Low-lying states of the102Rh nucleus

Zeitschrift für Physik A Hadrons and nuclei - The reaction32S+126Te has been used to determine theg-factor of theT 1/2=35 ns yrast isomeric state in154Er through the time-differential...     

Low-lying states of F2 +

Calculated potential energy curves for the 13 lowest electronic states of F₂ ⁺ are presented. Nine of the potential curves are found to possess substantial binding energies, while two others also display shallow, stable minima. The ordering, binding energies, relative equilibrium separations and vibrational frequencies of these curves should be of utility in helping to assign the large number of observed vibration-rotation lines in the electronic emission spectrum of F₂ ⁺. The calculated curves are in reasonable agreement with the available data on the two experimentally observed states.     

Low-lying states in112In

Low-lying states below 500 keV excitation in¹¹²In have been investigated via the¹¹²Cd(p, nγ) reaction. New levels have been established atE ^x=206.5keV and 456.1 keV from the measuredγ-ray excitation functions,γ?γ coincidences and the precision measurements of the (p, n) threshold energy of the ground state and of the 206.5 keV state of¹¹²In. Spins and parities of the 206.5 keV state (2⁺) and the 456.1 keV state (3⁺) and multipolarities and mixing ratios of the deexcitationγ-rays have been determined from the angular distributions and linear polarizations of the deexcitation γ-rays as well as the excitation functions of the residual levels. Possible configurations of the newly-found levels are discussed. Half-lives of two states have been remeasured:T _1/2=15.2±0.1 min for the ground state andT _1/2=20.9±0.1 min for the 156.4 keV (4⁺) state. The ground stateQ-value for the¹¹²Cd(p, n)¹¹² In reaction has been measured to be ?3.376±0.006 MeV.     

Low-lying vibrational states of145,147,149Nd

The fragmented neutron states in^145,147,149Nd detected through¹⁴⁴Nd(d, p) and^148,150Nd(d, t) reactions can be accounted for in terms of quasiparticles coupled with anharmonic vibrator model. The wave functions, obtained from diagonalisation of the Hamiltonian matrices are utilised to calculate B(E2), B(M1) and branching ratios in^145,147Nd. The calculated results are discussed in the light of the recent experimental findings.     

Low-lying electronic states of aluminum monoiodide

High-level ab initio calculations of aluminum monoiodide(AlI) molecule are performed by utilizing the multireference configuration interaction plus Davidson correction(MRCI+Q) method. The core-valence correlation(CV) and spin–orbit coupling(SOC) effect are considered. The adiabatic potential energy curves(PECs) of a total of 13 Λ–S states and 24 ? states are computed. The spectroscopic constants of bound states are determined, which are in accordance with the results of the available experimental and theoretical studies. The interactions between the Λ–S states are analyzed with the aid of the spin–orbit matrix elements. Finally, the transition properties including transition dipole moment(TDM),Frank–Condon factors(FCF) and radiative lifetime are obtained based on the computed PEC. Our study sheds light on the electronic structure and spectroscopy of low-lying electronic states of the AlI molecule.     

Low-lying two-particle states in the nucleus236Np

The ambiguities and the uncertainties about the energy levels of the doubly odd actinide nucleus ₉₃ ²³⁶ Np₁₄₃ are sought to be removed by determination of the bandhead energies of various two-particle configurations expected to appear in the low energy spectrum of this nucleus. The calculations involve quantitative evaluation of the zero range neutron-proton residual interaction energy contribution to the bandhead energy for each configuration. It is concluded that the ground state is the long-lived isomer with spin-parityI ^π=6^- arising from the configuration {5/2⁺[642] _p +7/2^?[743] _n }. Bandhead energies for eight two-particle states appearing upto an excitation energy of 400 keV are presented and the results are discussed in the context of the available and further experiments.     

Low-lying states and separabelized Skyrme interactions

A finite-rank separable approximation for the quasiparticle RPA calculations with Skyrme interactions that was proposed in our previous work is extended to take into account the coupling between one-and two-phonon terms in the wave functions of excited states. It is shown that the phonon-phonon coupling effect can be very important to reproduce experimental data.     

The electronic states of silicon monofluoride: Low-lying valence states

Hartree-Fock and configuration interaction calculations are reported for the lowest valence state of the SiF molecule. Deduced spectroscopic constants are in good agreement with the experimental values. The dipole moment calculated for SiF is consistent with a charge distribution corresponding to a Si⁺F^? configuration.     

