.19.     

Mössbauer effect and nuclear moments of the 75 keV state of Dy161 and the 81 keV state of Dy162

The Mössbauer effect of theγ rays from the 74.5 keV state of Dy¹⁶¹ and the 80.7 keV state of Dy¹⁶² has been investigated. From hyperfine splitting patterns the magnetic moments μ(75 keV)=?(0.39±0.04) nm, μ(81 keV)=+(0.74±0.08) nm and the quadrupole momentQ(75 keV)=+(1.4±0.2)b have been determined. For the odd neutron nucleus Dy¹⁶¹ an effective spin g factorg _{s, eff}=0.76 g_{s, free} is deduced for the 75 keV level.     

Multipole mixing ratios of transitions in168Er

Time-integral and time-differentialγ-γ directional correlation measurements were performed for cascades in¹⁶⁸Er populated from the electron-capture decay of¹⁶⁸Tm(87d). The¹⁶⁸Tm source was dissolved in HF acid to minimize extranuclear perturbations. The results of the time-differential experiment for the 448-99.3 keV and 448-198 keV cascades showed agreement with time dependent interaction and gaveλ ₂(1094)=(0.79±0.09) ×10⁷ sec^?1. The attenuation factors for the 80 keV level were determined asG ₂₂ (80)=0.90±0.01 and G₄₄(80)=0.94±0.01. OnlyI=4 spin value for the 1094 keV level is consistent with our measurements. The 632, 731, 741, and 816 keV transitions connecting theK=2⁺ andK = 0⁺ rotational bands were found to be of almost pureE2 character. The 99.3, 198, 547, 720, 830, and 1277 keV transitions are of practically pureE1 multipolarity. The 448 keVMl transition has (0.8 _?0.4 ^+2.0 )%E2 admixture. The results for the 1014?80keV cascade give (23±4)%E3 component in the 1014 keV transition.     

Levels in74As from the74Ge(p,nγe)74As reaction

The low-lying levels in⁷⁴As have been studied by means ofγ-ray and internal conversion electron spectroscopy following the⁷⁴Ge(p,n)⁷⁴As reaction. New levels at 372.7, 532.8, 632.1, 731.6, 752.7, 758.3, 801.6, 902.9 and 1128.5 keV, not observed in earlier studies, have been established.J ^π assignments have been made to several low-lying levels. An earlier ambiguity regarding the identification of an isomeric level has been clarified. The half-life of a level at 271.4 keV has been measured to be 1.0±0.1 nsec; in addition, limits on half-lives of levels at 182.7, 277.5 and 425.4 keV have been assigned. The level structure is discussed on the basis of available nuclear models.     

Mean life of the 854 keV 02+ state in 74Se and the coexistence model

The mean life of the first excited 0₂⁺ state in ⁷⁴Se, only 219 keV above the first excited 2⁺ state at 635 keV, was measured to be 1.2±0.2 nsec, with delayed coincidence techniques. The 0₂⁺ state was populated by the decay of ⁷⁴Br produced via the ⁶⁰Ni(¹⁶O, pn)⁷⁴Br reaction. The extracted B(E2; 0₂⁺ → 20₁⁺) value is 14±2 s.p.u. which suggests that the 0₂⁺ state is collective. Application of a coexistence model in terms of spherical and deformed shapes is discussed for ⁷⁴Se.     

In-beam study of74Br and a first cascade in75Kr

An in-beam study of⁷⁴Br has been carried out using γ-ray spectroscopy in connection with the reactions (³He,p2in) and (d,2n) on⁷⁴Se targets. Separate level schemes on top of the two β-decaying isomers of⁷⁴Br are proposed. Two cascades connecting highspin states are assigned to populate theI ^π=4⁽⁺⁾ isomer. In this level scheme, the excited states at 72.1, 188.3 and 472.0 keV are found to have half-lives of 13.3, 0.7 and 0.7 ns, respectively. The low-spin isomer of⁷⁴Br is tentatively assigned asI ^π=(0^?). This state is populated by two other cascades. For the low-spin levels two-particle configurations of proton and neutron Nilsson orbitals are proposed. The high-spin states are tentatively interpreted as arising from the configurations (πg _9/2,νg _9/2) and (πg _3/2,νg _9/2). As a by-product, a cascade of four transitions has been observed during the³He bombardment of⁷⁴Se and tentatively assigned to negative-parity states in⁷⁵Kr.     

Suche nach dem Isomer74mAs

An activity with the decay propertiesT _1/2=(8.0±0.3)sec andE _γ=(283±5)keV has been produced bySchardt andGoodman by proton irradiation of thin layers of evaporated⁷³Ge and⁷⁴Ge on thick gold backings. This activity was interpreted as the new isomer^74mAs. In the present experiment a search for^74mAs was carried out using the reactions⁷⁵As(n, 2n),⁷¹Ga(α, n) and⁷⁴Ge(d, 2n).^74mAs could not be detected. Upper limits for the reaction cross sections were determined. It is discussed that the reported properties of^74mAs resemble the known properties of^197mAu.     