The electronic states of carbon monofluoride: Low-lying valence states

Multiconfiguration Hartree-Fock calculations are reported on the low-lying valence states, the X²Π, ⁴Σ^?, B²Δ, and ²Σ^± states, of carbon monofluoride. The wavefunctions describe dissociation of the molecule to the correct atomic limits and take account of the atomic 2s-2p near-degeneracy effect. For the ground state the calculations give (with experimental values in parentheses): a bond length of 1.286 Å (1.2667 Å), a fundamental frequency of 1292 cm^?1 (1308 cm¹), and a dissociation energy of 3.93 eV (5.5 ± 0.1 eV). A ⁴Σ^? state arising from the $\text{C}\text{(}{}^3\text{P) +}\text{F}\text{(}{}^2\text{P)}$ manifold is calculated to lie just 2.66 eV above the ground state. The B²Δ state, calculated adiabatic excitation energy 6.59 eV (6.12 eV), is found to dissociate to $\text{C}\text{(}{}^1\text{D) +}\text{F}\text{(}{}^2\text{P)}$ via a potential maximum. Calculations are also reported on a repulsive ²Δ state arising from ground state atoms.     

Low-lying states and isospin excitation in the Ge isotopes

The level structure of ^64-70Ge isotopes has been studied within the framework of the interacting boson model-3（IBM-3） . The symmetry character in the proton and neutron degrees of freedom of the energy levels has been investigated. The isospin excitation states（T 〉 Tz） have been assigned for the ^64Ge（N = Z） nucleus. Some intruder states in these nuclei have been suggested. The calculated energy levels and transition probabilities are in good agreement with recent experimental data. The study indicates that the Ge isotopes are in transition from γ-unstable to vibrational.     

Low-lying states and isospin excitation in the Ge isotopes

The level structure of 64-70Ge isotopes has been studied within the framework of the interacting boson model-3 (IBM-3). The symmetry character in the proton and neutron degrees of freedom of the energy levels has been investigated. The isospin excitation states (T>Tz) have been assigned for the 64Ge (N=Z) nucleus. Some intruder states in these nuclei have been suggested. The calculated energy levels and transition probabilities are in good agreement with recent experimental data. The study indicates that the Ge isotopes are in transition from γ-unstable to vibrational.     

Low-lying excited states and photodissociation studies of cis-BrONO

A computational study of the low-lying singlet and triplet states of bromine nitrite, cis-BrONO, is presented. Calculations of excitation energies and oscillator strengths are reported using multi-reference configuration interaction, MRD-CI, methods in conjunction with the cc-pVDZ?+?sp and cc-pVTZ?+?sp basis sets. In agreement with recent experimental work the calculations find two important transitions, namely to the states 2¹ A′ at 3.99?eV and 4¹ A′ at 5.27?eV. The corresponding measurements obtained 3.87 and 5.44?eV, respectively. Both states show multi-reference character, representing a linear combination of 3a″?→?4a″ and 9a′?→?10a′ transitions. The potential energy curves for the Br+ONO dissociation are repulsive for both states indicating possible photodissociation. BrO+NO products are not favoured because the corresponding potential energy curves show barriers on the order of 0.5?eV.     

Low-lying states of the 16F nucleus

Low-lying proton-emitting states of ¹⁶F have been investigated through the sequential particle decay reactions ¹⁴N(³He, n)¹⁶F(p)¹⁵O. Excitation energies were determined by measuring outgoing proton energies. Estimations of proton decay widths and spin limitations were made from proton spectra and angular correlation data which were obtained by detecting the protons in time coincidence with the associated neutrons at θ_n = 0°. To date, the ground-state spin of ¹⁶F has been considered to be J = 0; however, the present work suggests J = 1 to be preferable.     

Low-lying nuclear deformed states and angular momentum projection

A fast computational method for approximate angular momentum projection is proposed for low-lying deformed nuclear states. The accuracy of the method is demonstrated by calculating the low-lying states of the ground-state band and the two 0⁺ excited bands in ¹⁶⁸Er with good experimental comparison.     

Vibrational states of a cobalt dimer on the (111) and (001) copper surfaces

The results of calculations of the total (lateral and vertical) relaxation of the (001) and (111) copper surfaces in the presence of a small cluster of cobalt adatoms, local vibrational density of states and polarizations of these states are presented. The calculations were performed using the atomic interaction potentials in a tight binding approximation. An analysis of the results obtained showed that the presence of a cobalt dimer gives rise to modification of the vibrational states of the copper surface and generation of new modes localized both on the adatoms of the cluster and the surface atoms of the substrate. The revealed anisotropy of surface relaxation along [001] results in deformation of atomic bonding and splitting of the vibrational modes of the dimer. The lifetimes of the vibrational states of the dimer are found to be nearly equal for both surfaces under study, with a frequency shift being however observed. Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 12, pp.73–78, December, 2008.