Nuclear structure effect on internal conversion ofl-forbidden transitions in139La,141Pr and203Tl

Accurate experimental internal conversion data have been used to study the effect of nuclear penetration in the case of thel-forbidden transitions in¹³⁹La (165.8 keV),¹⁴¹Pr (145.4 keV) and²⁰³Tl (279.2 keV). The nuclear penetration parameterλ and theE2/M 1 mixing ratioδ ² have been deduced by graphical analysis. Following results were obtained:λ=2.8±1.3,δ ² =(8.4 _?8.4 ^+14.0 )·10^?4 for¹³⁹La,λ=1.2±0.6,δ ²=(4.8±0.5)·10^?3 for¹⁴¹Pr, andλ=6.4±1.1,δ ²=1.36±0.12 for²⁰³Tl.     

Magnetic dipole moments of excited states of105Pd and other spectroscopic investigations in the decay of105g Ag

The IPAC-method has been used with the external magnetic field of 9.0 T of a split coil superconducting magnet and with the internal field of PdFe for a measurement of magnetic moments of¹⁰⁵Pd states populated in the decay of 41.29d¹⁰⁵Ag. The results are:μ _7/2 (645 keV)=?1.49(9) nmμ _5/2 (319 keV)=+0.95(20) nmμ _3/2 (280keV)=?0.074(13) nm. The half-life of the 645 keV state has been redetermined by use of cooled thallium free Nal detectors asT _1/2 (645 keV)=126(2) ps. γ-γ directional correlations were measured with a system of three large Ge planar diodes for the cascades 443–645 keV, 332–319 keV, 393–280 keV, and 64–280 keV and analyzed in terms of dipole quadrupole mixing ratios of theγ-lines involved. The spin of the 673 keV state was derived as l/2⁺.     

Electric quadrupole and magnetic dipole moments of the first excited 2+ states of186Os and188Os

The spectroscopic quadrupole moments and the magnetic dipole moments of the lowest 2⁺ states in¹⁸⁶Os (137 keV) and¹⁸⁸Os (155 keV) have been determined by Mößbauer transmission experiments. The electric quadrupole momentsQ ₂₊(Os 186)=? (1.80±0.22) b andQ ₂₊(Os 188)=?(1.81±0.24) b as well as their ratioQ ₂₊(Os 188)/Q ₂₊(Os 186)=1.00±0.07 within the limits of error agree withB(E2) data, if a comparison on the basis of the rotational model is made. For the g-factors and their ratio g₂₊(Os 186)=0.281±0.008, g₂₊(Os 188)=0.305±0.015 andg ₂₊(Os 188)/g ₂₊(Os 186)=1.08±0.05 was obtained. All results are compared with recent model calculations.     

70Ge(α, γ)74Se cross section measurements at energies of astrophysical interest

The cross section of the reaction⁷⁰Ge(α, γ)⁷⁴Se has been measured over the bombarding energy range of 5.05 MeV <E _α < 7.80 MeV using single and coincidence gamma spectroscopy techniques. The experimental S-factor values are in agreement with theoretical statistical-model calculations. Reaction rates for the⁷⁰Ge(α, γ)⁷⁴Se and the inverse (γ, α) reactions have been determined for appropriate temperatures.     

High spin states in77Se populated by the74Ge(α,n γ) reaction

⁷⁷Se has been investigated by the reaction⁷⁴Ge(α,nγ) at 14 MeV. Gamma singles spectra, gamma angular distributions and gamma-gamma coincidences have been taken. A level scheme has been established, spins and parities have been assigned. States of a rotational band on the 1/2^? ground state, a rotational band on the 5/2^? 249.7 keV state and an anormal band have been identified. Nuclear Reaction ⁷⁴Ge(α,n γ)E _α=14 MeV; measuredE _γ ,I _γ ,γ-γ-Coin.,γ-ang. distr.⁷⁷Se deduced levels,J, π. Enriched target, Ge (Li).     

Penetration effects in the internal conversion process of the 204 keV transition in205Tl

Penetration effects have been detected in²⁰⁵Tl by measuring theK, L and (M+N+...) internal conversion coefficients of the 204 keV, 3/2⁺→l/2⁺ transition. From the resulting values α _K =0.29±0.04, α _L =0.132±0.006 and α _M+N+...=0.0397±0.0034 the penetration parameter and the mixing ratio have been deduced to be λ=13.1±2.7 andδ ²=1.40±0.46, respectively.